We experimentally and theoretically demonstrate that nonlinear spin-wave interactions suppress the hybrid magnon-photon quasiparticle or "magnon polariton" in microwave spectra of an yttrium iron garnet film detected by an on-chip split-ring resonator. We observe a strong coupling between the Kittel and microwave cavity modes in terms of an avoided crossing as a function of magnetic fields at low microwave input powers, but a complete closing of the gap at high powers. The experimental results are well explained by a theoretical model including the three-magnon decay of the Kittel magnon into spin waves. The gap closure originates from the saturation of the ferromagnetic resonance above the Suhl instability threshold by a coherent back reaction from the spin waves.
Cavity spintronics explores light matter interactions at the interface between spintronic and quantum phenomena. Until now, studies have focused on the hybridization between ferromagnets and cavity photons.In this article, we realize antiferromagnetic cavity-magnon polaritons. The collective spin motion in single hematite crystals (α-Fe2O3) hybridizes with 18 - 45 GHz microwave cavity photons with required specific symmetries. We show theoretically and experimentally that the photon-magnon coupling in the collinear phase is mediated by the dynamical Neel vector and the weak magnetic moment in …
We formulate a scattering theory to study magnetic films in microwave cavities beyond the independent-spin and rotating wave approximations of the Tavis-Cummings model. We demonstrate that strong coupling can be realized not only for the ferromagnetic resonance (FMR) mode, but also for spin wave resonances (SWRs); the coupling strengths are mode dependent and decrease with increasing mode index. The strong coupling regime can be also accessed electrically by spin pumping into a metal contact.
Strong coupling in cavity-magnon systems has shown great potential for use in spintronics and information processing technologies due to the low damping rates and long coherence times. Although such systems are conceptually similar to those coupled by magnon-polaritons (MPs), the link between magnon-cavity coupling and MPs has not been explicitly defined. In this work we establish such a connection by studying the frequency-wavevector dispersion of a strongly coupled magnon-cavity system, using a height-adjustable microwave cavity, and by modelling the observed behaviour through the system's e…
We propose thermal induced generation of monochromatic microwave radiation in magnon-polariton. Mechanism of thermal to microwave energy transformation is based on intrinsic energy loss compensation of coupled magnon and microwave cavity oscillators by thermal induced "negative damping". A singularity at an exceptional point is achieved when at the critical value of "negative damping" the damping of the system is fully compensated. At the exceptional point, the input energy is equally distributed between the magnon and photon subsystems of the magnon-polariton. The efficiency of transformation…
We consider a hybrid structure formed by graphene and an insulating antiferromagnet, separated by a dielectric of thickness up to $d\simeq 500 \,nm$. When uncoupled, both graphene and the antiferromagnetic surface host their own polariton modes coupling the electromagnetic field with plasmons in the case of graphene, and with magnons in the case of the antiferromagnet. We show that the hybrid structure can host two new types of hybrid polariton modes. First, a surface magnon-plasmon polariton whose dispersion is radically changed by the carrier density of the graphene layer, including a change…
Magnon-polaritons are hybrid light-matter quasiparticles originating from the strong coupling between magnons and photons. They have emerged as a potential candidate for implementing quantum transducers and memories. Owing to the dampings of both photons and magnons, the polaritons have limited lifetimes. However, stationary magnon-polariton states can be reached by a dynamical balance between pumping and losses, so the intrinsical nonequilibrium system may be described by a non-Hermitian Hamiltonian. Here we design a tunable cavity quantum electrodynamics system with a small ferromagnetic sph…
We predict magnon polariton states circulating unidirectionally in a microwave cavity when loaded by a number of magnets on special lines. Realistic finite-element numerical simulations, including dielectric, time-dependent and non-linear effects, confirm the validity of the approximations of a fully analytical input-output model. We find that a phased antenna array can focus all power into a coherent microwave beam with controlled direction and an intensity that scales with the number of magnets.
The Rabi oscillations of a coupled spin-photon system are experimentally studied using time domain microwave transmission measurements. An external magnetic bias field is applied to control the amplitude and frequency of Rabi oscillations, which are a measure of the coherent spin-photon energy exchange and coupling strength respectively. The amplitude and frequency control is described in the time domain as the transient response of a two-level spin-photon system. This approach reveals the link between steady state and transient behaviour of the cavity-magnon-polariton, which is necessary to i…
Exceptional points (EPs) are singularities of energy levels in non-Hermitian systems. In this Letter, we demonstrate the surface of EPs on a magnon polariton platform composed of coupled magnons and microwave photons. Our experiments show that EPs form a three-dimensional exceptional surface (ES) when the system is tuned in a four-dimensional synthetic space. We demonstrated that there exists an exceptional saddle point (ESP) in the ES which originates from the unique couplings between magnons and microwave photons. Such an ESP exhibits unique anisotropic behaviors in both the real and imagina…
We have theoretically and experimentally investigated the dispersion of the cavity-magnon-polariton (CMP) in a 1D configuration, created by inserting a low damping magnetic insulator into a high-quality 1D microwave cavity. By simplifying the full-wave simulation based on the transfer matrix approach in the long wavelength limit, an analytic approximation of the CMP dispersion has been obtained. The resultant coupling strength of the CMP shows different dependence on the sample thickness as well as the permittivity of the sample, determined by the parity of the cavity modes. These scaling effe…
By connecting light to magnetism, cavity-magnon-polaritons (CMPs) can build links from quantum computation to spintronics. As a consequence, CMP-based information processing devices have thrived over the last five years, but almost exclusively been investigated with single-tone spectroscopy. However, universal computing applications will require a dynamic control of the CMP on demand and within nanoseconds. In this work, we perform fast manipulations of the different CMP modes with independent but coherent pulses to the cavity and magnon system. We change the state of the CMP from the energy e…
The dynamics of arbitrary-order quantum correlations in a cavity magnon-polariton system are investigated based on the quantum master equation in the coherent state representation. The phenomena of Rabi-like oscillation and level repulsion of the average cavity-photon number agree remarkably well with existing experimental observations. The competing nature of coherent and incoherent components in these two cases is further revealed by the second-order quantum coherence of the cavity photons and magnons, which can be systematically tuned by the driving microwave and thermal bath. Our results d…
We report the first observation of the magnon-polariton bistability in a cavity magnonics system consisting of cavity photons strongly interacting with the magnons in a small yttrium iron garnet (YIG) sphere. The bistable behaviors are emerged as sharp frequency switchings of the cavity magnon-polaritons (CMPs) and related to the transition between states with large and small number of polaritons. In our experiment, we align, respectively, the [100] and [110] crystallographic axes of the YIG sphere parallel to the static magnetic field and find very different bistable behaviors (e.g., clockwis…
Strong coupling between magnon and electromagnetic wave can lead to the formation of a coupled spinphoton quasiparticle named as magnon-polariton. The phenomenon is well studied for ferromagnetic systems inside microwave cavities in recent years. However, formation of magnon-polariton is rarely seen for an antiferromagnet (AFM) because the strong coupling condition is not easily fulfilled. Here we present time-domain terahertz measurement on a multiferroic polar antiferromagnet Fe2Mo3O8. We find clearly beating between two modes at frequencies above and below the electric-active magnon frequen…
Tripartite Phonon-Magnon-Plasmon Coupling, Parametric Amplification, and Formation of a Phonon-Magnon-Plasmon Polariton in a Two-Dimensional Periodic Array of Magnetostrictive/Plasmonic Bilayered Nanodots
Cavity-magnon polaritons (CMPs) are the associated quasiparticles of the hybridization between cavity photons and magnons in a magnetic sample placed in a microwave resonator. In the strong coupling regime, where the macroscopic coupling strength exceeds the individual dissipation, there is a coherent exchange of information. This renders CMPs as promising candidates for future applications such as in information processing. Recent advances on the study of the CMP now allow not only for creation of CMPs on demand, but also for tuning of the coupling strength - this can be thought of as enhanci…
Depending on the relative rates of coupling and dissipation, a light-matter coupled system is either in the weak- or strong-coupling regime. Here, we present a unique system where the coupling rate continuously increases with an externally applied magnetic field while the dissipation rate remains constant, allowing us to monitor a weak-to-strong coupling transition as a function of magnetic field. We observed a Rabi splitting of a terahertz magnon mode in yttrium orthoferrite above a threshold magnetic field of ~14 T. Based on a microscopic theoretical model, we show that with increasing magne…
For dipole-carrying excitations observed in a high-quality resonator, strong-coupling modes can appear as composite bosons with the spontaneous formation of quantized vortices in the condensed phase of a polariton fluid. In exciton-polaritons, in particular, it leads to sustained trapping of the emitted photon. In this paper, we show that magnon-polaritons can be realized due to magnon condensation caused by magnetic dipole-dipole interaction. In a quasi-2D ferrite disk placed in a microwave cavity, one observes quantum confinement effects of magnetic-dipolar-mode (MDM) oscillations. These mod…
Achieving magnetometers with ultrahigh sensitivity at room temperature is an outstanding problem in physical sciences and engineering. Recently developed non-Hermitian cavity spintronics offers new possibilities. In this work we predict an exceptional magnetic sensitivity of cavity magnon polaritons with the peculiar parity-time (PT) symmetry. Based on the input-output formalism, we demonstrate a "Z"-shape spectrum including two sideband modes and a dark-state branch with an ultranarrow linewidth in the exact PT phase. The spectrum evolves to a step function when the polariton touches the thir…
Polaritons in metals, semimetals, semiconductors, and polar insulators, with their extreme confinement of electromagnetic energy, provide many promising opportunities for enhancing typically weak light-matter interactions such as multipolar radiation, multiphoton spontaneous emission, Raman scattering, and material nonlinearities. These highly confined polaritons are quasi-electrostatic in nature, with most of their energy residing in the electric field. As a result, these "electric" polaritons are far from optimized for enhancing emission of a magnetic nature, such as spin relaxation, which i…
Cavity based sensing of antiferromagnetic canting and nonzero-momentum spin waves in a van der Waals cavity-magnon-polariton system
University of Illinois Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校）；Tata Institute of Fundamental Research（塔塔基础研究所）；Institute of Science and Technology Austria（奥地利科学技术研究所）；Indian Institute of Technology Palakkad（印度理工学院帕拉卡德分校）
Hybridized magnonic-photonic systems are key components for future information processing technologies such as storage, manipulation or conversion of data both in the classical (mostly at room temperature) and quantum (cryogenic) regime. In this work, we investigate a YIG sphere coupled strongly to a microwave cavity over the full temperature range from $290\,\mathrm{K}$ down to $30\,\mathrm{mK}$. The cavity-magnon polaritons are studied from the classical to the quantum regime where the thermal energy is less than one resonant microwave quanta, i.e. at temperatures below $1\,\mathrm{K}$. We c…
The full coherent control of hybridized systems such as strongly coupled cavity photon-magnon states is a crucial step to enable future information processing technologies. Thus, it is particularly interesting to engineer deliberate control mechanisms such as the full control of the coupling strength as a measure for coherent information exchange. In this work, we employ cavity resonator spectroscopy to demonstrate the complete control of the coupling strength of hybridized cavity photon-magnon states. For this, we use two driving microwave inputs which can be tuned at will. Here, only the fir…
Cavity control of quantum matter may offer new ways to study and manipulate many-body systems. A particularly appealing idea is to use cavities to enhance superconductivity, especially in unconventional or high-$T_c$ systems. Motivated by this, we propose a scheme for coupling Terahertz resonators to the antiferromagnetic fluctuations in a cuprate parent compound, which are believed to provide the glue for Cooper pairs in the superconducting phase. First, we derive the interaction between magnon excitations of the Neél-order and polar phonons associated with the planar oxygens. This mode also …
On-chip Dicke-type magnon polaritons in the ultrastrong coupling regime via spatially separated nanomagnets
Kyoto University（京都大学）；Center for Spintronics Research Network, Institute for Chemical Research, Kyoto University（京都大学化学研究所在旋电子学研究网络中心）；Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften（巴伐利亚科学院瓦尔特-迈斯纳研究所）；Technical University of Munich, TUM School of Natural Sciences, Physics Department（慕尼黑工业大学自然科学学院物理系）；Osaka Metropolitan University（大阪公立大学）；Munich Center for Quantum Science and Technology (MCQST)（慕尼黑量子科学与技术中心）
We report on the impact of nonlinear four-magnon scattering on magnon transport in microstructured Co25Fe75 waveguides with low magnetic damping. We determine the magnon propagation length with microfocused Brillouin light scattering over a broad range of excitation powers and detect a decrease of the attenuation length at high powers. This is consistent with the onset of nonlinear four-magnon scattering. Hence, it is critical to stay in the linear regime, when deriving damping parameters from the magnon propagation length. Otherwise, the intrinsic nonlinearity of magnetization dynamics may le…
Strong optical nonlinearities play a central role in realizing quantum photonic technologies. In solid state systems, exciton-polaritons, which result from the hybridization of material excitations and cavity photons, are an attractive candidate to realize such nonlinearities. Here, the interaction between excitons forms the basis of the polaritonic nonlinearity. While the interaction between ground state excitons generates a notable optical nonlinearity, the strength of such ground state interactions is generally not sufficient to reach the regime of quantum nonlinear optics and strong single…
When a magnon passes through two-dimensional magnetic textures, it will experience a fictitious magnetic field originating from the $3\times 3$ skew-symmetric gauge fields. To date, only one of the three independent components of the gauge fields has been found to play a role in generating the fictitious magnetic field while the rest two are perfectly hidden. In this work, we show that they are concealed in the nonlinear magnon transport in magnetic textures. Without loss of generality, we theoretically study the nonlinear magnon-skyrmion interaction in antiferromagnets. By analyzing the scatt…
Soft-X-ray momentum microscopy of nonlinear magnon interactions below 100-nm wavelength
Max-Born-Institut für Nichtlineare Optik & Kurzzeitspektroskopie（马克斯·玻恩非线性光学与超快光谱学研究所）；Helmholtz-Zentrum Berlin für Materialien & Energie GmbH（柏林亥姆霍兹材料与能源中心）；Dipartimento di Ingegneria Elettrica, Università di Napoli ”Federico II”（那不勒斯费德里科二世大学电气工程系）；Laboratory of Nanoscale Magnetic Materials & Magnonics, Institute of Materials (IMX), École Polytechnique Fédérale（洛桑联邦理工学院材料研究所纳米磁性材料与磁振学实验室）
In this Letter, we study the spin Nernst effect (SNE) of magnons in the nonlinear response regime. We derive the formula for the nonlinear magnon spin Nernst current by solving the Boltzmann equation and find out that it is described by an extended Berry curvature dipole of magnons. The nonlinear magnon SNE is expected to occur in various Néel antiferromagnets without Dzyaloshinskii-Moriya interaction. In particular, the nonlinear spin Nernst current in the honeycomb and diamond lattice antiferromagnets can be controlled by strain/pressure.
