Defect-free atom arrays are an important precursor for quantum information processing and quantum simulation. Yet, large-scale defect-free atom arrays can be challenging to realize, due to the losses encountered when rearranging stochastically loaded atoms to achieve a desired target array. Here, we demonstrate a novel parallel rearrangement algorithm that uses multiple mobile tweezers to independently sort and compress atom arrays in a way that naturally avoids atom collisions. With a high degree of parallelism, our algorithm offers a reduced move complexity compared to both single-tweezer algorithms and existing multi-tweezer algorithms. We further determine the optimal degree of parallelism to be a balance between an algorithmic speedup and multi-tweezer inhomogeneity effects. The defect-free probability for a 225-atom array is demonstrated to be as high as 33(1)% in a room temperature setup after multiple cycles of rearrangement. The algorithm presented here can be implemented for any target array geometry with an underlying periodic structure.
We report on improvements extending the capabilities of the atom-by-atom assembler described in [Barredo et al., Science 354, 1021 (2016)] that we use to create fully-loaded target arrays of more than 100 single atoms in optical tweezers, starting from randomly-loaded, half-filled initial arrays. We describe four variants of the sorting algorithm that (i) allow decrease the number of moves needed for assembly and (ii) enable the assembly of arbitrary, non-regular target arrays. We finally demonstrate experimentally the performance of this enhanced assembler for a variety of target arrays.
We show that with a purely blue-detuned cooling mechanism we can densely load single neutral atoms into large arrays of shallow optical tweezers. With this ability, more efficient assembly of larger ordered arrays will be possible - hence expanding the number of particles available for bottom-up quantum simulation and computation with atoms. Using Lambda-enhanced grey molasses on the D1 line of 87Rb, we achieve loading into a single 0.63 mK trap with 89% probability, and we further extend this loading to 100 atoms at 80% probability. The loading behavior agrees with a model of consecutive ligh…
We demonstrate the coherent creation of a single NaCs molecule in its rotational, vibrational, and electronic (rovibronic) ground state in an optical tweezer. Starting with a weakly bound Feshbach molecule, we locate a two-photon transition via the $|{c^3Σ,v'=26}\rangle$ excited state and drive coherent Rabi oscillations between the Feshbach state and a single hyperfine level of the NaCs rovibronic ground state $|{X^1Σ,v''=0,N''=0}\rangle$ with a binding energy of $D_0 = h \times 147038.30(2)$ GHz. We measure a lifetime of $3.4\pm1.6$ s for the rovibronic ground-state molecule, which possesses…
As a physically motivated and computationally simple model for cold atomic and molecular collisions, the multichannel quantum defect theory (MQDT) with frame transformation (FT) formalism provides an analytical treatment of scattering resonances in an arbitrary partial wave between alkali-metal atoms, leading to the experimental observation of $p-$ and $d-$wave resonances. However, the inconsistency of quantum defects for describing scattering resonances shows up when compared with experiments. Here, with two heteronuclear atoms in the ground state of an optical tweezer, the energy dependence …
We report on the realization of large assembled arrays of more than 300 single $^{87}$Rb atoms trapped in optical tweezers in a cryogenic environment at $\sim4$~K. For arrays with $N_{\rm a}=324$ atoms, the assembly process results in defect-free arrays in $\sim37\%$ of the realizations. To achieve this high assembling efficiency, we equalize the loading probability of the traps within the array using a closed-loop optimization of the power of each optical tweezers, based on the analysis of the fluorescence time-traces of atoms loaded in the traps.
The multichannel Na-Cs interactions are characterized by a series of measurements using two atoms in an optical tweezer, along with a multichannel quantum defect theory (MQDT). The triplet and singlet scattering lengths are measured by performing Raman spectroscopy of the Na-Cs motional states and least-bound molecular state in the tweezer. Magnetic Feshbach resonances are observed for only two atoms at fields which agree well with the MQDT. Our methodology, which promotes the idea of an effective theory of interaction, can be a key step towards the understanding and the description of more co…
Large arrays of individually controlled atoms trapped in optical tweezers are a very promising platform for quantum engineering applications. However, to date, only disordered arrays have been demonstrated, due to the non-deterministic loading of the traps. Here, we demonstrate the preparation of fully loaded, two-dimensional arrays of up to 50 microtraps each containing a single atom, and arranged in arbitrary geometries. Starting from initially larger, half-filled matrices of randomly loaded traps, we obtain user-defined target arrays at unit filling. This is achieved with a real-time contro…
Quantum walks provide a framework for understanding and designing quantum algorithms that is both intuitive and universal. To leverage the computational power of these walks, it is important to be able to programmably modify the graph a walker traverses while maintaining coherence. Here, we do this by combining the fast, programmable control provided by optical tweezer arrays with the scalable, homogeneous environment of an optical lattice. Using this new combination of tools we study continuous-time quantum walks of single atoms on a 2D square lattice, and perform proof-of-principle demonstra…
We demonstrate full quantum state control of two species of single atoms using optical tweezers and assemble the atoms into a molecule. Our demonstration includes 3D ground-state cooling of a single atom (Cs) in an optical tweezer, transport by several microns with minimal heating, and merging with a single Na atom. Subsequently, both atoms occupy the simultaneous motional ground state with 61(4)\% probability. This realizes a sample of exactly two co-trapped atoms near the phase-space-density limit of one, and allows for efficient stimulated-Raman transfer of a pair of atoms into a molecular …
We demonstrate single-atom resolved imaging with a survival probability of $0.99932(8)$ and a fidelity of $0.99991(1)$, enabling us to perform repeated high-fidelity imaging of single atoms in tweezers for thousands of times. We further observe lifetimes under laser cooling of more than seven minutes, an order of magnitude longer than in previous tweezer studies. Experiments are performed with strontium atoms in $813.4~\text{nm}$ tweezer arrays, which is at a magic wavelength for the clock transition. Tuning to this wavelength is enabled by off-magic Sisyphus cooling on the intercombination li…
We demonstrate rapid loading of a small array of optical tweezers with a single $^{87}$Rb atom per site. We find that loading efficiencies of up to 90% per tweezer are achievable in less than 170 ms for traps separated by more than $1.7 \,μ\text{m}$. Interestingly, we find the load efficiency is affected by nearby traps and present the efficiency as a function of the spacing between two optical tweezers. This enhanced loading, combined with subsequent rearranging of filled sites, will enable the study of quantum many-body systems via quantum gas assembly.
D1 magic wavelengths have been predicted for the alkali atoms but are not yet observed to date. We experimentally confirm a D1 magic wavelength that is predicted to lie at 615.87 nm for $^{23}$Na, which we then use to trap and image individual atoms with 80.0(6)% efficiency and without having to modulate the trapping and imaging light intensities. We further demonstrate that the mean loading efficiency remains as high as 74.2(7)% for a 1D array of eight atoms. Leveraging on the absence of trap intensity modulation and lower trap depths afforded by the D1 light, we achieve an order-of-magnitude…
Sorting atoms stochastically loaded in optical tweezer arrays via an auxiliary mobile tweezer is an efficient approach to preparing intermediate-scale defect-free atom arrays in arbitrary geometries. However, high filling fraction of atom-by-atom assemblers is impeded by redundant sorting moves with imperfect atom transport, especially for scaling the system size to larger atom numbers. Here, we propose a new sorting algorithm (heuristic cluster algorithm, HCA) which provides near-fewest moves in our tailored atom assembler scheme and experimentally demonstrate a $5\times6$ defect-free atom ar…
Optically trapped mixed-species single atom arrays with arbitrary geometries are an attractive and promising platform for various applications, because tunable quantum systems with multiple components provide extra degrees of freedom for experimental control. Here, we report the first demonstration of two-dimensional $6\times4$ dual-species atom assembly with a filling fraction of 0.88 (0.89) for $^{85}$Rb ($^{87}$Rb) atoms. This mixed-species atomic synthetic is achieved via rearranging initially randomly distributed atoms using a sorting algorithm (heuristic heteronuclear algorithm) which is…
We present an experimental system for Rydberg tweezer arrays with ytterbium (Yb) atoms featuring internal state manipulation between the ground ${}^1$S$_0$ and the metastable ${}^3$P$_2$ states, and single-photon excitation from the ${}^3$P$_2$ to Rydberg states. In the experiments, single Yb atoms are trapped in two-dimensional arrays of optical tweezers and are detected by fluorescence imaging with the intercombination ${}^1$S$_0 \leftrightarrow {}^3$P$_1$ transition, and the defect-free single atom arrays are prepared by the rearrangement with the feedaback. We successfully perform high-res…
The realization of large-scale fully controllable quantum systems is an exciting frontier in modern physical science. We use atom-by-atom assembly to implement a novel platform for the deterministic preparation of regular arrays of individually controlled cold atoms. In our approach, a measurement and feedback procedure eliminates the entropy associated with probabilistic trap occupation and results in defect-free arrays of over 50 atoms in less than 400 ms. The technique is based on fast, real-time control of 100 optical tweezers, which we use to arrange atoms in desired geometric patterns an…
