Imaging Chern mosaic and Berry-curvature magnetism in magic-angle graphene
Sameer Grover, Matan Bocarsly, Aviram Uri, Petr Stepanov, Giorgio Di Battista, Indranil Roy, Jiewen Xiao, Alexander Y. Meltzer, Yuri Myasoedov, Keshav Pareek, K… 展开作者
Sameer Grover, Matan Bocarsly, Aviram Uri, Petr Stepanov, Giorgio Di Battista, Indranil Roy, Jiewen Xiao, Alexander Y. Meltzer, Yuri Myasoedov, Keshav Pareek, Kenji Watanabe, Takashi Taniguchi, Binghai Yan, Ady Stern, Erez Berg, Dmitri K. Efetov, Eli Zeldov
备注：
29 pages, 5 main text figures and 8 supplementary figures
Charge carriers in magic angle graphene come in eight flavors described by a combination of their spin, valley, and sublattice polarizations. When the inversion and time reversal symmetries are broken by the substrate or by strong interactions, the degeneracy of the flavors can be lifted and their corresponding bands can be filled sequentially. Due to their non-trivial band topology and Berry curvature, each of the bands is classified by a topological Chern number, leading to the quantum anomalous Hall and Chern insulator states at integer fillings $ν$ of the bands. It has been recently predicted, however, that depending on the local atomic-scale arrangements of the graphene and the encapsulating hBN lattices, rather than being a global topological invariant, the Chern number C may become position dependent, altering transport and magnetic properties of the itinerant electrons. Using a SQUID-on-tip, we directly image the nanoscale Berry-curvature-induced equilibrium orbital magnetism, the polarity of which is governed by the local Chern number, and detect its two constituent components associated with the drift and the self-rotation of the electronic wave packets. At $ν=1$, we observe local zero-field valley-polarized Chern insulators forming a mosaic of microscopic patches of C=-1, 0, or 1, governed by the local sublattice polarization, consistent with predictions. Upon further filling, we find a first-order phase transition due to recondensation of electrons from valley K to K', which leads to irreversible flips of the local Chern number and the magnetization, and to the formation of valley domain walls giving rise to hysteretic global anomalous Hall resistance. The findings shed new light on the structure and dynamics of topological phases and call for exploration of the controllable formation of flavor domain walls and their utilization in twistronic devices.
The long wavelength moiré superlattices in twisted 2D structures have emerged as a highly tunable platform for strongly correlated electron physics. We study the moiré bands in twisted transition metal dichalcogenide homobilayers, focusing on WSe$_2$, at small twist angles using a combination of first principles density functional theory, continuum modeling, and Hartree-Fock approximation. We reveal the rich physics at small twist angles $θ<4^\circ$, and identify a particular magic angle at which the top valence moiré band achieves almost perfect flatness. In the vicinity of this magic angle, …
We present a systematic study of the low-energy collective modes for different insulating states at integer fillings in twisted bilayer graphene. In particular, we provide a simple counting rule for the total number of soft modes, and analyze their energies and symmetry quantum numbers in detail. To study the soft mode spectra, we employ time dependent Hartree-Fock whose results are reproduced analytically via an effective sigma model description. We find two different types of low-energy modes - (i) approximate Goldstone modes associated with breaking an enlarged U(4)$\times$U(4) symmetry and…
We show that in a layered metal, the angle dependent, finite frequency, interlayer magnetoresistance is altered due to the presence of a non-zero Berry curvature at the Fermi surface. At zero frequency, we find a conservation law which demands that the `magic angle' condition for interlayer magnetoresistance extrema as a function of magnetic field tilt angle is essentially both field and Berry curvature independent. In the finite frequency case, however, we find that surprisingly large signatures of a finite Berry curvature occur in the periodic orbit resonances. We outline a method whereby th…
Quantized Transport through a Supermoiré Chern Mosaic
Massachusetts Institute of Technology（麻省理工学院）；Stanford University（斯坦福大学）；SLAC National Accelerator Laboratory（SLAC国家加速器实验室）；National Institute for Materials Science（物质材料研究机构）；University of Texas at Dallas（德克萨斯大学达拉斯分校）
Fractional Chern insulators (FCIs) are lattice analogues of fractional quantum Hall states that may provide a new avenue toward manipulating non-abelian excitations. Early theoretical studies have predicted their existence in systems with energetically flat Chern bands and highlighted the critical role of a particular quantum band geometry. Thus far, however, FCI states have only been observed in Bernal-stacked bilayer graphene aligned with hexagonal boron nitride (BLG/hBN), in which a very large magnetic field is responsible for the existence of the Chern bands, precluding the realization of …
We consider a family of twisted graphene multilayers consisting of $n$-untwisted chirally stacked layers, e.g., AB, ABC, etc, with a single twist on top of $m$-untwisted {chirally stacked} layers. Upon neglecting both trigonal warping terms for the untwisted layers and the same sublattice hopping between all layers, the resulting models generalize several remarkable features of the chiral model of twisted bilayer graphene (CTBG). In particular, they exhibit a set of magic angles which are identical to those of CTBG at which a pair of bands (i) are perfectly flat, (ii) have Chern numbers in the…
We uncover topological features of neutral particle-hole pair excitations of correlated quantum anomalous Hall (QAH) insulators whose approximately flat conduction and valence bands have equal and opposite non-zero Chern number. Using an exactly solvable model we show that the underlying band topology affects both the center-of-mass and relative motion of particle-hole bound states. This leads to the formation of topological exciton bands whose features are robust to nonuniformity of both the dispersion and the Berry curvature. We apply these ideas to recently-reported broken-symmetry spontane…
We propose that the electronic structure of twisted bilayer graphene (TBG) can be understood as Dirac fermions coupled with opposite pseudo magnetic fields generated by the moiré pattern. The two low-energy flat bands from each monolayer valley originate from the two zeroth pseudo Landau levels of Dirac fermions under such opposite effective magnetic fields, which have opposite sublattice polarizations and carry opposite Chern numbers $\pm1$, giving rise to helical edge states in the gaps below and above the low-energy bulk bands near the first magic angle. We argue that small Coulomb interact…
We investigate the topological properties of Floquet-engineered twisted bilayer graphene above the magic angle driven by circularly polarized laser pulses. Employing a full Moiré-unit-cell tight-binding Hamiltonian based on first-principles electronic structure we show that the band topology in the bilayer, at twisting angles above 1.05$^\circ$, essentially corresponds to the one of single-layer graphene. However, the ability to open topologically trivial gaps in this system by a bias voltage between the layers enables the full topological phase diagram to be explored, which is not possible in…
Recently twisted bilayer graphene (t-BLG) emerges as a new strongly correlated physical platform near a magic twist angle, which hosts many exciting phenomena such as the Mott-like insulating phases, unconventional superconducting behavior and emergent ferromagnetism. Besides the apparent significance of band flatness, band topology may be another critical element in determining strongly correlated twistronics yet receives much less attention. Here we report compelling evidence for nontrivial noninteracting band topology of t-BLG moiré Dirac bands through a systematic nonlocal transport study,…
