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arXiv 2302.02175cond-mat.mes-hall
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分子纳米探针实验揭示的各向异性弹道输运

Anisotropic Ballistic Transport Revealed by Molecular Nanoprobe Experiments

Markus Leisegang, Robert Schindhelm, Jens Kügel, Matthias Bode

摘要:

原子尺度的电荷输运性质不仅具有重要的基本意义,而且与许多技术应用高度相关。然而,能够在相关的个位数纳米长度尺度上检测电荷传输的实验方法是稀缺的。在这里,我们报告的分子纳米探针(MONA)的实验,在Pd(110),我们利用电荷载流子驱动的开关的一个单一的顺式-2-丁烯分子检测弹道输运性质在几个纳米的长度尺度。我们的数据表明了一个惊人的角度依赖性与下降的电荷输运沿[1-10]取向的原子行和峰值在横向[001]方向。窄角宽度的功能和距离相关的测量表明,纳米尺度的弹道输运性能的金属表面的原子结构的显着影响。

英文摘要:

Atomic-scale charge transport properties are not only of significant fundamental interest but also highly relevant for numerous technical applications. However, experimental methods which are capable of detecting charge transport at the relevant single-digit nanometer length scales are scarce. Here we report on molecular nanoprobe (MONA) experiments on Pd(110) where we utilize the charge carrier-driven switching of a single cis-2-butene molecule to detect ballistic transport properties over length scales of a few nanometers. Our data demonstrate a striking angular dependence with a dip in charge transport along the [1-10]-oriented atomic rows and a peak in the transverse [001] direction. The narrow angular width of both features and distance-dependent measurements suggest that the nanometer-scale ballistic transport properties of metallic surfaces is significantly influenced by the atomic structure.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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