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arXiv 2103.13545cond-mat.str-elcond-mat.mtrl-sci
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质子插层CaRuO3中具有费米液体行为的突现铁磁性

Emergent ferromagnetism with Fermi-liquid behavior in proton intercalated CaRuO3

Shengchun Shen, Zhuolu Li, Zijun Tian, Weidong Luo, Satoshi Okamoto, Pu Yu

摘要:

关联电子系统中费米液态和非费米液态之间的相互作用是凝聚态物理的重要研究课题。探索非费米液体行为本质的一个有效途径是接近其相界。本文报道了金属CaRuO3在离子液体门控作用下,通过电场质子化,实现了从非费米液体到费米液体的转变。这种电子跃迁随后引发了一个可逆的磁跃迁,从这个顺磁性化合物中出现了一个奇异的铁磁态。我们的理论分析表明,氢掺入通过结构畸变和电子掺杂在电子和磁性相变中起着关键作用。这些观测结果不仅有助于理解钙钛矿双烯酸盐体系中相关的磁性和电子跃迁,而且为相关材料中电子相的设计提供了新的途径。

英文摘要:

The evolution between Fermi liquid and non-Fermi-liquid states in correlated electron systems has been a central subject in condensed matter physics because of the coupled intriguing magnetic and electronic states. An effective pathway to explore the nature of non-Fermi liquid behavior is to approach its phase boundary. Here we report a crossover from non-Fermi liquid to Fermi-liquid state in metallic CaRuO3 through ionic liquid gating induced protonation with electric field. This electronic transition subsequently triggers a reversible magnetic transition with the emergence of an exotic ferromagnetic state from this paramagnetic compound. Our theoretical analysis reveals that hydrogen incorporation plays a critical role in both the electronic and magnetic phase transitions via structural distortion and electron doping. These observations not only help understand the correlated magnetic and electronic transitions in perovskite ruthenate systems, but also provide novel pathways to design electronic phases in correlated materials.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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