In liquid argon TPCs for dark matter search and neutrino detection experiments, primary scintillation light is used as a prompt signal of particle scattering, being intensively produced in the vacuum ultraviolet (VUV) due to excimer emission mechanism. On the other hand, there were indications on the production of visible-light emission in liquid argon, albeit at a much lower intensity, the origin of which is still not clear. The closely related issue is visible-light emission in liquid argon doped with methane, the interest in which is due to the possible use in neutron veto detectors for those experiments. In this work we study in detail the properties of such light emission in pure liquid argon and its mixtures with methane. In particular, the absolute photon yield of visible-light emission in pure liquid argon was measured to be about 200 and 90 photon/MeV for X-rays and alpha particles respectively. In liquid argon doped with methane the photon yield dropped down significantly, by about an order of magnitude at a methane molar content varying from 0.01 to 1%, and then almost did not change when further increasing the methane content up to 10%.
Neutron veto detector based on liquid scintillator containing hydrogen atoms is an integral part of any underground experiment for dark matter search. So far, a flammable mixture of liquid hydrocarbons was used as a liquid scintillator in such detectors. A safe alternative might be a liquid scintillator based on liquid argon doped with methane. In this work, we have studied the primary scintillations in pure liquid argon and its mixtures with methane, the CH4 content varying from 100 ppm to 5%. The primary scintillations have for the first time been observed in liquid argon doped with methane,…
In this paper we report on measurements of the effects of dissolved methane upon argon scintillation light. We monitor the light yield from an alpha source held 20 cm from a cryogenic photomultiplier tube (PMT) assembly as methane is injected into a high-purity liquid argon volume. We observe significant suppression of the scintillation light yield by dissolved methane at the 10 part per billion (ppb) level. By examining the late scintillation light time constant, we determine that this loss is caused by an absorption process and also see some evidence of methane-induced scintillation quenchin…
Xenon-doped liquid argon has been proposed as a good alternative to pure liquid argon in scintillation detectors. In this study, we report on the measurement of the time profile of scintillation light emitted from xenon-doped liquid argon with molar concentrations up to 1600 ppm. A compact setup has been developed for this study, with silicon photomultiplier (SiPM) as the photosensor and $^{210}\mathrm{Po}$ and $^{90}\mathrm{Sr}$ as scintillation sources. An effective model based on the de-excitation processes has been developed to describe the data. The results show that xenon-doped liquid ar…
Liquid argon (LAr) is a common choice as detection medium in particle physics and rare-event searches. Challenges of LAr scintillation light detection include its short emission wavelength, long scintillation time and short attenuation length. The addition of small amounts of xenon to LAr is known to improve the scintillation and optical properties. We present a characterization campaign on xenon-doped liquid argon (XeDLAr) with target xenon concentrations ranging from 0 to 300 ppm by mass encompassing the measurement of the photoelectron yield $Y$ , effective triplet lifetime $τ_3$ and effect…
We have measured the properties of scintillation light in liquid argon doped with xenon concentrations from 165 ppm to 10,010 ppm using a $^{22}$Na source. The energy transfer processes in the xenon-doped liquid argon are discussed in detail, and a new waveform model is established and used to fit the average waveform. The time profile of the scintillation photon in the xenon-doped liquid argon and of the TPB emission are presented. The quantities of xenon-doped are controlled by a Mass Flow Controller which is calibrated via a Redusial Gas Analyzer to ensure that the xenon concentration is ac…
Measuring the scintillation light in noble gases is an important detection technique in particle physics. Numerous rare event searches like neutrino beam experiments, neutrino-less double beta-decay, and dark matter searches use argon-based detectors. In liquid argon, the light yield can be enhanced by the addition of a small quantity of xenon, where $\sim 10 - 1000$ ppm are added. The general enhancement mechanism and its pathway via an energy transfer between argon and xenon excimers is well known, however the importance of absorption of argon excimer emission by atomic xenon has not been fu…
Results of transmission experiments of vacuum ultraviolet light through a 11.6 cm long cell filled with pure and xenon-doped liquid argon are described. Pure liquid argon shows no attenuation down to the experimental short-wavelength cut-off at 118nm. Based on a conservative approach, a lower limit of 1.10 m for the attenuation length of its own scintillation light could be derived. Adding xenon to liquid argon at concentrations on the order of parts per million leads to strong xenon-related absorption features which are used for a tentative assignment of the recently found near-infrared emiss…
We present a comprehensive analysis of photon emission and atomic collision processes in two-phase argon doped with xenon and nitrogen. The dopants are aimed to convert the VUV emission of pure Ar to the UV emission of the Xe dopant in the liquid phase and to the near UV emission of the N2 dopant in the gas phase. Such a mixture is relevant to two-phase dark matter and low energy neutrino detectors, with enhanced photon collection efficiency for primary and secondary scintillation signals. Based on this analysis, we show that the recently proposed hypothesis of the enhancement of the excitatio…
Gas Electroluminescence in a Dual Phase Xenon-Doped Argon Detector
Lawrence Livermore National Laboratory（劳伦斯利弗莫尔国家实验室）；University of California Davis（加州大学戴维斯分校）；University of California San Diego（加州大学圣地亚哥分校）；University of California Riverside（加州大学河滨分校）
The use of xenon-doped liquid argon is a promising alternative for large pure liquid-argon TPCs. Not only xenon-doped liquid argon enhances the light production, mitigating the possible suppression due to impurities, but also it increases the wavelength of the scintillation light, enlarging the effective Rayleigh scattering length and improving the detection uniformity. ProtoDUNE Dual-Phase is a 300-ton active volume LAr TPC, a prototype for the Deep Underground Neutrino Experiment (DUNE), a dual-site experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon …
A two-phase Cryogenic Avalanche Detector (CRAD) with electroluminescence (EL) gap, operated in argon doped with a minor (49$\pm$7 ppm) admixture of nitrogen, has been studied. The EL gap was optically read out using cryogenic PMTs located on the perimeter of the gap. We present the results of the measurements of the N$_2$ content, detector sensitivity to X-ray-induced signals, EL gap yield and electron lifetime in the liquid. The detector sensitivity, at a drift field in liquid Ar of 0.6 kV/cm, was measured to be 9 and 16 photoelectrons recorded at the PMTs per keV of deposited energy at 23 an…
We present the first direct experimental confirmation of the fast component re-emission in liquid argon (LAr) doped with xenon (Xe). This effect was studied at various Xe concentrations up to $\sim$3000 ppm. The rate constant of energy transfer for the fast component was quantified. It was shown that LAr doped with a high concentration of Xe without TPB has a better PSD efficiency than pure LAr or Xe-doped LAr with TPB. The stability of LAr+Xe mixture was tested for the first time at high Xe concentration for long continuous runtimes.
Liquid argon detectors are employed in a wide variety of nuclear and particle physics experiments. The addition of small quantities of xenon to argon modifies its scintillation, ionization, and electroluminescence properties and can improve its performance as a detection medium. However, a liquid argon-xenon mixture can develop instabilities, especially in systems that require phase transitions or that utilize high xenon concentrations. In this work, we discuss the causes for such instabilities and describe a small (liter-scale) apparatus with a unique cryogenic circuit specifically designed t…
The Deep Underground Neutrino Experiment (DUNE) is a leading-edge experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon decay searches. ProtoDUNE-Dual Phase (DP) is a 6x6x6 m$^3$ liquid argon time-projection-chamber (LArTPC) operated at the CERN Neutrino Platform in 2019-2020 as a prototype of the DUNE Far Detector. In ProtoDUNE-DP, the scintillation and electroluminescence light produced by cosmic muons in the LArTPC is collected by photomultiplier tubes placed up to 7 m away from the ionizing track. In this paper, we present the performance of the Proto…
In this paper we report on the evidence for ionization track signals from cosmic ray muons and Compton electrons in a Time Projection Chamber (TPC) filled with liquid Argon and doped with different fractions of Nitrogen. This study has been conducted in view of the possible use of liquid Argon/Nitrogen TPCs for the detection of gamma rays in the resonant band of the Nitrogen absorbtion spectrum, a promising technology for security and medical applications.
Vacuum ultraviolet light emission from xenon-doped liquid argon is described in the context of liquid noble gas particle detectors. Xenon concentrations in liquid argon from 0.1 ppm to 1000 ppm were studied. The energy transfer from the second excimer continuum of argon ($\sim$127 nm) to the second excimer continuum of xenon ($\sim$174 nm) is observed by recording optical emission spectra. The transfer almost saturates at a xenon concentration of $\sim$10 ppm for which, in addition, an intense emission in the infrared at a peak wavelength of 1.17 $μ$m with (13000$\pm$4000) photons per MeV depo…
Liquid argon is being employed as a detector medium in neutrino physics and Dark Matter searches. A recent push to expand the applications of scintillation light in Liquid Argon Time Projection Chamber neutrino detectors has necessitated the development of advanced methods of simulating this light. The presently available methods tend to be prohibitively slow or imprecise due to the combination of detector size and the amount of energy deposited by neutrino beam interactions. In this work we present a semi-analytical model to predict the quantity of argon scintillation light observed by a ligh…
Liquid argon is used as active medium in a variety of neutrino and Dark Matter experiments thanks to its excellent properties of charge yield and transport and as a scintillator. Liquid argon scintillation photons are emitted in a narrow band of 10~nm centered around 127 nm and with a characteristic time profile made by two components originated by the decay of the lowest lying singlet and triplet state of the excimer Ar$_2^*$ to the dissociative ground state. A model is proposed which takes into account the quenching of the long lived triplet states through the self-interaction with other tri…
We describe a technique, applicable to liquid-argon-based dark matter detectors, allowing for discrimination of alpha-decays in detector regions with incomplete light collection from nuclear-recoil-like events. Nuclear recoils and alpha events preferentially excite the liquid argon (LAr) singlet state, which has a decay time of ~6 ns. The wavelength-shifter TPB, which is typically applied to the inside of the active detector volume to make the LAr scintillation photons visible, has a short re-emission time that preserves the LAr scintillation timing. We developed a wavelength-shifting polymeri…
Proportional electroluminescence (EL) in gaseous Ar has for the first time been systematically studied in the two-phase mode, at 87 K and 1.00 atm. Liquid argon had a minor (56 ppm) admixture of nitrogen, which allowed to understand, inter alia, the effect of N2 doping on the EL mechanism in rare-event experiments using two-phase Ar detectors. The measurements were performed in a two-phase Cryogenic Avalanche Detector (CRAD) with EL gap located directly above the liquid-gas interface. The EL gap was optically read out in the Vacuum Ultraviolet (VUV), near 128 nm (Ar excimer emission), and in t…
In liquid argon-based particle detectors, slow wavelength shifters (WLSs) could be used alongside the common, nanosecond scale, WLS tetraphenyl butadiene (TPB) for background mitigation purposes. At room temperature, pyrene has a moderate fluorescence light yield (LY) and a time constant of the order of hundreds of nanoseconds. In this work, four pyrene-doped polystyrene films with various purities and concentrations were characterized in terms of LY and decay time constants in a range of temperature between 4 K and 300 K under ultraviolet excitation. These films were found to have a LY betwee…
DUNE is a dual-site experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon decay searches. ProtoDUNE Dual Phase (DP) is a 6x6x6m3 liquid argon time-projection-chamber (LArTPC) that recorded cosmic-muon data at the CERN Neutrino Platform in 2019-2020 as a prototype of the DUNE Far Detector. Charged particles propagating through the LArTPC produce ionization and scintillation light. The scintillation light signal in these detectors can provide the trigger for non-beam events. In addition, it adds precise timing capabilities and improves the calorimetry measu…
