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arXiv 2207.04020cond-mat.str-elcond-mat.mtrl-sci
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Cr$_2$Ge$_2$Te$_6$中强单轴压力依赖性证明自旋-晶格耦合与自旋涨落

Strong uniaxial pressure dependencies evidencing spin-lattice coupling and spin fluctuations in Cr$_2$Ge$_2$Te$_6$

S. Spachmann, S. Selter, B. Büchner, S. Aswartham, R. Klingeler

AI总结:

本研究通过高分辨率电容测膨胀法测量Cr$_2$Ge$_2$Te$_6$单晶,发现其相图存在三临界点,且面内压力下磁化强度与相变表现出极强依赖性,证明了自旋-晶格耦合与临界涨落的重要作用。

摘要:

通过高分辨率电容测膨胀法对Cr$_2$Ge$_2$Te$_6$单晶进行研究,获得了2至300 K温度及最高15 T磁场下面内($B\parallel ab$)与面外($B\parallel c$)的热膨胀与磁致伸缩数据。响应函数中的反常现象构建了“磁弹性”相图,并划分出顺磁(PM)、铁磁低温/低场(LTF)与取向铁磁(FM)相。在$B\parallel ab$小场下观察到两个具有不同磁场依赖性的独立热膨胀反常,支持PM与LTF相间存在中间区域的图景,并表明存在三临界点。利用Stoner-Wohlfarth模型模拟单轴各向异性磁致伸缩表明,LTF相中观察到的磁场二次方行为与自旋从优先$c$方向旋转至$ab$面内一致。LTF相及靠近T$_{\rm C}$的PM相均表现出极强的磁化强度压力依赖性${\partial}\ln{M_{\rm ab}}/{\partial}p_{\rm ab}$(达数百%/GPa),且LTF到FM相的转变也强烈依赖于$p_{\rm ab}$(约$-$280%/GPa),表明面内压力下单轴各向异性显著降低。数据明确证明了Cr$_2$Ge$_2$Te$_6$中临界涨落与磁弹性耦合的重要性。

英文摘要:

Single crystals of Cr$_2$Ge$_2$Te$_6$ were studied by high-resolution capacitance dilatometry to obtain in-plane ($B\parallel ab$) and out-of-plane ($B\parallel c$) thermal expansion and magnetostriction at temperatures between 2 and 300 K and in magnetic fields up to 15 T. The anomalies in both response functions lead to the 'magnetoelastic' phase diagrams and separate the paramagnetic (PM), ferromagnetic low-temperature/low-field (LTF) and aligned ferromagnetic (FM) phases. The presence of two distinct thermal expansion anomalies at small fields $B\parallel ab$ of different magnetic field dependence clearly supports the scenario of an intermediate region separating PM and LTF phases and is indicative of a tricritical point. Simulations of the magnetostriction using the Stoner-Wohlfarth model for uniaxial anisotropy demonstrate that the observed quadratic-in-field behavior in the LTF phase is in line with a rotation of the spins from the preferred $c$ direction into the $ab$ plane. Both the LTF and the PM phase close to T$_{\rm C}$ exhibit very strong pressure dependencies of the magnetization, ${\partial}\ln{M_{\rm ab}}/{\partial}p_{\rm ab}$, of several hundred %/GPa and also the transition from the LTF to the FM phase strongly depends on $p_{\rm ab}$ ($\sim -$280%/GPa), indicating a strong decrease of the uniaxial anisotropy under applied in-plane pressure. Our data clearly demonstrate the relevance of critical fluctuations and magnetoelastic coupling in Cr$_2$Ge$_2$Te$_6$.

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