We numerically investigate the effects of fiber aspect ratio, roughness, flexibility, and flow inertia on the rheology of concentrated suspensions. We perform direct numerical simulations modeling the fibers, suspended in an incompressible Newtonian fluid, as continuous flexible slender bodies obeying the Euler-Bernoulli beam equation. An immersed Boundary Method (IBM) is employed to solve for the motion of fibers. In concentrated suspensions, fibers come into contact due to the presence of asperities on their surface. We assume a normal load-dependent friction coefficient to model contact dynamics and friction, which successfully recovers the shear-thinning behaviour observed in experiments. First, we report the shear rate dependent behavior and the increase in the suspension viscosity with the increasing volume fraction of fibers, fiber roughness, and rigidity. The increase in the viscosity is stronger at a lower shear rate and finite inertia. Simulation results indicate that for the concentrated suspensions, contact stresses between fibers form the dominant contribution to the viscosity. Moreover, we find the first normal stress difference to be positive and to increase with the Reynolds number for flexible fibers. Lastly, we explore the divergence of viscosity for different aspect ratios and roughness of the fibers and predict the jamming volume fraction by fitting the data to the Maron-Pierce law. The jamming volume fraction decreases with increasing the aspect ratio and roughness. We conclude that the contact forces and interparticle friction become one of the crucial factors governing the rheology of flexible fiber suspensions at high concentrations.
As a paradigmatic model of active fluids, bacterial suspensions show intriguing rheological responses drastically different from their counterpart colloidal suspensions. Although the flow of bulk bacterial suspensions has been extensively studied, the rheology of bacterial suspensions under confinement has not been experimentally explored. Here, using a microfluidic viscometer, we systematically measure the rheology of dilute E. coli suspensions under different degrees of confinement. Our study reveals a strong confinement effect: the viscosity of bacterial suspensions decreases substantially …
Short-time dynamics and high-frequency rheology for suspensions of non-overlapping core-shell particles with thin shells were analyzed. In the thin-shell limit, the single-particle scattering coefficients were derived and shown to define a unique effective radius. This result was used to justify theoretically (in the thin-shell limit) the accuracy of the annulus approximation with the inner radius equal to the effective hydrodynamic radius of the core-shell particle. The two-particle virial expansion of the translational & rotational self-diffusion, sedimentation and viscosity was performed. T…
Rheology of dense suspensions of granular spherocylinders by particle-based simulation
School of Engineering, University of Edinburgh（爱丁堡大学工程学院）；Syngenta Jealott’s Hill International Research Centre（先正达乔洛特山国际研究中心）；School of Physics and Astronomy, The University of Edinburgh（爱丁堡大学物理与天文学院）
The rheology of non-colloidal suspensions under cyclic shear is studied numerically. The main findings are a strain amplitude ($γ_0$) dependent response in the shear stress and second normal stress difference ($N_2$). Specifically, we find a reduced viscosity, an enhanced intracycle shear thinning, the onset of a finite $N_2$ and its frequency doubling, all near a critical strain amplitude $γ_c$ that scales with the volume fraction $ϕ$ as $γ_c \sim ϕ^{-2}$. These rheological changes also signify a reversible-irreversible transition (RIT), dividing stroboscopic particle dynamics into a reversib…
We explain the origins of yield stress, shear-thinning, and normal stress differences in rigid fiber suspensions. We investigate the interplay between the hydrodynamic, colloidal attractive and repulsive, and inter-fiber contact interactions. The shear-thinning viscosity and finite yield stress obtained from the computational model are in quantitative agreement with experiential results from the literature. In this study, we show that attractive interactions result in yield stress and shear-thinning rheology in the suspensions of rigid fibers. This is an important finding, given the ongoing di…
We study suspensions of deformable (viscoelastic) spheres in a Newtonian solvent in plane Couette geometry, by means of direct numerical simulations. We find that in the limit of vanishing inertia the effective viscosity $μ$ of the suspension increases as the volume-fraction occupied by the spheres $Φ$ increases and decreases as the elastic modulus of the spheres $G$ decreases; the function $μ(Φ,G)$ collapses to an universal function, $μ(Φ_e)$, with a reduced effective volume fraction $Φ_e(Φ,G)$. Remarkably, the function $μ(Φ_e)$ is the well-known Eilers fit that describes the rheology of susp…
We investigate the rheology of strain-hardening spherical capsules, from the dilute to the concentrated regime under a confined shear flow using three-dimensional numerical simulations. We consider the effect of capillary number, volume fraction and membrane inextensibility on the particle deformation and on the effective suspension viscosity and normal stress differences of the suspension. The suspension displays a shear-thinning behaviour which is a characteristic of soft particles such as emulsion droplets, vesicles, strain-softening capsules, and red blood cells. We find that the membrane …
We study the effect of magnetic field on the rheology of magnetic micro-swimmers suspensions. We use a model of a dilute suspension under simple shear and subjected to a constant magnetic field. Particle shear stress is obtained for both pusher and puller types of micro-swimmers. In the limit of low shear rate, the rheology exhibits a constant shear stress, called actuated stress, which only depends on the swimming activity of the particles. This stress is induced by the magnetic field and can be positive (brake state) or negative (motor state). In the limit of low magnetic fields, a scaling r…
The microstructure and rheological properties of suspensions of neutrally buoyant hard spherical particles in Newtonian fluid under conditions of finite inertia are studied using the lattice-Boltzmann method (LBM), which is based on a discrete Boltzmann model for the fluid and Newtonian dynamics for the particles. The suspensions are subjected to simple-shear flow and the properties are studied as a function of Reynolds number and volume fraction, $ϕ$. The inertia is characterized by the particle-scale shear flow Reynolds number $Re = \frac{ρ\dotγa^{2}}μ$, where $a$ is the particle radius, $\d…
We study the effect of isotropic porous walls on a plane Couette flow laden with spherical and rigid particles. We perform a parametric study varying the volume fraction between $0$ and $30\%$, the porosity between $0.3$ and $0.9$ and the non-dimensional permeability between $0$ and $7.9 \times 10^{-3}$ We find that the porous walls induce a progressive decrease in the suspension effective viscosity as the wall permeability increases. This behavior is explained by the weakening of the wall-blocking effect and by the appearance of a slip velocity at the interface of the porous medium, which red…
Suspensions of self-motile, elongated particles are a topic of significant current interest, exemplifying a form of `active matter'. Examples include self-propelling bacteria, algae and sperm, and artificial swimmers. Ericksen's model of a transversely-isotropic fluid [J. L. Ericksen, Colloid Polym. Sci. 173(2):117-122 (1960)] treats suspensions of non-motile particles as a continuum with an evolving preferred direction; this model describes fibrous materials as diverse as extracellular matrix, textile tufts and plant cell walls. Director-dependent effects are incorporated through a modified s…
We investigate the shear thinning of red blood cell - dextran suspensions. Microscopic images show that at low polymer concentration, aggregation increases with increasing concentration until it reaches a maximum and then decreases again to non-aggregation. This bell shape dependency is also deduced from the rheological measurements, if the data are correctly normalized by the viscosity of the suspending phase since a significant amount of polymers adsorb to the cell surfaces. We find that the position of the maximum of this shear rate dependent bell shape increases with increasing viscosity o…
We study the shearing rheology of dense suspensions of elastic capsules, taking aggregation-free red blood cells as a physiologically relevant example. Particles are non-Brownian and interact only via hydrodynamics and short-range repulsive forces. An analysis of the different stress mechanisms in the suspension shows that the viscosity is governed by the shear elasticity of the capsules, whereas the repulsive forces are subdominant. Evidence for a dynamic yield stress above a critical volume fraction is provided and related to the elastic properties of the capsules. The shear stress is found …
Similarly to their biological counterparts, suspensions of chemically-active autophoretic swimmers exhibit nontrivial dynamics involving self-organization processes as a result of inter-particle interactions. Using a kinetic model for a dilute suspension of autochemotactic Janus particles, we analyse the effect of a confined pressure-driven flow on these collective behaviours and the impact of chemotactic aggregation on the effective viscosity of the active fluid. Four dynamic regimes are identified when increasing the strength of the imposed pressure-driven flow, each associated with a differ…
Granular suspensions present a transition from a Newtonian rheology in the Stokes limit to a Bagnoldian rheology when inertia is increased. A custom rheometer which can be run in a pressure or a volume-imposed mode is used to examine this transition in the dense regime close to jamming. By varying systematically the interstitial fluid, shear rate, and packing fraction in volume-imposed measurements, we show that the transition takes place at a Stokes number of 10 independent of the packing fraction. Using pressure-imposed rheometry, we investigate whether the inertial and viscous regimes can b…
We investigate the steady-state extensional rheology of a dilute suspension of spherical particles in a dilute polymer solution. For a particle-free polymeric fluid, in addition to the solvent viscosity, the extensional viscosity due to the polymers, $μ^\text{poly}$, contributes to the total non-dimensionalized extensional viscosity $1+μ^\text{poly}$. When a small volume fraction, $ϕ$, of spheres is added to a polymeric fluid, the stress is altered by the Einstein viscosity of 2.5$ϕ$ and two additional stress contributions: the interaction stresslet and the particle-induced polymer stress (PIP…
The agglomeration of particles caused by the formation of capillary bridges has a decisive impact on the transport properties of a variety of at a first sight very different systems such as capillary suspensions, fluidized beds in chemical reactors, or even sand castles. Here, we study the connection between the microstructure of the agglomerates and the rheology of fluidized suspensions using a coupled lattice Boltzmann and discrete element method approach. We address the influence of the shear rate, the secondary fluid surface tension, and the suspending liquid viscosity. The presence of cap…
The dynamics of an adhesive two-dimensional vesicle doublet under various flow conditions is investigated numerically using a high-order, adaptive-in-time boundary integral method. In a quiescent flow, two nearby vesicles move slowly towards each other under the adhesive potential, pushing out fluid between them to form a vesicle doublet at equilibrium. A lubrication analysis on such draining of a thin film gives the dependencies of draining time on adhesion strength and separation distance that are in good agreement with numerical results. In a planar extensional flow we find a stable vesicle…
The present study deals with the effect of interfacial slip on the deformation and emulsion rheology of a dilute suspension of droplets in a linear flow. The droplets are laden with surfactants that are bulk-insoluble and get transported only along the interface. An asymptotic approach is adopted for the present analysis in order to tackle the nonlinearity present due to deformation of droplets. The analysis is carried out under two different limiting scenarios namely: surface diffusion-dominated-surfactant transport and surface convection-dominated surfactant transport. For either of the limi…
A cutting-edge software is presented to tackle the Newton-Euler equations governing the dynamics of granular flows and dense suspensions in Newtonian fluids. In particular, we propose an implementation of a fixed-radius near neighbours search based on an efficient counting sort algorithm with an improved symmetric search. The adopted search method drastically reduces the computational cost and allows an efficient parallelisation even on a single node through the multi-threading paradigm. Emphasis is also given to the memory efficiency of the code since the history of the contacts among particl…
The dynamics of ideally polarizable spherical particles in concentrated suspensions under the effects of nonlinear electrokinetic phenomena is analysed using large-scale numerical simulations. Particles are assumed to carry no net charge and considered to undergo the combination of dielectrophoresis and induced-charge electrophoresis termed dipolophoresis. Chaotic motion and resulting hydrodynamic diffusion are known to be driven by the induced-charge electrophoresis, which dominates the dielectrophoresis. Up to a volume fraction $ϕ\approx 35\%$, the particle dynamics seems to be hindered by t…
We experimentally investigate the rheology and stress fluctuations of granules densely suspended in silicone oil. We find that both thickening strength and stress fluctuations significantly weaken with oil viscosity $η_0$. Comparison of our rheological results to the Wyart-Cates model for describing different dynamic jamming states suggests a transition from frictional contacts to lubrication interactions as $η_0$ increases. To clarify the contribution from viscous interactions to the rheology, we systematically measure stress fluctuations in various flow states. Reduction of stress fluctuatio…
Three-phase suspensions, of liquid that suspends dispersed solid particles and gas bubbles, are common in both natural and industrial settings. Their rheology is poorly constrained, particularly for high total suspended fractions ($\gtrsim 0.5$). We use a dam-break consistometer to characterize the rheology of suspensions of (Newtonian) corn syrup, plastic particles, and CO$_2$ bubbles. The study is motivated by a desire to understand the rheology of magma and lava. Our experiments are scaled to the volcanic system: they are conducted in the non-Brownian, non-inertial regime; bubble capillary …
Particle motion in non-Newtonian fluids can be markedly different than in Newtonian fluids. Here we look at the change in dynamics for a few problems involving rigid spherical particles in shear-thinning fluids in the absence of inertia. We give analytical formulas for sedimenting spheres, obtained by means of the reciprocal theorem, and demonstrate quantitively differences in comparison to a Newtonian fluid. We also calculate the first correction to the suspension viscosity, the Einstein viscosity, for a dilute suspension of spheres in a weakly shear-thinning fluid.
We study the impact between a plate and a drop of non-colloidal solid particles suspended in a Newtonian liquid, with a specific attention to the case when the particle volume fraction, $ϕ$, is close to - or even exceeds - the critical volume fraction, $ϕ_c$, at which the steady effective viscosity of the suspension diverges. We use a specific concentration protocol together with an accurate determination of $ϕ$ for each drop and we measure the deformation $β$ for different liquid viscosities, impact velocities and particle sizes. At low volume fractions, $β$ is found to follow closely an effe…
The response of a suspension under a variety of static or alternating external fields strongly depends on the equilibrium electric double layer that surrounds the colloidal particles in the suspension. The theoretical models for salt-free suspensions can be improved by incorporating non-uniform size effects and orientational ordering of water dipoles neglected in previous mean-field approaches, which are based on the Poisson-Boltzmann approach. Our model including non-uniform size effects and orientational ordering of water dipoles seems to have quite a promising effect because the model can p…
We investigate theoretically and experimentally how the hydrodynamically correlated lateral motion of particles in a suspension confined between two surfaces is affected by the suspension concentration. Despite the long range of the correlations (decaying as 1/r^2 with the inter-particle distance r), the concentration effect is present only at short inter-particle distances for which the static pair correlation is nonuniform. This is in sharp contrast with the effect of hydrodynamic screening present in unconfined suspensions, where increasing the concentration changes the prefactor of the lar…
In our recent work on concentrated suspensions of uniformly porous colloidal spheres with excluded volume interactions, a variety of short-time dynamic properties were calculated, except for the rotational self-diffusion coefficient. This missing quantity is included in the present paper. Using a precise hydrodynamic force multipole simulation method, the rotational self-diffusion coefficient is evaluated for concentrated suspensions of permeable particles. Results are presented for particle volume fractions up to 45%, and for a wide range of permeability values. From the simulation results an…
A concentrated, vertical monolayer of identical spherical squirmers, which may be bottom-heavy, and which are subjected to a linear shear flow, is modelled computationally by two different methods: Stokesian dynamics, and a lubrication-theory-based method. Inertia is negligible. The aim is to compute the effective shear viscosity and, where possible, the normal stress differences as functions of the areal fraction of spheres $ϕ$, the squirming parameter $β$ (proportional to the ratio of a squirmer's active stresslet to its swimming speed), the ratio $Sq$ of swimming speed to a typical speed of…
Blood is a complex suspension that demonstrates several non-Newtonian rheological characteristics such as deformation-rate dependency, viscoelasticity and yield stress. In this paper we outline some issues related to the non-Newtonian effects in blood circulation system and present modeling approaches based mostly on the past work in this field.
The stability of two-dimensional Poiseuille flow and plane Couette flow for concentrated suspensions is investigated. Linear stability analysis of the two-phase flow model for both flow geometries shows the existence of a convectively driven instability with increasing growth rates of the unstable modes as the particle volume fraction of the suspension increases. In addition it is shown that there exists a bound for the particle phase viscosity below which the two-phase flow model may become ill-posed as the particle phase approaches its maximum packing fraction. The case of two-dimensional Po…
A new two-phase model for concentrated suspensions is derived that incorporates a constitutive law combining the rheology for non-Brownian suspension and granular flow. The resulting model exhibits a yield-stress behavior for the solid phase depending on the collision pressure. This property is investigated for the simple geometry of plane Poiseuille flow, where an unyielded or jammed zone of finite width arises in the center of the channel. For the steady states of this problem, the governing equations are reduced to a boundary value problem for a system of ordinary differential equations and…
We give the first correction to the suspension viscosity due to fluid elasticity for a dilute suspension of spheres in a viscoelastic medium. Our perturbation theory is valid to $O(ϕ\mathrm{Wi}^2)$ in the Weissenberg number $\mathrm{Wi}=\dotγλ$, where $\dotγ$ is the typical magnitude of the suspension velocity gradient, and $λ$ is the relaxation time of the viscoelastic fluid. For shear flow we find that the suspension shear-thickens due to elastic stretching in strain hot spots near the particle, despite the fact that the stress inside the particles decreases relative to the Newtonian case. W…
We consider suspensions of deformable particles in a Newtonian fluid by means of fully Eulerian numerical simulations with a one-continuum formulation. We study the rheology of the visco-elastic suspension in plane Couette flow in the limit of vanishing inertia and examine the dependency of the effective viscosity $μ$ on the solid volume-fraction $Φ$, the capillary number $\mbox{Ca}$, and the solid to fluid viscosity ratio $\mbox{K}$. The suspension viscosity decreases with deformation and applied shear (shear-thinning) while still increasing with volume fraction. We show that $μ$ collapses to…
This paper reports experiments on the shear transient response of concentrated non-Brownian suspensions. The shear viscosity of the suspensions is measured using a wide-gap Couette rheometer equipped with a Particle Image Velocimetry (PIV) device that allows measuring the velocity field. The suspensions made of PMMA particles (31$μ$m in diameter) suspended in a Newtonian index- and density-matched liquid are transparent enough to allow an accurate measurement of the local velocity for particle concentrations as high as 50%. In the wide-gap Couette cell, the shear induced particle migration is …
