Observation of a critical prethermal discrete time crystal created by two-frequency driving
William Beatrez, Christoph Fleckenstein, Arjun Pillai, Erica Sanchez, Amala Akkiraju, Jesus Alcala, Sophie Conti, Paul Reshetikhin, Emanuel Druga, Marin Bukov, Ashok Ajoy
备注：
8 pages, 5 figures. SI: 15 pages, 19 figures. 4 anc movie files (also available on Youtube)
We report the observation of long-lived Floquet prethermal discrete time crystalline (PDTC) order in a three-dimensional position-disordered lattice of interacting dipolar-coupled 13C nuclei in diamond at room temperature. We demonstrate a novel strategy of "two-frequency" driving, involving an interleaved application of slow and fast drives that simultaneously prethermalize the spins with an emergent quasi-conserved magnetization along the x-axis, while enabling continuous and highly resolved observation of their dynamic evolution when periodically kicked away from x. The PDTC order manifests itself in a robust period doubling response of this drive-induced quasi-conserved spin magnetization interchanging between x and -x; our experiments allow a unique means to study the formation and melting of PDTC order. We obtain movies of the time-crystalline response with a clarity and throughput orders of magnitude greater than previous experiments. Parametric control over the drive frequencies allows us to reach PDTC lifetimes up to 396 Floquet cycles which we measure in a single-shot experiment. Such rapid measurement enables detailed characterization of the entire PDTC phase diagram, rigidity and lifetime, informing on the role of prethermalization towards stabilizing the DTC response. The two-frequency drive approach represents the simplest generalization of DTCs to multi-frequency drives; it expands the toolkit for realizing and investigating long-lived non-equilibrium phases of matter stabilized by emergent quasi-conservation laws.
Prethermalization, by introducing emergent quasiconserved observables, plays a crucial role in protecting Floquet many-body phases over exponentially long time, while the ultimate fate of such quasiconserved operators can signal thermalization to infinite temperature. To elucidate the properties of prethermal quasiconservation in many-body Floquet systems, here we systematically analyze infinite temperature correlations between observables. We numerically show that the late-time behavior of the autocorrelations unambiguously distinguishes quasiconserved observables from non-conserved ones, all…
Driven quantum systems may realize novel phenomena absent in static systems, but driving-induced heating can limit the time-scale on which these persist. We study heating in interacting quantum many-body systems driven by random sequences with $n-$multipolar correlations, corresponding to a polynomially suppressed low frequency spectrum. For $n\geq1$, we find a prethermal regime, the lifetime of which grows algebraically with the driving rate, with exponent ${2n+1}$. A simple theory based on Fermi's golden rule accounts for this behaviour. The quasiperiodic Thue-Morse sequence corresponds to t…
Periodic driving has emerged as a powerful tool in the quest to engineer new and exotic quantum phases. While driven many-body systems are generically expected to absorb energy indefinitely and reach an infinite-temperature state, the rate of heating can be exponentially suppressed when the drive frequency is large compared to the local energy scales of the system -- leading to long-lived 'prethermal' regimes. In this work, we experimentally study a bosonic cloud of ultracold atoms in a driven optical lattice and identify such a prethermal regime in the Bose-Hubbard model. By measuring the ene…
Periodically driven Floquet quantum systems provide a promising platform to investigate novel physics out of equilibrium. Unfortunately, the drive generically heats up the system to a featureless infinite temperature state. For large driving frequency, the heat absorption rate is predicted to be exponentially small, giving rise to a long-lived prethermal regime which exhibits all the intriguing properties of Floquet systems. Here we experimentally observe Floquet prethermalization using nuclear magnetic resonance techniques. We first show the relaxation of a far-from-equilibrium initial state …
Long-range interacting systems such as nitrogen vacancy centers in diamond and trapped ions serve as useful experimental setups to probe a range of nonequilibrium many-body phenomena. In particular, via driving, various effective Hamiltonians with physics potentially quite distinct from short-range systems can be realized. In this Letter, we derive general bounds on the linear response energy absorption rates of periodically driven systems of spins or fermions with long-range interactions that are sign changing and fall off as $1/r^α$ with $α> d/2$. We show that the disordered averaged energy …
The conventional framework for defining and understanding phases of matter requires thermodynamic equilibrium. Extensions to non-equilibrium systems have led to surprising insights into the nature of many-body thermalization and the discovery of novel phases of matter, often catalyzed by driving the system periodically. The inherent heating from such Floquet drives can be tempered by including strong disorder in the system, but this can also mask the generality of non-equilibrium phases. In this work, we utilize a trapped-ion quantum simulator to observe signatures of a non-equilibrium driven …
While a clean driven system generically absorbs energy until it reaches `infinite temperature', it may do so very slowly exhibiting what is known as a prethermal regime. Here, we show that the emergence of an additional approximately conserved quantity in a periodically driven (Floquet) system can give rise to an analogous long-lived regime. This can allow for non-trivial dynamics, even from initial states that are at a high or infinite temperature with respect to an effective Hamiltonian governing the prethermal dynamics. We present concrete settings with such a prethermal regime, one with a …
The manipulation of many-body systems often involves time-dependent forces that cause unwanted heating. One strategy to suppress heating is to use time-periodic (Floquet) forces at large driving frequencies. For quantum spin systems with bounded spectra, it was shown rigorously that the heating rate is exponentially small in the driving frequency. Recently, the exponential suppression of heating has also been observed in an experiment with ultracold atoms, realizing a periodically driven Bose-Hubbard model. This model has an unbounded spectrum and, hence, is beyond the reach of previous theore…
We study the microscopic dynamics of competing ordered phases in a two-dimensional correlated electron model, which is driven with a pulsed electric field of finite duration. In order to go beyond a mean-field treatment of the electronic interactions we adopt a large-$N$ generalization of the Hubbard model and combine it with the semiclassical fermionic truncated Wigner approximation as a time evolution method. This allows us to calculate dephasing corrections to the mean-field dynamics and to obtain stationary states, which we interpret as prethermal order. We use this framework to simulate t…
The use of periodic driving for synthesizing many-body quantum states depends crucially on the existence of a prethermal regime, which exhibits drive-tunable properties while forestalling the effects of heating. This motivates the search for direct experimental probes of the underlying localized nonergodic nature of the wave function in this metastable regime. We report experiments on a many-body Floquet system consisting of atoms in an optical lattice subjected to ultrastrong sign-changing amplitude modulation. Using a double-quench protocol we measure an inverse participation ratio quantifyi…
Heating to high-lying states strongly limits the experimental observation of driving induced non-equilibrium phenomena, particularly when the drive has a broad spectrum. Here we show that, for entire families of structured random drives known as random multipolar drives, particle excitation to higher bands can be well controlled even away from a high-frequency driving regime. This opens a window for observing drive-induced phenomena in a long-lived prethermal regime in the lowest band.
Localization may survive in periodically driven (Floquet) quantum systems, but is generally unstable for aperiodic drives. In this work, we identify a hidden conservation law originating from a chiral symmetry in a disordered spin-1/2 XX chain. This protects indefinitely long-lived localization for general--even aperiodic--drives. Therefore, rather counter-intuitively, adding further potential disorder which spoils the conservation law delocalizes the system, via a controllable parametrically long-lived prethermal regime. This provides a first example of persistent single-particle `localizatio…
The stabilization of steady state entanglement caused by action of a classical driving field in the system of two-level atoms with the dipole interaction accompanied by spontaneous emission is discussed. An exact solution shows that the maximum amount of concurrence that can be achieved in Lamb-Dicke limit is 0.43, which corresponds to the entanglement $\mathcal{E}_{max}=0.285$ ebit. Dependence of entanglement on interatomic distance and classical driving field is examined numerically.
The control of many-body quantum dynamics in complex systems is a key challenge in the quest to reliably produce and manipulate large-scale quantum entangled states. Recently, quench experiments in Rydberg atom arrays (Bluvstein et. al., arXiv:2012.12276) demonstrated that coherent revivals associated with quantum many-body scars can be stabilized by periodic driving, generating stable subharmonic responses over a wide parameter regime. We analyze a simple, related model where these phenomena originate from spatiotemporal ordering in an effective Floquet unitary, corresponding to discrete time…
The nonequilibrium quantum dynamics of closed many-body systems is a rich yet challenging field. While recent progress for periodically driven (Floquet) systems has yielded a number of rigorous results, our understanding on quantum many-body systems driven by rapidly varying but a- and quasi-periodic driving is still limited. Here, we derive rigorous, non-perturbative, bounds on the heating rate in quantum many-body systems under Thue-Morse quasi-periodic driving and under random multipolar driving, the latter being a tunably randomized variant of the former. In the process, we derive a static…
We discuss the universal nature of relaxation in isolated many-body quantum systems subjected to global and strong periodic driving. Our rigorous Floquet analysis shows that the energy of the system remains almost constant up to an exponentially long time in frequency for arbitrary initial states and that an effective Hamiltonian obtained by a truncation of the Floquet-Magnus expansion is a quasi-conserved quantity for long time scale. These two general properties lead to intriguing classification on the initial stage of relaxation, one of which is similar to the prethermalization phenomenon i…
Ultracold atomic gas provides a useful tool to explore many-body physics. One of the recent additions to this experimental toolbox is the Floquet engineering, where periodic modulation of the Hamiltonian allows the creation of effective potentials that do not exist otherwise. When subject to external modulations, however, generic interacting many-body systems absorb energy, thus posing a heating problem that may impair the usefulness of this method. For discrete systems with bounded local energy, an exponentially suppressed heating rate with the driving frequency has been observed previously, …
Two-mode squeezing and entanglement is obtained in a atom-cavity system cosisting a three-level atom and a two-mode cavity with driving laser fields. Here non-resonatn dressed-state transitions between the cavity modes and atom are used to get the effective Hamiltonian.
We present a detailed theoretical analysis of a multi-level quantum system coupled to two radiation fields and subject to decoherence. We concentrate on an effect known from quantum optics as the Autler-Townes splitting, which has been recently demonstrated experimentally [M. A. Sillanpaa et al., Phys. Rev. Lett. 103, 193601 (2009)] in a superconducting phase qubit. In the three-level approximation, we derive analytical solutions and describe how they can be used to extract the decoherence rates and to account for the measurement data. Better agreement with the experiment can be obtained by ex…
In the framework of the nonlinear $Λ$-model we investigate propagation of a slow-light soliton in atomic vapors and Bose-Einstein condensates. The velocity of the slow-light soliton is controlled by a time-dependent background field created by a controlling laser. For a fairly arbitrary time dependence of the field we find the dynamics of the slow-light soliton inside the medium. We provide an analytical description for the nonlinear dependence of the velocity of the signal on the controlling field. If the background field is turned off at some moment of time, the signal stops. We find the loc…
Discrete time crystals are periodically driven systems characterized by a response with periodicity $nT$, with $T$ the period of the drive and $n>1$. Typically, $n$ is an integer and bounded from above by the dimension of the local (or single particle) Hilbert space, the most prominent example being spin-$1/2$ systems with $n$ restricted to $2$. Here we show that a clean spin-$1/2$ system in the presence of long-range interactions and transverse field can sustain a huge variety of different `higher-order' discrete time crystals with integer and, surprisingly, even fractional $n > 2$. We charac…
This work explores a fundamental dynamical structure for a wide range of many-body quantum systems under periodic driving. Generically, in the thermodynamic limit, such systems are known to heat up to infinite temperature states after infinite-time evolution, irrespective of dynamical details. In the present study, instead of considering infinitely long-time scale, we aim to provide a framework to understand the long but finite time behavior, namely the transient dynamics. In the analysis, we focus on the Floquet-Magnus (FM) expansion that gives a formal expression of the effective Hamiltonian…
We propose a scheme to create distant entangled atomic states. It is based on driving two (or more) atoms with a weak laser pulse, so that the probability that two atoms are excited is negligible. If the subsequent spontaneous emission is detected, the entangled state is created. We have developed a model to analyze the fidelity of the resulting state as a function of the dimensions and location of the detector, and the motional properties of the atoms.
Emergent Self-Similar Quantum Revivals in Spiral Drives
Max Planck Institute for the Physics of Complex Systems（马克斯·普朗克复杂系统物理研究所）；Princeton University（普林斯顿大学）；Peking University（北京大学）；École Normale Supérieure (ENS), Université PSL（巴黎高等师范学院，PSL大学）
Discrete time crystals represent a paradigmatic nonequilibrium phase of periodically driven matter. Protecting its emergent spatiotemporal order necessitates a mechanism that hinders the spreading of defects, such as localization of domain walls in disordered quantum spin chains. In this work, we establish the effectiveness of a different mechanism arising in clean spin chains: the confinement of domain walls into ``mesonic'' bound states. We consider translationally invariant quantum Ising chains periodically kicked at arbitrary frequency, and discuss two possible routes to domain-wall confin…
