Imaging through scattering and random media is an outstanding problem that to date has been tackled by either measuring the medium transmission matrix or exploiting linear correlations in the transmitted speckle patterns. However, transmission matrix techniques require interferometric stability and linear correlations, such as the memory effect, can be exploited only in thin scattering media. Here we show the existence of a statistical dependency in strongly scattered optical fields in a case where first-order correlations are not expected. We also show that this statistical dependence and the related information transport is directly linked to artificial neural network imaging in strongly scattering, dynamic media. These non-trivial dependencies provide a key to imaging through dynamic and thick scattering media with applications for deep-tissue imaging or imaging through smoke or fog
We review our recent theoretical results on multiple scattering of waves in nonlinear disordered media. In particular, we discuss angular correlations of scattered waves, coherent backscattering cone, and the new phenomenon of temporal instability of multiply scattered waves in disordered media with sufficiently strong nonlinearity. Instability threshlod is derived, dynamics of speckle pattern beyond the threshold is discussed.
We experimentally measure the monochromatic transmission matrix (TM) of an optical multiple scattering medium using a spatial light modulator together with a phase-shifting interferometry measurement method. The TM contains all information needed to shape the scattered output field at will or to detect an image through the medium. We confront theory and experiment for these applications and we study the effect of noise on the reconstruction method. We also extracted from the TM informations about the statistical properties of the medium and the light transport whitin it. In particular, we are …
Spatial field correlation functions represent a key quantity for the description of mesoscopic phenomena in disordered media and the optical characterization of complex materials. Yet many aspects related to the vector nature of light waves have not been investigated so far. We study theoretically the polarization and coherence properties of electromagnetic waves produced by a dipole source in a three-dimensional uncorrelated disordered medium. The spatial field correlation matrix is calculated analytically using a multiple scattering theory for polarized light. This allows us to provide a for…
We develop a self-consistent theory of temporal fluctuations of a speckle pattern resulting from the multiple scattering of a coherent wave in a weakly nonlinear disordered medium. The speckle pattern is shown to become unstable if the nonlinearity exceeds a threshold value. The instability is due to a feedback provided by the multiple scattering and manifests itself in spontaneous fluctuations of the scattered intensity. The development of instability is independent of the sign of nonlinearity.
We consider the multiple scattering of a scalar wave in a disordered medium with a weak nonlinearity of Kerr type. The perturbation theory, developed to calculate the temporal autocorrelation function of scattered wave, fails at short correlation times. A self-consistent calculation shows that for nonlinearities exceeding a certain threshold value, the multiple-scattering speckle pattern becomes unstable and exhibits spontaneous fluctuations even in the absence of scatterer motion. The instability is due to a distributed feedback in the system "coherent wave + nonlinear disordered medium". The…
Disordered packings of colloidal spheres show angle-independent structural color when the particles are on the scale of the wavelength of visible light. Previous work has shown that the positions of the peaks in the reflectance spectra can be predicted accurately from a single-scattering model that accounts for the effective refractive index of the material. This agreement shows that the main color peak arises from short-range correlations between particles. However, the single-scattering model does not quantitatively reproduce the observed color: the main peak in the reflectance spectrum is m…
The irradiation of a dilute cloud of cold atoms with a coherent light field produces a random intensity distribution known as laser speckle. Its statistical fluctuations contain information about the mesoscopic scattering processes at work inside the disordered medium. Following up on earlier work by Assaf and Akkermans [Phys.\ Rev.\ Lett.\ \textbf{98}, 083601 (2007)], we analyze how static speckle intensity correlations are affected by an internal Zeeman degeneracy of the scattering atoms. It is proven on general grounds that the speckle correlations cannot exceed the standard Rayleigh law. O…
The polarization of a coherent depolarized incident light beam passing through a disordered medium is investigated. The local polarization of the scattered far field and the probability density function are calculated and show an excellent agreement with experiment. It is demonstrated that complex media may confer high degree of polarization (0.75 DOP average) to the incident unpolarized light.
Speckle patterns generated in a disordered medium carry a lot of information despite the apparent complete randomness in the intensity pattern. When the medium possesses $χ^{(2)}$ nonlinearity, the speckle is sensitive to the phase of the incident fundamental light, as well as the light generated within. Here, we examine the speckle decorrelation in the fundamental and second-harmonic transmitted light as a function of varying power in the fundamental beam. At low incident powers, the speckle patterns produced by successive pulses exhibit strong correlations, that decrease with increasing powe…
We consider the information content h of a scalar multiple-scattered, diffuse wave field $ψ(\vec{r})$ and the information capacity C of a communication channel that employs diffuse waves to transfer the information through a disordered medium. Both h and C are shown to be directly related to the mesoscopic correlations between the values of $ψ(\vec{r})$ at different positions $\vec{r}$ in space, arising due to the coherent nature of the wave. For the particular case of a communication channel between two identical linear arrays of $n \gg 1$ equally-spaced transmitters/receivers (receiver spaci…
The reflection and transmission amplitudes of waves in disordered multimode waveguides are studied by means of numerical simulations based on the invariant embedding equations. In particular, we analyze the influence of surface-type disorder on the behavior of the ensemble average and fluctuations of the reflection and transmission coefficients, reflectance, transmittance, and conductance. Our results show anomalous effects stemming from the combination of mode dispersion and rough surface scattering: For a given waveguide length, the larger the mode transverse momentum is, the more strongly i…
The purpose of this work is to understand the fundamental connection between structural correlations and light localization in three-dimensional (3D) open scattering systems of finite size. We numerically investigate the transport of vector electromagnetic waves scattered by resonant electric dipoles spatially arranged in 3D space by stealthy hyperuniform disordered point patterns. Three-dimensional stealthy hyperuniform disordered systems (3D-SHDS) are engineered with different structural correlation properties determined by their degree of stealthiness $χ$. Such fine control of exotic states…
The propagation of light through a random medium is an important problem in photonics. When the random fluctuations of the orientation for individual rods were introduced to the ideal woodpile photonic structure, a crossover from Laue diffraction to randomly scattered fields which is similar in appearance to speckle patterns was observed and investigated. Unexpected interplay between order and disorder was discovered from anisotropic glassy samples when orientational disorder was added only in one direction of square woodpile structure. It is found that the ordered sets of rods produced disord…
Strong suppression of the photonic density of states in three-dimensional disordered silicon networks
University of Fribourg（弗里堡大学）；Université Côte d’Azur（蔚蓝海岸大学）；CNRS, Institut de Physique de Nice – INPHYNI（法国国家科学研究中心，尼斯物理研究所-INPHYNI）；Optoelectronics Research Centre, University of Southampton（南安普顿大学光电研究中心）
Disordered optical media are an emerging class of materials capable of strongly scattering light. Their study is relevant to investigate transport phenomena and for applications in imaging, sensing and energy storage. While such materials can be used to generate coherent light, their directional emission is typically hampered by their very multiple scattering nature. Here, we tune the out-of-plane directionality of coherent Raman light scattered by a fractal network of silicon nanowires. By visualizing Rayleigh scattering, photoluminescence and weakly localized Raman light from the random netw…
We report a method to characterize the propagation of an ultrashort pulse of light through a multiple scattering medium by measuring its time-resolved transmission matrix. This method is based on the use of a spatial light modulator together with a coherent time-gated detection of the transmitted speckle field. Using this matrix, we demonstrate the focusing of the scattered pulse at any arbitrary position in space and time after the medium. Our approach opens new perspectives for both fundamental studies and applications in imaging and coherent control in disordered media.
Understanding the scattering properties of various media is of critical importance in many applications, from secure, high-bandwidth communications to extracting information about biological and mineral particles dissolved in sea water. In this paper we demonstrate how beams carrying orbital angular momentum (OAM) can be used to detect the presence of symmetric or chiral subsets of particles in disordered media. Using a generalized Mie theory we calculate analytical expressions for quasi-monochromatic structured light scattered by dilute distributions of micro- and nanoparticles. These allow u…
Complex dielectric media often appear opaque because light traveling through them is scattered multiple times. Although the light scattering is a random process, different paths through the medium can be correlated encoding information about the medium. Here, we present spectroscopic measurements of nonuniversal intensity correlations that emerge when embedding quantum emitters inside a disordered photonic crystal that is found to Anderson-localize light. The emitters probe in-situ the microscopic details of the medium, and imprint such near-field properties onto the far-field correlations. Ou…
On the basis of general theoretical results developed previously in [JETP 112, 246 (2011)], we analyze the reflection of quasiresonant light from a plane surface of dense and disordered ensemble of motionless point scatters. Angle distribution of the scattered light is calculated both for s and p polarizations of the probe radiation. The ratio between coherent and incoherent (diffuse) components of scattered light is calculated. We analyze the contributions of scatters located at different distances from the surface and determine on this background the thickness of surface layer responsible fo…
Transmission eigenchannels are building blocks of coherent wave transport in diffusive media, and selective excitation of individual eigenchannels can lead to diverse transport behavior. An essential yet poorly understood property is the transverse spatial profile of each eigenchannel, which is critical for coupling into and out of it. Here, we discover that the transmission eigenchannels of a disordered slab possess localized incident and outgoing profiles, even in the diffusive regime far from Anderson localization. Such transverse localization arises from a combination of reciprocity, local…
We present angular-resolved correlation measurements between photons after propagation through a three-dimensional disordered medium. The multiple scattering process induces photon correlations that are directly measured for light sources with different photon statistics. We find that multiple scattered photons between different angular directions with angles much larger than the average speckle width are strongly correlated. The time dependence of the angular photon correlation function is investigated and the coherence time of the light source is determined. Our results are found to be in ex…
Scattering has usually be considered as detrimental for optical focusing or imaging. Recently, more and more research has shown that strongly scattering materials can be utilized to focus coherent light by controlling or shaping the incident light. Here, purposeful focusing of second-harmonic waves, which are generated and scattered from nonlinear turbid media via feedback-based wavefront shaping is presented. This work shows a flexible manipulation of both disordered linear and nonlinear scattering signals, indicating more controllable degrees of freedom for the description of turbid media. T…
Focusing light inside scattering media in a freely addressable fashion is challenging, as the wavefront of the scattered light is highly disordered. Recently developed ultrasound-guided wavefront shaping methods are addressing this challenge, albeit with relatively low modulation efficiency and resolution limitations. In this paper, we present a new technique, time-reversed ultrasound microbubble encoded (TRUME) optical focusing, which is able to focus light with improved efficiency and sub-ultrasound wavelength resolution. This method ultrasonically destructs microbubbles, and measures the wa…
The brilliant white appearance of ultrathin scattering media with low refractive index contrast and the underlying radiative transport phenomena fascinate scientists for more than a decade. Examples of such systems are the scales of beetles of the genus Cyphochilus, photonic network structures or disordered Bragg stacks (DBS). While previous studies relate the highly efficient scattering in the scales to the anisotropy of the intra-scale network and diffusive light transport, the coherent radiation propagation dynamics remained unaccounted for. Here, we identify different coherent light transp…
We show that coherent multiple light scattering, or diffuse light propagation, in a disordered atomic medium, prepared at ultra-low temperatures, can be be effectively delayed in the presence of a strong control field initiating a stimulated Raman process. On a relatively short time scale, when the atomic system can preserve its configuration and effects of atomic motion can be ignored, the scattered signal pulse, diffusely propagating via multiple coherent scattering through the medium, can be stored in the spin subsystem through its stimulated Raman-type conversion into spin coherence. We de…
We introduce a numerical method that enables efficient modelling of light scattering by large, disordered ensembles of non-spherical particles incorporated in stratified media, including when the particles are in close vicinity to each other, to planar interfaces and/or to localized light sources. The method consists in finding a small set of fictitious polarizable elements -- or numerical dipoles -- that quantitatively reproduces the field scattered by an individual particle for any excitation and at an arbitrary distance from the particle surface. The set of numerical dipoles is described by…
New materials aim at exploiting the great control of living organisms over molecular architectures and minerals. Optical biomimetics has been widely developed by microengineering, leading to photonic components with order resembling those found in plants and animals. These systems, however, are realized by complicated and adverse processes. Here we show how biomineralization might enable the one-step generation of components for amorphous photonics, in which light is made to travel through disordered scattering systems, and particularly of active devices such as random lasers, by using electro…
An optical imaging system forms an object image by recollecting light scattered by the object. However, intact optical information of the object delivered through the imaging system is deteriorated by imperfect optical elements and unwanted defects. Image deconvolution, also known as inverse filtering, has been widely exploited as a recovery technique because of its practical feasibility, and operates by assuming the linear shift-invariant property of the imaging system. However, shift invariance is not rigorously hold in all imaging situations and it is not a necessary condition for solving t…
The coupling of atomic arrays and one-dimensional subwavelength waveguides gives rise to in- teresting photon transport properties, such as recent experimental demonstrations of large Bragg reflection and paves the way for a variety of potential applications in the field of quantum non-linear optics. Here, we present a theoretical analysis for the process of single-photon scattering in this configuration using a full microscopic approach. Based on this formalism, we analyze the spectral dependencies for different scattering channels from either ordered or disordered arrays. The de- veloped app…
Light scattering in disordered media has been studied extensively due to its prevalence in natural and artificial systems [1]. In the field of photonics most of the research has focused on understanding and mitigating the effects of scattering, which are often detrimental. For certain applications, however, intentionally introducing disorder can actually improve the device performance, e.g., in photovoltaics optical scattering improves the efficiency of light harvesting [2-5]. Here, we utilize multiple scattering in a random photonic structure to build a compact on-chip spectrometer. The probe…
