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arXiv 2301.04673cond-mat.str-el
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掺杂应变扭转双层石墨烯中的对称近藤晶格态

Symmetric Kondo Lattice States in Doped Strained Twisted Bilayer Graphene

H. Hu, G. Rai, L. Crippa, J. Herzog-Arbeitman, D. Călugăru, T. Wehling, G. Sangiovanni, R. Valenti, A. M. Tsvelik, B. A. Bernevig

AI总结:

该研究利用THF模型、KL表述、平均场与DMFT计算,揭示扭转双层石墨烯中对称近藤相在整数填充受抑制,而可通过非整数掺杂或C3z破缺应变稳定。

摘要:

我们使用拓扑重费米子(THF)模型及其近藤晶格(KL)表述来研究扭转双层石墨烯中的对称近藤态。通过大N近似,我们在填充数ν=0、±1、±2的KL模式中发现了一个对称近藤(SK)态。在SK态中,所有对称性均得到保留,且局域磁矩被传导电子近藤屏蔽。在ν=0、±1、±2、±3时THF模型的平均场层面,我们也发现了类似的对称态。我们通过比较对称态与有序态的能量来研究对称态的稳定性,发现有序态具有更低的能量。然而,当通过向轻带掺杂空穴而偏离整数填充时,我们发现能量差减小,这表明有序性丧失并出现趋向近藤屏蔽的趋势。为了纳入平均场近似之外的多体效应,我们对THF模型进行了动力学平均场理论(DMFT)计算。我们发现,在ν=0、±1、±2时,自旋磁化率一直到约2 K都遵循居里行为,在该温度下局域磁矩的屏蔽开始显现。这暗示这些填充数下存在非常低的近藤温度,与我们的平均场计算结果一致。在非整数填充ν=±0.5、±0.8、±1.2时,DMFT显示磁化率在高得多的温度下偏离1/T行为,表明掺杂对局域磁矩产生了更有效的屏蔽。最后,我们通过平均场方法研究了破坏C3z旋转对称性的应变效应,发现在ν=0、±1、±2时,足够大的应变可以稳定一个仅破坏C3z对称性的对称相。我们的结果表明,对称近藤相在整数填充时受到强烈抑制,但可以在非整数填充或施加应变时得到稳定。

英文摘要:

We use the topological heavy fermion (THF) model and its Kondo Lattice (KL) formulation to study the symmetric Kondo state in twisted bilayer graphene. Via a large-N approximation, we find a symmetric Kondo (SK) state in KL mode at fillings $ν=0,\pm 1,\pm 2$. In the SK state, all symmetries are preserved and the local moments are Kondo screened by the conduction electrons. At the mean-field level of the THF model at $ν=0,\pm 1, \pm 2, \pm 3$, we also find a similar symmetric state. We study the stability of the symmetric state by comparing its energy with the ordered states and find the ordered states to have lower energy. However, moving away from integer fillings by doping holes to the light bands, we find the energy difference is reduced, which suggests the loss of ordering and a tendency towards Kondo screening. In order to include many-body effects beyond the mean-field approximation, we perform dynamical mean-field theory (DMFT) calculations on the THF model. We find the spin susceptibility follows a Curie behavior at $ν=0, \pm 1,\pm 2$ down to $\sim 2\text{K}$ where the onset of screening of the local moment becomes visible. This hints to very low Kondo temperatures at these fillings, in agreement with the outcome of our mean-field calculations. At non-integer filling $ν=\pm 0.5,\pm 0.8,\pm 1.2$ DMFT shows deviations from a $1/T$-susceptibility at much higher temperatures, suggesting a more effective screening of local moments with doping. Finally, we study the effect of a $C_{3z}$-rotational-symmetry-breaking strain via mean-field approaches and find that a symmetric phase (that only breaks $C_{3z}$ symmetry) can be stabilized at sufficiently large strain at $ν=0,\pm 1, \pm 2$. Our results suggest that a symmetric Kondo phase is strongly suppressed at integer fillings, but could be stabilized either at non-integer fillings or by applying strain.

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