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arXiv 2301.05038cond-mat.mtrl-scicond-mat.mes-hall
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GaAs中Mn受主的交换相互作用:揭示其强烈的形变依赖性

Exchange interaction for Mn acceptor in GaAs: revealing its strong deformation dependence

I. V. Krainov, K. A. Baryshnikov, A. A. Karpova, N. S. Averkiev

AI总结:

本文利用微观多粒子波函数计算了GaAs中锰离子与价带束缚空穴的交换相互作用常数,揭示了其对晶格形变的强烈依赖性,并解释了高温下Mn离子静态磁化率降低的物理机制。

摘要:

本文利用微观多粒子波函数,计算了锰离子内电子d壳层与GaAs价带束缚空穴之间的交换相互作用常数。我们揭示了其对晶格形变的参数依赖性,并发现在应变张量达到$10^{-3} ÷10^{-2}$时,该变化可达甚至超过数十个百分点。这一事实与先前通过拉曼光谱获得的GaAs中Mn受主精细能级结构存在形变依赖性的假设相符,且我们表明该依赖性具有相同的量级。此外,我们解决了GaAs中Mn离子静态磁化率在高温下成熟理论与实验数据存在显著不匹配的问题。通过数值估计和计算,我们表明,GaAs晶格膨胀对交换耦合值的强烈参数依赖性同样决定了高温($50~$K以上)磁化率的降低。

英文摘要:

In this paper we calculate exchange interaction constant between manganese ion inner electronic $d$-shell and GaAs valence band bounded hole using their microscopic multiparticle wave functions. We reveal its parametric dependence on crystal lattice deformations and find out that it could be about and even more than dozens percent when the strain tensor reaches values of $10^{-3} ÷10^{-2}$. This fact is in accordance with the previous hypothesis of deformation dependence of Mn acceptors in GaAs fine energy structure obtained from Raman spectroscopy, and we show that this dependence has the same magnitude. Also, we resolve here the problem of a substantial high temperature mismatch between well-developed theory and experimental data for the static magnetic susceptibility of Mn ions in GaAs. We show by numerical estimates and calculations that quite a strong parametric dependence of the exchange coupling value on GaAs lattice expansion determines the high temperature (above $50~$K) magnetic susceptibility reduction as well.

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