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arXiv 2311.03435cond-mat.mes-hallcond-mat.str-el

来自非线性霍尔效应的隐藏八极序特征

Signatures of hidden octupolar order from nonlinear Hall effects

Sopheak Sorn, Adarsh S. Patri

AI总结:

针对磁学中隐藏多极序难探测的问题,提出用非线性霍尔效应作为金属体系多极序的新探针,构建相关模型并证明贝里曲率四极子可产生可测的霍尔电压三次谐波,为多极序研究开辟新方向。

摘要:

用传统探针探测对称性破缺的隐藏序一直是磁学领域的长期挑战。高阶多极序——由自旋轨道耦合与晶体环境共同作用产生的各向异性电荷和磁化分布——是这类隐藏序的典型例子,目前仍亟需新的直接探测方案。在本研究中,我们提出将非线性霍尔效应作为金属体系中多极序的新型探测手段。受Pr基重费米子化合物家族Pr(Ti,V)$_2$Al$_{20}$的启发,我们构建了一个与铁八极序参量耦合的传导电子最小立方晶格模型。这种破坏时间反演对称性的序会产生支持强贝里曲率(BC)四极矩的能带结构。结合半经典玻尔兹曼形式理论与对称性分析,我们证明贝里曲率四极子会产生可在交流霍尔实验中测量的霍尔电压三次谐波$[V_H(3 ω)]$。我们还研究了霍尔响应的各向异性、无耗散性及其对序参量的依赖等性质。本工作为通过非线性输运实验研究多极序开辟了新方向。

英文摘要:

Detecting symmetry-breaking hidden orders with conventional probes has been a long-standing challenge in the field of magnetism. Higher-rank multipolar ordering $-$ anisotropic charge and magnetization distributions arising from a combination of spin-orbit coupling and crystalline environments $-$ is a quintessential example of such hidden orders, where new protocols of direct detection remain highly desirable. In this work, we propose non-linear Hall effects as a novel probe for multipolar ordering in metallic systems. Taking inspiration from the family of Pr-based heavy-fermion compounds, Pr(Ti,V)$_2$Al$_{20}$, we formulate a minimal cubic-lattice model of conduction electrons coupled to a ferro-octupolar order parameter. The time-reversal-breaking order leads to a band structure that supports strong quadrupolar moments of the Berry curvature (BC). Using a semi-classical Boltzmann formalism in conjunction with a symmetry analysis, we demonstrate that the BC quadrupoles produce a third harmonic generation of the Hall voltage $[V_H(3 ω)]$ measurable in an AC Hall experiment. Properties of the Hall response such as its anisotropy, its dissipationlessness, and its dependence on the order parameter are also examined. Our work encourages a new realm of investigation of multipolar ordering from non-linear transport experiments.

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