We propose experimental measurements of the logarithmic negativity, which quantifies quantum correlations using Gouy phase measurements in an asymmetric double-slit interference experiment for twin photons. This is possible because both quantities have analogous dependence with the spatial confinement by the slits and enables one to manipulate the portion of entanglement by the Gouy phase. In order to obtain those measurements, we need to work in a regime where the position correlations between particles are strong, therefore we investigate such correlations for biphotons. Since we would like to handle entanglement quantifiers through the Gouy phase, we analyze the Gouy phase difference for two entangled photons in an asymmetric double-slit interference experiment.
Using a basic Mach-Zehnder interferometer, we demonstrate experimentally the measurement of the photonic de Broglie wavelength of an entangled photon pair (a biphoton) generated by spontaneous parametric down-conversion. The observed interference manifests the concept of the photonic de Broglie wavelength. The result also provides a proof-of-principle of the quantum lithography that utilizes the reduced interferometric wavelength.
We verified operational approach based on direct measurement of entanglement degree for bipartite systems. In particular spectral distributions of single counts and coincidence for pure biphoton states generated by train of short pump pulses have been measured and entanglement quantifier calculated. The approach gives upper bound of entanglement stored in total biphoton states, which can reach extremely high value up to $10^{4}-10^{5}$.
We analyze spontaneous parametric down-conversion in various experimentally feasible 1D quadratic nonlinear waveguide arrays, with emphasis on the relationship between the lattice's topological invariants and the biphoton correlations. Nontrivial topology results in a nontrivial "winding" of the array's Bloch waves, which introduces additional selection rules for the generation of biphotons. These selection rules are in addition to, and independent of existing control using the pump beam's spatial profile and phase matching conditions. In finite lattices, nontrivial topology produces single ph…
We show that the wave packet of a biphoton generated via spontaneous parametric down conversion is strongly anisotropic. Its anisotropic features manifest themselves very clearly in comparison of measurements performed in two different schemes: when the detector scanning plane is perpendicular or parallel to the plane containing the crystal optical axis and the laser axis. The first of these two schemes is traditional whereas the second one gives rise to such unexpected new results as anomalously strong narrowing of the biphoton wave packet measured in the coincidence scheme and very high degr…
Spontaneous parametric down-conversion (SPDC) is a widely used source for photonic entanglement. Years of focused research have led to a solid understanding of the process, but a cohesive analytical description of the paraxial biphoton state has yet to be achieved. We derive a general expression for the spatio-temporal biphoton state that applies universally across common experimental settings and correctly describes the non-separability of spatial and spectral modes. We formulate a criterion on how to decrease the coupling of the spatial from the spectral degree of freedom by taking into acco…
The nonlinear optical process of spontaneous parametric down-conversion (SPDC) is widely studied for applications in quantum information science due to its ability to produce two photons that can be entangled in many degrees of freedom. For applications in quantum communication, two metrics of this process are particularly important: heralding efficiency and total joint rate. Here, we derive expressions for both quantities for a variety of different beam geometries and frequencies. We pay specific attention to the spectrum of both biphotons and individual photons. We reveal the underlying mech…
As a tutorial to the spatial aspects of Spontaneous Parametric Downconversion (SPDC), we present a detailed first-principles derivation of the transverse correlation width of photon pairs in degenerate collinear SPDC. This width defines the size of a biphoton birth zone, the region where the signal and idler photons are likely to be found when conditioning on the position of the destroyed pump photon. Along the way, we discuss the quantum-optical calculation of the amplitude for the SPDC process, as well as its simplified form for nearly collinear degenerate phase matching. Following this, we …
Analytical expressions are derived for the distribution rates of spatial coincidences in the counting of photons produced by spontaneous parametric down conversion (SPDC). Gaussian profiles are assumed for the wave function of the idler and signal light created in type-I SPDC. The distribution rates describe ellipses on the detection planes that are oriented at different angles according to the photon coincidences in either horizontal-horizontal, vertical-vertical, horizontal-vertical or vertical-horizontal position variables. The predictions are in agreement with the experimental data obtaine…
We calculate the properties of a biphoton source based on resonant backward-wave spontaneous parametric down-conversion. We show that the biphotons are generated in a single longitudinal mode having a subnatural linewidth and a Glauber correlation time exceeding 65 ns.
We provide a toolbox for continuous variables quantum state engineering and characterization of biphoton states produced by spontaneous parametric down conversion in a transverse pump configuration. We show that the control of the pump beam's incidence spot and angle corresponds to phase space displacements of conjugate collective continuous variables of the biphoton. In particular, we illustrate with numerical simulations on a semiconductor device how this technique can be used to engineer and characterize arbitrary states of the frequency and time degrees of freedom.
Polarization state of biphoton light generated via collinear frequency-degenerate spontaneous parametric down-conversion is considered. A biphoton is described by a three-component polarization vector, its arbitrary transformations relating to the SU(3) group. A subset of such transformations, available with retardation plates, is realized experimentally. In particular, two independent orthogonally polarized beams of type-I biphotons are transformed into a beam of type-II biphotons. Polarized biphotons are suggested as ternary analogs of two-state quantum systems (qubits).
A double-Gaussian model and the Schmidt modes are found for the biphoton wave function characterizing spontaneous parametric down-conversion with the degenerate collinear phase-matching of the type I and with a pulsed pump. The obtained results are valid for all durations of the pump pulses, short, long and intermediately long.
We study the theory of linearly chirped biphoton wave-packets produced in two basic quasi-phase-matching configurations: chirped photonic-like crystals and aperiodically poled crystals. The novelty is that these structures are considered as definite assembles of nonlinear layers that leads to detailed description of spontaneous parametric down-conversion (SPDC) processes through the discrete Gauss sums. We demonstrate that biphoton spectra for chirped photonic crystals involving a small number of layers consist from definite well-resolved spectral lines. We also discuss the forming of broadban…
In this paper, we investigate the influence of the symmetry of the biphoton wavefunction on the coincidence measurement of the generalized Mach-Zehnder (MZ) interferometer, where there are a temporal and frequency shift operations between the two beam-splitters. We show that the generalized MZ interferometer is the measurement of the short-time Fourier transform of the function modeling the energy conservation of a spontaneous parametric down-conversion process if the full biphoton state is symmetric, and of the symmetric characteristic distribution of the phase-matching function if the state …
We show that broadband biphoton wavepackets produced via Spontaneous Parametric Down-Conversion (SPDC) in crystals with linearly aperiodic poling can be easily compressed in time using the effect of group-velocity dispersion in optical fibres. This result could foster important developments in quantum metrology and lithography.
We consider a double Gaussian approximation to describe the wavefunction of twin photons (also called a biphoton) created in a nonlinear crystal via a type-I spontaneous parametric downconversion (SPDC) process. We find that the wavefunction develops a Gouy phase while it propagates, being dependent of the two-photon correlation through the Rayleigh length. We evaluate the covariance matrix and show that the logarithmic negativity, useful in quantifying entanglement in Gaussian states, although Rayleigh-dependent, does not depend on the propagation distance. In addition, we show that the two-p…
Quantum correlations encoded in photonic Laguerre-Gaussian modes were shown to be related to the Gouy phase shifts (D. Kawase et al., Phys. Rev. Lett. 101, 050501 (2008)) allowing for a non-destructive manipulation of photonic quantum states. In this work we exploit the relation between phase space correlations of biphotons produced by spontaneously parametric down conversion (SPDC) as encoded in the logarithmic negativity (LN) and the Gouy phase as they are diffracted through an asymmetrical double slit setup. Using an analytical approach based on a double-gaussian approximation for type-I SP…
Spectral and temporal coincidence and single-particle photon wave packets are described and their widths and durations are found. The degree of entanglement is characterized by the experimentally measurable parameter R defined as the ratio of the coincidence and single-particle spectral widths. In the frequency representation, this parameter is found as a function of the pump-pulse duration. This function is shown to have a minimum and even in the minimum, at rather natural conditions, the parameter R is found to be very high (R=73>>1). The Schmidt number K is found for both short and long pum…
We utilized the all-copropagating scheme, which maintains the phase-match condition, in the spontaneous four-wave mixing (SFWM) process to generate biphotons from a hot atomic vapor. The scheme enables our biphotons not only to surpass those in the previous works of hot-atom SFWM, but also to compete with the biphotons that are generated by either the cold-atom SFWM or the cavity-assisted spontaneous parametric down conversion. The biphoton linewidth in this work is tunable for an order of magnitude. As we tuned the linewidth to 610 kHz, the maximum two-photon correlation function, $g_{s,as}^{…
In this work we study the spatio-temporal correlations of photons produced by spontaneous parametric down conversion. In particular, we study how the waists of the detection and pump beams impact on the spectral bandwidth of the photons. Our results indicate that this parameter is greatly affected by the spatial properties of the detection beam, while not as much by the pump beam. This allows for a simple experimental implementation to control the bandwidth of the biphoton spectra, which only entails modifying the optical configuration to collect the photons. Moreover, we have performed Hong-O…
We demonstrate one- and two-photon diffraction and interference experiments utilizing parametric down-converted photon pairs (biphotons) and a transmission grating. With two-photon detection, the biphoton exhibits a diffraction-interference pattern equivalent to that of an effective single particle that is associated with half the wavelength of the constituent photons. With one-photon detection, however no diffraction-interference pattern is observed. We show that these phenomena originate from the spatial quantum correlation between the down-converted photons.
We report on controlling the bi-photon orbital angular momentum (OAM) eigenmodes in the spontaneous parametric down conversion process by simply adjusting the asymmetry of the pump vortex beam. Adjusting the optic axis of the spiral phase plate (SPP) of phase winding corresponding to OAM mode, l, with respect to the beam propagation axis, we have transformed a Gaussian beam into an asymmetric vortex beam with OAM modes, l, l-1, l-2, 0 with different weightages. Pumping the nonlinear crystal with such asymmetric vortices and controlling their asymmetry we have tailored the spiral spectrum of th…
Indistinguishable single photons are key ingredient for a plethora of quantum information processing applications ranging from quantum communications to photonic quantum computing. A mainstream platform to produce indistinguishable single photons over a wide spectral range is based on biphoton generation through spontaneous parametric down-conversion (SPDC) in nonlinear crystals. The purity of the SPDC biphotons, however, is limited by their spectral correlations. Here, we present a design recipe, based on a machine-learning framework, for the engineering of biphoton joint spectrum amplitudes …
High-dimensional biphoton states are promising resources for quantum applications, ranging from high-dimensional quantum communications to quantum imaging. A pivotal task is fully characterising these states, which is generally time-consuming and not scalable when projective measurement approaches are adopted. However, new advances in coincidence imaging technologies allow for overcoming these limitations by parallelising multiple measurements. Here, we introduce biphoton digital holography, in analogy to off-axis digital holography, where coincidence imaging of the superposition of an unknown…
We describe spontaneous parametric down-conversion experiments in which induced coherence across two coupled interferometers results in high-visibility single-photon interference. Opening additional photon channels allows "which-path" information and reduces the visibility of the singlephoton interference, but results in nearly perfect visibility when photons are counted in coincidence. A simplified theoretical model accounts for these complementary observations and attributes them directly to the relations among the vacuum fields at the different crystals.
We report results of two-photon quantum holography where spatial information stored in phase holograms is retrieved by measuring quantum spatial correlations between two images formed by spatially entangled twin photons with a dimensionality of 1790 in the two-dimensional transverse space. In our experiments, the entire flux of spontaneous down converted photons illuminates the phase holograms and the photons of pairs signal-idler transmitted by the holograms are detected separately in far field on two electron-multiplying charge coupled device cameras.
In this work, we present a theoretical and experimental study about the spatial correlations of paired photons generated by type-II spontaneous parametric down-conversion. In particular, we show how these correlations can be positive or negative depending on the direction in which the far field plane is scanned and the polarization post-selected. Our results provide a straightforward way to observe different kind of correlations, that complement other well known methods to tune the spatial correlations of paired photons.
We demonstrate the generation of narrowband biphotons with polarization-frequency coupled hy- perentanglement from spontaneous four-wave mixing in cold atoms. The coupling between polariza- tion and frequency is realized through a frequency shifter and linear optics. When the polarization- frequency degrees of freedom are decoupled, it is robust to create polarization and frequency Bell states, confirmed by the polarization quantum-state tomography and the two-photon temporal quan- tum beating. Making use of the polarization-frequency coupling to transfer polarization phase retard to the entan…
We report a scalable linear optical scheme for generating entangled states of multiple ququarts in which the individual single-ququart state is prepared with the biphoton polarization state of frequency-nondegenerate spontaneous parametric down-conversion. The output state is calculated with the full consideration of the higher order effect (double-pair events) of spontaneous parametric down-conversion. Scalability to multiple-ququart entanglement is demonstrated with examples: linear optical entanglement of three and four individual biphoton ququarts.
We theoretically investigate the preparation of mid-infrared (MIR) spectrally-uncorrelated biphotons from a spontaneous parametric down-conversion process using doped LN crystals, including MgO doped LN, ZnO doped LN, and In2O3 doped ZnLN with doping ratio from 0 to 7 mol%. The tilt angle of the phase-matching function and the corresponding poling period are calculated under type-II, type-I, and type-0 phase-matching conditions. We also calculate the thermal properties of the doped LN crystals and their performance in Hong-Ou-Mandel interference. It is found that the doping ratio has a substan…
Biphotons of narrow bandwidth and long temporal length play a crucial role in long-distance quantum communication (LDQC) and linear optical quantum computing (LOQC). However, generation of these photons usually requires atomic ensembles with high optical depth or spontaneous parametric down-conversion with sophisticated optical cavity. By manipulating the two-component biphoton wavefunction generated from a low-optical-depth (low-OD) atomic ensemble, we demonstrate biphotons with subnatural linewidth in the sub-MHz regime. The potential of shaping and manipulating the quantum wavepackets of th…
We present the first observation of two-photon polarization interference structure in the second-order Glauber's correlation function of two-photon light generated via type-II spontaneous parametric down-conversion. In order to obtain this result, two-photon light is transmitted through an optical fibre and the coincidence distribution is analyzed by means of the START-STOP method. Beyond the experimental demonstration of an interesting effect in quantum optics, these results also have considerable relevance for quantum communications.
We systematically studied the temporal profile of biphotons, i.e., pairs of time-correlated single photons, generated from a hot atomic vapor via the spontaneous four-wave mixing process. The measured temporal width of biphoton wave packet or two-photon correlation function against the coupling power was varied from about 70 to 580 ns. We derived an analytical expression of the biphoton's spectral profile in the Doppler-broadened medium. The analytical expression reveals that the spectral profile is mainly determined by the effect of electromagnetically induced transparency (EIT), and behaves …
In spontaneous parametric down-conversion photons are known to be created coherently and with equal probability over the entire length of the crystal. Then, there is no particular position in the crystal where a photon pair is created. We make the seemingly contradictory observation that we can control the time delay with the crystal position along the propagation direction. We resolve this contradiction by showing that the spatio-temporal correlations critically affect the temporal properties of the pair of photons, when using a finite detector size. We expect this to have important implicati…
We investigate the transverse spatial profile of down-converted light produced by noncollinear, degenerate, Type-I spontaneous parametric down-conversion in two types of nonlinear crystals. We find that the pattern produced by one crystal, beta barium borate (BBO), produces a circular down-conversion pattern while the other crystal, bismuth triborate (BiBO) produces an elliptical pattern. We show this difference is due to the angle-independent refractive index experienced by the daughter photons in BBO, while they experience an angle-dependent refractive index in BiBO. We image the transverse …
We measure the transverse entanglement of photon pairs on their propagation from the near to the far field of spontaneous parametric downconversion (SPDC). The Fedorov ratio, depending on the widths of conditional and unconditional intensity measurements, is shown to be only able to characterize entanglement in the near and far field zones of the source. Therefore we also follow a different approach. By evaluating the first-order coherence of a subsystem of the state we can quantify its entanglement. Unlike previous measurements, which determine the Fedorov ratio via intensity correlations, ou…
As a tutorial, we examine the absolute brightness and number statistics of photon pairs generated in Spontaneous Parametric Down-Conversion (SPDC) from first principles. In doing so, we demonstrate how the diverse implementations of SPDC can be understood through a single common framework, and use this to derive straightforward formulas for the biphoton generation rate (pairs per second) in a variety of different circumstances. In particular, we consider the common cases of both collimated and focused gaussian pump beams in a bulk nonlinear crystal, as well as in nonlinear waveguides and micro…
3D imaging of the biphoton spatiotemporal wave packet
University of Science and Technology of China（中国科学技术大学）；Laboratory of Quantum Information, University of Science and Technology of China（中国科学技术大学量子信息实验室）；Anhui Province Key Laboratory of Quantum Network, University of Science and Technology of China（中国科学技术大学安徽省量子网络重点实验室）；CAS Center for Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China（中国科学技术大学中科院量子信息与量子物理卓越创新中心）；Hefei National Laboratory, University of Science and Technology of China（中国科学技术大学合肥国家实验室）
The requirement on the symmetry of the biphoton wave function results in a double peak structure of the coincidence spectra of Spontaneous Parametric Down Conversion (SPDC) [1]. In this work we report the experimental observation of this effect by careful tailoring parameters of the SPDC crystal, the ultra-fast pump laser, and the measurement setup. The results are shown to be relevant to quantum state engineering of ultra-fast polarization-, or frequency-entangled mixed states.
We show that, when the integration time of the single photon detectors is longer than the correlation time of the biphoton, the attainable spatial resolution in ghost imaging with entangled signal idler pairs generated in type II spontaneous parametric down conversion is limited by the angular spread of single-frequency-signal idler pairs. If, however, the detector integration time is shorter than the biphoton correlation time, the transverse k-vectors of different spectral components combine coherently in the image, improving the spatial resolution.
Spontaneous parametric down conversion has been shown to be a reliable source of entangled photons. Amongst the wide range of properties that have been shown to be entangled, it is the orbital angular momentum that is the focus of our study. We investigate, in particular, the bi-photon state generated using a Gaussian pump beam. We derive an expression for the simultaneous correlations in the orbital angular momentum and radial momentum of the down-converted Laguerre-Gaussian beams. Our result allows us, for example, to calculate the spiral bandwidth with no restriction on the geometry of the …
We demonstrate Einstein-Podolsky-Rosen (EPR) entanglement by detecting purely spatial quantum correlations in the near and far fields of spontaneous parametric down-conversion generated in a type-2 beta barium borate crystal. Full-field imaging is performed in the photon-counting regime with an electron-multiplying CCD camera. The data are used without any postselection, and we obtain a violation of Heisenberg inequalities with inferred quantities taking into account all the biphoton pairs in both the near and far fields by integration on the entire two-dimensional transverse planes. This ensu…
We report a proof-of-principle experiment demonstrating that appropriately chosen set of Hermite-Gaussian modes constitutes a Schmidt decomposition for transverse momentum states of biphotons generated in the process of spontaneous parametric down conversion. We experimentally realize projective measurements in Schmidt basis and observe correlations between appropriate pairs of modes. We perform tomographical state reconstruction in the Schmidt basis, by direct measurement of single-photon density matrix eigenvalues.
We study first-order interference in spontaneous parametric down-conversion generated by two pump pulses that do not overlap in time. The observed modulation in the angular distribution of the signal detector counting rate can only be explained in terms of a quantum mechanical description based on biphoton states. The condition for observing interference in the signal channel is shown to depend on the parameters of the idler radiation.
