Attaining viable thermoelectric cooling at cryogenic temperatures is of major fundamental and technological interest for novel electronics and quantum materials applications. In-device temperature control can provide a more efficient and precise thermal environment management as compared to the conventional global cooling. Here we develop nanoscale cryogenic imaging of a magneto-thermoelectric effect and demonstrate absolute cooling and an ultrahigh Ettingshausen effect in exfoliated WTe2 Weyl semimetal flakes at liquid He temperatures. Application of a current and perpendicular magnetic field gives rise to cooling via generation of electron-hole pairs on one side of the sample and heating by their recombination at the opposite side. In contrast to bulk materials, the cooling process is found to be nonmonotonic in magnetic field and device size. The derived model of magneto-thermoelectricity in mesoscopic semimetal devices shows that the cooling efficiency and the induced temperature profiles are governed by the interplay between sample geometry, electron-hole recombination length, magnetic field, and flake and substrate heat conductivities. The findings open the way for direct integration of microscopic thermoelectric cooling and for temperature landscape engineering in novel van der Waals devices.
The ideal reversible thermodynamic cycle visualization of the Nernst effect in Laughlin geometry, excluding the kinetic contribution is proposed. The Ettingshausen effect is also treated in the fashion using the reverse cycle. The corresponding values of the off-diagonal thermoelectric coefficients are expressed through the ratio of the entropy budget per magnetic flux. Our approach enlightens the profound thermodynamic origin of the relation between the Nernst effect and magnetization currents.
We investigate whether there could exist topological invariants of gapped 2D materials related to dissipationless thermoelectric transport at low temperatures. We give both macroscopic and microscopic arguments showing that thermoelectric transport coefficients vanish in the limit of zero temperature and thus topological invariants arise only from the electric Hall conductance and the thermal Hall conductance. Our arguments apply to systems with arbitrarily strong interactions. We also show that there is no analog of the Thouless pump for entropy.
Thermocurrent flowing through a single-molecule device contains valuable information about the quantum properties of the molecular structure and, in particular, on its electronic and phononic excitation spectra, and entropy. Furthermore, accessing the thermoelectric heat-to-charge conversion efficiency experimentally can help to select suitable molecules for future energy conversion devices, which - predicted by theoretical studies - could reach unprecedented efficiencies. However, one of the major challenges in quantifying thermocurrents in nanoscale devices is to determine the exact temperat…
Coherent Absorption Synergizes with Plasmon-Enhanced Graphene Terahertz Photo-thermoelectric Response
State Key Laboratory of Optoelectronic Materials and Technologies, Guangdong Province Key Laboratory of Display Material and Technology, and School of Electronics and Information Technology, Sun Yat-sen University（中山大学光电材料与技术国家重点实验室、广东省显示材料技术重点实验室、电子与信息学院）
