Scalable spin squeezing in a dipolar Rydberg atom array
Guillaume Bornet, Gabriel Emperauger, Cheng Chen, Bingtian Ye, Maxwell Block, Marcus Bintz, Jamie A. Boyd, Daniel Barredo, Tommaso Comparin, Fabio Mezzacapo, To… 展开作者
Guillaume Bornet, Gabriel Emperauger, Cheng Chen, Bingtian Ye, Maxwell Block, Marcus Bintz, Jamie A. Boyd, Daniel Barredo, Tommaso Comparin, Fabio Mezzacapo, Tommaso Roscilde, Thierry Lahaye, Norman Y. Yao, Antoine Browaeys
The standard quantum limit bounds the precision of measurements that can be achieved by ensembles of uncorrelated particles. Fundamentally, this limit arises from the non-commuting nature of quantum mechanics, leading to the presence of fluctuations often referred to as quantum projection noise. Quantum metrology relies on the use of non-classical states of many-body systems in order to enhance the precision of measurements beyond the standard quantum limit. To do so, one can reshape the quantum projection noise -- a strategy known as squeezing. In the context of many-body spin systems, one typically utilizes all-to-all interactions (e.g. the one-axis twisting model) between the constituents to generate the structured entanglement characteristic of spin squeezing. Motivated by recent theoretical work, here we explore the prediction that short-range interactions -- and in particular, the two-dimensional dipolar XY model -- can also enable the realization of scalable spin squeezing. Working with a dipolar Rydberg quantum simulator of up to 100 atoms, we demonstrate that quench dynamics from a polarized initial state lead to spin squeezing that improves with increasing system size up to a maximum of -3.5 dB (prior to correcting for detection errors, or approximately -5 dB after correction). Finally, we present two independent refinements: first, using a multistep spin-squeezing protocol allows us to further enhance the squeezing by approximately 1 dB, and second, leveraging Floquet engineering to realize Heisenberg interactions, we demonstrate the ability to extend the lifetime of the squeezed state by freezing its dynamics.
We analyze spin squeezing via Rydberg dressing in optical lattice clocks with random fractional filling. We compare the achievable clock stability in different lattice geometries, including unity-filled tweezer clock arrays and fractionally filled lattice clocks with varying dimensionality. We provide practical considerations and useful tools in the form of approximate analytical expressions and fitting functions to aid in the experimental implementation of Rydberg-dressed spin squeezing. We demonstrate that spin squeezing via Rydberg dressing in one-, two-, and three-dimensional optical latti…
This review summarizes experimental works performed over the last decade by several groups on the manipulation of a few individual interacting Rydberg atoms. These studies establish arrays of single Rydberg atoms as a promising platform for quantum state engineering, with potential applications to quantum metrology, quantum simulation and quantum information.
We demonstrate a cooperative optical non-linearity caused by dipolar interactions between Rydberg atoms in an ultra-cold atomic ensemble. By coupling a probe transition to the Rydberg state we map the strong dipole-dipole interactions between Rydberg pairs onto the optical field. We characterize the non-linearity as a function of electric field and density, and demonstrate the enhancement of the optical non-linearity due to cooperativity.
We experimentally study the effects of the anisotropic Rydberg-interaction on $D$-state Rydberg polaritons slowly propagating through a cold atomic sample. In addition to the few-photon nonlinearity known from similar experiments with Rydberg $S$-states, we observe the interaction-induced dephasing of Rydberg polaritons at very low photon input rates into the medium. We develop a model combining the propagation of the two-photon wavefunction through our system with nonperturbative calculations of the anisotropic Rydberg-interaction to show that the observed effect can be attributed to pairwise…
How do isolated quantum systems approach an equilibrium state? We experimentally and theoretically address this question for a prototypical spin system formed by ultracold atoms prepared in two Rydberg states with different orbital angular momenta. By coupling these states with a resonant microwave driving we realize a dipolar XY spin-1/2 model in an external field. Starting from a spin-polarized state we suddenly switch on the external field and monitor the subsequent many-body dynamics. Our key observation is density dependent relaxation of the total magnetization much faster than typical de…
We study the effect of dipolar interactions on the level of squeezing in spin-1 Bose-Einstein condensates by using the single mode approximation. We limit our consideration to the $\mathfrak{su}(2)$ Lie subalgebra spanned by spin operators. The biaxial nature of dipolar interactions allows for dynamical generation of spin-squeezed states in the system. We analyze the phase portraits in the reduced mean-filed space in order to determine positions of unstable fixed points. We calculate numerically spin squeezing parameter showing that it is possible to reach the strongest squeezing set by the tw…
We show that the interaction between Rydberg atomic states can provide continuous spin squeezing of atoms with two ground states. The interaction prevents the simultaneous excitation of more than a single atom in the sample to the Rydberg state, and we propose to utilize this blockade effect to realize an effective collective spin hamiltonian J_x^2-J_y^2. With this hamiltonian the quantum mechanical uncertainty of the spin variable J_x+J_y can be reduced significantly.
We examine interactions between atoms continuously and coherently driven between the ground state and a Rydberg state, producing "Rydberg-dressed atoms." Because of the large dipolar coupling between two Rydberg atoms, a small admixture of Rydberg character into a ground state can produce an atom with a dipole moment of a few Debye, the appropriate size to observe interesting dipolar physics effects in cold atom systems. We have calculated the interaction energies for atoms that interact via the dipole-dipole interaction and find that due to blockade effects, the R-dependent two-atom interacti…
We propose a Rydberg molecule dressing scheme to create strong and long-ranged interactions at selective distances. This is achieved through laser coupling ground-state atoms off-resonantly to an attractive molecular curve of two interacting Rydberg atoms. Although dephasing due to Rydberg state decay occurs in all dressing schemes, an advantage of the molecule dressing is that a large ratio of dressed interaction to dephasing rate can be realized at large atomic separations. In an optical lattice or tweezer setting, we show that the strong interaction permits the fast generation of spin squee…
We investigate the dipole mediated transport of Rydberg impurities through an ultracold gas of atoms excited to an auxiliary Rydberg state. In one experiment we continuously probe the system by coupling the auxiliary Rydberg state to a rapidly decaying state which realizes a dissipative medium. In-situ imaging of the impurities reveals diffusive spreading controlled by the intensity of the probe laser. By preparing the same density of hopping partners but then switching off the dressing fields the spreading is effectively frozen. This is consistent with numerical simulations which indicate the…
We study the quantum critical effect enhanced spin-nematic squeezing and quantum Fisher information (QFI) in the spin-1 dipolar atomic Bose-Einstein condensate. We show that the quantum phase transitions can improve the squeezing and QFI in the nearby regime of critical point, and the Heisenberg-limited high-precision metrology can be obtained. The different properties of the ground squeezing and entanglement under even and odd number of atoms are further analyzed, by calculating the exact analytical expressions.We also demonstrate the squeezing and entanglement generated by the spin-mixing dy…
We study a bulk fermionic dipolar molecular gas in the quantum degenerate regime confined in a two-dimensional geometry. We consider two rotational states that encode a spin 1/2 degree of freedom. We derive a long-range interacting XXZ model describing the many-body spin dynamics of the molecules valid in the regime where motional degrees of freedom are frozen. Due to the spatially extended nature of the harmonic oscillator modes, the interactions in the spin model are very long-ranged and the system behaves close to the collective limit, resulting in robust dynamics and generation of entangle…
A scheme is proposed to prepare squeezed states and Schrödinger cat-like states of the collective spin degrees of freedom associated with a pair of ground states in an atomic ensemble. The scheme uses an effective Jaynes-Cummings interaction which can be provided by excitation of the atoms to Rydberg states and an effective J_x interaction implemented by a resonant Raman coupling between the atomic ground states. Both dynamical evolution with a constant Hamiltonian and with adiabatic variation of the two interaction terms are studied. We show that by the application of further resonant laser f…
We investigate the process of spin squeezing in a ferromagnetic dipolar spin-1 Bose-Einstein condensate under the driven oneaxis twisting scheme, with emphasis on the detrimental effect of noisy environments (stray magnetic fields) which completely destroy the spin squeezing. By applying concatenated dynamical decoupling pulse sequences with a moderate bias magnetic field to suppress the effect of the noisy environments, we faithfully reconstruct the spin squeezing process under realistic experimental conditions. Our noise-resistant method is ready to be employed to generate the spin squeezed …
We present a theoretical analysis of the implementation of an entangling quantum gate between two trapped Ca$^+$ ions which is based on the dipolar interaction among ionic Rydberg states. In trapped ions the Rydberg excitation dynamics is usually strongly affected by mechanical forces due to the strong couplings between electronic and vibrational degrees of freedom in inhomogeneous electric fields. We demonstrate that this harmful effect can be overcome by using dressed states that emerge from the microwave coupling of nearby Rydberg states. At the same time these dressed states exhibit long r…
A three-level atomic medium can be made transparent to a resonant probe field in the presence of a strong control field acting on an adjacent atomic transition to a long-lived state, which can be represented by a highly excited Rydberg state. The long-range interactions between the Rydberg state atoms then translate into strong, non-local, dispersive or absorptive interactions between the probe photons, which can be used to achieve deterministic quantum logic gates and single photon sources. Here we show that long-range dipole-dipole exchange interaction with one or more spins -- two-level sys…
We propose a simple setup of Rydberg atoms in a honeycomb lattice which gives rise to topologically protected edge states. The proposal is based on the combination of dipolar exchange interaction, which couples the internal angular momentum and the orbital degree of freedom of a Rydberg excitation, and a static magnetic field breaking time reversal symmetry. We demonstrate that for realistic experimental parameters, signatures of topologically protected edge states are present in small systems with as few as 10 atoms. Our analysis paves the way for the experimental realization of Rydberg syste…
We propose an experiment to demonstrate a novel blockade mechanism caused by long-range anisotropic interactions in an ultracold dipolar gas composed of the recently observed "butterfly" Rydberg molecules. At the blockade radius, the strong intermolecular interaction between two adjacent molecules shifts their molecular states out of resonance with the photoassociation laser, preventing their simultaneous excitation. When the molecules are prepared in a quasi-one-dimensional (Q1D) trap, the interaction's strength can be tuned via a weak external field. The molecular density thus depends strong…
In this chapter, we present an overview of experiments with trapped Rydberg ions and outline the advantages and challenges of developing applications of this new platform for quantum computing, sensing and simulation. Trapped Rydberg ions feature several important properties, unique in their combination: they are tightly bound in a harmonic potential of a Paul trap, in which their internal and external degrees of freedom can be controlled in a precise fashion. High fidelity state preparation of both internal and motional states of the ions has been demonstrated, and the internal states have be…
The quest to realize topological band structures in artificial matter is strongly focused on lattice systems, and only quantum Hall physics is known to appear naturally also in the continuum. In this letter, we present a proposal based on a two-dimensional cloud of atoms dressed to Rydberg states, where excitations propagate by dipolar exchange interaction, while the Rydberg blockade phenomenon naturally gives rise to a characteristic length scale, suppressing the hopping on short distances. Then, the system becomes independent of the atoms' spatial arrangement and can be described by a contin…
We investigate the coupling of a nanomechanical oscillator in the quantum regime with molecular (electric) dipoles. We find theoretically that the cantilever can produce single-mode squeezing of the center-of-mass motion of an isolated trapped molecule and two-mode squeezing of the phonons of an array of molecules. This work opens up the possibility of manipulating dipolar crystals, which have been recently proposed as quantum memory, and more generally, is indicative of the promise of nanoscale cantilevers for the quantum detection and control of atomic and molecular systems.
We study interactions between polaritons, arising when photons strongly couple to collective excitations in an array of two-level atoms trapped in an optical lattice inside a cavity. We consider two types of interactions between atoms: Dipolar forces and atomic saturability, which ranges from hard-core repulsion to Rydberg blockade. We show that, in spite of the underlying repulsion in the subsystem of atomic excitations, saturability induces a broadband bunching of photons for two-polariton scattering states. We interpret this bunching as a result of interference, and trace it back to the mis…
Feshbach resonances in ultra-cold atomic gases have led to some of the most important advances in atomic physics. They did not only enable ground breaking work in the BEC-BCS crossover regime [1], but are also widely used for the association of ultra-cold molecules [2], leading to the formation of molecular Bose-Einstein condensates [3,4] and ultra-cold dipolar molecular systems [5]. Here, we demonstrate the experimental realization of an optical Feshbach resonance using ultra-long range Rydberg molecules [6]. We show their practical use by tuning the revival time of a quantum many-body system…
We discuss a candidate solution for the controlled trapping and manipulation of two individual Rydberg atoms by means of a magnetic Ioffe-Pritchard trap that is superimposed by a constant electric field. In such a trap Rydberg atoms experience a permanent electric dipole moment that can be of the order of several hundred Debye. The interplay of electric dipolar repulsion and three dimensional magnetic confinement leads to a well controllable equilibrium configuration with tunable trap frequency and atomic distance. We thoroughly investigate the trapping potentials and analyze the interaction-i…
Mach-Zehnder interferometer, a powerful tool for a wide variety of measurements, has been realized with Bose-Einstein condensates in recent experiments. In this report, we propose and analyze a realizable scheme for performing a Heisenberg-limited Mach-Zehnder interferometry with dipolar spin-1 condensate. Based upon adiabatic processes of sweeping the transverse magnetic field, we demonstrate a perfect phase transition, which accomplishes the beam splitter, phase shifter and recombiner as for a Mach-Zehnder interferometer. The attractive dipolar interaction ensures the existence of a path-ent…
We put forward and discuss in detail a scheme to achieve Bose-Einstein condensation of stationary-light dark-state polaritons with dipolar interaction. To this end we have introduced a diamond-like coupling scheme in a vapor of Rydberg atoms under the frozen gas approximation. To determine the system's dynamics we employ normal modes and identify the dark-state polariton corresponding to one of the modes. We show that in contrast to atomic dipolar ultra-cold vapors dark-state polariton Bose-Einstein condensates proposed here can be stable for a negative dipolar interaction constant.
We propose a scheme for realizing fractional quantum Hall states of light. In our scheme, photons of two polarizations are coupled to different atomic Rydberg states to form two flavors of Rydberg polaritons that behave as an effective spin. An array of optical cavity modes overlapping with the atomic cloud enables the realization of an effective spin-1/2 lattice. We show that the dipolar interaction between such polaritons, inherited from the Rydberg states, can be exploited to create a flat, topological band for a single spin-flip excitation. At half filling, this gives rise to a photonic (o…
The concept of topological phases is a powerful framework to characterize ground states of quantum many-body systems that goes beyond the paradigm of symmetry breaking. While a few topological phases appear in condensed matter systems, a current challenge is the implementation and study of such quantum many-body ground states in artificial matter. Here, we report the experimental realization of a symmetry protected topological phase of interacting bosons in a one-dimensional lattice, and demonstrate a robust ground state degeneracy attributed to protected edge states. The setup is based on ato…
We experimentally realize a Peierls phase in the hopping amplitude of excitations carried by Rydberg atoms, and observe the resulting characteristic chiral motion in a minimal setup of three sites. Our demonstration relies on the intrinsic spin-orbit coupling of the dipolar exchange interaction combined with time-reversal symmetry breaking by a homogeneous external magnetic field. Remarkably, the phase of the hopping amplitude between two sites strongly depends on the occupancy of the third site, thus leading to a correlated hopping associated to a density-dependent Peierls phase. We experimen…
We show how to realize quantum state transfer between distant qubits using the chiral edge states of a two-dimensional topological spin system. Our implementation based on Rydberg atoms allows to realize the quantum state transfer protocol in state of the art experimental setups. In particular, we show how to adapt the standard state transfer protocol to make it robust against dispersive and disorder effects.
Expanding the Neutral Atom Gate Set: Native iSWAP and Exchange Gates from Dipolar Rydberg Interactions
Institute for Theoretical Physics, University of Innsbruck（因斯布鲁克大学理论物理研究所）；Parity Quantum Computing GmbH（Parity量子计算有限公司）；Parity Quantum Computing Germany GmbH（Parity量子计算德国有限公司）；Parity Quantum Computing France SAS（Parity量子计算法国股份有限公司）
We report on the realization of long-range Ising interactions in a cold gas of cesium atoms by Rydberg dressing. The interactions are enhanced by coupling to Rydberg states in the vicinity of a Förster resonance. We characterize the interactions by measuring the mean-field shift of the clock transition via Ramsey spectroscopy, observing one-axis twisting dynamics. We furthermore emulate a transverse-field Ising model by periodic application of a microwave field and detect dynamical signatures of the paramagnetic-ferromagnetic phase transition. Our results highlight the power of optical address…
We propose a new protocol for preparing spin squeezed states in controllable atomic, molecular, and optical systems, with particular relevance to emerging optical clock platforms compatible with Rydberg interactions. By combining a short-ranged, soft-core potential with an external drive, we can transform naturally emerging Ising interactions into an XX spin model while opening a many-body gap. The gap helps maintain the system within a collective manifold of states where metrologically useful spin squeezing can be generated at a level comparable to the spin squeezing generated in systems with…
We demonstrate spatially resolved, coherent excitation of Rydberg atoms on an atom chip. Electromagnetically induced transparency (EIT) is used to investigate the properties of the Rydberg atoms near the gold coated chip surface. We measure distance dependent shifts (~10 MHz) of the Rydberg energy levels caused by a spatially inhomogeneous electric field. The measured field strength and distance dependence is in agreement with a simple model for the electric field produced by a localized patch of Rb adsorbates deposited on the chip surface during experiments. The EIT resonances remain narrow (…
We discuss laser dressed dipolar and Van der Waals interactions between atoms and polar molecules, so that a cold atomic gas with laser admixed Rydberg levels acts as a designed reservoir for both elastic and inelastic collisional processes. The elastic scattering channel is characterized by large elastic scattering cross sections and repulsive shields to protect from close encounter collisions. In addition, we discuss a dissipative (inelastic) collision where a spontaneously emitted photon carries away (kinetic) energy of the collision partners, thus providing a significant energy loss in a s…
We present a setup with Rydberg atoms for the realization of a bosonic fractional Chern insulator in artificial matter. The suggested setup relies on Rydberg atoms arranged in a honeycomb lattice, where excitations hop through the lattice by dipolar exchange interactions, and can be interpreted as hard-core bosons. The quantum many-body Hamiltonian is studied within exact diagonalization and DMRG. We identify experimentally accessible parameters where all signatures indicate the appearance of a fractional state with the same topological properties as the $ν=1/2$ bosonic Laughlin state. We demo…
