Physical properties of single-electron devices in the week Coulomb blockade regime are significantly dependent on non-perturbative effects. They arise as instanton solutions of equations of motion for the corresponding Ambegaokar-Eckern-Schoen action. In equilibrium those solutions are known as Korshunov instantons. In this paper we study non-equilibrium Ambegaokar-Eckern- Schoen action using Keldysh technique. We found instantons for the most general stationary out-of equilibrium state. We also found that action saddle-point value assumes a universal value irrespective of the stationary non-equilibrium state.
We develop the two-instanton approximation to the current-voltage characteristic of a single electron transistor within the Ambegaokar-Eckern-Schön model. We determine the temperature and gate voltage dependence of the Coulomb blockade oscillations of the conductance and the effective charge. We find that a small (in comparison with the charging energy) bias voltage leads to significant suppression of the Coulomb blockade oscillations and to appearance of the bias-dependent phase shift.
We study many-body corrections to the cotunneling current via a localized state with energy $ε_d$ at large bias voltages $V$. We show that the transfer of {\em electron pairs}, enabled by the Coulomb repulsion in the localized level, results in ionization resonance peaks in the third derivative of the current with respect to $V$, centered at $eV=\pm 2ε_d/3$. Our results predict the existence of previously unnoticed structure within Coulomb-blockade diamonds.
The charging of a quantum box connected to a lead by a single-mode point contact is solved for arbitrary temperatures, tunneling amplitudes, and gate voltages, using a variant of Wilson's numerical renormalization group. The charge inside the box and the capacitance of the junction are calculated on equal footing for all physical regimes, including weak tunneling, near perfect transmission, and the crossover regime in between. At the charge plateaus, perturbation theory is found to break down at fairly small tunneling amplitudes. Near perfect transmission, we confirm Matveev's scenario for the…
Carbon nanotubes provide a new class of molecular wires that display new and exciting mesoscopic transport properties. We provide a detailed theoretical description for transport in multi-wall nanotubes, where both disorder and strong interactions are important. The interplay of both aspects leads to a particularly effective intrinsic Coulomb blockade for tunneling. The relation to recent experiments is discussed.
We derive a closed expression for the linear conductance through a quantum dot in the Coulomb-blockade regime in the presence of a constant exchange interaction. With this expression we calculate the temperature dependence of the conductance peak-height and peak-spacing statistics. Using a realistic value of the exchange interaction, we find significantly better agreement with experimental data as compared with the statistics obtained in the absence of an exchange interaction.
In this paper, we ask the question: How well can Coulomb blockade experiments correctly identify and distinguish between different topological orders in quantum Hall states? We definitively find the answer to be: Quite poorly. In particular, we write the general expression for the spacing of resonance peaks in a simple form that explicitly displays its dependence on the conformal scaling dimensions of the systems' edge modes. This form makes transparent the general argument that the Coulomb blockade peak spacings do not provide a strongly indicative signature of the topological order of the sy…
The non-linear current-voltage characteristic of a tunnel junction between two Luttinger systems is calculated for an interaction with finite range. Coulomb blockade features are found. The dissipative resistance, the capacitance and the external impedance, which were introduced ad hoc in earlier theories, are obtained in terms of the electron-electron interaction. The frequency dependence of the impedance is given by the excitation spectrum of the electrons.
Above the Kondo temperature, the Kohn-Sham zero-bias conductance of an Anderson junction has been shown to completely miss the Coulomb blockade. Within a standard model for the spectral function, we deduce a parameterization for both the onsite exchange-correlation potential and the bias drop as a function of the site occupation that applies for all correlation strengths. We use our results to sow doubt on the common interpretation of such corrections as arising from dynamical exchange-correlation contributions.
We discuss some recent results on the statistics of the Coulomb Blockade in disordered quantum dots containing spinless interacting fermions using the self-consistent Hartree-Fock approximation. We concentrate on the regime r_s >~1, with finite dimensionless conductance g. We present significantly different results for the cases of a Coulomb and a nearest-neighbour bare interaction. We show that neglecting rearrangements when the particle number is changed (Koopmans' approximation) can lead to large errors, and show how the spectral statistics of the self-consistent single particle orbitals ev…
We study the conductance spectrum of graphene quantum dots, both single and multiple cases. The single electron tunneling phenomenon is investigated and the periodicity, amplitude and line shape of the Coulomb blockade oscillations at low temperatures are obtained. Further, we discuss the transport behavior when multiple dots are assembled in array and find a phase transition of conductance spectra from individual Coulomb blockade to collective Coulomb blockade.
We use chiral Luttinger liquid theory to study transport through a quantum dot in the fractional quantum Hall effect regime and find rich non-Fermi-liquid tunneling characteristics. In particular, we predict a remarkable Coulomb-blockade-type energy gap that is quantized in units of the noninteracting level spacing, new power-law tunneling exponents for voltages beyond threshold, and a line shape as a function of gate voltage that is dramatically different than that for a Fermi liquid. We propose experiments to use these unique spectral properties as a new probe of the fractional quantum Hall …
A new theoretical method is introduced to study coherent electron transport in an interacting multilevel quantum dot. The method yields the correct behavior both in the limit of weak and strong coupling to the leads, giving a unified description of Coulomb blockade and the Kondo effect. Results for the density of states and the temperature dependent conductance for a two- level dot are presented. The relevance of these results in connection to recent experiments on the Kondo effect in semiconducting quantum dots is discussed.
We study the mechanism of nuclear spin relaxation in quantum dots due to the electron exchange with 2D gas. We show that the nuclear spin relaxation rate is dramatically affected by the Coulomb blockade and can be controlled by gate voltage. In the case of strong spin-orbit coupling the relaxation rate is maximal in the Coulomb blockade valleys whereas for the weak spin-orbit coupling the maximum of the nuclear spin relaxation rate is near the Coulomb blockade peaks.
We study the dissipation in a system consisting of a small metallic island coupled to a gate electrode and to a massive reservoir via single tunneling junction. The dissipation of energy is caused by a slowly oscillating gate voltage. We compute it in the regimes of weak and strong Coulomb blockade. We focus on the regime of not very low temperatures when electron coherence can be neglected but quantum fluctuations of charge are strong due to Coulomb interaction. The answers assume a particularly transparent form while expressed in terms of specially chosen physical observables. We discovered …
Tunneling spectroscopy measurements of single tunnel junctions formed between multiwalled carbon nanotubes (MWNTs) and a normal metal are reported. Intrinsic Coulomb interactions in the MWNTs give rise to a strong zero-bias suppression of a tunneling density of states (TDOS) that can be fitted numerically to the environmental quantum-fluctuation (EQF) theory. An asymmetric conductance anomaly near zero bias is found at low temperatures and interpreted as Fano resonance in the strong tunneling regime.
We study the interplay between Coulomb blockade and the Kondo effect in quantum dots. We use a self-consistent scheme which describes mesoscopic devices in terms of a collective phase variable (slave rotor) and quasiparticle degrees of freedom. In the strong Coulomb blockade regime, we recover the description of metallic islands in terms of a phase only action. For a dot with well-separated levels, our method leads to the Kondo effect. We identify the regime where a crossover between the Coulomb blockade regime at high temperatures and the formation of a Kondo resonance at lower temperature ta…
Signatures of the non-Abelian statistics of quasi-particles in the $ν=5/2$ quantum Hall state are predicted to be present in the current-voltage characteristics of tunneling through one or two quantum Hall puddles of Landau filling $ν_a$ embedded in a bulk of filling $ν_b$ with $(ν_a,ν_b)=(2,5/2)$ and $(ν_a,ν_b)=(5/2,2)$.
We study theoretically the spin-dependent transport in ferromagnet/normal-metal/ferromagnet double tunnel junctions by special attention to cotunneling in the Coulomb blockade region. The spin accumulation caused by cotunneling squeezes the Coulomb blockade region when the magnetizations in the ferromagnetic electrodes are antiparallel. Outside the squeezed Coulomb blockade region, we propose a new anomalous region, where the sequential tunneling in one of the spin bands is suppressed by the Coulomb blockade and that in the other is not. In this region, the tunnel magnetoresistance oscillates …
We report on Coulomb blockade and Coulomb diamond measurements on an etched, tunable single-layer graphene quantum dot. The device consisting of a graphene island connected via two narrow graphene constrictions is fully tunable by three lateral graphene gates. Coulomb blockade resonances are observed and from Coulomb diamond measurements a charging energy of ~3.5 meV is extracted. For increasing temperatures we detect a peak broadening and a transmission increase of the nanostructured graphene barriers.
Amplitude of the Coulomb blockade oscillations is calculated for a single-mode Josephson junction with arbitrary electron transparency $D$. It is shown that the Coulomb blockade is suppressed in ballistic junctions with $D\to 1$. The suppression is described quantitatively as the Landau-Zener transition in imaginary time.
We investigate theorerically the non-equilibrium transport through a molecular quantum dot as a function of gate and bias voltage, taking into account the typical situation in molecular electronics. In this respect, our study includes asymmetries both in the capacitances and tunneling rates to the source and drain electrodes, as well as an infinitely large charging energy on the molecule. Our calculations are based on the out-of-equilibrium Non-Crossing-Approximation (NCA), which is a reliable technique in the regime under consideration. We find that Coulomb blockade edges and Kondo peaks disp…
We present a theory of zero-bias anomalies and dephasing rates for a Coulomb-blockaded quantum dot, driven out of equilibrium by coupling to voltage biased source and drain leads. We interpret our results in terms of the statistics of voltage fluctuations in the system.
We study the fluctuations of an energy level as a function of the number of electrons $m$ added to a Coulomb-blockade quantum dot. A microscopic calculation in the limit of Koopmans' theorem predicts that the standard deviation of these fluctuations behaves as $\sqrt{m}$ in the absence of surface charge but is linear in $m$ when the effect of a surface charge in a finite geometry is included. The microscopic results are compared to a parametric random-matrix approach. We estimate the number of electrons it takes to scramble the spectrum completely in terms of the interaction strength, the dime…
Disordered granular systems, at temperatures where charging effects are important, are studied, by means of an effective medium approximation. The intragrain charging energy leads to insulating behavior at low temperatures, with a well defined Coulomb gap. Non equilibrium effects can give rise to a zero temperature transition between a metallic, gapless phase, and an insulating phase.
We report that the conductance of macroscopic multiwall nanotube (MWNT) bundles under pressure shows power laws in temperature and voltage, as corresponding to a network of bulk-bulk connected Tomonaga-Luttinger Liquids (LL). Contrary to individual MWNT, where the observed power laws are attributed to Coulomb blockade, the measured ratio for the end and bulk obtained exponents, ~2.4, can only be accounted for by LL theory. At temperatures characteristic of interband separation, it increases due to thermal population of the conducting sheets unoccupied bands.
We find that tunnel junctions are not needed to provide single electron effects in a metallic island. Eventually the tunnel junction may be replaced by an arbitrary scatterer. It is important that even a {\it diffusive} scatterer provides a sufficient isolation for single electron effects to persist. To formulate this in exact terms, we derive and analyze the effective action that describes an arbitrary scatterer. We also consider the fluctuations of the effective charging energy.
We explore electron transport through a quantum dot coupled to the source and drain charge reservoirs We trace the transition from the Coulomb blockade regime to Kondo regime in the electron transport through the dot occuring when we gradually strengthen the coupling of the dot to the charge reservoirs. The current-voltage $(I-V)$ characteristics are calculated using the equations of motion approach within the nonequilibrium Green's functions formalism (NEGF) beyond the Hartree-Fock approximation. We show that within the Coulomb blockade regime the $I-V$ characteristics for the quantum dot con…
Graphene nanodisk is a graphene derivative with a closed edge. The trigonal zigzag nanodisk with size $N$ has $N$-fold degenerated zero-energy states. We investigate electron-electron interaction effects in the zero-energy sector. We explicitely derive the direct and exchange interactions, which are found to have no SU($N$) symmetry. Then, regarding a nanodisk as a quantum dot with an internal degree of freedom, we analyze the nanodisk-lead system consisting of a nanodisk and two leads. Employing the standard Green function method, we reveal novel Coulomb blockade effects in the system. The oc…
We performed electronic transport measurements on 1D InAs quantum wires. In sufficiently disordered wires, transport is dominated by Coulomb blockade, and the conductance can be well described by tunneling through a quantum dot embedded between two one-dimensional Luttinger liquid wires. In contrast to previous experiments in other material systems, in our system the conductance difference between peak to valley decreases with decreasing temperature for several consecutive peaks. This phenomenon is theoretically expected to occur only for strongly interacting systems with small Luttinger inter…
Transport through two quantum dots laterally embedded in Aharonov-Bohm interferometry with infinite intradot and arbitrary interdot Coulomb repulsion is analyzed in the weak coupling and Coulomb blockade regime. By employing the modified quantum rate equations and the slave-boson approach, we establish a general dc current formula at temperatures higher than the Kondo temperature for the case that the spin degenerate levels of two dots are close to each other. We examine two simple examples for identical dots - no doubly occupied states and no empty state. In the former, completely destructive…
Motivated by the discovery of superconductivity in the infinite-layer nickelate family, we report an experimental endeavor to clean the surface of nickelate superconductor Pr0.8Sr0.2NiO2 films by Ar+ ion sputtering and subsequent annealing, and we study their electronic structures by cryogenic scanning tunneling microscopy and spectroscopy. The annealed surfaces are characterized by nano-sized clusters and Coulomb staircases with periodicity inversely proportional to the projected area of the nanoclusters, consistent with a double-barrier tunneling junction model. Moreover, the dynamical Coulo…
We study the Coulomb blockade in a chaotic cavity connected to a lead by a perfectly transmitting quantum channel. In contrast to the previous theories, we show that the quantum fluctuations of charge, resulting from the perfect transmission, do not destroy the Coulomb blockade completely. The oscillatory dependence of all the observable characteristics on the gate voltage persists, its period is not affected; however, phases of the oscillations are random, reflecting the chaotic electron motion in the cavity. Because of this randomness, the Coulomb blockade shows up not in the averages but in…
We report the observation of Coulomb blockade in a quantum dot contacted by two quantum point contacts each with a single fully-transmitting mode, a system previously thought to be well described without invoking Coulomb interactions. At temperatures below 50 mK we observe a periodic oscillation in the conductance of the dot with gate voltage that corresponds to a residual quantization of charge. From the temperature and magnetic field dependence, we infer the oscillations are Mesoscopic Coulomb Blockade, a type of Coulomb blockade caused by electron interference in an otherwise open system.
We study conductance through a quantum dot under Coulomb blockade conditions in the presence of an external periodic perturbation. The stationary state is determined by the balance between the heating of the dot electrons by the perturbation and cooling by electron exchange with the cold contacts. We show that Coulomb blockade peak can have a peculiar shape if heating is affected by dynamic localization, which can be an experimental signature of this effect.
We demonstrate single electron shuttling through two coupled nanomechanical pendula. The pendula are realized as nanopillars etched out of the semiconductor substrate. Coulomb blockade is found at room temperature, allowing metrological applications. By controlling the mechanical shuttling frequency we are able to validate the different regimes of electron shuttling.
I. Introduction (Preface, Basic properties of semiconductor nanostructures). II. Theory of Coulomb-blockade oscillations (Periodicity of the oscillations, Amplitude and lineshape). III. Experiments on Coulomb-blockade oscillations (Quantum dots, Disordered quantum wires, Relation to earlier work on disordered quantum wires). IV. Quantum Hall effect regime (The Aharonov-Bohm effect in a quantum dot, Coulomb blockade of the Aharonov-Bohm effect, Experiments on quantum dots, Experiments on disordered quantum wires).
We study Coulomb charging effects for transport through a topologically nontrivial superconducting wire, where Majorana bound states are present at the interface to normal-conducting leads. We construct the general Keldysh functional integral representation, and provide detailed results for the nonlinear current-voltage relation under weak Coulomb blockade conditions.
We demonstrate experimentally a precise realization of Coulomb Blockade Thermometry (CBT) working at temperatures up to 60 K. Advances in nano fabrication methods using electron beam lithography allow us to fabricate a uniform arrays of sufficiently small tunnel junctions to guarantee an overall temperature reading uncertainty of about 1\%
Coherent electronic transport in single-molecule junctions is investigated in the Coulomb blockade regime. Both the transmission phase and probability are calculated for junctions with various contact symmetries. A dramatic suppression of the Coulomb blockade peaks is predicted for junctions where multiple atomic orbitals of the molecule couple to a single electrode although the charging steps are unaffected.
Quantum transport through single molecules is very sensitive to the strength of the molecule-electrode contact. When a molecular junction weakly coupled to external electrodes, charging effects do play an important role (Coulomb blockade regime). In this regime, the non-equilibrium Green function is usually substituted with master equation approaches, which prevents the density functional theory from describing Coulomb blockade in non-equilibrium case. Last year, we proposed an Ansatz to combine the non-equilibrium Green function technique with the equation of motion method. With help of it, C…
Coulomb blockade resonances are measured in a GaAs quantum dot in which both shape deformations and interactions are small. The parametric evolution of the Coulomb blockade peaks shows a pronounced pair correlation in both position and amplitude, which is interpreted as spin pairing. As a consequence, the nearest-neighbor distribution of peak spacings can be well approximated by a smeared bimodal Wigner surmise, provided that interactions which go beyond the constant interaction model are taken into account.
The distribution of Coulomb blockade peak heights as a function of magnetic field is investigated experimentally in a Ge-Si nanowire quantum dot. Strong spin-orbit coupling in this hole-gas system leads to antilocalization of Coulomb blockade peaks, consistent with theory. In particular, the peak height distribution has its maximum away from zero at zero magnetic field, with an average that decreases with increasing field. Magnetoconductance in the open-wire regime places a bound on the spin-orbit length ($l_{so}$ < 20 nm), consistent with values extracted in the Coulomb blockade regime ($l_{s…
A new field electron emission (FE) mechanism, which includes Coulomb blockade and quantum confinement effects, is revealed for heterostructured emitters composed of quantum dots and nanowires self-assembled at diamond nanotips. The total energy distributions of the emitted electrons show multiple peaks attributed to the discrete electronic states of the quantum-confined emitter with the corresponding energy levels oscillating as a function of the applied voltage due to the Coulomb blockade. The FE current-voltage characteristics exhibit a modified Coulomb staircase with additional steps becomi…
A tunable directional coupler based on Coulomb Blockade effect is presented. Two electron waveguides are coupled by a quantum dot to an injector waveguide. Electron confinement is obtained by surface Schottky gates on single GaAs/AlGaAs heterojunction. Magneto-electrical measurements down to 350 mK are presented and large transconductance oscillations are reported on both outputs up to 4.2 K. Experimental results are interpreted in terms of Coulomb Blockade effect and the relevance of the present design strategy for the implementation of an electronic multiplexer is underlined.
Motivated by recent experiments, we have studied transport behavior of coupled quantum dot systems in the Coulomb blockade regime using the master (rate) equation approach. We explore how electron-electron interactions in a donor-acceptor system, resembling weakly coupled quantum dots with varying charging energy, can modify the systems response to an external bias, taking it from normal Coulomb blockade behavior to negative differential resistance (NDR) in the curent-voltage characteristics.
We extend the theory of Coulomb blockade oscillations to quantum dots which are deformed by the confining potential. We show that shape deformations can generate sequences of conductance resonances which carry the same internal wavefunction. This fact may cause strong correlations of neighboring conductance peaks. We demonstrate the relevance of our results for the interpretation of recent experiments on semiconductor quantum dots.
We develop a theory of the reversible switching of the magnetic state of the ferromagnet-insulator-normal metalferromagnet (FINF) nanostructure. The switching is controlled by tuning the Coulomb blockade strength via the gate voltage on the normal metal granule. The proposed mechanism allows for realizing the switching without passing a dissipative current through the structure.
A magnet with precessing magnetization pumps a spin current into adjacent leads. As a special case of this spin pumping, a precessing macrospin (magnetization) can assist electrons in tunneling. In small systems, however, the Coulomb blockade effect can block the transport of electrons. Here, we investigate the competition between macrospin-assisted tunneling and Coulomb blockade for the simplest system where both effects meet; namely, for a single tunnel junction between a normal metal and a metallic ferromagnet with precessing magnetization. By combining Fermi's golden rule with magnetizatio…
What quantity controls the Coulomb blockade oscillations if the dot--lead conductance is essentially frequency--dependent ? We argue that it is the ac dissipative conductance at the frequency given by the effective charging energy. The latter may be very different from the bare charging energy due to the interface--induced capacitance (or inductance). These observations are supported by a number of examples, considered from the weak and strong coupling (perturbation theory vs. instanton calculus) perspectives.
We report the observation of Coulomb blockade in field electron emission (FE) from single-wall carbon nanotubes (SWCNTs), which is manifested as pronounced steps in the FE current-voltage curves and oscillatory variations in the energy distribution of emitted electrons. The appearance of the Coulomb blockade is explained by the formation of nanoscale protrusions at the apexes of SWCNTs due to the electric field-assisted surface diffusion of adsorbates and carbon adatoms. The proposed adsorbate-assisted FE mechanism is substantially different from the well-known resonant tunneling associated wi…
Signatures of "mesoscopic Coulomb blockade" are reported for quantum dots with one fully transmitting point-contact lead, T1 = 1, T2 << 1. Unlike Coulomb blockade (CB) in weak-tunneling devices (T1, T2 << 1), one-channel CB is a mesoscopic effect requiring quantum coherence. Several distinctive features of mesoscopic CB are observed, including a reduction in CB upon breaking time-reversal symmetry with a magnetic field, relatively large fluctuations of peak position as a function of magnetic field, and strong temperature dependence on the scale of the quantum level spacing.
By using bosonization method and unitary transformation, we give a general relation between the dimensionless tunneling conductance and the fractional Coulomb blockade conductance peak splitting which is valid both for weak and strong transmission between two quantum dots, and show that the tunneling conductance has a linear temperature dependence in the low energy and low temperature limit.
We have investigated one and two dimensional (1D and 2D) arrays of tunnel junctions in partial Coulomb blockade regime. The absolute accuracy of the Coulomb blockade thermometer is influenced by the external impedance of the array, which is not the same in the different topologies of 1D and 2D arrays. We demonstrate, both by experiment and by theoretical calculations in simple geometries, that the 1D structures are better in this respect. Yet in both 1D and 2D, the influence of the environment can be made arbitrarily small by making the array sufficiently large.
We investigate temperature errors of Coulomb blockade thermometer (CBT) arising from inevitable non-uniformities in tunnel junction arrays. The errors are proportional to the junction resistance variance in the universal operation regime and this result holds approximately also beyond this originally studied high temperature range. We present both analytical and numerical results, and discuss briefly their implications on achievable uniformity based on state-of-the-art fabrication of sensors.
We determine the zero-bias anomaly of the conductance of tunnel junctions by an approach unifying the conventional Coulomb blockade theory for ultrasmall junctions with the diffusive anomalies in disordered conductors. Both, electron-electron interactions within the electrodes and electron-hole interactions between the electrodes are taken into account nonperturbatively. Explicit results are given for one- and two-dimensional junctions, and the crossover to ultrasmall junctions is discussed.
We propose that recent transport experiments revealing the existence of an energy gap in graphene nanoribbons may be understood in terms of Coulomb blockade. Electron interactions play a decisive role at the quantum dots which form due to the presence of necks arising from the roughness of the graphene edge. With the average transmission as the only fitting parameter, our theory shows good agreement with the experimental data.
The quantum theory for mesoscopic electric circuit is briefly described. The uncertainty relation for electric charge and current modifies the tranditional Heisenberg uncertainty relation. The mesoscopic ring is regarded as a pure L-design, and the persistent current is obtained explicitly. The Coulomb blockade phenomenon appears when applying to the pure C-design.
We study conductance through a quantum dot under Coulomb blockade conditions in the presence of an external periodic perturbation. The stationary state is determined by the balance between the heating of the dot electrons by the perturbation and cooling. We analyze two cooling mechanisms: electron exchange with the cold contacts and emission of phonons. Together with the usual linear Ohmic heating of the dot electrons we consider possible effects of dynamic localization. The combination of the abovementioned factors may result in a drastic change of the shape of the Coulomb blockade peak with …
