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arXiv 2312.03215cond-mat.supr-con
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块体极限下2H-NbSe₂中新型轨道Fulde-Ferrell-Larkin-Ovchinnikov态的证据

Evidence for the novel type of orbital Fulde-Ferrell-Larkin-Ovchinnikov state in the bulk limit of 2H-NbSe2

Chang-woo Cho, Timothée T. Lortz, Kwan To Lo, Cheuk Yin Ng, Shek Hei Chui, Abdel Rahman Allan, Mahmoud Abdel-Hafiez, Jaemun Park, Beopgil Cho, Keeseong Park, No… 展开作者

Chang-woo Cho, Timothée T. Lortz, Kwan To Lo, Cheuk Yin Ng, Shek Hei Chui, Abdel Rahman Allan, Mahmoud Abdel-Hafiez, Jaemun Park, Beopgil Cho, Keeseong Park, Noah F. Q. Yuan, Rolf Lortz

AI总结:

本研究通过高分辨率直流磁化和磁扭矩实验,发现块体2H-NbSe₂在4T及以上平行基面磁场中存在轨道FFLO态的证据,其磁扭矩异常及上临界场6重对称性与薄层样品的轨道FFLO态特征一致。

摘要:

Fulde-Ferrell-Larkin-Ovchinnikov(FFLO)态是一种特殊的超导态,能抵抗超过泡利顺磁极限的强磁场,其超导序参量在实空间呈现空间调制,极为罕见。近期,一种更奇特的变体——轨道FFLO态在过渡金属二硫化物超导体2H-NbSe₂中被预测并识别,该态出现于厚度约40 nm以下的薄样品中,处于二维与三维的边界。伊辛自旋轨道耦合与泡利顺磁效应的复杂相互作用,可在磁相图的较大范围内稳定FFLO态,甚至远低于泡利极限。本研究提供了块体2H-NbSe₂样品中形成轨道FFLO态的实验证据,这些证据通过在严格平行于NbSe₂基面的磁场中进行高分辨率直流磁化和磁扭矩实验获得。在4 T及以上磁场中,这两个量在正常态边界处均显示出向不连续一级超导转变的交叉,这通常被视为泡利顺磁对断裂效应影响超导态的标志。磁扭矩揭示了一个小的阶梯状可逆异常,表明磁场诱导了超导态内的热力学相变,该异常与其他FFLO超导体中的FFLO转变有许多相似之处,暗示块体2H-NbSe₂样品中可能存在轨道FFLO态。此外,我们观察到该相变以上磁场范围内上临界场具有明显的面内6重对称性,这此前被解释为薄2H-NbSe₂中轨道FFLO态的标志。

英文摘要:

The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state, an unusual superconducting state, defies high magnetic fields beyond the Pauli paramagnetic limit. It exhibits a spatial modulation of the superconducting order parameter in real space and is exceptionally rare. Recently, an even more exotic variant - the orbital FFLO state - was predicted and identified in the transition metal dichalcogenide superconductor 2H-NbSe2. This state emerges in thin samples with thicknesses below ~40 nm, at the boundary between two and three dimensions. The complex interplay between Ising spin orbit coupling and the Pauli paramagnetic effect can lead to a stabilization of the FFLO state in a relatively large range of the magnetic phase diagram, even well below the Pauli limit. In this study, we present experimental evidence of the formation of this orbital FFLO state in bulk 2H-NbSe2 samples. This evidence was obtained using high-resolution DC magnetization and magnetic torque experiments in magnetic fields applied strictly parallel to the NbSe2 basal plane. Both quantities display a crossover to a discontinuous first-order superconducting transition at the normal state boundary in magnetic fields of 4 T and above. This is usually seen as a sign that Pauli paramagnetic pair breaking effects affect the superconducting state. The magnetic torque reveals a small step-like reversible anomaly, indicating a magnetic field-induced thermodynamic phase transition within the superconducting state. This anomaly bears many similarities to the FFLO transitions in other FFLO superconductors, suggesting the potential existence of an orbital FFLO state in bulk 2H-NbSe2 samples. Additionally, we observe a pronounced in-plane 6-fold symmetry of the upper critical field in the field range above this phase transition, which has previously been interpreted as a hallmark of the orbital FFLO state in thin 2H-NbSe2.

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