Kondo effect and spin-orbit coupling in graphene quantum dots
Annika Kurzmann, Yaakov Kleeorin, Chuyao Tong, Rebekka Garreis, Angelika Knothe, Marius Eich, Christopher Mittag, Carolin Gold, Folkert K. de Vries, Kenji Watan… 展开作者
Annika Kurzmann, Yaakov Kleeorin, Chuyao Tong, Rebekka Garreis, Angelika Knothe, Marius Eich, Christopher Mittag, Carolin Gold, Folkert K. de Vries, Kenji Watanabe, Takashi Taniguchi, Vladimir Fal'ko, Yigal Meir, Thomas Ihn, Klaus Ensslin
The Kondo effect is a cornerstone in the study of strongly correlated fermions. The coherent exchange coupling of conduction electrons to local magnetic moments gives rise to a Kondo cloud that screens the impurity spin. Whereas complete Kondo screening has been explored widely, realizations of the underscreened scenario - where only some of several Kondo channels participate in the screening - remain rare. Here we report the observation of fully screened and underscreened Kondo effects in quantum dots in bilayer graphene. More generally, we introduce a unique platform for studying Kondo physics. In contrast to carbon nanotubes, whose curved surfaces give rise to strong spin-orbit coupling breaking the SU(4) symmetry of the electronic states relevant for the Kondo effect, we study a nominally flat carbon material with small spin-orbit coupling. Moreover, the unusual two-electron triplet ground state in bilayer graphene dots provides a route to exploring the underscreened spin-1 Kondo effect.
The observation of the Kondo effect in quantum dots has provided new opportunities to finally observe the controversial Kondo screening cloud. We study how screening cloud effects appear in the conductance through a quantum wire containing a quantum dot when the length of the wire is comparable to the size of the screening cloud.
We demonstrate a tunable Kondo effect realized in small quantum dots. We can switch our dot from a Kondo impurity to a non-Kondo system as the number of electrons on the dot is changed from odd to even. We show that the Kondo temperature can be tuned by means of a gate voltage as a single-particle energy state nears the Fermi energy. Measurements of the temperature and magnetic field dependence of a Coulomb-blockaded dot show good agreement with predictions of both equilibrium and non-equilibrium Kondo effects.
Anderson impurity model for semiconductor quantum dot is extended to take into account both particle and hole branches of charge excitations. It is shown that in dots with even number of electrons where the Kondo effect is absent in the ground state, novel midgap excitonic states emerge in the energy spectrum due to Kondo-type shake-up processes. The relevance of the model to rare earth ions adsorbed on metallic surfaces is discussed.
Quantum dots in the quantum Hall regime can have pairs of single Slater determinant states that are degenerate in energy. We argue that these pairs of many body states may give rise to a Kondo effect which can be mapped into an ordinary Kondo effect in a fictitious magnetic field. We report on several properties of this Kondo effect using scaling and numerical renormalization group analysis. We suggest an experiment to investigate this Kondo effect.
We report theoretical investigations of indirectly coupled double quantum dots (QD) side connected to an one-dimensional quantum wire. Due to quantum interference controlled by the parameter $k_F L$, with $k_F$ the Fermi wave number of the wire and $L$ the distance between the two QDs, distinctly different Kondo resonances are predicted depending on the range of $k_F L$. A true bound Kondo states is found while an anomalous Kondo resonance gives rise to both reduction and enhancement of conductance.
We theoretically study enhancement mechanisms of the Kondo effect in multilevel quantum dots. In quantum dots fabricated on semiconductors, the energy difference between discrete levels Δis tunable by applying a magnetic field. With two orbitals and spin 1/2 in the quantum dots, we evaluate the Kondo temperature T_K as a function of Δ, using the scaling method. T_K is maximal around Δ=0 and decreases with increasing |Δ|, following a power law, T_K(Δ)=T_K(0) (T_K(0)/|Δ|)^γ, which is understood as a crossover from SU(4) to SU(2) Kondo effect. The exponents on both sides of a level crossing, γ_L …
We study two double dot systems, one with dots in parallel and one with dots in series, and argue they admit an exact solution via the Bethe ansatz. In the case of parallel dots we exploit the exact solution to extract the behavior of the linear response conductance. The linear response conductance of the parallel dot system possesses multiple Kondo effects, including a Kondo effect enhanced by a nonpertubative antiferromagnetic RKKY interaction, has conductance zeros in the mixed valence regime, and obeys a non-trivial form of the Friedel sum rule.
We have observed the Kondo effect in strongly coupled semiconducting nanowire quantum dots. The devices are made from indium arsenide nanowires, grown by molecular beam epitaxy, and contacted by titanium leads. The device transparency can be tuned by changing the potential on a gate electrode, and for increasing transparencies the effects dominating the transport changes from Coulomb Blockade to Universal Conductance Fluctuations with Kondo physics appearing in the intermediate region.
In this Letter we study thermoelectric effects in ultra small quantum dots. We study the behaviour of the thermopower, Peltier coefficient and thermal conductance both in the sequencial tunneling regime and in the regime where Kondo correlations develope. Both cases of linear response and non-equilibrium induced by strong temperature gradients are considered. The thermopower is a very sensitive tool to detect Kondo correlations. It changes sign both as a function of temperature and temperature gradient. We also discuss violations of the Wiedemann-Franz law.
We show that the numerical method [M.E. Torio, K. Hallberg, A.H. Ceccatto, and C.R. Proetto, Phys. Rev. B 65, 085302 (2002), cond-mat/0108167v2] does not reproduce correctly the Kondo physics in quantum dot systems with interaction.
The Kondo effect in coupled quantum dots is investigated theoretically under magnetic fields. We show that the magnetoconductance (MC) illustrates peak structures of the Kondo resonant spectra. When the dot-dot tunneling coupling $V_C$ is smaller than the dot-lead coupling $Δ$ (level broadening), the Kondo resonant levels appear at the Fermi level ($E_F$). The Zeeman splitting of the levels weakens the Kondo effect, which results in a negative MC. When $V_{C}$ is larger than $Δ$, the Kondo resonances form bonding and anti-bonding levels, located below and above $E_F$, respectively. We observe …
We systematically investigate electron transport through double quantum dots with particular emphasis on interference induced via multiple paths of electron propagation. By means of the slave-boson mean-field approximation, we calculate the conductance, the local density of states, the transmission probability in the Kondo regime at zero temperature. It is clarified how the Kondo-assisted transport changes its properties when the system is continuously changed among the serial, parallel and T-shaped double dots. The obtained results for the conductance are explained in terms of the Kondo reson…
The Kondo effect in coupled quantum dots is investigated from the viewpoint of transmission spectroscopy using the slave-boson formalism of the Anderson model. The antiferromagnetic spin-spin coupling $J$ between the dots is taken into account. Conductance $G$ through the dots connected in a series is characterized by the competition between the dot-dot tunneling coupling $V_{C}$ and the level broadening $Δ$ in the dots (dot-lead coupling). When $V_{C}/Δ< 1$, the Kondo resonance is formed between each dot and lead, which is replaced by a spin-singlet state in the dots at low gate voltages. The…
We have fabricated single electron tunneling structures by forming nanogap metallic electrodes directly upon single self-assembled InAs quantum dots (QDs). The fabricated samples exhibited clear Coulomb blockade effects. Furthermore, a clear Kondo effect was observed when strong coupling between the electrodes and the QDs was realized using a large QD with a diameter of ~ 100 nm. From the temperature dependence of the linear conductance at the Kondo valley, the Kondo temperature TK was determined to be ~ 81 K. This is the highest TK ever reported for artificial quantum nanostructures.
Exchange interaction within a quantum dot strongly affects the transport through it in the Kondo regime. In a striking difference with the results of the conventional model, where this interaction is neglected, here the temperature and magnetic field dependence of the conductance may become non-monotonic: its initial increase follows by a drop when temperature and magnetic field are lowered.
We analyze the full counting statistics (FCS) of quantum dots in the Kondo regime contacted by normal and superconducting leads or an STM tip. To describe the Kondo resonance we use an effective model for the quantum dot in the Kondo regime in combination with the FCS for tunneling contacts calculated using the Hamiltonian approach. We show that the situation of weak coupling to the superconducting electrode in the case of superconductor gap being larger than the Kondo resonance width can be easily handled and verify the method by comparing our theoretical predictions to experimental data. Thi…
We experimentally verify hitherto untested theoretical predictions about the thermoelectric properties of Kondo correlated quantum dots (QDs). The specific conditions required for this study are obtained by using QDs epitaxially grown in nanowires, combined with a recently developed method for controlling and measuring temperature differences at the nanoscale. This makes it possible to obtain data of very high quality both below and above the Kondo temperature, and allows a quantitative comparison with theoretical predictions. Specifically, we verify that Kondo correlations can induce a polari…
A path integral approach is used to derive a closed analytical expression for the Kondo temperature of the SU(4) symmetrical Anderson model. In contrast to the SU(2) case, the prefactor of the Kondo temperature is found to display a peculiar orbital energy (gate voltage) dependence, reflecting the presence of various SU(4) mixed valence fixed points. Our analytical expressions are tested against and confirmed by numerical renormalization group computations.
Properties of the Kondo effect in quantum dots depend sensitively on the coupling parameters and so on the realization of the quantum dot -- the Kondo temperature itself becomes a mesoscopic quantity. Assuming chaotic dynamics in the dot, we use random matrix theory to calculate the distribution of both the Kondo temperature and the conductance in the Coulomb blockade regime. We study two experimentally relevant cases: leads with single channels and leads with many channels. In the single-channel case, the distribution of the conductance is very wide as $T_K$ fluctuates on a logarithmic scale.…
We address a recent theoretical discrepancy concerning the Kondo effect in quantum dots with an even number of electrons where spin-singlet and -triplet states are nearly degenerate. We show that the discrepancy arises from the fact that the Kondo scaling involves many parameters, which makes the results depend on concrete microscopic models. We illustrate this by the scaling calculations of the Kondo temperature, $T_K$, as a function of the energy difference between the singlet and triplet states $Δ$. $T_K(Δ)$ decreases with increasing $Δ$, showing a crossover from a power law with a universa…
We study the interplay of the Kondo effect and spin-polarized tunneling in a class of systems exhibiting uniaxial magnetic anisotropy, such as magnetic molecules, magnetic adatoms, or quantum dots coupled to a single localized magnetic moment. Using the numerical renormalization group method we calculate the spectral functions and linear conductance in the Kondo regime. We show that the exchange coupling between conducting electrons and localized magnetic core generally leads to suppression of the Kondo effect. We also predict a nontrivial dependence of the tunnel magnetoresistance on the stre…
We review mechanisms of low-temperature electronic transport through a quantum dot weakly coupled to two conducting leads. Transport in this case is dominated by electron-electron interaction. At temperatures moderately lower than the charging energy of the dot, the linear conductance is suppressed by the Coulomb blockade. Upon further lowering of the temperature, however, the conductance may start to increase again due to the Kondo effect. We concentrate on lateral quantum dot systems and discuss the conductance in a broad temperature range, which includes the Kondo regime.
Strong electron correlations and interference effects are discussed in capacitively coupled side attached and embedded quantum dots. The finite - U mean field slave boson approach is used to study many-body effects. In the linear range the many-body resonances exhibit SU(4) Kondo or Kondo-Fano like character and their properties in the corresponding arms are close to the properties of embedded or T- shape double dot systems respectively. Breaking of the spin symmetry in one of the arms or in both allows for the formation of many-body resonances of SU(3) or SU(2) symmetries in the linear range.
We study the interaction between graphene and a single-molecule-magnet, [Fe4(L)2(dpm)6]. Focusing on the closest Iron ion in a hollow position with respect to the graphene sheet, we derive a channel selective tunneling Hamiltonian, that couples different d orbitals of the Iron atom to precise independent combinations of sublattice and valley degrees of freedom of the electrons in graphene. When looking at the spin-spin interaction between the molecule and the graphene electrons, close to the Dirac point the channel selectivity results in a channel decoupling of the Kondo interaction, with two …
We discuss the difficulties to discover Kondo effect in the resistivity of graphene. Similarly to the Kondo effect, electron-electron interaction effects and weak localization appear as logarithmic corrections to the resistance. In order to disentangle these contributions, a refined analysis of the magnetoconductance and the magnetoresistance is introduced. We present numerical simulations which display the discrimination of both effects. Further, we present experimental data of magnetotransport. When magnetic molecules are added to graphene, a logarithmic correction to the conductance occurs,…
We report measurements of the nonlinear conductance of InAs nanowire quantum dots coupled to superconducting leads. We observe a clear alternation between odd and even occupation of the dot, with sub-gap-peaks at $|V_{sd}|=Δ/e$ markedly stronger(weaker) than the quasiparticle tunneling peaks at $|V_{sd}|=2Δ/e$ for odd(even) occupation. We attribute the enhanced $Δ$-peak to an interplay between Kondo-correlations and Andreev tunneling in dots with an odd number of spins, and substantiate this interpretation by a poor man's scaling analysis.
We investigate the Kondo effect in a quadruple quantum dot device of coupled-double quantum dots (DQDs), which simultaneously contains intra-DQDs and inter-DQDs coupling. A variety of novel behaviors are observed. The differential conductance dI/dV is measured in the upper DQDs as a function of source drain bias. It is found to exhibit multiple peaks, including a zero-bias peak, where the number of peaks exceeds five. Alternatively, tuning the lower DQDs yielded regions of four peaks. In addition, a Kondo-effect switcher is demonstrated, using the lower DQDs as the controller.
We use co-tunneling spectroscopy to investigate spin-, orbital-, and spin-orbital Kondo transport in a strongly confined system of InAs double quantum dots (QDs) parallel-coupled to source and drain. In the one-electron transport regime, the higher symmetry spin-orbital Kondo effect manifests at orbital degeneracy and no external magnetic field. We then proceed to show that the individual Kondo contributions can be isolated and studied separately; either by orbital detuning in the case of spin-Kondo transport, or by spin splitting in the case of orbital Kondo transport. By varying the inter-do…
The out-of-equilibrium transport properties of a double quantum dot system in the Kondo regime are studied theoretically by means of a two-impurity Anderson hamiltonian with interimpurity hopping. The hamiltonian is solved by means of a non-equilibrium generalization of the slave-boson mean-field theory. It is demonstrated that measurements of the differential conductance dI/dV, for the appropriate values of voltages and tunneling couplings, can give a direct observation of the coherent superposition between the many-body Kondo states of each dot. For large voltages and arbitrarily large inter…
The Fano-Kondo effect in zero-bias conductance is investigated based on a theoretical model for the T-shaped quantum dot. The conductance as a function of the gate voltage is generally characterized by a Fano asymmetric parameter q. With varying temperature the conductance shows a crossover between the high and low temperature regions compared with the Kondo temperature T_K: two Fano asymmetric peaks at high temperatures and the Fano-Kondo plateau inside a Fano peak at low temperatures. Temperature dependence of conductance is calculated numerically by the Finite temperature density matrix ren…
We study magnetoconductance of the small bandgap carbon nanotube quantum dots in the presence of spin-orbit coupling in the strong correlations regime. The finite-U mean field slave boson approach is used to study many-body effects. Different degeneracies are restored in magnetic field and Kondo effects of different symmetries arise including SU(3) effects of different types. Full spin-orbital degeneracy might be recovered for zero field and correspondingly SU(4) Kondo effect sets in. We point out on the possibility of the occurrence of electron-hole Kondo effects in slanting magnetic fields, …
Electronic transport through a triple quantum dot system, with only a single dot coupled directly to external leads, is considered theoretically. The model includes Coulomb correlations in the central dot, while such correlations in the two side-coupled dots are omitted. The infinite-U mean-field slave-boson approach is used to obtain basic transport characteristics in the Kondo regime. When tuning position of the side-coupled dots' levels, transition from subradiant to superradiant like mode (and vice versa) has been found in the spectral function, in analogy to the Dicke effect in atomic phy…
We investigate quantum dots in clean single-wall carbon nanotubes with ferromagnetic PdNi-leads in the Kondo regime. In most odd Coulomb valleys the Kondo resonance exhibits a pronounced splitting, which depends on the tunnel coupling to the leads and an external magnetic field $B$, and only weakly on gate voltage. Using numerical renormalization group calculations, we demonstrate that all salient features of the data can be understood using a simple model for the magnetic properties of the leads. The magnetoconductance at zero bias and low temperature depends in a universal way on $g μ_B (B-B…
I reply to the new arguments of Muñoz et al. (arXiv:1308.0638) regarding our controversy on non-equilibrium Green functions of the impurity Anderson model, and to new unfounded criticism to my paper Ref. 1 (arXiv:1110.0816). In particular, I show that the lesser self energy given in Ref. 1 does satisfy a Ward identity. References are updated.
We report measurements consistent with the valley Kondo effect in Si/SiGe quantum dots, evidenced by peaks in the conductance versus source-drain voltage that show strong temperature dependence. The Kondo peaks show unusual behavior in a magnetic field that we interpret as arising from the valley degree of freedom. The interplay of valley and Zeeman splittings is suggested by the presence of side peaks, revealing a zero-field valley splitting between 0.28 to 0.34 meV. A zero-bias conductance peak for non-zero magnetic field, a phenomenon consistent with valley non- conservation in tunneling, i…
We consider electrons confined to a quantum dot interacting antiferromagnetically with a spin-$\half$ Kondo impurity. The electrons also interact among themselves ferromagnetically with a dimensionless coupling $\tilde{J}$, where $\tilde{J}=1$ denotes the bulk Stoner transition. We show that as $\tilde{J}$ approaches 1 there is a regime with enhanced Kondo correlations, followed by one where the Kondo effect is destroyed and impurity is spin polarized opposite to the dot electrons. The most striking signature of the first, Stoner-enhanced Kondo regime, is that a Zeeman field increases the Kond…
We study the conductance of an electron interferometer formed in a two dimensional electron gas between a nanostructured quantum contact and the charged tip of a scanning gate microscope. Measuring the conductance as a function of the tip position, thermally induced rings may be observed in addition to Fabry-Pérot interference fringes spaced by half the Fermi wavelength. If the contact is made of a quantum dot opened in the middle of a Kondo valley, we show how the location of the rings allows to measure by electron interferometry the magnetic moment of the dot above the Kondo temperature.
We study the spin-resolved transport through single-level quantum dots strongly coupled to ferromagnetic leads in the Kondo regime, with a focus on contact and material asymmetry-related effects. By using the numerical renormalization group method, we analyze the dependence of relevant spectral functions, linear conductance and tunnel magnetoresistance on the system asymmetry parameters. In the parallel magnetic configuration of the device the Kondo effect is generally suppressed due to the presence of exchange field, irrespective of system's asymmetry. In the antiparallel configuration, on th…
Spin-polarized transport through a quantum dot strongly coupled to ferromagnetic electrodes with non-collinear magnetic moments is analyzed theoretically in terms of the non-equilibrium Green function formalism. Electrons in the dot are assumed to be coupled to a phonon bath. The influence of electron-phonon coupling on tunnelling current, linear and nonlinear conductance, and on tunnel magnetoresistance is studied in detail. Variation of the main Kondo peaks and phonon satellites with the angle between magnetic moments of the leads is analyzed.
We investigate the effects induced by spin polarization in the contacts attached to a serial double quantum dot. The polarization generates effective magnetic fields and suppresses the Kondo effect in each dot. The super-exchange interaction ($J_{\mathrm{AFM}}$), tuned by the inter-dot tunnelling rate $t$, can be used to compensate the effective fields and restore the Kondo resonance when the contact polarizations are aligned. As a consequence, the direction of the spin conductance can be controlled and even reversed using electrostatic gates alone. Furthermore, we study the associated two-imp…
Many-body entanglement is at the heart of the Kondo effect, which has its hallmark in quantum dots as a zero-bias conductance peak at low temperatures. It signals the emergence of a conducting singlet state formed by a localized dot degree of freedom and conduction electrons. Carbon nanotubes offer the possibility to study the emergence of the Kondo entanglement by tuning many-body correlations with a gate voltage. Here we quantitatively show an undiscovered side of Kondo correlations, which counterintuitively tend to block conduction channels: inelastic cotunneling lines in the magnetospectru…
In this article, we review recent work about time dependent quantum transport through a quantum dot in Kondo regime. This represents a major step towards designing next generation transistors that are expected to replace current MOSFET's in a few years. We first discuss the effects of the density of states of gold contacts on the instantaneous conductance of an asymmetrically coupled quantum dot that is abruptly moved into Kondo regime via a gate voltage. Next, we investigate the effect of strong electron-phonon coupling on the dot on the instantaneous conductance. Finally, we discuss thermoel…
Magnetic impurity adsorbed on one of the carbon planes of a bilayer graphene is studied. The formation of the many-body SU(2) and SU(4) resonances close to the bandgap is analyzed within the mean field Kotliar-Ruckenstein slave boson approach. Impact of enhanced hybridization and magnetic instability of bilayer doped near the Van Hove singularity on the screening of magnetic moment is discussed.
We present lateral transport measurements on strongly, vertically coupled quantum dots formed in separate quantum wells in a GaAs/AlGaAs heterostructure. Coulomb oscillations are observed forming a honeycomb lattice consistent with two strongly coupled dots. When the tunnel barriers in the upper well are reduced we observe the Fano effect due to the interfering paths through a resonant state in the lower well and a continuum state in the upper well. In both regimes an in plane magnetic field reduces the coupling between the wells when the magnetic length is comparable to the center to center s…
We investigate the enhancement of the Kondo effect in quantum dots with an even number of electrons, using a scaling method and a mean field theory. We evaluate the Kondo temperature $T_K$ as a function of the energy difference between spin-singlet and triplet states in the dot, $Δ$, and the Zeeman splitting, $E_Z$. If the Zeeman splitting is small, $E_Z \ll T_K$, the competition between the singlet and triplet states enhances the Kondo effect. $T_K$ reaches its maximum around $Δ=0$ and decreases with $Δ$ obeying a power law. If the Zeeman splitting is strong, $E_Z \gg T_K$, the Kondo effect o…
We analyze the interactions between two Kondo Quantum Dots connected to a Rashba-active Quantum Wire. We find that the Kondo-doublet interaction, at an inter-dot distance of the order of the wire Fermi length, is over an order of magnitude greater than the RKKY interaction. The effects induced on the Kondo-doublet interaction by the wire spin-orbit coupling can be used to control the Quantum Dots spin-spin correlation. These results imply that the widely used assumption that the RKKY is the dominant interaction between Anderson impurities must be revised.
Low temperature zero-bias conductance through two side-coupled quantum dots is investigated using Wilson's numerical renormalization group technique. A low-temperature phase diagram is computed. Near the particle-hole symmetric point localized electrons form a spin-singlet associated with weak conductance. For weak inter-dot coupling we find enhanced conductance due to the two-stage Kondo effect when two electrons occupy quantum dots. When quantum dots are populated with a single electron, the system enters Kondo regime with enhanced conductance. Analytical expressions for the width of the Kon…
Based on ab-initio calculations we discuss Kondo effect due to Co adatom on graphene zigzag nanoribbon. Co atom located at hollow site behaves as spin S = 1/2 impurity with dxz and dyz orbitals contributing to magnetic moment. Dynamical correlations are analyzed with the use of complementary approximations: mean field slave boson approach, noncrossing approximation and equation of motion method. The impact of interplay between spin and orbital degrees of freedom together with the effect of peculiarities of electronic and magnetic structure of nanoribbon on many-body resonances is examined.
We analyze the transport properties of a double quantum dot device in the side-coupled configuration. A small quantum dot (QD), having a single relevant electronic level, is coupled to source and drain electrodes. A larger QD, whose multilevel nature is considered, is tunnel-coupled to the small QD. A Fermi liquid analysis shows that the low temperature conductance of the device is determined by the total electronic occupation of the double QD. When the small dot is in the Kondo regime, an even number of electrons in the large dot leads to a conductance that reaches the unitary limit, while fo…
Anderson's orthogonality catastrophe in graphene, at energies close to the Dirac point, is analyzed. It is shown that, in clean systems, the orthogonality catastrophe is suppressed, due to the vanishing density of states at the Dirac point. In the presence of preexisting localized states at the Dirac energy, the orthogonality catastrophe shows similar features to those found in normal metals with a finite density of states at the Fermi level. The implications for the Kondo effect induced by magnetic impurities, and for the Fermi edge singularities in tunneling processes are also discussed.
Strong electron correlations and interference effects are discussed in parallel-coupled single-level and orbitally doubly degenerate quantum dots. The finite-U mean-field slave boson approach is used to study many-body effects. The analysis is carried out in a wide range of parameter space including both atomic-like and molecular-like Kondo regimes and taking into account various perturbations, like interdot tunneling, interdot interaction, mixing of the electrode channels and exchange interaction. We also discuss the influence of singularities of electronic structure and the impact of polariz…
We calculate the conductance through strongly correlated T-shaped molecular or quantum dot systems under the influence of phonons. The system is modelled by the extended Anderson-Holstein Hamiltonian. The finite-U mean-field slave boson approach is used to study many-body effects. Phonons influence both interference and correlations. Depending on the dot unperturbed energy and the strength of electron-phonon interaction the system is occupied by a different number of electrons which effectively interact with each other repulsively or attractively. This leads together with the interference effe…
We demonstrate delicate control over the Kondo effect and its interplay with quantum interference in an Aharonov-Bohm interferometer containing one Kondo dot and one noninteracting dot. It is shown that the Kondo resonance undergoes a dramatic evolution as the interdot tunnel coupling progressively increases. A novel triple Kondo splitting occurs from the interference between constant and Lorentzian conduction bands that cooperate in forming the Kondo singlet. The device also manifests a highly controllable Fano-Kondo effect in coherent electronic transport, and can be tuned to a regime where …
We explore the finite bias DC differential conductance of a correlated quantum dot under the influence of an AC field, from the low-temperature Kondo to the finite temperature Coulomb blockade regime. Real-time simulations are performed using a time-dependent generalization of the steady-state density functional theory (i-DFT) [Nano Lett. {\bf 15}, 8020 (2015)]. The numerical simplicity of i-DFT allows for unprecedented long time evolutions. Accurate values of average current and density are obtained by integrating over several periods of the AC field. We find that (i) the zero-temperature Kon…
We investigate electronic transport through parallel double quantum dot(DQD) system with strong on-site Coulomb interaction and capacitive interdot coupling. By applying numerical renormalization group(NRG) method, the ground state of the system and the transmission probability at zero temperature have been obtained. For a system of quantum dots with degenerate energy levels and small interdot tunnel coupling, the spin correlations between the DQDs is ferromagnetic, and the ground state of the system is a spin 1 triplet state. The linear conductance will reach the unitary limit ($2e^2/h$) due …
We present a general description of low temperature transport through a quantum dot with any number of electrons at filling factor $1<ν<2$. We provide a general description of a novel Kondo effect which is turned on by application of an appropriate magnetic field. The spin-flip scattering of carriers by the quantum dot only involves two states of the scatterer which may have a large spin. This process is described by spin-flip Hubbard operators, which change the angular momentum, leading to a Kondo Hamiltonian. We obtain antiferromagnetic exchange couplings depending on tunneling amplitudes an…
Quantum dots connected to larger systems containing a continuum of states like charge reservoirs allow the theoretical study of many-body effects such as the Coulomb blockade and the Kondo effect. Here, we analyze the nonequilibrium Kondo effect and transport phenomena in a quantum dot coupled to pure monolayer graphene electrodes under external magnetic fields for finite on-site Coulomb interaction. The system is described by the pseudogap Anderson Hamiltonian. We use the equation of motion technique to determine the retarded Green's function of the quantum dot. An analytical formula for the …
We study the Kondo effect in a quantum dot which is coupled to ferromagnetic leads and analyse its properties as a function of the spin polarization of the leads. Based on a scaling approach we predict that for parallel alignment of the magnetizations in the leads the strong-coupling limit of the Kondo effect is reached at a finite value of the magnetic field. Using an equation-of-motion technique we study nonlinear transport through the dot. For parallel alignment the zero-bias anomaly may be split even in the absence of an external magnetic field. For antiparallel spin alignment and symmetri…
Orbital Kondo effect in a system of two single-level quantum dots attached to external electron reservoirs is considered theoretically. The dots are coupled via direct hoping term and Coulomb interaction. The Kondo temperature is evaluated from the scaling approach and slave boson technique. The later method is also used to calculate linear conductance of the system. Nonlinear conductance, in turn, is calculated in terms of the nonequilibrium Green function formalism.
