Long-range spatial coherence can be induced in thermal emitters by embedding a periodic grating into a material supporting propagating polaritons or dielectric modes. However, the emission angle and frequency cannot be defined simultaneously and uniquely, resulting in emission at unusable angles or frequencies. Here, we explore superstructure gratings (SSGs) to control the spatial and spectral properties of thermal emitters. SSGs have long-range periodicity, but a unit cell that provides tailorable Bragg components to interact with light. These Bragg components allow simultaneous launching of polaritons with different frequencies/wavevectors in a single grating, manifesting as additional spatial and spectral bands upon the emission profile. As the unit cell period approaches the spatial coherence length, the coherence properties of the superstructure will be lost. Whilst the 1D k-space representation of the grating provides insights into the emission, the etch depth of the grating can result in strong polariton-polariton interactions. An emergent effect of these interactions is the creation of polaritonic band gaps, and defect states that can have a well-defined frequency and emission angle. In all, our results show experimentally how even in simple 1D gratings there is significant design flexibility for engineering the profile of thermal emitters, bound by finite coherence length.
The interaction of magnetic dipole (MD) emitters and common photonic cavities is usually weak, which is partially due to the low magnetic near field enhancements of the cavities. Here, we show that whispering gallery modes (WGMs) of a subwavelength dielectric cavity can not only greatly boost the emission rate of a MD emitter but also bring efficient couplings between coherent MD emitters. In a WGM cavity, the maximal emission rate (γmax) of a single emitter occurs at an antinode of the field pattern. The emission of the MD emitter can also be greatly affected by another coherent one depending…
The thermal emission of refractory plasmonic metamaterial - a titanium nitride 1D grating - is studied at high operating temperature (540 °C). By choosing a refractory material, we fabricate thermal gratings with high brightness that are emitting mid-infrared radiation centered around 3 $μ$m. We demonstrate experimentally that the thermal excitation of plasmon-polariton on the surface of the grating produces a well-collimated beam with a spatial coherence length of 32λ (angular divergence of 1.8°) which is quasi-monochromatic with a full width at half maximum of 70 nm. These experimental resul…
We provide a general theoretical platform based on quantized radiation in absorptive and inhomogeneous media for investigating the coherent interaction of light with metallic structures in the immediate vicinity of quantum emitters. In the case of a very small metallic cluster, we demonstrate extreme regimes where a single emitter can either counteract or enhance particle absorption by three orders of magnitude. For larger structures, we show that an emitter can eliminate both scattering and absorption and cloak a plasmonic antenna. We provide physical interpretations of our results and discus…
We study the dynamics of single-photon absorption by a single emitter coupled to a one-dimensional waveguide that simultaneously provides channels for spontaneous emission decay and a channel for the input photon. We have developed a time-dependent theory that allows us to specify any input single-photon wavepacket guided by the waveguide as initial condition, and calculate the excitation probability of the emitter, as well as the time evolution of the transmitted and reflected field. For single-photon wavepackets with a gaussian spectrum and temporal shape, we obtain analytical solutions for …
We study the dynamics of single-photon absorption by a single emitter coupled to a one-dimensional waveguide that simultaneously provides channels for spontaneous emission decay and a channel for the input photon. We have developed a time-dependent theory that allows us to specify any input single-photon wavepacket guided by the waveguide as initial condition, and calculate the excitation probability of the emitter, as well as the time evolution of the transmitted and reflected field. For single-photon wavepackets with a gaussian spectrum and temporal shape, we obtain analytical solutions for …
Rapid progress in silicon photonics has fostered numerous chip-scale sensing, computing, and signal processing technologies. However, many crucial filtering and signal delay operations are difficult to perform with all-optical devices. Unlike photons propagating at luminal speeds, GHz-acoustic phonons with slow velocity allow information to be stored, filtered, and delayed over comparatively smaller length-scales with remarkable fidelity. Hence, controllable and efficient coupling between coherent photons and phonons enables new signal processing technologies that greatly enhance the performan…
We theoretically demonstrate the generation and radiation of coherent nanoplasmons powered by a single three-level quantum emitter on a plasmonic nanoresonator. By pumping the three-level emitter in a Raman configuration, we show a pathway to achieve macroscopic accumulation of nanoplasmons due to stimulated emission in the nanoresonator despite their fast relaxation. Thanks to the antenna effect of the nanoresonator, the system acts as an efficient and bright nanoscopic coherent light source with a photon emission rate of hundreds of Terahertz and could be realized with solid-state emitters a…
The control and manipulation of quantum-entangled non-local states is a crucial step for the development of quantum information processing. A promising route to achieve such states on a wide scale is to couple solid-state quantum emitters through their coherent dipole-dipole interactions. Entanglement in itself is challenging, as it requires both nanometric distances between emitters and nearly degenerate electronic transitions. Implementing hyperspectral imaging to identify pairs of coupled organic molecules trapped in a low temperature matrix, we reach distinctive spectral signatures of maxi…
A portion of the electromagnetic wave spectrum between $\sim 0.1$ and $\sim 10$ terahertz (THz) suffers from the lack of powerful, effective, easy-to-use and inexpensive emitters, detectors and mixers. We propose a multilayer graphene -- boron-nitride heterostructure which is able to emit radiation in the frequency range $\sim 0.1-30$ THz with the power density up to $\sim 0.5$ W/cm$^2$ at room temperature. The proposed device is extremely thin, light, flexible, almost invisible and may completely cover the needs of science and technology in the sources of terahertz radiation.
Polarization control of THz light is of paramount interest for the numerous applications offered in this frequency range. Recent developments in THz spintronic emitters allow for a very efficient broadband emission, and especially unique is their ability of THz polarization switching through magnetization control of the ferromagnetic layer. Here we present an improved scheme to achieve full 360° nearly coherent polarization rotation that does not require multipolar or rotating external magnetic bias nor complex cascaded emitters. By replacing the FM layer of the spintronic emitter with a caref…
We report on the coherent internal-state control of single crystalline nanodiamonds, containing on average 1200 nitrogen-vacancy (NV) centers, embedded in three-dimensional direct-laser-written waveguides. We excite the NV centers by light propagating through the waveguide, and we show that emitted fluorescence can be efficiently coupled to the waveguide modes. We find an average coupling efficiency of 21.6% into all guided modes. Moreover, we investigate optically-detected magnetic-resonance spectra as well as Rabi oscillations recorded through the waveguide-coupled signal. Our work shows tha…
Long-range coherent interactions between quantum emitters are instrumental for quantum information and simulation technologies, but they are generally difficult to isolate from dissipation. Here, we show how such interactions can be obtained in photonic Weyl environments due to the emergence of an exotic bound state whose wavefunction displays power-law spatial confinement. Using an exact formalism, we show how this bound state can mediate coherent transfer of excitations between emitters, with virtually no dissipation and with a transfer rate that follows the same scaling with distance as the…
We investigate a nonlinear localization microscopy method based on Rabi oscillations of single emitters. We demonstrate the fundamental working principle of this new technique using a cryogenic far-field experiment in which subwavelength features smaller than $λ$/10 are obtained. Using Monte Carlo simulations, we show the superior localization accuracy of this method under realistic conditions and a potential for higher acquisition speed or a lower number of required photons as compared to conventional linear schemes. The method can be adapted to other emitters than molecules and allows for th…
In a quantum network, coherent emitters can be entangled over large distances using photonic channels. In solid-state devices, the required efficient light-emitter interface can be implemented by confining the light in nanophotonic structures. However, fluctuating charges and magnetic moments at the nearby interface then lead to spectral instability of the emitters. Here we avoid this limitation when enhancing the photon emission up to 70(12)-fold using a Fabry-Perot resonator with an embedded 19 micrometer thin crystalline membrane, in which we observe around 100 individual erbium emitters. I…
In a recent Letter [Phys. Rev. Lett. 126, 063902 (2021)], M. A. Carroll et al. derived a model to analytically determine regimes of thermal, collective anti-bunching, and laser emission for emitters in a cavity. According to their model, nanolasers exhibit a distinct threshold at which the coherent laser field emerges from a bifurcation at a finite pump rate. The amplitude of this coherent field increases with a further increase in the pump rate. Such a behavior contrasts the usual view of the transition to lasing in single-mode high-$β$ nanolasers, according to which strong spontaneous emissi…
In this Letter we show that the strong coupling between a disordered set of molecular emitters and surface plasmons leads to the formation of spatially coherent hybrid states extended on acroscopic distances. Young type interferometric experiments performed on a system of J-aggregated dyes spread on a silver layer evidence the coherent emission from different molecular emitters separated by several microns. The coherence is absent in systems in the weak coupling regime demonstrating the key role of the hybridization of the molecules with the plasmon.
Resonant excitation of solid-state quantum emitters enables coherent control of quantum states and generation of coherent single photons, which are required for scalable quantum photonics applications. However, these systems can often decay to one or more intermediate dark states or spectrally jump, resulting in the lack of photons on resonance. Here, we present an optical co-excitation scheme which uses a weak non-resonant laser to reduce transitions to a dark state and amplify the photoluminescence from quantum emitters in hexagonal boron nitride (hBN). Utilizing a two-laser repumping scheme…
We propose a novel type of optomechanical coupling which enables a tripartite interaction between a quantum emitter, an optical mode and a macroscopic mechanical oscillator. The interaction uses a mechanism we term mode field coupling: mechanical displacement modifies the spatial distribution of the optical mode field, which in turn modulates the atom-photon coupling rate. In properly designed multimode optomechanical systems, we can achieve situations in which mode field coupling is the only possible interaction pathway for the system. This enables, for example, swapping of a single excitatio…
Hexagonal boron nitride is an emerging two-dimensional material with far-reaching applications in fields like nanophotonics or nanomechanics. Its layered architecture plays a key role for new materials such as Van der Waals heterostructures. The layered structure has also unique implications for hosted, optically active defect centers. A very special type of defect center arises from the possibility to host mechanically isolated orbitals localized between the layers. The resulting absence of coupling to low-frequency acoustic phonons turns out to be the essential element to protect the coheren…
In a preceding paper we introduced a formalism to study the scattering of low intensity fields from a system of multi-level emitters embedded in a $3$D dielectric medium. Here we show how this photon-scattering relation can be used to analyze the scattering of single photons and weak coherent states from any generic multi-level quantum emitter coupled to a $1$D waveguide. The reduction of the photon-scattering relation to $1$D waveguides provides for the first time a direct solution of the scattering problem involving low intensity fields in the waveguide QED regime. To show how our formalism …
We report on a quantitative measurement of the spatial coherence of electrons emitted from a sharp metal needle tip. We investigate the coherence in photoemission using near-ultraviolet laser triggering with a photon energy of 3.1 eV and compare it to DC-field emission. A carbon-nanotube is brought in close proximity to the emitter tip to act as an electrostatic biprism. From the resulting electron matter wave interference fringes we deduce an upper limit of the effective source radius both in laser-triggered and DC-field emission mode, which quantifies the spatial coherence of the emitted ele…
A simple calculation method for photon statistics of frequency-filtered fields is proposed. This method, based on eigenvalue decompositions of superoperators, allows us to study effects on the photon statistics of spectral filtering by various types of filters, such as Gaussian and rectangular filters as well as Lorentzian filters, which is not possible by conventional approaches. As an example, this method is applied to a simulation of quantum dot single-photon emitters, where we found the efficient choice of the filter types to have pure single photons depends on the excitation conditions i.…
Extinction spectroscopy is a powerful tool for demonstrating the coupling of a single quantum emitter to a photonic structure. However, it can be challenging in all but the simplest of geometries to deduce an accurate value of the coupling efficiency from the measured spectrum. Here we develop a theoretical framework to deduce the coupling efficiency from the measured transmission and reflection spectra without precise knowledge of the photonic environment. We then consider the case of a waveguide interrupted by a transverse cut in which an emitter is placed. We apply that theory to a silicon …
Advances in nanotechnology provide techniques for the realisation of integrated quantum-optical circuits for on-chip quantum information processing(QIP). The indistinguishable single photons, required for such devices can be generated by parametric down-conversion, or from quantum emitters such as colour centres and quantum dots(QDs). Among these, semiconductor QDs offer distinctive capabilities including on-demand operation, coherent control, frequency tuning and compatibility with semiconductor nanotechnology. Moreover, the coherence of QD photons can be significantly enhanced in resonance f…
This is the third of a series of papers devoted to develop a microscopical approach to the dipole emission process and its relation to coherent transport in random media. In this paper, we compute the power emitted by an induced dipole and the spontaneous decay rate of a Lorentzian-type dipole. In both cases, the emitter is placed at the center of a real cavity drilled in a continuous medium.
This is the first of a series of papers devoted to develop a microscopical approach to the dipole emission process and its relation to coherent transport in random media. In this Letter, we deduce general expressions for the decay rate of spontaneous emitters and the power emission of induced dipoles embedded in homogenous dielectric media. We derive formulae which apply generically to virtual cavities and, in the continuum approximation, to small real cavities.
Single-photon emitters in solid-state systems are important building blocks for scalable quantum technologies. Recently, quantum light emitters have been discovered in the wide-gap van der Waals insulator hBN. These color centers have attracted considerable attention due to their quantum performance at elevated temperatures and wide range of transition energies. Here, we demonstrate coherent state manipulation of a single hBN color center with ultrafast laser pulses and investigate in our joint experiment-theory study the coupling between the electronic system and phonons. We demonstrate that …
