Tuning of dipolar interactions and evaporative cooling in a three-dimensional molecular quantum gas
Jun-Ru Li, William G. Tobias, Kyle Matsuda, Calder Miller, Giacomo Valtolina, Luigi De Marco, Reuben R. W. Wang, Lucas Lassablière, Goulven Quéméner, John L. Bohn, Jun Ye
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Main text 27 pages (4+1 figures) + 8 pages Supplementary Information
Ultracold polar molecules possess long-range, anisotropic, and tunable dipolar interactions, providing the opportunities to probe quantum phenomena inaccessible with existing cold gas platforms. However, experimental progress has been hindered by the dominance of two-body loss over elastic interactions, which prevents efficient evaporative cooling. Though recent work has demonstrated controlled interactions by confining molecules to a two-dimensional geometry, a general approach for tuning molecular interactions in a three-dimensional (3D), stable system has been lacking. Here, we demonstrate tunable elastic dipolar interactions in a bulk gas of ultracold 40K87Rb molecules in 3D, facilitated by an electric field-induced shielding resonance which suppresses the reactive loss by a factor of thirty. This improvement in the ratio of elastic to inelastic collisions enables direct thermalization. The thermalization rate depends on the angle between the collisional axis and the dipole orientation controlled by an external electric field, a direct manifestation of the anisotropic dipolar interaction. We achieve evaporative cooling mediated by the dipolar interactions in three dimensions. This work demonstrates full control of a long-lived bulk quantum gas system with tunable long-range interactions, paving the way for the study of collective quantum many-body physics.
Atomic physics was revolutionized by the development of forced evaporative cooling: it led directly to the observation of Bose-Einstein condensation, quantum-degenerate Fermi gases, and ultracold optical lattice simulations of condensed matter phenomena. More recently, great progress has been made in the production of cold molecular gases, whose permanent electric dipole moment is expected to generate rich, novel, and controllable phases, dynamics, and chemistry in these ultracold systems. However, while many strides have been made in both direct cooling and cold-association techniques, evapor…
Recent experimental developments in the loading of ultracold KRb molecules into quasi-two-dimensional traps, combined with the ability to tune the ratio between elastic and loss (inelastic/reactive) collisions through application of an external electric field, are opening the door to achieving efficient evaporative cooling of reactive polar molecules. In this paper, we use Monte Carlo simulations and semianalytic models to study theoretically the experimental parameter regimes in which evaporative cooling is feasible under current trapping conditions. We investigate the effect of the anisotrop…
To achieve Bose-Einstein condensation, one may implement evaporative cooling by dynamically regulating the power of laser beams forming the optical dipole trap. We propose and experimentally demonstrate a protocol of Bayesian optimization of Bose-Einstein condensation via the evaporative cooling model. Applying this protocol, pure Bose-Einstein condensate of 87Rb with 2.4X10e4 atoms can be produced via evaporative cooling from the initial stage when the number of atoms is 6.0X10e5 at a temperature of 12μK. In comparison with Bayesian optimization via blackbox experiment, our protocol only need…
In this paper, we numerically studied the effects of mechanical vibration and magnetic fields on evaporative cooling process carried in space station by direct simulation Monte Carlo method. Simulated with the vibration data of international space station, we found that the cooling process would suffer great atomic losses until the accelerations reduced tenfold at least. In addition, if we enlarge the s-wave scattering length five times by Feshbach resonance, the PSD increased to 50 compared to 3 of no magnetic fields situation after 5 seconds evaporative cooling. We also simulated the two sta…
We report the realization of Bose-Einstein condensates of 39K atoms without the aid of an additional atomic coolant. Our route to Bose-Einstein condensation comprises Sub Doppler laser cooling of large atomic clouds with more than 10^10 atoms and evaporative cooling in optical dipole traps where the collisional cross section can be increased using magnetic Feshbach resonances. Large condensates with almost 10^6 atoms can be produced in less than 15 seconds. Our achievements eliminate the need for sympathetic cooling with Rb atoms which was the usual route implemented till date due to the unfav…
We demonstrate experimentally the evaporative cooling of a few hundred rubidium 87 atoms in a single-beam microscopic dipole trap. Starting from 800 atoms at a temperature of 125microKelvins, we produce an unpolarized sample of 40 atoms at 110nK, within 3s. The phase-space density at the end of the evaporation reaches unity, close to quantum degeneracy. The gain in phase-space density after evaporation is 10^3. We find that the scaling laws used for much larger numbers of atoms are still valid despite the small number of atoms involved in the evaporative cooling process. We also compare our re…
We present a combined computational and experimental study to optimize the efficiency of evaporative cooling for atoms in optical dipole traps. By employing a kinetic model of evaporation, we provide a strategy for determining the optimal relation between atom temperature, trap depth, and average trap frequency during evaporation given experimental initial conditions. We then experimentally implement a highly efficient evaporation process in an optical dipole trap, showing excellent agreement between the theory and experiment. This method has allowed the creation of pure Bose-Einstein condensa…
We calculate the evaporative cooling dynamics of trapped one-dimensional Bose-Einstein condensates for parameters leading to a range of condensates and quasicondensates in the final equilibrium state. We confirm that solitons are created during the evaporation process, but always eventually dissipate during thermalisation. The distance between solitons at the end of the evaporation ramp matches the coherence length in the final thermal state. Calculations were made using the classical fields method. They bridge the gap between the phase defect picture of the Kibble-Zurek mechanism and the long…
In recent years, cold atoms could prove their scientific impact not only on ground but in microgravity environments such as the drop tower in Bremen, sounding rockets and parabolic flights. We investigate the preparation of cold atoms in an optical dipole trap, with an emphasis on evaporative cooling under microgravity. Up to $ 1\times10^{6} $ rubidium-87 atoms were optically trapped from a temporarily dark magneto optical trap during free fall in the droptower in Bremen. The efficiency of evaporation is determined to be equal with and without the effect of gravity. This is confirmed using num…
Degenerate quantum gases are instrumental in advancing many-body quantum physics and underpin emerging precision sensing technologies. All state-of-the-art experiments use evaporative cooling to achieve the ultracold temperatures needed for quantum degeneracy, yet evaporative cooling is extremely lossy: more than 99.9% of the gas is discarded. Such final particle number limitations constrain imaging resolution, gas lifetime, and applications leveraging macroscopic quantum coherence. Here we show that atomic Bose gases can be cooled to quantum degeneracy using real-time feedback, an entirely ne…
We theoretically show how to obtain a long one-dimensional crystal near its quantum ground state. We rely on an evaporative cooling scheme applicable to many-body systems with nonzero-ranged interactions. Despite the absence of periodic potentials, the final state is a crystal which exhibits long-range spatial order. We describe the scheme thermodynamically, applying the truncated Boltzmann distribution to the collective excitations of the chain, and show that it leads to a novel quasi-equilibrium many-body state. For longer chains, comprising about 1000 atoms, we emphasize the quasi-universal…
We study depletion dynamics of an open system of weakly interacting fermions with two-body random interactions. In this model fermions are escaping from the high-energy one-particle orbitals, that mimics the evaporation process used in laboratory experiments with neutral atoms to cool them to ultra-low temperatures. It is shown that due to dynamical thermalization the system instantaneously adjusts to the new chemical potential and temperature, so that occupation numbers of the one-particle orbitals always obey the Fermi-Dirac distribution. In this way we are able to describe the evaporation p…
Semi-classical evaporative cooling: classical and quantum distributions
Centro de Investigación en Computación, Instituto Politénico Nacional（国家理工学院计算研究中心）；Facultad de Ciencias, Universidad Nacional Autónoma de México（墨西哥国立自治大学理学院）；Instituto de Química, Universidad Nacional Autónoma de México（墨西哥国立自治大学化学研究所）；Instituto de Física, Universidad Nacional Autónoma de México（墨西哥国立自治大学物理研究所）；Investigador por México - Instituto de Física, Universidad Nacional Autónoma de México（墨西哥研究者计划-墨西哥国立自治大学物理研究所）
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Bose-Einstein condensation (BEC) is a powerful tool for a wide range of research activities, a large fraction of which are related to quantum simulations. Various problems may benefit from different atomic species, but cooling down novel species interesting for quantum simulations to BEC temperatures requires a substantial amount of optimization and is usually considered as a hard experimental task. In this work, we implemented the Bayesian machine learning technique to optimize the evaporative cooling of thulium atoms and achieved BEC in an optical dipole trap operating near 532 nm. The devel…
