Multiband superconductors have featured one of the main challenges to achieve a comprehensive understanding of unconventional superconductivity. Here, the multiband character is studied separately as orbital and sublattice degrees of freedom, as they have different effects for the superconducting and magnetic or charge orders. We build on the framework of the matrix random-phase approximation (RPA), which accounts for the RPA Feynman diagrams and also vertex corrections, to treat the electron-electron interactions in an off-site degenerate Hubbard model. As a result, systems without a sublattice degree of freedom tend to be dominated by spin fluctuations, while systems with multiple sublattice sites and orbitals have the charge fluctuations favored. Finally, we explicitly demonstrate that the known suppression of the superconducting pairing strength $λ$ by spin fluctuations from repulsive interactions at zero momentum transfer $\boldsymbol{q}$ is countered by the finite-$\boldsymbol{q}$ pairing, which always improves $λ$.
The ruthenate family of layered perovskites has been a topic of intense interest with much work dedicated to understanding the superconducting state of the single layer, Sr$_2$RuO$_4$. Another longstanding puzzle is the lack of superconductivity in its sister compound, Sr$_3$Ru$_2$O$_7$, which constrains the possible superconducting mechanisms of Sr$_2$RuO$_4$. Here we address a microscopic mechanism that unifies superconducting and spin-density wave order in this family of materials. Beginning from a model of Sr$_2$RuO$_4$ featuring intraband pseudospin-singlet superconductivity originating f…
The calculations of the local and global properties of two band superconductors have been presented with particular attention to the role of the inter-orbital scattering of pairs. The properties of such superconductors are very different from a single band or typical two band systems with dominant intra-band pairing interactions. The role of Van Hove singularity in one of the bands on the properties of intra-band clean superconductor has been discussed. It leads to marked increase of superconducting transition temperature in the weak coupling limit. We study the inhomogeneous systems in which …
Even-parity interorbital spin-triplet pairing emerges as an intriguing candidate in multiorbital superconductors with significant Hund's and spin-orbit coupling. Within such a state, the pairing is dominated by the intraband pseudospin-singlet component via the spin-orbit coupling, distinguishing it from a pure spin triplet and motivating the name, shadowed triplet. With atomic spin-orbit coupling, it was shown that this pairing exhibits an anisotropic $s$-wave character, while higher angular momentum pairing symmetries such as $d$- or $g$-wave have been proposed based on phenomenological anal…
We study s-wave Cooper pairing in heavy-fermion systems. We analyze the periodic Anderson model by means of the variational cluster approach (VCA) focusing on the interorbital Cooper pairing between a conduction electron ($c$ electron) and an $f$ electron, called the "$c$-$f$ pairing." It is shown that the s-wave superconductivity appears coexisting with long-range antiferromagnetic order when electrons or holes are doped into the system at half filling. The antiferromagnetic order vanishes when the doping concentration exceeds a certain critical value, leading to a pure s-wave superconducting…
Orbital-selective Mottness Driven by Geometric Frustration of Interorbital Hybridization in Pr4Ni3O10
Tsinghua University（清华大学）；ShanghaiTech University（上海科技大学）；Songshan Lake Materials Laboratory（松山湖材料实验室）；Yale University（耶鲁大学）；Diamond Light Source（钻石光源）；University of Oxford（牛津大学）；Lanzhou University（兰州大学）；Shanghai Advanced Research Institute, Chinese Academy of Sciences（中国科学院上海高等研究院）；University of Science and Technology of China（中国科学技术大学）；SLAC National Accelerator Laboratory（斯坦福直线加速器中心）；Hefei National Laboratory（合肥国家实验室）
We investigate the Josephson transport properties in a Josephson junction consisting of a conventional $s$-wave superconductor coupled to a multi-orbital noncentrosymmetric superconductor marked by an orbitally driven inversion asymmetry and isotropic interorbital spin-triplet pairing. Contrary to the canonical single band noncentrosymmetric superconductor, we demonstrate that the local interorbital spin-triplet pairing is tied to the occurrence of sign-changing spin-singlet pair amplitude on different bands with $d$-wave symmetry. Such multi-band $d^{\pm}$-wave state is a unique superconducti…
We theoretically examine the orbital excitations coupled to the spin degree of freedom in the parent state of the iron-arsenide superconductor, based on the calculation in a five-band itinerant model. The calculated Fe $L_3$-edge resonant inelastic x-ray scattering (RIXS) spectra disclose the presence of spin-flip excitations involving several specific orbitals. Magnon excitations predominantly composed of a single orbital component can be seen in experiments, although its spectral weight is smaller than spin-flipped interorbital high-energy excitations. The detailed polarization and momentum …
We investigate the impact of impurity scattering on superconductivity in an anisotropic multi-orbital model with spin-orbit coupling which describes the electron fluid at two-dimensional oxide interfaces. As the pairing mechanism is under debate, both conventional and unconventional superconducting states are analyzed. We consider magnetic and nonmagnetic spin-dependent intra- and interorbital scattering and discuss possible microscopic realizations leading to these processes. It is found that, for magnetic disorder, the unconventional superconductor is protected against interband scattering a…
We extend the rotationally invariant formulation of the slave-boson method to superconducting states. This generalization, building on the recent work by Lechermann et al. [Phys. Rev. B {\bf 76}, 155102 (2007)], allows to study superconductivity in strongly correlated systems. We apply the formalism to a specific case of strongly correlated superconductivity, as that found in a multi-orbital Hubbard model for alkali-doped fullerides, where the superconducting pairing has phonic origin, yet it has been shown to be favored by strong correlation owing to the symmetry of the interaction. The metho…
We study superconductivity in the two-dimensional 16-band d-p model extracted from a tight-binding fit to the band structure of LaFeAsO, using the random phase approximation. When the intraorbital repulsion U is larger than the interorbital one U', an extended s-wave (s+--wave) pairing with sign reversal of order parameter is mediated by antiferromagnetic spin fluctuations, while when U<U' another kind of s-wave (s++-wave) pairing without sign reversal is mediated by ferro-orbital fluctuations. The s++-wave pairing is enhanced due to the electron-phonon coupling and then can be expanded over t…
Based on the effective four-band model we analyze the spin response in the normal and superconducting states of the Fe-pnictide superconductors. While the normal state spin excitations are dominated by the continuum of the interorbital antiferromagnetic fluctuations and the intraband spin density wave fluctuations, the unconventional superconductivity yields different feedback. The resonance peak in form of the well-defined spin exciton occurs {\it only} for the interband scattering at the antiferromagnetic momentum ${\bf Q}_{AFM}$ for the $s_\pm$ (extended s-wave) superconducting order parame…
Transverse Magnetic Response from Orbitally Polarized Cooper Pairs in Elemental Superconductors
CNR-SPIN, c/o Università di Salerno（意大利国家研究委员会自旋物理中心，萨莱诺大学）；Dipartimento di Fisica “E. R. Caianiello”, Università di Salerno（萨莱诺大学 E.R. 凯亚涅洛物理学系）；Wigner Research Centre for Physics, Institute for Solid State Physics and Optics（维格纳物理学研究中心，固体物理与光学研究所）
Time-reversal-invariant topological superconductors have a full paring gap in the bulk and gapless Majorana states at the edge or on the surface. Here, we theoretically propose topological superconductivity in a doped quantum spin Hall insulator. We study the pairing symmetry of doped Sn$X$ film within a two-orbital model, and show that it realizes a topological superconductor when the intraorbital attractive interaction is stronger than the interorbital interaction, which is generic for a doped quantum spin Hall insulator with strong spin-orbit coupling. Edge channels are studied in a tight-b…
Electronic structure, dimer physics, orbital-selective behavior, and magnetic tendencies in the bilayer nickelate superconductor La$_3$Ni$_2$O$_7$ under pressure
基于{\it ab initio}技术，研究了双层La$_3$Ni$_2$O$_7$在压力下的电子结构与磁性，揭示了其由$d_{3z^2-r^2}$轨道形成的二聚体晶格、双轨道最小模型、异常的轨道间跃迁及主导的自旋条纹序。
There is increasing recognition that the multiorbital nature of the 3d electrons is important to the proper description of the electronic states in the normal state of the iron-based superconductors. Earlier studies of the pertinent multiorbital Hubbard models identified an orbital-selective Mott phase, which anchors the orbital-selective behavior seen in the overall phase diagram. An important characteristics of the models is that the orbitals are kinetically coupled -- i.e. hybridized -- to each other, which makes the orbital-selective Mott phase especially nontrivial. A U(1) slave-spin meth…
We report a $μ$SR investigation of a non-centrosymmetric superconductor (LaNiC$_2$) in single crystal form. Compared to previous $μ$SR studies of non-centrosymmetric superconducting polycrystalline and powder samples, the unambiguous orientation of single crystals enables a simultaneous determination of the absolute value of the magnetic penetration depth and the vortex core size from measurements that probe the magnetic field distribution in the vortex state. The magnetic field dependence of these quantities unambiguously demonstrates the presence of two nodeless superconducting energy gaps. …
General trends of electronic structures, superconducting pairing, and magnetic correlations in the Ruddlesden-Popper nickelate $m$-layered superconductors La$_{m+1}$Ni$_{m}$O$_{3m+1}$
