arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2109.11286cond-mat.supr-con
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可果美金属RbV $_3$ Sb $_5$的电子结构演化

Evolution of electronic structure in pristine and hole-doped kagome metal RbV$_3$Sb$_5$

Jiawei Yu, Kebin Xiao, Yonghao Yuan, Qiangwei Yin, Zhiqiang Hu, Chunsheng Gong, Yunkai Guo, Zhijun Tu, Hechang Lei, Qi-Kun Xue, Wei Li

摘要:

本文报道了用原位低温(4 K)扫描隧道显微镜对碱金属可果美RbV $_3$ Sb $_5$单晶解理面的原子和电子结构的测量。我们发现,占主导地位的原始表面呈现Rb-1x 1结构,其中一个独特的单向$\sqrt{3}a_0$电荷秩序被发现。当样品温度稍升高时,由于表面Rb原子的脱附,形成Rb- $\sqrt{3}$ x1和Rb- $\sqrt{3}$ x $\sqrt{3}$重构。我们的电导映射结果表明,Rb脱附不仅引起空穴掺杂,但也重整电子能带结构。令人惊讶的是,我们发现一个普遍存在的能隙开放附近的费米能级的隧道光谱在所有的表面上,尽管它们的空穴载流子浓度的巨大差异,表明轨道选择性带重建在RbV $_3$ Sb $_5$。

英文摘要:

We report on in situ low-temperature (4 K) scanning tunneling microscope measurements of atomic and electronic structures of the cleaved surfaces of an alkali-based kagome metal RbV$_3$Sb$_5$ single crystals. We find that the dominant pristine surface exhibits Rb-1x1 structure, in which a unique unidirectional $\sqrt{3}a_0$ charge order is discovered. As the sample temperature slightly rises, Rb-$\sqrt{3}$x1 and Rb-$\sqrt{3}$x$\sqrt{3}$ reconstructions form due to desorption of surface Rb atoms. Our conductance mapping results demonstrate that Rb desorption not only gives rise to hole doping, but also renormalizes the electronic band structures. Surprisingly, we find a ubiquitous gap opening near the Fermi level in tunneling spectra on all the surfaces despite their large differences of hole-carrier concentration, indicating an orbital-selective band reconstruction in RbV$_3$Sb$_5$.

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