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arXiv 2308.03483cond-mat.mtrl-sci
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如何增强磁性外尔半金属Co$_3$Sn$_2$S$_2$中的反常霍尔效应?

How to enhance anomalous Hall effects in magnetic Weyl semimetal Co$_3$Sn$_2$S$_2$?

Shivam Rathod, Megha Malasi, Archana Lakhani, Devendra Kumar

AI总结:

本文通过选择性和共化学掺杂调控Co₃Sn₂S₂的化学势与Berry曲率,在In掺杂中协同增强AHA和AHC,并在电子-空穴等量共掺杂保持化学势不变时使内禀AHC提升约116%。

摘要:

大的自旋轨道耦合、kagome晶格、具有能带反转反交叉的非平庸拓扑能带结构以及外尔节点,是获得最大反常霍尔效应(AHE)所理想需要的关键要素,这些要素同时存在于Co$_3$Sn$_2$S$_2$中。它是同时展示大内禀反常霍尔电导率(AHC)和巨反常霍尔角(AHA)的领先平台,且所需磁场很低。Co$_3$Sn$_2$S$_2$中的巨AHE对小尺度掺杂相关的化学势变化具有鲁棒性。在本工作中,我们揭示了一种选择性和共化学掺杂路线,以最大化Co$_3$Sn$_2$S$_2$中的AHE。首先,在Co$_3$Sn$_{2-x}$In$_x$S$_2$中,我们将化学势置于Berry曲率热点处,同时在高迁移率区域获得最大的非对称杂质散射。结果在x=0.05时,由于带隙节点线修正的Berry曲率中外禀和内禀机制的协同增强,我们发现AHA(95%)和AHC(190%)显著增强。随后,预期AHE进一步改善,我们生长了空穴共掺杂的Co$_{3-y}$Fe$_y$Sn$_{2-x}$In$_x$S$_2$晶体,却发现AHE反而受到抑制。当掺杂后化学势不发生变化时,可以更好地理解掺杂剂在提供外禀效应或能带展宽方面的作用。通过在Co$_{3-y-z}$Fe$_y$Ni$_z$Sn$_2$S$_2$中同时等量共掺杂电子和空穴,我们保持了化学势不变。此后,我们发现由于kagome能带中的无序展宽,内禀AHC显著增强了约116%。

英文摘要:

Large spin-orbit coupling, kagome lattice, nontrivial topological band structure with inverted bands anti-crossings, and Weyl nodes are essential ingredients, ideally required to obtain maximal anomalous Hall effect (AHE) are simultaneously present in Co$_3$Sn$_2$S$_2$. It is a leading platform to show large intrinsic anomalous Hall conductivity (AHC) and giant anomalous Hall angle (AHA) simultaneously at low fields. The giant AHE in Co$_3$Sn$_2$S$_2$ is robust against small-scale doping-related chemical potential changes. In this work, we unveil a selective and co-chemical doping route to maximize AHEs in Co$_3$Sn$_2$S$_2$. To begin with, in Co$_3$Sn$_{2-x}$In$_x$S$_2$, we brought the chemical potential at the hotspot of Berry curvature along with a maximum of asymmetric impurity scattering in high mobility region. As a result at x=0.05, we found a significant enhancement of AHA (95%) and AHC (190%) from the synergistic enhancement of extrinsic and intrinsic mechanisms from modified Berry curvature of gaped nodal lines. Later, with anticipation of further improvements in AHE, we grew hole-co-doped Co$_{3-y}$Fe$_y$Sn$_{2-x}$In$_x$S$_2$ crystals, where we found rather a suppression of AHEs. The role of dopants in giving extrinsic effects or band broadening can be better understood when chemical potential does not change after doping. By simultaneous and equal co-doping with electrons and holes in Co$_{3-y-z}$Fe$_y$Ni$_z$Sn$_2$S$_2$, we kept the chemical potential unchanged. Henceforth, we found a significant enhancement in intrinsic AHC $\sim$116% due to the disorder broadenings in kagome bands

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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