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arXiv 2108.09679cond-mat.str-el
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Metastable antiphase boundary ordering in CaFe$_{2}$O$_{4}$

H. Lane, E. E. Rodriguez, H. C. Walker, Ch. Niedermayer, U. Stuhr, R. I. Bewley, D. J. Voneshen, M. A. Green, J. A. Rodriguez-Rivera, P. Fouquet, S. -W. Cheong,… 展开作者

H. Lane, E. E. Rodriguez, H. C. Walker, Ch. Niedermayer, U. Stuhr, R. I. Bewley, D. J. Voneshen, M. A. Green, J. A. Rodriguez-Rivera, P. Fouquet, S. -W. Cheong, J. P. Attfield, R. A. Ewings, C. Stock

英文摘要:

CaFe$_{2}$O$_{4}$ is an $S=5/2$ antiferromagnet exhibiting two magnetic orders which shows regions of coexistence at some temperatures. Using a Green's function formalism, we model neutron scattering data of the spin wave excitations in this material, ellucidating the microscopic spin Hamiltonian. In doing so, we suggest that the low temperature A phase order $(\uparrow\uparrow\downarrow\downarrow)$ finds its origins in the freezing of antiphase boundaries created by thermal fluctuations in a parent B phase order $(\uparrow\downarrow\uparrow\downarrow)$. The low temperature magnetic order observed in CaFe$_{2}$O$_{4}$ is thus the result of a competition between the exchange coupling along $c$, which favors the B phase, and the single-ion anisotropy which stabilizes thermally-generated antiphase boundaries, leading to static metastable A phase order at low temperatures.

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