Charge radii of exotic potassium isotopes challenge nuclear theory and the magic character of $N = 32$
Á. Koszorús, X. F. Yang, W. G. Jiang, S. J. Novario, S. W. Bai, J. Billowes, C. L. Binnersley, M. L. Bissell, T. E. Cocolios, B. S. Cooper, R. P. de Groote, A. … 展开作者
Á. Koszorús, X. F. Yang, W. G. Jiang, S. J. Novario, S. W. Bai, J. Billowes, C. L. Binnersley, M. L. Bissell, T. E. Cocolios, B. S. Cooper, R. P. de Groote, A. Ekström, K. T. Flanagan, C. Forssén, S. Franchoo, R. F. Garcia Ruiz, F. P. Gustafsson, G. Hagen, G. R. Jansen, A. Kanellakopoulos, M. Kortelainen, W. Nazarewicz, G. Neyens, T. Papenbrock, P. -G. Reinhard, B. K. Sahoo, C. M. Ricketts, A. R. Vernon, S. G. Wilkins
备注:
submitted version; revision accepted in Nature Physics
Nuclear charge radii are sensitive probes of different aspects of the nucleon-nucleon interaction and the bulk properties of nuclear matter; thus, they provide a stringent test and challenge for nuclear theory. The calcium region has been of particular interest, as experimental evidence has suggested a new magic number at $N = 32$ [1-3], while the unexpectedly large increases in the charge radii [4,5] open new questions about the evolution of nuclear size in neutron-rich systems. By combining the collinear resonance ionization spectroscopy method with $β$-decay detection, we were able to extend the charge radii measurement of potassium ($Z =19$) isotopes up to the exotic $^{52}$K ($t_{1/2}$ = 110 ms), produced in minute quantities. Our work provides the first charge radii measurement beyond $N = 32$ in the region, revealing no signature of the magic character at this neutron number. The results are interpreted with two state-of-the-art nuclear theories. For the first time, a long sequence of isotopes could be calculated with coupled-cluster calculations based on newly developed nuclear interactions. The strong increase in the charge radii beyond $N = 28$ is not well captured by these calculations, but is well reproduced by Fayans nuclear density functional theory, which, however, overestimates the odd-even staggering effect. These findings highlight our limited understanding on the nuclear size of neutron-rich systems, and expose pressing problems that are present in some of the best current models of nuclear theory.
We present precision Penning-trap mass measurements of neutron-rich calcium and potassium isotopes in the vicinity of neutron number N=32. Using the TITAN system the mass of $^{51}$K was measured for the first time, and the precision of the $^{51,52}$Ca mass values were improved significantly. The new mass values show a dramatic increase of the binding energy compared to those reported in the atomic mass evaluation. In particular, $^{52}$Ca is more bound by 1.74 MeV, and the behavior with neutron number deviates substantially from the tabulated values. An increased binding was predicted recent…
We report on the measurement of optical isotope shifts for $^{38,39,42,44,46\text{-}51}$K relative to $^{47}$K from which changes in the nuclear mean square charge radii across the N=28 shell closure are deduced. The investigation was carried out by bunched-beam collinear laser spectroscopy at the CERN-ISOLDE radioactive ion-beam facility. Mean square charge radii are now known from $^{37}$K to $^{51}$K, covering all $νf_{7/2}$-shell as well as all $νp_{3/2}$-shell nuclei. These measurements, in conjunction with those of Ca, Cr, Mn and Fe, provide a first insight into the $Z$ dependence of the…
\item[Background] Ground-state spins and magnetic moments are sensitive to the nuclear wave function, thus they are powerful probes to study the nuclear structure of isotopes far from stability. \item[Purpose] Extend our knowledge about the evolution of the $1/2^+$ and $3/2^+$ states for K isotopes beyond the $N = 28$ shell gap. \item[Method] High-resolution collinear laser spectroscopy on bunched atomic beams. \item[Results] From measured hyperfine structure spectra of K isotopes, nuclear spins and magnetic moments of the ground states were obtained for isotopes from $N = 19$ up to $N = 32$. …
The recently confirmed neutron-shell closure at N = 32 has been investigated for the first time below the magic proton number Z = 20 with mass measurements of the exotic isotopes 52,53K, the latter being the shortest-lived nuclide investigated at the online mass spectrometer ISOLTRAP. The resulting two-neutron separation energies reveal a 3 MeV shell gap at N = 32, slightly lower than for 52Ca, highlighting the doubly-magic nature of this nuclide. Skyrme-Hartree-Fock-Boguliubov and ab initio Gorkov-Green function calculations are challenged by the new measurements but reproduce qualitatively t…
Using inelastic $α$-scattering at extremely forward angles, including $0^\circ$, the strength distributions of the isoscalar giant monopole resonance (ISGMR) have been measured in the $^{204,206,208}$Pb isotopes in order to examine the proposed mutually enhanced magicity (MEM) effect on the nuclear incompressibility. The MEM effect had been suggested as a likely explanation of the "softness" of nuclear incompressibility observed in the ISGMR measurements in the Sn and Cd isotopes. Our experimental results rule out any manifestation of the MEM effect in nuclear incompressibility and leave the q…
Two-neutron transfer associated with the pair correlation in superfluid neutron-rich nuclei is studied with focus on low-lying $0^+$ states in Sn isotopes beyond the N=82 magic number. We describe microscopically the two-neutron addition and removal transitions by means of the Skyrme-Hartree-Fock-Bogoliubov mean-field model and the continuum quasiparticle random phase approximation formulated in the coordinate space representation. It is found that the pair transfer strength for the transitions between the ground states becomes significantly large for the isotopes with $A \ge 140$, reflecting …
Levels of trace radiopurity in active detector materials is a subject of major concern in low-background experiments. Among the radio-isotopes, $\k40$ is one of the most abundant and yet whose signatures are difficult to reject. Procedures were devised to measure trace potassium concentrations in the inorganic salt CsI as well as in organic liquid scintillator (LS) with Accelerator Mass Spectrometry (AMS), giving, respectively, the $\k40$-contamination levels of $\sim 10^{-10}$ and $\sim 10^{-13}$ g/g. Measurement flexibilities and sensitivities are improved over conventional methods. The proj…
The variation of E(2+_1) of (134-140)Sn calculated with empirical SMPN interaction has striking similarity with that of experimental E(2+_1) of even-even (18-22)O and (42-48)Ca, showing clearly that N=84-88 spectra exhibit the effect of gradual filling up of ν(2f_{7/2}) orbital which finally culminates in a new shell closure at N=90. Realistic two-body interaction CWG does not show this feature. Spin-tensor decomposition of SMPN and CWG interactions and variation of their components with valence neutron number reveals that the origin of the shell closure at 140Sn lies in the three body effects…
The nuclear shell structure, which originates in the nearly independent motion of nucleons in an average potential, provides an important guide for our understanding of nuclear structure and the underlying nuclear forces. Its most remarkable fingerprint is the existence of the so-called `magic numbers' of protons and neutrons associated with extra stability. Although the introduction of a phenomenological spin-orbit (SO) coupling force in 1949 helped explain the nuclear magic numbers, its origins are still open questions. Here, we present experimental evidence for the smallest SO-originated ma…
Despite being a complex many-body system, the atomic nucleus exhibits simple structures for certain "magic" numbers of protons and neutrons. The calcium chain in particular is both unique and puzzling: evidence of doubly-magic features are known in 40,48Ca, and recently suggested in two radioactive isotopes, 52,54Ca. Although many properties of experimentally known Ca isotopes have been successfully described by nuclear theory, it is still a challenge to predict their charge radii evolution. Here we present the first measurements of the charge radii of 49,51,52Ca, obtained from laser spectrosc…
N=Z nuclei above Ni are understood to be waiting-point nuclei in the rp-process nucleosynthesis. Investigating the experimental isotope shifts in Kr isotopes near the proton drip-line, we have discovered that N=Z rp-process nuclei $^{68}$Se, $^{72}$Kr, $^{76}$Sr and $^{80}$Zr exhibit a significant shell gap both at the proton and neutron numbers in the deformed space with the consequence that pairing correlations for protons and neutrons vanish, thus lending a double-magic character to these nuclei. A significant number of nuclei in this region are also shown to exhibit neutron magicity at N =…
Understanding and predicting the formation of shell structure from nuclear forces is a central challenge for nuclear physics. While the magic numbers N=2,8,20 are generally well understood, N=28 is the first standard magic number that is not reproduced in microscopic theories with two-nucleon forces. In this Letter, we show that three-nucleon forces give rise to repulsive interactions between two valence neutrons that are key to explain 48Ca as a magic nucleus, with a high 2+ excitation energy and a concentrated magnetic dipole transition strength. The repulsive three-nucleon mechanism improve…
The shapes of neutron-rich exotic Ni isotopes are studied. Large-scale shell model calculations are performed by advanced Monte Carlo Shell Model (MCSM) for the $pf$-$g_{9/2}$-$d_{5/2}$ model space. Experimental energy levels are reproduced well by a single fixed Hamiltonian. Intrinsic shapes are analyzed for MCSM eigenstates. Intriguing interplays among spherical, oblate, prolate and gamma-unstable shapes are seen including shape fluctuations, $E$(5)-like situation, the magicity of doubly-magic $^{56,68,78}$Ni, and the coexistence of spherical and strongly deformed shapes. Regarding the last …
We link the structure of nuclei around $^{100}$Sn, the heaviest doubly magic nucleus with equal neutron and proton numbers ($N=Z=50$), to nucleon-nucleon ($NN$) and three-nucleon ($NNN$) forces constrained by data of few-nucleon systems. Our results indicate that $^{100}$Sn is doubly magic, and we predict its quadrupole collectivity. We present precise computations of $^{101}$Sn based on three-particle--two-hole excitations of $^{100}$Sn, and reproduce the small splitting between the lowest $J^π=7/2^+$ and $5/2^+$ states. Our results are consistent with the sparse available data.
New data on proton and neutron single-particle energies $E_{nlj}$ of Si isotopes with neutron number $N$ from 12 to 28 as well as occupation probabilities $N_{nlj}$ of single particle states of stable isotopes $^{28,30}$Si near the Fermi energy were obtained by the joint evaluation of the stripping and pick-up reaction data and excited state decay schemes of neighboring nuclei. The evaluated data indicate following features of single-particle structure evolution: persistence of $Z = 14$ subshell closure with $N$ increase, the new magicity of the number $N = 16$, and the conservation of the mag…
The paper reports on the first observation of doubly-magic Nickel-48 in an experimental at the SISSI/LISE3 facility of GANIL. Four Nickel-48 isotopes were identified. In addition, roughly 100 Nickel-49, 50 Iron-45, and 290 Chromium-42 isotopes were observed. This opens the possibility to search for two-proton emission from these nuclei.
Using two theoretical models (the post form finite range distorted wave Born approximation and the adiabatic model) we calculate the parallel momentum distribution of the charged core in the Coulomb breakup of Be isotopes on a heavy target at 100 MeV/u. We show that the full width at half maxima of the parallel momentum distribution can be used to study the breakdown of N = 8 magic number away from the valley of stability.
In this paper, we present direct mass measurements of neutron-rich $^{86}$Kr projectile fragments conducted at the HIRFL-CSR facility in Lanzhou by employing the Isochronous Mass Spectrometry (IMS) method. The new mass excesses of $^{52-54}$Sc nuclides are determined to be -40492(82), -38928(114), -34654(540) keV, which show a significant increase of binding energy compared to the reported ones in the Atomic Mass Evaluation 2012 (AME12). In particular, $^{53}$Sc and $^{54}$Sc are more bound by 0.8 MeV and 1.0 MeV, respectively. The behavior of the two neutron separation energy with neutron num…
In this paper we study the issue of the puzzle of the radii of calcium isotopes. Despite an excess of eight neutrons, strangely $^{48}{\rm Ca}$ exhibits essentially the same charge radius as $^{40}{\rm Ca}$ does. A fundamental microscopic description of this is still lacking. Also strange is a peak in charge radius of calcium at N = 24. The $^{52}{\rm Ca}$ (N = 32) nucleus, well known to be doubly magical, amazingly has recently been found to have a very large charge radius. Also amazing is the property of $^{42}_{14}{\rm Si}_{28}$ which simultaneously appears to be both magical/spherical and …
The self-consistent Theory of Finite Fermi Systems based on the Energy Density Functional by Fayans et al. with the set DF3-a of parameters fixed previously is used to calculate three kinds of quadrupole moments. At first, we examined systematically quadrupole moments of odd neighbors of semi-magic lead and tin isotopes and $N=50,N=82$ isotones. Second, we found quadrupole moments of the first $2^+$ states in the same two chains of isotopes. Finally, we evaluated quadrupole moments of odd-odd nuclei neighboring to double magic ones. Reasonable agreement with available experimental data has bee…
Interaction cross sections for $^{42\textrm{-}51}$Ca on a carbon target at 280 MeV/nucleon have been measured for the first time. The neutron number dependence of derived root-mean-square matter radii shows a significant increase beyond the neutron magic number $N=28$. Furthermore, this enhancement of matter radii is much larger than that of the previously measured charge radii, indicating a novel growth in neutron skin thickness. A simple examination based on the Fermi-type distribution, and the Mean-Field calculations point out that this anomalous enhancement of the nuclear size beyond $N=28…
In rapid-proton capture (rp-process), N=Z nuclei above Ni are understood to act as waiting-point nuclei. The N=Z nuclei 68Se, 72Kr, 76Sr and 80Zr among others are known to give rise to a large-energy x-ray flux and peaks in abundances of these nuclei synthesized in the astrophysical rp-process. Investigating the experimental isotope shifts in Kr isotopes near the proton drip-line within the framework of the deformed Relativistic Hartree-Bogoliubov theory, we have discovered that N=Z rp-process nuclei 68Se, 72Kr, 76Sr and 80Zr exhibit large shell gap both at the proton and neutron numbers in th…
$β$-decay rates play a decisive role in understanding the nucleosynthesis of heavy elements and are governed by microscopic nuclear-structure information. A sudden shortening of the half-lives of Ni isotopes beyond $N=50$ was observed at the RIKEN-RIBF. This is considered due to the persistence of the neutron magic number $N=50$ in the very neutron-rich Ni isotopes. By systematically studying the $β$-decay rates and strength distributions in the neutron-rich Ni isotopes around $N=50$, I try to understand the microscopic mechanism for the observed sudden shortening of the half-lives. The $β$-st…
We present the first ab initio calculations for open-shell nuclei past the tin isotopic line, focusing on Xe isotopes as well as doubly-magic Sn isotopes. We show that, even for moderately hard interactions, it is possible to obtain meaningful predictions and that the NNLOsat chiral interaction predicts radii and charge density distributions close to the experiment. We then make a new prediction for ${}^{100}$Sn. This paves the way for ab initio studies of exotic charge density distributions at the limit of the present ab initio mass domain, where experimental data is becoming available. The p…
Recent experimental observation of magicity in $^{78}$Ni has infused the interest to examine the persistence of the magic character across the N$=$50 shell gap in extremely neutron rich exotic nucleus $^{78}$Ni in ground as well as excited states. A systematic study of Ni isotopes and N$=$50 isotones in ground state is performed within the microscopic framework of relativistic mean-field (RMF) and the triaxially deformed Nilson Strutinsky model (NSM). Ground state density distributions, charge form factors, radii, separation energies, pairing energies, single particle energies and the shell co…
High-precision mass measurements of more than thirty neutron-rich nuclides around the Z=28 closed proton shell were performed with the triple-trap mass spectrometer ISOLTRAP at ISOLDE/CERN to address the question of a possible neutron shell closure at N=40. The results, for 57,60,64-69Ni (Z=28), 65-74,76Cu (Z=29), and 63-65,68-78Ga (Z=31), have a relative uncertainty of the order of 10^8. In particular, the masses of 72-74,76Cu have been measured for the first time. We analyse the resulting mass surface for signs of magicity, comparing the behavior of N=40 to that of known magic numbers and to…
The exotic phenomenon of two-neutron halos and 2n-radioactivity are explored in the neutron-rich $^{40,42,44}$Mg by employing various variants of the relativistic mean-field approach. The extended tail of spatial density distributions including the enhanced neutron radii and skin thickness, pairing correlations, single-particle spectrum and wave functions predict $^{40,42,44}$Mg to be strong candidates for deformed neutron halos. Weakening of magicity at N$=$28 plays a significant role in the existence of a weakly bound halo in $^{40}$Mg which is currently the heaviest isotope of Mg accessible…
The study of high-spin states in regions of doubly-magic nuclei performed with the use of deep-inelastic heavy ion reactions is reviewed. New and tentative results concerning high-spin states in the 48Ca and yrast structures in 47Ca, 47K, 49Ca and 49Sc isotopes are presented. The status of the high-spin state study in the region of 132Sn and 208Pb is outlined, including discussion of recently obtained results in the 208Pb core and the 206Hg two-proton-hole nucleus.
Doubly magic nuclei have a simple structure and are the cornerstones for entire regions of the nuclear chart. Theoretical insights into the supposedly doubly magic $^{78}$Ni and its neighbors are challenging because of the extreme neutron-to-proton ratio and the proximity of the continuum. We predict the $J^π=2_1^+$ state in $^{78}$Ni from a correlation with the $J^π=2_1^+$ state in $^{48}$Ca using chiral nucleon-nucleon and three-nucleon interactions. Our results confirm that $^{78}$Ni is doubly magic, and the predicted low-lying states of $^{79,80}$Ni open the way for shell-model studies of …
Systematic trends in nuclear charge radii are of great interest due to universal shell effects and odd-even staggering (OES). The modified root mean square (rms) charge radius formula, which phenomenologically accounts for the formation of neutron-proton ($np$) correlations, is here applied for the first time to the study of odd-$Z$ copper and indium isotopes. Theoretical results obtained by the relativistic mean field (RMF) model with NL3, PK1 and NL3$^{*}$ parameter sets are compared with experimental data. Our results show that both OES and the abrupt changes across $N=50$ and $82$ shell cl…
We study the spectra of neutron-rich oxygen isotopes based on chiral two- and three-nucleon interactions. First, we benchmark our many-body approach by comparing ground-state energies to coupled-cluster results for the same two-nucleon interaction, with overall good agreement. We then calculate bound excited states in 21,22,23O, focusing on the role of three-nucleon forces, in the standard sd shell and an extended sdf7/2p3/2 valence space. Chiral three-nucleon forces provide important one- and two-body contributions between valence neutrons. We find that both these contributions and an extende…
We probe the $N=82$ nuclear shell closure by mass measurements of neutron-rich cadmium isotopes with the ISOLTRAP spectrometer at ISOLDE-CERN. The new mass of $^{132}$Cd offers the first value of the $N=82$, two-neutron shell gap below $Z=50$ and confirms the phenomenon of mutually enhanced magicity at $^{132}$Sn. Using the recently implemented phase-imaging ion-cyclotron-resonance method, the ordering of the low-lying isomers in $^{129}$Cd and their energies are determined. The new experimental findings are used to test large-scale shell-model, mean-field and beyond-mean-field calculations, a…
We report high-precision mass measurements of $^{50-55}$Sc isotopes performed at the LEBIT facility at NSCL and at the TITAN facility at TRIUMF. Our results provide a substantial reduction of their uncertainties and indicate significant deviations, up to 0.7 MeV, from the previously recommended mass values for $^{53-55}$Sc. The results of this work provide an important update to the description of emerging closed-shell phenomena at neutron numbers $N=32$ and $N=34$ above proton-magic $Z=20$. In particular, they finally enable a complete and precise characterization of the trends in ground stat…
The evolution of quadrupole and octupole collectivity in neutron-deficient Xe, Ba, Ce, and Nd nuclei near the "octupole magic" neutron number $N=56$ is investigated within the mapped $sdf$-IBM framework. Microscopic input is obtained via quadrupole and octupole constrained Hartree-Fock-Bogoliubov calculations, based on the parametrization D1M of the Gogny energy density functional. Octupole-deformed mean-field ground states are predicted for Ba and Ce isotopes near $N=56$. Excitation energies of positive- and negative-parity states as well as electric transition rates are computed with wave fu…
Nuclear magic numbers, which emerge from the strong nuclear force based on quantum chromodynamics, correspond to fully occupied energy shells of protons, or neutrons inside atomic nuclei. Doubly magic nuclei, with magic numbers for both protons and neutrons, are spherical and extremely rare across the nuclear landscape. While the sequence of magic numbers is well established for stable nuclei, evidence reveals modifications for nuclei with a large proton-to-neutron asymmetry. Here, we provide the first spectroscopic study of the doubly magic nucleus $^{78}$Ni, fourteen neutrons beyond the last…
Photoneutron cross sections were measured for $^{137}$Ba and $^{138}$Ba at energies below two-neutron threshold using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The photoneutron data are used to constrain the $γ$-ray strength function on the basis of the Hartree-Fock-Bogolyubov plus quasi-particle random phase approximation using the Gogny D1M interaction. Supplementing the experimentally constrained $γ$-ray strength function with the zero-limit E1 and M1 contributions which are unique to the deexcitation mode, we dis…
Rare isotope beams of neutron-deficient $^{106,108,110}$Sn nuclei from the fragmentation of $^{124}$Xe were employed in an intermediate-energy Coulomb excitation experiment yielding $B(E2, 0^+_1 \to 2^+_1)$ transition strengths. The results indicate that these $B(E2,0^+_1 \to 2^+_1)$ values are much larger than predicted by current state-of-the-art shell model calculations. This discrepancy can be explained if protons from within the Z = 50 shell are contributing to the structure of low-energy excited states in this region. Such contributions imply a breaking of the doubly-magic $^{100}$Sn cor…
We report first precision mass measurements of the $1/2^-$ isomeric and $9/2^+$ ground states of $^{101}$In. The determined isomeric excitation energy continues a smooth trend of odd-$A$ indium isotopes up to the immediate vicinity of $N=50$ magic number. This trend can be confirmed by dedicated shell model calculations only if the neutron configuration mixing is considered. We find that the single particle energies are different for different states of the same isotope. The presented configuration-dependent shell evolution, type II shell evolution, in odd-$A$ nuclei is discussed for the first…
Accurate atomic mass measurements of neutron-deficient and neutron-rich nuclides around the doubly-magic 208Pb and of neutron-rich cesium isotopes were performed with the Penning trap mass spectrometer ISOLTRAP at ISOLDE/CERN. The masses of 145,147Cs, 181,183Tl, 186Tlm, 187Tl, 196Tlm, 205Tl, 197Pbm, 208Pb, 190 to 197Bi, 209,215,216Bi, 203,205,229Fr, and 214,229,230Ra were determined. The obtained relative mass uncertainty in the range of $2 \cdot 10^{-7}$ to $2 \cdot 10^{-8}$ is not only required for safe identification of isomeric states but also allows mapping the detailed structure of the m…
Nuclear charge radii of $^{55,56}$Ni were measured by collinear laser spectroscopy. The obtained information completes the behavior of the charge radii at the shell closure of the doubly magic nucleus $^{56}$Ni. The trend of charge radii across the shell closures in calcium and nickel is surprisingly similar despite the fact that the $^{56}$Ni core is supposed to be much softer than the $^{48}$Ca core. The very low magnetic moment $μ(^{55}\mathrm{Ni})=-1.108(20)\,μ_N$ indicates the impact of M1 excitations between spin-orbit partners across the $N,Z=28$ shell gaps. Our charge-radii results are…
Nuclear spins and precise values of the magnetic dipole and electric quadrupole moments of the ground-states of neutron-rich $^{76-78}$Cu isotopes were measured using the Collinear Resonance Ionization Spectroscopy (CRIS) experiment at ISOLDE, CERN. The nuclear moments of the less exotic $^{73,75}$Cu isotopes were re-measured with similar precision, yielding values that are consistent with earlier measurements. The moments of the odd-odd isotopes, and $^{78}_{29}$Cu ($N=49$) in particular, are used to investigate excitations of the assumed doubly-magic $^{78}$Ni core through comparisons with l…
The electric quadrupole moment of $^{49}$Sc was measured by collinear laser spectroscopy at CERN-ISOLDE to be $Q_{\rm s}=-0.159(8)$ $e$b, and a nearly tenfold improvement in precision was reached for the electromagnetic moments of $^{47,49}$Sc. The single-particle behavior and nucleon-nucleon correlations are investigated with the electromagnetic moments of $Z=21$ isotopes and $N=28$ isotones as valence neutrons and protons fill the distinctive $0f_{7/2}$ orbit, respectively, located between magic numbers, 20 and 28. The experimental data are interpreted with shell-model calculations using an …
The nuclear potential and resulting shell structure are well established for the valley of stability, however, dramatic modifications to the familiar ordering of single-particle orbitals in rare isotopes with a large imbalance of proton and neutron numbers have been found: new shell gaps emerge and conventional magic numbers are no longer valid. This article outlines some of the recent in-beam gamma-ray spectroscopy measurements at NSCL aimed at shedding light on the evolution of nuclear structure around neutron number N = 28 in neutron-rich Ar and S isotopes.
We present the results of precision mass measurements of neutron-rich cadmium isotopes. These nuclei approach the $N=82$ closed neutron shell and are important to nuclear structure as they lie near doubly-magic $^{132}$Sn on the chart of nuclides. Of particular note is the clear identification of the ground state mass in $^{127}$Cd along with the isomeric state. We show that the ground state identified in a previous mass measurement which dominates the mass value in the Atomic Mass Evaluation is an isomeric state. In addition to $^{127/m}$Cd, we present other cadmium masses measured ($^{125/m}…
Mass measurements on radionuclides along the potassium isotope chain have been performed with the ISOLTRAP Penning trap mass spectrometer. For 35K T1/2=178ms) to 46K (T1/2=105s) relative mass uncertainties of 2x10-8 and better have been achieved. The accurate mass determination of 35K (dm=0.54keV) has been exploited to test the Isobaric Multiplet Mass Equation (IMME) for the A=35, T=3/2 isospinquartet. The experimental results indicate a deviation from the generally adopted quadratic form.
Characterizing the nature of single-particle states outside of double shell closures is essential to a fundamental understanding of nuclear structure. This is especially true for those doubly magic nuclei that lie far from stability and where the shell closures influence nucleo-synthetic pathways. The region around $^{100}$Sn is one of the most important due to the proximity of the N=Z=50 magic numbers, the proton-drip line, and the end of the rp-process. However, owing to the low production rates, there is a lack of spectroscopic information and no firm spin-parity assignment for ground state…