We demonstrate that the electronic structure of a material can be deformed into Floquet pseudo-bands with arbitrarily tailored shapes. We achieve this goal with a novel combination of quantum optimal control theory and Floquet engineering. The power and versatility of this framework is demonstrated here by utilizing the independent-electron tight-binding description of the $π$ electronic system of graphene. We show several prototype examples focusing on the region around the K (Dirac) point of the Brillouin zone: creation of a gap with opposing flat valence and conduction bands, creation of a gap with opposing concave symmetric valence and conduction bands -- which would correspond to a material with an effective negative electron-hole mass --, or closure of the gap when departing from a modified graphene model with a non-zero field-free gap. We employ time periodic drives with several frequency components and polarizations, in contrast to the usual monochromatic fields, and use control theory to find the amplitudes of each component that optimize the shape of the bands as desired. In addition, we use quantum control methods to find realistic switch-on pulses that bring the material into the predefined stationary Floquet band structure, i.e. into a state in which the desired Floquet modes of the target bands are fully occupied, so that they should remain stroboscopically stationary, with long lifetimes, when the weak periodic drives are started. Finally, we note that although we have focused on solid state materials, the technique that we propose could be equally used for the Floquet engineering of ultracold atoms in optical lattices, and to other non-equilibrium dynamical and correlated systems.
We review recent work on low-frequency Floquet engineering and its application to quantum materials driven by light, emphasizing van der Waals systems hosting Moiré superlattices. These non-equilibrium systems combine the twist-angle sensitivity of the band structures with the flexibility of light drives. The frequency, amplitude, and polarization of light can be easily tuned in experimental setups, leading to platforms with on-demand properties. First, we review recent theoretical developments to derive effective Floquet Hamiltonians in different frequency regimes. We apply some of these theo…
Dynamic manipulation of magnetism in topological materials is demonstrated here via a Floquet engineering approach using circularly polarized light. Increasing the strength of the laser field, besides the expected topological phase transition, the magnetically doped topological insulator thin film also undergoes a magnetic phase transition from ferromagnetism to paramagnetism, whose critical behavior strongly depends on the quantum quenching. In sharp contrast to the equilibrium case, the non-equilibrium Curie temperatures vary for different time scale and experimental setup, not all relying o…
Using Floquet theory, we investigate the effect of light on triple fold fermions. We study a low energy model as well as a simplified tight binding model under illumination. We find that the three fold degeneracy remains symmetry protected even after applying light if the original band structure is rotationally symmetric around the degeneracy. Otherwise, light can lift the degeneracy and open up a gap. We further investigate the effect of light on the topological Fermi arcs by means of numerical computations. The changes caused by illumination are reflected in experimentally detectable signatu…
Floquet engineering, modulating quantum systems in a time periodic way, lies at the central part for realizing novel topological dynamical states. Thanks to the Floquet engineering, various new realms on experimentally simulating topological materials have emerged. Conventional Floquet engineering, however, only applies to time periodic non-dissipative Hermitian systems, and for the quantum systems in reality, non-Hermitian process with dissipation usually occurs. So far, it remains unclear how to characterize topological phases of periodically driven non-Hermitian systems via the frequency sp…
Tsinghua University（清华大学）；State Key Laboratory of Low-Dimensional Quantum Physics, Tsinghua University（清华大学低维量子物理国家重点实验室）；Frontier Science Center for Quantum Information（量子信息前沿科学中心）
We present a new scheme to control the spin exchange interactions between two magnetic ions by manipulating the orbital degrees of freedom using a periodic drive. We discuss two different protocols for orbital Floquet engineering. In one case, we modify the properties of the ligand orbitals which mediate magnetic interactions between two transition metal ions. While in the other case, we mix the d orbitals on each magnetic ion. In contrast to previous works on Floquet engineering of magnetic properties, the present scheme makes use of the AC Stark shift of the states involved in the exchange p…
We introduce the concept of Floquet odd-frequency superconducting pairs and establish their emergence in time-periodic conventional superconductors, where the continuous time-translation invariance is broken. We show that these exotic Cooper pairs are possible because the Floquet modes in time-periodic systems provide an additional index (a Floquet index) that broadens the classification of pair symmetries, with no analog in the static regime. Our results thus put forward a different route for odd-frequency superconducting pairs and pave the way for Floquet engineered dynamical superconducting…
In this paper, we theoretically study the Floquet engineering of two dimensional photonic waveguide arrays in three types of lattices: honeycomb lattice with Kekule distortion, breathing square lattice and breathing Kagome lattice. The Kekule distortion factor or the breathing factor in the corresponding lattice is periodically changed along the axial direction of the photonic waveguide with frequency $ω$. Within certain ranges of $ω$, the Floquet corner states in the Floquet band gap of quasi-energy spectrum are found, which are localized at the corner of the finite two-dimensional arrays. Du…
Motivated by the recent experimental realization of twisted double bilayer graphene (TDBG) samples we study, both analytically and numerically, the effects of circularly polarized light propagating in free space and confined into a waveguide on the band structure and topological properties of these systems. These two complementary Floquet protocols allow us to selectively tune different parameters of the system by varying the intensity and the frequency of the light. For the drive protocol in free space, in the high-frequency regime, we find that in TDBG with AB/BA stacking, we can selectively…
Floquet engineering is the concept of tailoring a system by a periodic drive. It has been very successful in opening new classes of Hamiltonians to the study with ultracold atoms in optical lattices, such as artificial gauge fields, topological band structures and density-dependent tunneling. Furthermore, driven systems provide new physics without static counterpart such as anomalous Floquet topological insulators. In this review article, we provide an overview of the exciting developments in the field and discuss the current challenges and perspectives.
We investigate the topological properties of Floquet-engineered twisted bilayer graphene above the magic angle driven by circularly polarized laser pulses. Employing a full Moiré-unit-cell tight-binding Hamiltonian based on first-principles electronic structure we show that the band topology in the bilayer, at twisting angles above 1.05$^\circ$, essentially corresponds to the one of single-layer graphene. However, the ability to open topologically trivial gaps in this system by a bias voltage between the layers enables the full topological phase diagram to be explored, which is not possible in…
Prethermalization, where quasi-steady states are realized in the intermediate long time regime (prethermal regime), in periodically driven (Floquet) systems is an important phenomenon since it provides a platform of nontrivial Floquet many-body physics. In this Letter, we consider Floquet systems with dual energy scales: the Hamiltonian consists of two different terms whose amplitude is either comparable or much smaller than the frequency. As a result, when the larger-amplitude drive induces a $\mathbb{Z}_N$ symmetry operation, we obtain the effective static Hamiltonian respecting a new emerge…
Within the Floquet theory of periodically driven quantum systems, we demonstrate that a high-frequency electromagnetic field can be used as an effective tool to control excitonic properties of semiconductor quantum dots (QDs). It is shown, particularly, that the field both decreases the exciton binding energy and dynamically stabilizes the exciton, increasing its radiative lifetime. The developed theory can serve as a basis for the ultrafast method to tune spectral characteristics of the QD-based photon emitters by a high-frequency field.
Floquet engineering provides a toolbox for the realization of novel quantum phases without static counterparts, while conventionally the realization may rely on the manipulation of complex temporal evolution. Here we propose a systematic and high-precision scheme to realize unconventional Floquet topological phases by engineering local band structures in particular momentum subspace called band inversion surfaces (BISs). This scheme is based on a new bulk-boundary correspondence that for a class of generic $d$-dimensional periodically driven systems, the local topological structure formed in e…
We demonstrate the emergence of a non-equilibrium superradiant phase in the dissipative Rabi-Dicke model. This phase is characterized by a photonic steady state that oscillates with a frequency close to the cavity frequency, in contrast to the constant photonic steady state of the equilibrium superradiant phase in the Dicke model. We relate this superradiant phase to the population inversion of Floquet states by introducing a Schwinger representation of the driven two-level systems in the cavity. This inversion is depleted near Floquet energies that are resonant with the cavity frequency to su…
This work provides a convenient and powerful means towards the engineering of Floquet bands via Bloch oscillations, by adding a tilted linear potential to periodically driven lattice systems. The added linear field not only restricts the spreading of a time-evolving wavepacket but also, depending on the ratio between the Bloch oscillation frequency and the modulation frequency of the periodic driving, dramatically modifies the band profile and topology. Specifically, we consider a driven Aubry-André-Harper model as a working example, in the presence of a linear field. Almost flat Floquet bands…
The coupling of monochromatic light fields and solids introduces nonequilibrium Floquet states, offering opportunities to create and explore new topological phenomena. Using combined first-principles and Floquet analysis we show that one can freely engineer Floquet-Dirac fermions (FDFs) in graphene by tuning the frequency and intensity of linearly polarized light. Not only type-II FDFs are created, but they also coexist with type-I FDFs near the Fermi level. Intriguingly, novel topologically nontrivial edge states connecting type-I and type-II Floquet-Dirac points emerge in photodriven graphen…
In Hermitian topological systems, the bulk-boundary correspondence strictly constraints boundary transport to values determined by the topological properties of the bulk. We demonstrate that this constraint can be lifted in non-Hermitian Floquet insulators. Provided that the insulator supports an anomalous topological phase, non-Hermiticity allows us to modify the boundary states independently of the bulk, without sacrificing their topological nature. We explore the ensuing possibilities for a Floquet topological insulator with non-Hermitian time-reversal symmetry, where the helical transport …
Magnetism and Topology from Circularly Polarized Phonon Floquet Engineering
RIKEN Center for Emergent Matter Science (CEMS)（RIKEN 涌现物质科学中心）；Institute of Theoretical Physics, Chinese Academy of Sciences（中国科学院理论物理研究所）；The Institute for Solid State Physics, The University of Tokyo（东京大学固体物理研究所）；Department of Physics, Institute of Science Tokyo（东京科学大学物理系）
We consider asymmetric and symmetric dimerized two-leg ladders, comprising of four different lattice points per unit cell, illuminated by circularly polarized light. In the asymmetric dimerized ladder case, rungs are not perpendicular to the ladder's legs whereas the rungs are perpendicular to the legs for the symmetric one. Using the Floquet theory, we obtain an effective Hamiltonian to study topological properties of the systems. Depending on the dimerization strength and driving amplitude, it is shown that topologically protected edge states manifest themselves not only as a zero-energy ban…
Floquet engineering is one of the most vigorous fields in periodically driven (Floquet) systems, with which we can control phases of matter usually by high-frequency drives. In this paper, with Floquet engineering by a combination of high-frequency drives and resonant drives, we propose a way to realize nontrivial topological phases protected by a $\mathbb{Z}_2 \times \mathbb{Z}_2$ symmetry only in the presence of a $\mathbb{Z}_2$ symmetry, using a robust emergent $\mathbb{Z}_2$ symmetry induced by the resonant drives. Moreover, the symmetry protected topological (SPT) phases are switchable be…
It is generally believed that non-Hermiticity can transform Weyl semimetals into Weyl-exceptional-ring semimetals. However, this belief is from the systems without skin effect. We investigate the non-Hermitian Weyl semimental and its Floquet engineering in a system with skin effect, which breaks the bulk-boundary correspondence in its Hermitian counterpart. It is found in both the static and periodically driven cases that the skin effect makes this general belief no longer valid. We discover that exotic non-Hermitian topological matters, e.g., a composite phase of Weyl semimetal and topologica…
We discuss Floquet engineering of dissipative molecular systems through periodic driving of an infrared-active vibrational transition, either directly or via a cavity mode. Following a polaron quantum Langevin equations approach, we derive correlation functions and stationary quantities showing strongly modified optical response of the infrared-dressed molecule. The coherent excitation of molecular vibrational modes, in combination with the modulation of electronic degrees of freedom due to vibronic coupling can lead to both enhanced vibronic coherence as well as control over vibrational sideb…
We present an experimental proposal to tune the effective lattice structure in twisted transition metal dichalcogenide (TMD) heterobilayers with time-periodic Floquet drive. We show that elliptically polarized light with sub-terahertz frequencies $\hbarω\sim 1$ meV and moderate electric fields $E\sim0.2$~MV/cm allows tuning between the native triangular lattice and a square lattice, while linearly polarized light enables dimensional reduction to a quasi-one-dimensional geometry. Without drive, these twisted TMDs simulate the single band Fermi-Hubbard model; we show that this approximation stil…
Time-periodic driving in the form of coherent radiation provides powerful tool for the manipulation of topological materials or synthetic quantum matter. In this paper we propose a scheme to realize non-Hermitian semimetals exhibiting exceptional rings in the spectra through Floquet engineering. A transition from a concentric pair of the rings to a dipolar pair is observed. The concentric pair carries only a quantized Berry phase while the dipolar pair possesses opposite Chern numbers in addition, signaling a topological Lifshitz transition of the Fermi surface. The transport properties of the…
The insertion of a local magnetic flux, as the one created by a thin solenoid, plays an important role in gedanken experiments of quantum Hall physics. By combining Floquet engineering of artificial magnetic fields with the ability of single-site addressing in quantum-gas microscopes, we propose a scheme for the realization of such local solenoid-type magnetic fields in optical lattices. We show that it can be employed to manipulate and probe elementary excitations of a topological Chern insulator. This includes quantized adiabatic charge pumping along tailored paths inside the bulk, as well a…
We derive a theory for the generation of arbitrary spin-spin interactions in superconducting circuits via periodic time modulation of the individual qubits or the qubit-qubit interactions. The modulation frequencies in our approach are in the microwave or radio frequency regime so that the required fields can be generated with standard generators. Among others, our approach is suitable for generating spin lattices that exhibit quantum spin liquid behavior such as Kitaev's honeycomb model.
Quantum simulators based on atoms or molecules often have long-range interactions due to dipolar or Coulomb interactions. We present a method based on Floquet engineering to turn a long-range interaction into a short-range one. By modulating a magnetic-field gradient with one or a few frequencies, one reshapes the interaction profile, such that the system behaves as if it only had nearest-neighbor interactions. Our approach works in both one and two dimensions and for both spin-1/2 and spin-1 systems. It does not require individual addressing, and is applicable to all experimental systems with…
Floquet engineering is an important way to manipulate the electronic states of condensed matter physics. Recently, the discovery of the magnetic topological insulator MnBi$_2$Te$_4$ and its family provided a valuable platform to study magnetic topological phenomena, such as, the quantum anomalous Hall effect, the axion insulator state and the topological magnetoelectric effect. In this work, based on the effective model and first-principles calculations in combination with the Floquet theory, we reveal that the circularly polarized light (CPL) induces the sign reversal of the Chern number of o…
Electric polarization is a geometric phenomenon in solids and has a close relationship to the symmetry of the system. Here we propose a mechanism to dynamically induce and manipulate electric polarization by using an external light field. Specifically, we show that application of bicircular lights (BCLs) control the rotational symmetry of the system and can generate electric polarization. To this end, we use Floquet theory to study a system subjected to a two-frequency drive. We derive an effective Hamiltonian with high frequency expansions, for which the electric polarization is computed with…
We analyze, analytically and numerically, a periodically driven Rashba nanowire proximity coupled to an $s$-wave superconductor using bosonization and renormalization group analysis in the regime of strong electron-electron interactions. Due to the repulsive interactions, the superconducting gap is suppressed, whereas the Floquet Zeeman gap is enhanced, resulting in a higher effective value of $g$-factor compared to the non-interacting case. The flow equations for different coupling constants, velocities, and Luttinger-liquid parameters explicitly establish that even for small initial values o…
Within the Floquet theory of periodically driven quantum systems, we developed the theory of light-induced modification of electronic states in semiconductor materials described by the Luttinger Hamiltonian (the electronic term $Γ_8$). Particularly, exact solutions of the Floquet problem are found for the band edge in the cases of linearly and circularly polarized irradiation. It is shown that the irradiation changes electron effective masses near the band edge, induces anisotropy of the electron dispersion and splits the bands. It is demonstrated that the light-induced band splitting strongly…
Exotic topological states of matter such as Floquet topological insulator or Floquet Weyl semimetal can be induced by periodic driving. This work proposes a Floquet semimetal with Floquet-band holonomy. That is, the system is gapless, but as a periodic parameter viewed as quasimomentum of a synthetic dimension completes an adiabatic cycle, each Floquet band as a whole exchanges with other Floquet bands. The dynamical manifestations of such Floquet-band holonomy are studied. Under open boundary conditions, we discover anomalous chiral edge modes localized only at one edge, winding around the en…
Floquet engineering is a convenient strategy to induce nonequilibrium phenomena in molecular and solid-state systems, or to dramatically alter the physicochemical properties of matter, bypassing costly and time-consuming synthetic modifications. In this article, we investigate theoretically some interesting consequences of the fact that an originally achiral molecular system can exhibit nonzero circular dichroism (CD) when it is driven with elliptically polarized light. More specifically, we consider an isotropic ensemble of small cyclic molecular aggregates in solution whose local low-frequen…
Here we present a theoretical investigation of the Floquet spectrum in multiterminal quantum dot Josephson junctions biased with commensurate voltages. We first draw an analogy between the electronic band theory and superconductivity which enlightens the time-periodic dynamics of the Andreev bound states. We then show that the equivalent of the Wannier-Stark ladders observed in semiconducting superlattices via photocurrent measurements, appears as specific peaks in the finite frequency current fluctuations of superconducting multiterminal quantum dots. In order to probe the Floquet-Wannier-Sta…
Hamiltonians which are inaccessible in static systems can be engineered in periodically driven many-body systems, i.e., Floquet many-body systems. We propose to use interacting particles in a one-dimensional (1D) harmonic potential with periodic kicking to investigate two-dimensional (2D) topological and many-body physics. Depending on the driving parameters, the Floquet Hamiltonian of single kicked harmonic oscillator has various lattice structures in phase space. The noncommutative geometry of phase space gives rise to the topology of the system. We investigate the effective interactions of …
It has been shown that long-range {\it p}-wave superconductivity in a Kitaev chain can be engineered via an ac field with a high frequency [Benito et al., Phys. Rev. B 90, 205127 (2014)]. For its experimental realization, however, theoretical understanding of Floquet engineering with a broader range of driving frequencies becomes important. In this work, focusing on the ac-driven tunneling interactions of a Kitaev chain, we investigate effects from the leading correction to the high-frequency limit on the emergent {\it p}-wave superconductivity. Importantly, we find new engineered long-range {…
We propose to Floquet-engineer Dirac cones at the surface of a three-dimensional topological insulator. We show that a large tunability of the Fermi velocity can be achieved as a function of the polarization, direction and amplitude of the driving field. Using this external control, the Dirac cones in the quasienergy spectrum may become elliptic or massive, in accordance to experimental evidences. These results help us to understand the interplay of surface states and external ac driving fields in topological insulators. In our work we use the full Hamiltonian for the three-dimensional system …
