In a magnetic field few-layer graphene supports, at the lowest Landau level, a multiplet of zero-mode levels nearly degenerate in orbitals as well as in spins and valleys. Those pseudo-zero-mode (PZM) levels are generally sensitive to interactions and external perturbations, and have a crossing among themselves or with other higher Landau levels when an external field is swept over a certain range. A close study is made of how such PZM levels evolve when they are gradually brought from empty to filled levels under many-body interactions. It is pointed out that the level spectra generally avoid a crossing via orbital level mixing and that orbital mixing is governed by a non-Abelian Berry phase that derives from an approximate degeneracy and interactions. A look is also taken into evolution/crossing of many-body ground states with increasing external bias in bilayer graphene.
The Berry phase of π in graphene is derived in a pedagogical way. The ambiguity of how to calculate this value properly is clarified. Its connection with the unconventional quantum Hall effect in graphene is discussed.
The Berry phase and the group-velocity-based traversal time have been calculated for an asymmetric non-contacted or contacted graphene structure, and significant differences have been observed compared to semiconductor heterostructures. These differences are related to the specific, Dirac-like evolution law of charge carriers in graphene, which introduces a new type of asymmetry. When contacted with electrodes, the symmetry of the Dirac equation is broken by the Schrodinger-type electrons in contacts, so that the Berry phase and traversal time behavior in contacted and non-contacted graphene d…
We derive a semiclassical expression for the Green's function in graphene, in which the presence of a semiclassical phase is made apparent. The relationship between this semiclassical phase and the adiabatic Berry phase, usually referred to in this context, is discussed. These phases coincide for the perfectly linear Dirac dispersion relation. They differ however when a gap is opened at the Dirac point. We furthermore present several applications of our semiclassical formalism. In particular we provide, for various configurations, a semiclassical derivation of the electron's Landau levels, ill…
We show that in gapped bilayer graphene, quasiparticle tunneling and the corresponding Berry phase can be controlled such that it exhibits features of single layer graphene such as Klein tunneling. The Berry phase is detected by a high-quality Fabry-Pérot interferometer based on bilayer graphene. By raising the Fermi energy of the charge carriers, we find that the Berry phase can be continuously tuned from $2π$ down to $0.68π$ in gapped bilayer graphene, in contrast to the constant Berry phase of $2π$ in pristine bilayer graphene. Particularly, we observe a Berry phase of $π$, the standard val…
Hamiltonian and eigenstate problem is formulated for a bilayer graphene in terms of Clifford's geometric algebra \textit{Cl}$_{3,1}$. It is shown that such approach allows to perform analytical calculations in a simple way if geometrical algebra rotors are used. The measured quantities are express through spectrum and rotation half-angle of the pseudospin that appears in geometric algebra rotors. Properties of free charge carriers -- pseudospin, velocity and Berry phase -- in a bilayer graphene are investigated in the presence of the external voltage applied between the two layers.
Recent experiments have measured local uniaxial strain fields in twisted bilayer graphene (TBG). Our calculations found that the finite Berry curvature generated by breaking the sublattice symmetry and the band proximity between narrow bands in these TBG induces a giant Berry dipole of order 10\,nm or larger. The large Berry dipole leads to transverse topological non-linear charge currents which dominates over the linear bulk valley current at experimentally accessible crossover in-plane electric field of $\sim 0.1 {\rm mV} / μ\rm{m}$. This anomalous Hall effect, due to Berry dipole, is strong…
We have observed the quantum Hall effect (QHE) and Shubnikov-de Haas (SdH) oscillations in highly disordered graphene at magnetic fields up to 65 T. Disorder was introduced by hydrogenation of graphene up to a ratio H/C $\approx 0.1\%$. The analysis of SdH oscillations and QHE indicates that the topological part of the Berry phase, proportional to the pseudo-spin winding number, is robust against introduction of disorder by hydrogenation in large scale graphene.
The magnetic effects in ferromagnetic graphene basically depend on the principle of exchange interaction when ferromagntism is induced by depositing an insulator layer on graphene. Here we deal with the consequences of non-uniformity in the exchange coupling strength of the ferromagnetic graphene. We discuss how the in- homogeneity in the coordinate and momentum of the exchange vector field can provide interesting results in the conductivity analysis of the ferromagnetic graphene. Our analysis is based on the Kubo formalism of quantum transport.
High-order terahertz (THz) sideband generation (HSG) in semiconductors is a phenomenon with physics similar to high-order harmonic generation but in a much lower frequency regime. It was found that the electron-hole pairs excited by a weak optical laser can accumulate Berry phases along a cyclic path under the driving of a strong THz field. The Berry phases appear as the Faraday rotation angles of the emission signal under short-pulse excitation in monolayer MoS$_2$. In this paper, the theory of Berry phase in THz extreme nonlinear optics is applied to biased bilayer graphene with Bernal stack…
It has been recently established that optoelectronic and non-linear transport experiments can give direct access to the dipole moment of the Berry curvature in non-magnetic and non-centrosymmetric materials. Thus far, non-vanishing Berry curvature dipoles have been shown to exist in materials with substantial spin-orbit coupling where low-energy Dirac quasiparticles form tilted cones. Here, we prove that this topological effect does emerge in two-dimensional Dirac materials even in the complete absence of spin-orbit coupling. In these systems, it is the warping of the Fermi surface that trigge…
We propose a general framework of nonlinear optics induced by non-Abelian Berry curvature in time-reversal-invariant (TRI) insulators. We find that the third-order response of a TRI insulator under optical and terahertz light fields is directly related to the integration of the non-Abelian Berry curvature over the Brillouin zone. We apply the result to insulators with rotational symmetry near the band edge. Under resonant excitations, the optical susceptibility is proportional to the flux of the Berry curvature through the iso-energy surface, which is equal to the Chern number of the surface t…
We study the influence of a magnetic flux tube on the possibility to electrostatically confine electrons in a graphene quantum dot. Without magnetic flux tube, the graphene pseudospin is responsible for a quantization of the total angular momentum to half-integer values. On the other hand, with a flux tube containing half a flux quantum, the Aharonov-Bohm phase and Berry phase precisely cancel, and we find a state at zero angular momentum that cannot be confined electrostatically. In this case, true bound states only exist in regular geometries for which states without zero-angular-momentum co…
We present an approach to the computation of the non-Abelian statistics of quasiholes in quantum Hall states, such as the Pfaffian state, whose wavefunctions are related to the conformal blocks of minimal model conformal field theories. We use the Coulomb gas construction of these conformal field theories to formulate a plasma analogy for the quantum Hall states. A number of properties of the Pfaffian state follow immediately, including the Berry phases which demonstrate the quasiholes' fractional charge, the abelian statistics of the two-quasihole state, and equal-time ground state correlatio…
There are known two distinct types of the integer quantum Hall effect. One is the conventional quantum Hall effect, characteristic of two-dimensional semiconductor systems, and the other is its relativistic counterpart recently observed in graphene, where charge carriers mimic Dirac fermions characterized by Berry's phase pi, which results in a shifted positions of Hall plateaus. Here we report a third type of the integer quantum Hall effect. Charge carriers in bilayer graphene have a parabolic energy spectrum but are chiral and exhibit Berry's phase 2pi affecting their quantum dynamics. The L…
Since its discovery, Berry phase has been demonstrated to play an important role in many quantum systems. In gapped Bernal bilayer graphene, the Berry phase can be continuously tuned from zero to 2pi, which offers a unique opportunity to explore the tunable Berry phase on the physical phenomena. Here, we report experimental observation of Berry phases-induced valley splitting and crossing in moveable bilayer graphene p-n junction resonators. In our experiment, the bilayer graphene resonators are generated by combining the electric field of scanning tunneling microscope tip with the gap of bila…
Ever since the novel quantum Hall effect in bilayer graphene was discovered, and explained by a Berry phase of 2pi [K. S. Novoselov et al., "Unconventional quantum Hall effect and Berry's phase of 2pi in bilayer graphene", Nature Phys. 2, 177 (2006)], it has been widely accepted that the low-energy electronic wavefunction in this system is described by a non-trivial Berry phase of 2pi, different from the zero phase of a conventional two-dimensional electron gas. Here, we show that (i) the relevant Berry phase for bilayer graphene is not different from that for a conventional two-dimensional el…
Valley is a useful degree of freedom for non-dissipative electronics since valley current that can flow even in an insulating material does not accompany electronic current. We use dual-gated bilayer graphene in the Hall bar geometry to electrically control broken inversion symmetry or Berry curvature as well as the carrier density to generate and detect the pure valley current. We find a large nonlocal resistance and a cubic scaling between the nonlocal resistance and the local resistivity in the insulating regime at zero-magnetic field and 70 K as evidence of the pure valley current. The ele…
Non-trivial Berry phase of graphene leads to unusual quantum correction to the conductivity. Berry phase of pi in single layer graphene (SLG) and 2pi in bi-layer graphene (BLG) is expected to reveal weak anti-localization (WAL) and weak localization (WL), respectively. However, experimentally both WAL and WL have been observed in graphene devices depending on the strength of different scattering mechanisms. Graphene superlattice having multiple Dirac cones is expected to exhibit pi to 2pi Berry phase transition from primary Dirac cone (PDC) to cloned Dirac cone (CDC). However, its effect on lo…
We show that the spectrum of subbands in an electrostatically defined quantum wire in gapped bilayer graphene directly manifests the minivalley structure and reflects Berry curvature via the associated magnetic moment of the states in the low-energy bands of this two-dimensional material. We demonstrate how these appear in degeneracies of the low-energy minibands and their valley splitting, which develops linearly in a weak magnetic field. Consequently, magneto-conductance of a ballistic point contact connecting two non-gapped areas of a bilayer through a gapped (top and bottom gated) barrier …
Real magnetic and lattice deformation gauge fields have been investigated in honeycomb lattice of graphene. The coexistence of these two gauges will induce a gap difference between two valley points ($K$ and $K'$) of system. This gap difference allows us to study the possible topological valley Hall current and valley polarization in the graphene sheet. In the absence of magnetic field, the strain alone could not generate a valley polarization when the Fermi energy coincides exactly with the Dirac points. Since in this case there is not any imbalance between the population of the valley points…
Berry phase plays an important role in determining many physical properties of quantum systems. However, a Berry phase altering energy spectrum of a quantum system is comparatively rare. Here, we report an unusual tunable valley polarized energy spectra induced by continuously tunable Berry phase in Bernal-stacked bilayer graphene quantum dots. In our experiment, the Berry phase of electron orbital states is continuously tuned from about pi to 2pi by perpendicular magnetic fields. When the Berry phase equals pi or 2pi, the electron states in the two inequivalent valleys are energetically degen…
When a gap of tunable size opens at the conic band intersections of graphene, the Berry phase does not vanish abruptly, but progressively decreases as the gap increases. The phase depends on the reciprocal-space path radius, i.e., for a doped system, the Fermi wave vector. The phase and its observable consequences can thus be tuned continuously via gap opening --by a modulating potential induced by strain, epitaxy, or nanostructuration-- and doping adjustment.
Brillouin zones of graphene systems possess Dirac points, where band degeneracies occur. We study the variety of (and large magnitude) phases that the electronic states can acquire when a uniform time-dependent electric field carries the electrons around one or more Dirac points in a non-concentric fashion. An experimentally accessible determination of excess Berry phases is proposed involving the Zitterbewegung of electronic current near an orthogonality point in adiabatic motion.
We describe a method for measuring the Berry curvature from the wave-packet dynamics in perturbed arrays of evanescently coupled optical waveguides with honeycomb lattice structure. To disentangle the effects of the Berry curvature and the energy dispersion we utilize a difference measurement by propagating the wave packet under the influence of a constant external force back and forth. In this way a non-vanishing Berry curvature is obtained for photonic graphene with small sublattice bias or strain, where the relative error between the exact Berry curvature and the one derived from the semicl…
We point out a practical way to induce a finite charge Hall conductivity in graphene via an off-diagonal strain. Our conclusions are based on a general analysis and supported by numerical examples. The interplay between a substrate-induced gap and the strain is discussed. We show that the substrate-induced gap itself does not break the symmetry that maps one valley onto the other, and hence does not yield a net charge Hall effect. The net charge Hall conductivity is found to be sizable and should be observable in the presence of both the gap and the strain. The sign of the Hall conductivity ca…
Klein tunneling in gapless bilayer graphene, perfect reflection of electrons injecting normal to a pn junction, is expected to disappear in the presence of energy band gap induced by external gates. We theoretically show that the Klein effect still exists in gapped bilayer graphene, provided that the gaps in the n and p regions are balanced such that the polarization of electron pseudospin has the same normal component to the bilayer plane in the regions. We attribute the Klein effect to Berry phase $π$ (rather than the conventional value $2 π$ of bilayer graphene) and to electron-hole and tim…
We have found that the Berry phase of bilayer graphene becomes from 2$π$ estimated by Shubnikov-de Haas oscillations when the A-B stacked pristine bilayer graphene experiences the Li-intercalation and sequential Li-desorption process in ultrahigh vacuum. Furthermore, the mobility of such processed bilayer graphene increases around four times larger, ~ 8,000 cm2/V$\cdot$s, than that of the pristine bilayer graphene. This is mainly due to increment of the scattering time and decrement of the cyclotron mass, which can be interpreted as a result of the change of the stacking structure of bilayer g…
We consider gated graphene nanoribbons subject to Berry-Mondragon boundary conditions in the presence of weak impurities. Using field--theoretical methods, we calculate the density of charge carriers (and, thus, the quantum capacitance) as well as the optical and DC conductivities at zero temperature. We discuss in detail their dependence on the gate (chemical) potential, and reveal a non-linear behaviour induced by the quantization of the transversal momentum.
Standing waves near the zigzag and armchair edges, and their Berry's phases are investigated. It is suggested that the Berry's phase for the standing wave near the zigzag edge is trivial, while that near the armchair edge is non-trivial. A non-trivial Berry's phase implies the presence of a singularity in parameter space. We have confirmed that the Dirac singularity is absent (present) in the parameter space for the standing wave near the zigzag (armchair) edge. The absence of the Dirac singularity has a direct consequence in the local density of states near the zigzag edge. The transport prop…
Chiral quasiparticles in Bernal-stacked bilayer graphene have valley-contrasting Berry phases of 2π. This nontrival topological structure, associated with the pseudospin winding along a closed Fermi surface, is responsible for various novel electronic properties, such as anti-Klein tunneling, unconventional quantum Hall effect, and valley Hall effect1-6. Here we show that the quantum interference due to intervalley scattering induced by atomic defects/impurities provides further insights into the topological nature of the bilayer graphene. The scattered chiral quasiparticles between distinct v…
We study the quantum nonlinear planar Hall effect in bilayer graphene under a steady in-plane magnetic field. When time-reversal symmetry is broken by the magnetic field, a charge current occurs in the second-order response to an external electric field, as a result of the Berry curvature dipole in momentum space. We have shown that a nonlinear planar Hall effect originating from the anomalous velocity is deduced by an orbital effect of an in-plane magnetic field on electrons in bilayer graphene in the complete absence of spin-orbit coupling. Taking into account the symmetry analysis, we deriv…
We present a quantized non-Abelian Berry phase for time reversal invariant systems such as quantum spin Hall effect. Ordinary Berry phase is defined by an integral of Berry's gauge potential along a loop (an integral of the Chern-Simons one-form), whereas we propose that a similar integral but over five dimensional parameter space (an integral of the Chern-Simons five-form) is suitable to define a non-Abelian Berry phase. We study its global topological aspects and show that it is indeed quantized into two values. We also discuss its close relationship with the nonperturbative anomalies.
The phase of a quantum state may not return to its original value after the system's parameters cycle around a closed path; instead, the wavefunction may acquire a measurable phase difference called the Berry phase. Berry phases typically have been accessed through interference experiments. Here, we demonstrate an unusual Berry-phase-induced spectroscopic feature: a sudden and large increase in the energy of angular-momentum states in circular graphene p-n junction resonators when a small critical magnetic field is reached. This behavior results from turning on a $π$-Berry phase associated wit…
Electronic band structures dictate the mechanical, optical and electrical properties of crystalline solids. Their experimental determination is therefore of crucial importance for technological applications. While the spectral distribution in energy bands is routinely measured by various techniques, it is more difficult to access the topological properties of band structures such as the Berry phase γ. It is usually thought that measuring the Berry phase requires applying external electromagnetic forces because these allow realizing the adiabatic transport on closed trajectories along which qua…
We consider the anomalous thermoelectric transport in gapped single and bilayer graphene where the gap may be due to broken inversion symmetry. In the presence of the gap, non-trivial Berry phase effects can be shown to mediate a transverse thermoelectric voltage in response to an applied temperature gradient even in the absence of a perpendicular magnetic field. This spontaneous, anomalous Nernst effect is nonzero for non-uniform chemical potential in the two inequivalent valleys in the graphene band structure. Conversely, the Nernst response can be used to create a valley-index polarization …
When electrons are confined in two-dimensional (2D) materials, quantum mechanically enhanced transport phenomena, as exemplified by the quantum Hall effects (QHE), can be observed. Graphene, an isolated single atomic layer of graphite, is an ideal realization of such a 2D system. Here, we report an experimental investigation of magneto transport in a high mobility single layer of graphene. Adjusting the chemical potential using the electric field effect, we observe an unusual half integer QHE for both electron and hole carriers in graphene. Vanishing effective carrier masses is observed at Dir…
We demonstrate that dislocations in the graphene lattice give rise to electron Berry phases equivalent to quantized values {0,1/3,-1/3} in units of the flux quantum, but with an opposite sign for the two valleys. An elementary scale consideration of a graphene Aharonov-Bohm ring equipped with valley filters on both terminals, encircling a dislocation, says that in the regime where the intervalley mean free path is large compared to the intravalley phase coherence length, such that the valley quantum numbers can be regarded as conserved on the relevant scale, the coherent valley-polarized curre…
We have investigated pumping in quantum dots from the perspective of non-Abelian (matrix) Berry phases by solving the time dependent Schr{ö}dinger equation exactly for adiabatic changes. Our results demonstrate that a pumped charge is related to the presence of a finite matrix Berry phase. When consecutive adiabatic cycles are performed the pumped charge of each cycle is different from the previous ones.
The electronic dispersion of a graphene bilayer is highly dependent on rotational mismatch between layers and can be further manipulated by electrical gating. This allows for an unprecedented control over electronic properties and opens up the possibility of flexible band structure engineering. Here we present novel magnetotransport data in a twisted bilayer, crossing the energetic border between decoupled monolayers and coupled bilayer. In addition a transition in Berry phase between pi and 2pi is observed at intermediate magnetic fields. Analysis of Fermi velocities and gate induced charge c…
Periodicity of long wavelength moiré patterns is very often destroyed by the inhomogeneous strain introduced in fabrications of van der Waals layered structures. We present a framework to describe massive Dirac fermions in such distorted moiré pattern of transition metal dichalcogenides homobilayers, accounting for the dynamics of layer pseudospin. In decoupled bilayers, we show two causes of in-plane layer pseudospin precession: By the coupling of layer antisymmetric strain to valley magnetic moment; and by the Aharonov-Bohm effect in the SU(2) gauge potential for the case of R-type bilayer u…
Here, we introduce and apply non-Abelian tensor Berry connections to topological phases in multi-band systems. These gauge connections behave as non-Abelian antisymmetric tensor gauge fields in momentum space and naturally generalize Abelian tensor Berry connections and ordinary non-Abelian (vector) Berry connections. We build these novel gauge fields from momentum-space Higgs fields, which emerge from the degenerate band structure of degenerate-band models. Firstly, we show that the conventional topological invariants of two-dimensional topological insulators and three-dimensional Dirac semim…
We show that the non-Abelian Berry phase emerges naturally in the s-wave and spin quintet pairing channel of spin-3/2 fermions. The topological structure of this pairing condensate is characterized by the second Chern number. This topological structure can be realized in ultra-cold atomic systems and in solid state systems with at least two Kramers doublets.
We propose that n-type semiconductor quantum dots with the Rashba and Dresselhaus spin orbit interactions may be used for single electron manipulation through adiabatic transformations between degenerate states. All the energy levels are discrete in quantum dots and possess a double degeneracy due to time reversal symmetryin the presence of the Rashba and/or Dresselhaus spin orbit coupling terms. We find that the presence of double degeneracy does not necessarily give rise to a finite non-Abelian (matrix) Berry phase. We show that a distorted two-dimensional harmonic potential may give rise to…
We demonstrate that flat bands with local Berry curvature arise naturally in chiral (ABC) multilayer graphene placed on a boron nitride (BN) substrate. The degree of flatness can be tuned by varying the number of graphene layers N. For N = 7 the bands become nearly flat, with a small bandwidth of 3.6 meV. The two nearly flat bands coming from the K and K' valleys cross along lines in the reduced zone. Weak intervalley tunneling turns the bandcrossing into an avoided crossing, producing two nearly flat bands with global Chern number zero, but with local Berry curvature. The flatness of the band…
In the present paper we have directly computed the Berry curvature terms relevant for Graphene in the presence of an \textit{inhomogeneous} lattice distortion. We have employed the generalized Foldy Wouthuysen framework, developed by some of us \cite{ber0,ber1,ber2}. We show that a non-constant lattice distortion leads to a valley-orbit coupling which is responsible to a valley-Hall effect. This is similar to the valley-Hall effect induced by an electric field proposed in \cite{niu2} and is the analogue of the spin-Hall effect in semiconductors \cite{MURAKAMI, SINOVA}. Our general expressions …
We study the energy spectrum of a graphene bilayer in the presence of transverse electric and magnetic fields. We find that the resulting Landau levels exhibit a nonmonotonic dependence on the electric field, as well as numerous level crossings. This behavior is explained using quasiclassical quantization rules that properly take into account the pseudospin of the quasiparticles. The pseudospin generates the Berry phase, which leads to a shift in energy quantization and results in a pseudo-Zeeman effect. The latter depends on the electric field, alternates in sign among the two valleys, and al…
Single-layer carbon, or graphene, demonstrates amazing transport properties, such as the minimum conductivity near $\frac{4e^2}{h}$ independent of shapes and mobility of samples. This indicates there exist some unusual effects due to specific Dirac dispersion relation of fermion in two dimensions. By deriving fermion-lattice interaction Hamiltonian we show that Berry phases can be produced in fermion states around two Dirac points by relative rotations of two sublattices. The Berry phases in turn remove the degeneracies of energies for states near the Fermi surface, leading to a dynamical inst…
The electronic band structure of ABC-stacked multilayer graphene is studied within an effective mass approximation. The electron and hole bands touching at zero energy support chiral quasiparticles characterized by Berry's phase N pi for N-layers, generalizing the low-energy band structure of monolayer and bilayer graphene. We investigate the trigonal-warping deformation of the energy bands and show that the Lifshitz transition, in which the Fermi circle breaks up into separate parts at low energy, reflects Berry's phase N pi. It is particularly prominent in trilayers, N=3, with the Fermi circ…
