A semiclassical theory for the orbital magnetization due to adiabatic evolutions of Bloch electronic states is proposed. It renders a unified theory for the periodic-evolution pumped orbital magnetization and the orbital magnetoelectric response in insulators by revealing that these two phenomena are the only instances where the induced magnetization is gauge invariant. This theory also accounts for the electric-field induced intrinsic orbital magnetization in two-dimensional metals and Chern insulators. We illustrate the orbital magnetization pumped by microscopic local rotations of atoms, which correspond to phonon modes with angular momentum, in toy models based on honeycomb lattice, and the results are comparable to the pumped spin magnetization via strong Rashba spin orbit coupling. We also show the vital role of the orbital magnetoelectricity in validating the Mott relation between the intrinsic nonlinear anomalous Hall and Ettingshausen effects.
We show that a slowly decaying current pulse can lead to nearly deterministic precessional switching in the presence of noise. We consider a biaxial macrospin, with an easy axis in the plane and a hard axis out-of-the plane, typical of thin film nanomagnets patterned into asymmetric shapes. Out-of-plane precessional magnetization orbits are excited with a current pulse with a component of spin polarization normal to the film plane. By numerically integrating the stochastic Landau-Lifshitz-Gilbert-Slonczewski equation we show that thermal noise leads to strong dephasing of the magnetization orb…
The spin orbit effect in graphene is too muted to have any observable significance with respect to its application in spintronics. However, graphene technology is too valuable to be rendered impotent to spin transport. In this communication we look at the effect of adiabatically twisting a single molecule magnet embedded in a graphene monolayer. Surprisingly, we see that pure spin currents (zero charge current) can be generated from the system via quantum pumping. In addition we also see spin selective current can also be pumped from the system. The pure spin current seen is quite resilient to…
We propose a robust and highly efficient NMR technique to create singlet spin order from longitudinal spin magnetization in coupled spin-1/2 pairs and to perform backward conversion (singlet order)$\to$magnetization. In this method we exploit adiabatic switching of an RF-field in order to drive transitions between the singlet state and the $T_\pm$ triplet states of a spin pair under study. We demonstrate that the method works perfectly for both strongly and weakly coupled spin pairs, providing a conversion efficiency between the singlet spin order and magnetization, which is equal to the theor…
We study the anomalous Hall effect and orbital magnetization in chiral antiferromagnets, constructing a simple tight-binding model on a stacked Kagome lattice structure with spin-orbit coupling and the exchange interaction between the localized spins and itinerant electrons. It is shown that the ground state is an orbital ferromagnet with the easy-plane anisotropy. The relation between the orbital magnetization and the configuration of the Weyl points are discussed.
We calculate orbital spin-dependent magnetization in a two-dimensional electron gas with spin-orbit interaction of Rashba type. Such an orbital magnetization is admitted by the time-reversal symmetry of the system, and gives rise to spin currents when the system is not in thermal equilibrium. The theoretical approach is based on the linear response theory and the Matsubara Green's function formalism. To account for the spin-resolved orbital magnetization a spin-dependent vector potential has been introduced. The spin currents which appear in thermal nonequilibrium due to the spin-resolved orbi…
We investigate the induced orbital magnetization density in a Rashba electron gas with magnetic impurities. Relying on classical electrodynamics, we obtain this quantity through the bound currents composed of a paramagnetic and a diamagnetic-like contribution which emerge from the spin-orbit interaction. Similar to Friedel charge ripples, the bound currents and the orbital magnetization density oscillate as function of distance away from the impurity with characteristic wavelengths defined by the Fermi energy and the strength of the Rashba spin-orbit interaction. The net induced orbital magnet…
We consider periodic adiabatic processes of gapped many-body spinless electrons. We find an additional contribution to the orbital magnetization due to the adiabatic time evolution, dubbed \textit{geometric} orbital magnetization, which can be expressed as derivative of the many-body Berry phase with respect to an external magnetic field. For two-dimensional band insulators, we show that the geometric orbital magnetization generally consists of two pieces, the topological piece that is expressed as third Chern-Simons form in $(t,k_x,k_y)$ space, and the non-topological piece that depends on Bl…
Recently, signatures of quantum anomalous Hall states with spontaneous ferromagnetism were observed in twisted bilayer graphenes (TBGs) near 3/4 filling [1, 2]. Importantly, it was demon-strated that an extremely small current can switch the direction of the magnetization. This offers the prospect of realizing low energy dissipation magnetic memories. However, the mechanism of the current-driven magnetization switching is poorly understood as the charge currents in graphene layers are generally believed to be non-magnetic. In this work, we demonstrate that, in TBGs, the twist-induced reduction…
We theoretically show that in a crystal with a helical lattice structure, orbital and spin magnetizations along a helical axis are induced by an electric current along the helical axis. We propose a simple tight-binding model for calculations, and the results can be generalized to any helical crystals. The induced magnetizations are opposite for right-handed and left-handed helices. The current-induced spin magnetization along the helical axis comes from a radial spin texture on the Fermi surface. This is in sharp contrast to Rashba systems where the induced spin magnetization is perpendicular…
We present a magnetization measurement probing the transition from a quantum Hall to insulating (QH-I) state for a two-dimensional electron gas in a disordered GaAs/AlGaAs heterostructure. Using a highly sensitive DC torque magnetometer, we discover an abrupt change in the orbital magnetization precisely at the critical point for the QH-I transition. Since this transition is predicted to be a second order quantum phase transition, a thermodynamic signature in magnetization is totally unexpected. The observed feature is reminiscent of the well-known de Haas-van Alphen oscillations arising from …
Both spin and orbital degrees of freedom contribute to the magnetic moment of isolated atoms. However, when inserted in crystals, atomic orbital moments are quenched because of the lack of rotational symmetry that protects them when isolated. Thus, the dominant contribution to the magnetization of magnetic materials comes from electronic spin. Here we show that nanoislands of quantum spin Hall insulators can host robust orbital edge magnetism whenever their highest occupied Kramers doublet is singly occupied, upgrading the spin edge current into a charge current. The resulting orbital magnetiz…
The intrinsic orbital magnetization of a TMD monolayer is usually calculated for a plane unbounded system without mentioning the geometrical shape of samples and boundary conditions (BCs) for electron wave functions. The method of calculations includes allowing for the Berry curvature contribution also in the case when the system is described by the two-band minimal model [9]. In the present paper, we show that the geometrical and topological properties of the specimen, as well as the BCs, play an important role in the problem of magnetization even for a macroscopic specimen.
The orbital magnetic moment of a finite piece of matter is expressed in terms of the one-body density matrix as a simple trace. We address a macroscopic system, insulating in the bulk, and we show that its orbital moment is the sum of a bulk term and a surface term, both extensive. The latter only occurs when the transverse conductivity is nonzero and owes to conducting surface states. Simulations on a model Hamiltonian validate our theory.
The modern expressions for polarization $¶$ and orbital magnetization $\M$ are $\k$-space integrals. But a genuine bulk property should also be expressible in $\r$-space, as unambiguous function of the ground-state density matrix, "nearsighted" in insulators, independently of the boundary conditions---either periodic or open. While $¶$---owing to its "quantum" indeterminacy---is {\it not} a bulk property in this sense, $\M$ is. We provide its $\r$-space expression for any insulator, even with nonzero Chern invariant. Simulations on a model Hamiltonian validate our theory.
Based on standard perturbation theory, we present a full quantum derivation of the formula for the orbital magnetization in periodic systems. The derivation is generally valid for insulators with or without a Chern number, for metals at zero or finite temperatures, and at weak as well as strong magnetic fields. The formula is shown to be valid in the presence of electron-electron interaction, provided the one-electron energies and wave functions are calculated self-consistently within the framework of the exact current and spin density functional theory.
Staggered orbital magnetization from itinerant electrons: orbital antiferro- and ferrimagnetic phases
Instituto de Física, Universidade Federal Fluminense（弗鲁米嫩塞联邦大学物理研究所）；International Iberian Nanotechnology Laboratory (INL)（伊比利亚纳米技术国际实验室）；Centro Brasileiro de Pesquisas Físicas (CBPF)（巴西物理研究中心）；Physics Center of Minho and Porto Universities (CF-UM-UP)（米尼奥与波尔图大学物理中心）
Theory of In-Plane Orbital Magnetization with Layer Hybridization
The Hong Kong University of Science and Technology（香港科技大学）；RIKEN Center for Emergent Matter Science (CEMS)（理化学研究所新兴物质科学中心）；Beijing Institute of Technology（北京理工大学）
We propose an orbital magnetothermal effect wherein a temperature gradient generates an orbital magnetization (OM) for Bloch electrons, and we present a unified theory for electrically and thermally induced OM, valid for both metals and insulators. We reveal that there exists an intrinsic response of OM, for which the susceptibilities are completely determined by the band geometric quantities such as interband Berry connections, interband orbital moments, and the quantum metric. The theory can be readily combined with first-principles calculations to study real materials. As an example, we cal…
Real-Space Spectral Approach to Orbital Magnetization
International Iberian Nanotechnology Laboratory (INL)（伊比利亚纳米技术国际实验室）；Centro de Física das Universidades do Minho e Porto（米尼奥和波尔图大学物理中心）；Universidade do Porto（波尔图大学）；University of York（约克大学）；Centro Brasileiro de Pesquisas Físicas (CBPF)（巴西物理研究中心）；Universidade Federal Fluminense（弗鲁米嫩塞联邦大学）；Physics Center of Minho and Porto Universities (CF-UM-UP)（米尼奥和波尔图大学物理中心）
We calculate the orbital magnetization of single and double quantum dots coupled both by Coulomb interaction and by electron tunneling. The electronic states of the quantum dots are calculated in a tight-binding model and the magnetization is discussed in relation to the energy spectrum and to the edge and bulk states. We identify effects of chirality of the electronic orbits and of the anti-crossing of the energy levels when the magnetic field is varied. We also consider the effects of detuning the energy spectra of the quantum dots by an external gate potential. We compare our results with t…
A valley-contrasting Berry curvature in bilayer transition metal dichalcogenides with spin-orbit coupling can generate valley magnetization when the inversion symmetry is broken, for example, by an electric field, regardless of time-reversal symmetry. A nontrivial Berry curvature can also lead to anomalous transport responses, such as the anomalous Hall effect and the anomalous Nernst effect. Applied to a bilayer WSe$_2$, an electric field can tune the Berry curvature and orbital magnetic moment, which has important consequences for the orbital magnetization and the anomalous Nernst responses.…
The orbital magnetization of the electron gas on a two-dimensional kagome lattice under a perpendicular magnetic field is theoretically investigated. The interplay between the lattice geometry and magnetic field induce nontrivial $k$-space Chern invariant in the magnetic Brillouin zone, which turns to result in profound effects on the magnetization properties. We show that the Berry-phase term in the magnetization gives a paramagnetic contribution, while the conventional term brought about by the magnetic response of the magnetic Bloch bands produces a diamagnetic contribution. As a result, th…
We theoretically demonstrate that 100\% valley-polarized transport in monolayers of MoS$_{2}$ and other group-VI dichalcogenides can be obtained using off-resonant circularly polarized light. By tuning the intensity of the off-resonant light the intrinsic band gap in one valley is reduced, while it is enhanced in the other valley, enabling single valley quantum transport. As a consequence, we predict (i) enhancement of the longitudinal electrical conductivity, accompanied by an increase in the spin-polarization of the flowing electrons, (ii) enhancement of the intrinsic spin Hall effect, toget…
Ensembles of gold nanoparticles present a magnetic behavior which is at odds with the weakly diamagnetic response of bulk gold. In particular, an unusual ferromagnetic order has been unveiled by several experiments. Here we investigate if the combined effect of orbital magnetism of conduction electrons and interparticle dipolar interaction can lead to magnetic ordering. Using different model systems of interacting mesoscopic magnetic dipoles, together with a microscopic description of the electron dynamics within the nanoparticles, we find that a spontaneous magnetic moment may arise in dimers…
Theory of local orbital magnetization: local Berry curvature
CPHT, CNRS, École polytechnique, Institut Polytechnique de Paris（法国国家科学研究中心，巴黎综合理工学院，巴黎理工学院）；Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS（巴黎-萨克雷大学，法国国家科学研究中心）
In order to understand the orbital and spin magnetization of a confined electronic system we analyze these ground state properties in the transition from a quantum dot to a quantum ring of finite thickness. The Coulomb interaction between the electrons is treated in the Hartree and Hartree-Fock approximations and special care is taken to include also the contributions of the nonlocal current to the summation of the magnetic moments of the occupied states. We identify changes in the many-body structure of the ground state and in the magnetization curves versus the magnetic field and other param…
We theoretically study current-induced orbital magnetization in a chiral crystal. This phenomenon is an orbital version of the Edelstein effect. We propose an analogy between the current-induced orbital magnetization and an Ampère field in a solenoid in classical electrodynamics. In order to quantify this effect, we define a dimensionless parameter from the response coefficient relating a current density with an orbital magnetization. This dimensionless parameter can be regarded as a number of turns within a unit cell when the crystal is regarded as a solenoid, and it represents how "chiral" t…
A general expression for the orbital magnetization of a Floquet system is derived. The expression holds for a clean system, and is valid for any driving protocol, and arbitrary occupation of the bands. The orbital magnetization is shown to be large not only for Chern insulators, but also for anomalous phases where the Chern number does not fully account for the topology. In addition, the orbital magnetization is shown to take significant values both for a thermal equilibrium occupation of the Floquet bands, and for occupations determined by a quantum quench from an initial state with zero orbi…
We theoretically investigate spin current and magnetic response induced by the twisting phonon mode in carbon nanotubes via the spin-rotation coupling. An effective magnetic field due to the twisting mode induces both spin and orbital magnetizations. The induced spin and orbital magnetizations have both radial and axial components. We show that ac pure spin current is generated by the twisting phonon mode. The magnitude of the spin current and orbital magnetization for a (10,10) armchair nanotube is estimated as an example. We find that the ac pure spin current is detectable in magnitude when …
We study orbital magnetism in a three-dimensional (3D) quantum dot with a parabolic confining potential. We calculate the free energy of the system as a function of the magnetic field and the temperature. By this, we show that the temperature-field plane can be classified into three regions in terms of the characteristic behavior of the magnetization: the Landau diamagnetism, de Haas-van Alphen oscillation and mesoscopic fluctuation of magnetization. We also calculate numerically the magnetization of the system and then the current density distribution. As for the oscillation of the magnetizat…
The real space formalism of orbital magnetization (OM) is an average of the local OM over some appropriate region of the system. Previous studies prefer a bulk average (i.e., without including boundaries). Based on a bilayer model with an adjustable Chern number at half filling, we numerically investigate the effects from boundaries on the real space expressions of OM. The size convergence processes of its three constituent terms $M_{\mathrm{LC}}$, $M_{\mathrm{IC}}$, $M_{\mathrm{BC}}$ are analysed. The topological term $M_{\mathrm{BC}}$ makes a nonnegligible contribution from boundaries as a m…
The observed magnetization switching by circularly polarized ultrafast laser pulses has been attributed to the inverse Faraday effect in which the induced non-equilibrium orbital momentum serves as an effective magnetic filed via spin-orbit coupling for magnetization rotation and switching. We critically examine this scenario by explicitly calculating the magnitude of the induced orbital momentum for generic itinerant band. We show that the calculated induced angular momentum is not large enough for reversing the magnetization in one laser pulse with the order of 100 femtosecond duration. Inst…
We show how the orbital magnetization of an interacting disordered diffusive electron gas can be simply related to the magnetization of the non-interacting system having the same geometry. This result is applied to the persistent current of a mesoscopic ring and to the relation between Landau diamagnetism and the interaction correction to the magnetization of diffusive systems. The field dependence of this interaction contribution can be deduced directly from the de Haas-van Alphen oscillations of the free electron gas. Known results for the free orbital magnetism of finite systems can be used…
Recently, Berry phase in the semiclassical dynamical of Bloch electrons has been found to make a correction to the phase-space density of states and a general multi-band formula for finite-temperature orbital magnetization has been given [Phys. Rev. Lett. \textbf{97}, 026603 (2006)], where the orbital magnetization $\mathcal{M}$ consists of two parts, i.e., the conventional part $M_{c}$ and the Berry-phase correction part $M_Ω$. Using this general formula, we theoretically investigate the orbital magnetization and its effects on thermoelectric transport and magnetic susceptibility properties o…
The modern theory of orbital magnetization addresses crystalline materials at the noninteracting level: therein the observable is the k-space integral of a geometrical integrand. Alternatively, magnetization admits a local representation in r space, i.e. a "density" which may address noncrystalline and/or inhomogeneous materials as well; the Chern number admits an analogous density. Here we provide the formulation for ribbons, polymers, and layered materials, where both k-space and r-space integrations enter the definition of the two observables.
The orbital magnetization and its effects on the two-dimensional kagomé lattice with spin anisotropies included in the general Hund's coupling region have been theoretically studied. The results show that the strength of the Hund's coupling, as well as the spin chirality, contributes to the orbital magnetization $\mathcal{M}$. Upon varying both these parameters, it is found that the two parts of $\mathcal{M}$, i.e., the conventional part $\mathbf{M}_{c}$ and the Berry-phase correction part $\mathbf{M}_Ω$, oppose each other. The anomalous Nernst conductivity is also calculated and a peak-valley…
Working in the Wannier representation, we derive an expression for the orbital magnetization of a periodic insulator. The magnetization is shown to be comprised of two contributions, an obvious one associated with the internal circulation of bulk-like Wannier functions in the interior, and an unexpected one arising from net currents carried by Wannier functions near the surface. Each contribution can be expressed as a bulk property in terms of Bloch functions in a gauge-invariant way. Our expression is verified by comparing numerical tight-binding calculations for finite and periodic samples.
The Berry curvature dipole is a physical quantity that is expected to allow various quantum geometrical phenomena in a range of solid-state systems. Monolayer transition metal dichalcogenides provide an exceptional platform to modulate and investigate the Berry curvature dipole through strain. Here we theoretically demonstrate and experimentally verify for monolayer MoS$_\rm{2}$ the generation of valley orbital magnetization as a response to an in-plane electric field due to the Berry curvature dipole. The measured valley orbital magnetization shows excellent agreement with the calculated Berr…
Under suitable conditions, some twisted graphene multilayers and transition-metal dichalcogenides become Chern insulators, exhibiting the anomalous quantum Hall effect and orbital magnetization due to spontaneous valley polarization. We study interaction of a Chern insulator with circularly polarized light. The interaction energy contains an antisymmetric term that couples to the helicity of incident light. For a two-band Chern insulator, this term is expressed as an integral involving the Berry curvature of the system. Taking advantage of this interaction, we propose an experimental protocol …
Quantum Geometric Origin of Nonlinear Current Induced Orbital Magnetization
University of Macau（澳门大学）；Great Bay University（大湾区大学）；Great Bay Institute for Advanced Study（大湾区高等研究院）；Fudan University（复旦大学）；Max Planck Institute for Chemical Physics of Solids（马克斯·普朗克固体化学物理研究所）；University of Science and Technology of China（中国科学技术大学）；The Hong Kong Polytechnic University（香港理工大学）
Using a multi-orbital tight-binding model, we have studied the edge states of zigzag silicene, germanene, and stanene nanoribbons (ZSiNRs, ZGeNRs and ZSnNRs, respectively) in the presence of the Coulomb interaction and a vertical electric field. The resulting edge states have non-linear energy dispersions due to multi-orbital effects, and the nanoribbons show induced magnetization at the edges. Owing to this non-linear dispersion, ZSiNRs, ZGeNRs and ZSnNRs may not provide superior performance in field effect transistors, as has been proposed from single-orbital tight-binding model calculations…
Results are presented for Floquet systems in two spatial dimensions where the Floquet driving breaks an effective time reversal symmetry. The driving protocol also induces flat bands that correspond to anomalous Floquet phases where the Chern number is zero and yet chiral edge modes exist. Analytic expressions for the edge modes, Berry curvature, and the orbital magnetization are derived for the flat bands. Results are also presented for the static Haldane model for parameters when the bands are flat. Floquet driving of the same model is shown to give rise to Chern insulators as well as anomal…
