Impurity physics is a traditional topic in condensed matter physics that nowadays is being explored in the field of ultracold gases. Among the different classes of impurities, we focus on charged impurities in an ultracold bath. When a single ion is brought in contact with an ultracold gas it is subjected to different reactive processes that can be understood from a cold chemistry approach. In this work, we present an outlook of approaches for the dynamics of a single ion in a bath of ultracold atoms or molecules, complementing the usual many-body approaches characteristic of impurity physics within condensed matter physics. In particular, we focus on the evolution of a charged impurity in different baths, including external time-dependent trapping potentials and we explore the effect of the external laser sources present in ion-neutral hybrid traps into the lifetime of an impurity.
We report on controlled doping of an ultracold Rb gas with single neutral Cs impurity atoms. Elastic two-body collisions lead to a rapid thermalization of the impurity inside the Rb gas, representing the first realization of an ultracold gas doped with a precisely known number of impurity atoms interacting via s-wave collisions. Inelastic interactions are restricted to a single three-body recombination channel in a highly controlled and pure setting, which allows to determine the Rb-Rb-Cs three-body loss rate with unprecedented precision. Our results pave the way for a coherently interacting h…
We study the transport, decoherence and dissipation of an impurity interacting with a bath of free fermions in a one-dimensional lattice. Numerical simulations are made with the time-evolving block decimation method. We introduce a mass imbalance between the impurity and bath particles and find that the fastest decoherence occurs for a light impurity in a bath of heavy particles. By contrast, the fastest dissipation of energy occurs when the masses are equal. We present a simple model for decoherence in the heavy bath limit, and a linear density response description of the interaction which pr…
We consider a localized impurity atom that interacts with a cloud of fermions in the paired state. We develop an effective scattering length description of the interaction between an impurity and a fermionic atom using their vacuum scattering length. Treating the pairing of fermions at the mean-field level, we show that the impurity atom acts like a magnetic impurity in the condensed matter context, and leads to the formation of a pair of Shiba bound states inside the superconducting gap. In addition, the impurity atom can lead to the formation of deeply bound states below the Fermi sea.
In their Comment [1] Giraud and Combescot point out that the contribution to the impurity-boson distribution function $ρ_{bi}(x-y)$ of a term we dropped is not negligible, rather than being negligible in the thermodynamic limit as we had conjectured. We now agree with them, but nevertheless our results for $ρ_{bi}$ are highly accurate for large impurity-boson mass ratio $m_i/m$ and remain qualitatively correct for all values of $m_i/m$ and all values of the boson-impurity coupling constant.
Very recently Girardeau and Minguzzi [arXiv:0807.3366v2, Phys. Rev. A 79, 033610 (2009)] have studied an impurity in a one-dimensional gas of hard-core bosons. In particular they deal with the general case where the mass of the impurity is different from the mass of the bosons and the impurity-boson interaction is not necessarily infinitely repulsive. We show that one of their initial step is erroneous, contradicting both physical intuition and known exact results. Their results in the general case apply only actually when the mass of the impurity is infinite.
Mobile-impurity dynamics in a non-Hermitian Stark-localised bath
Institute of Atomic and Molecular Sciences, Academia Sinica（台湾中央研究院原子与分子科学研究所）；Department of Physics, National Central University（中原大学物理系）；Physics Division, National Center for Theoretical Sciences（国家理论科学中心物理组）；Department of Physics, National Taiwan Normal University（台湾师范大学物理系）
We report Ramsey spectroscopy on the clock states of individual Cs impurities immersed in an ultracold Rb bath. We record both the interaction-driven phase evolution and the decay of fringe contrast of the Ramsey interference signal to obtain information about bath density or temperature nondestructively. The Ramsey fringe is modified by a differential shift of the collisional energy when the two Cs states superposed interact with the Rb bath. This differential shift is directly affected by the mean gas density and the details of the Rb-Cs interspecies scattering length, affecting the phase ev…
We study a single impurity driven by a constant force through a 1D Bose gas using a Lieb-Liniger based approach. Our calculaton is exact in the interaction amongst the particles in the Bose gas, and is perturbative in the interaction between the gas and the impurity. In contrast to previous studies of this problem, we are able to handle arbitrary interaction strength for the Bose gas. We find very good agreement with recent experiments [Phys. Rev. Lett. 103, 150601 (2009)].
The role of impurities as experimental probes in the detection of quantum material properties is well appreciated. Here we study the effect of a single classical magnetic impurity in trapped ultracold Fermi superfluids. Depending on its shape and strength, a magnetic impurity can induce single or multiple mid-gap bound states in a superfluid Fermi gas. The multiple mid-gap states could coincide with the development of a Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase within the superfluid. As an analog of the Scanning Tunneling Microscope, we propose a modified RF spectroscopic method to measure…
By means of time-dependent density-matrix renormalization-group (TDMRG) we are able to follow the real-time dynamics of a single impurity embedded in a one-dimensional bath of interacting bosons. We focus on the impurity breathing mode, which is found to be well-described by a single oscillation frequency and a damping rate. If the impurity is very weakly coupled to the bath, a Luttinger-liquid description is valid and the impurity suffers an Abraham-Lorentz radiation-reaction friction. For a large portion of the explored parameter space, the TDMRG results fall well beyond the Luttinger-liquid…
We explore the dynamical transport of an impurity between different embedding majority species which are spatially separated in a double well. The transfer and storage of the impurity is triggered by dynamically changing the interaction strengths between the impurity and the two majority species. We find a simple but efficient protocol consisting of linear ramps of majority-impurity interactions at designated times to pin or unpin the impurity. Our study of this highly imbalanced few-body triple mixture is conducted with the multi-layer multi-configuration time-dependent Hartree method for ato…
We explore the dynamics and the steady state of a driven quantum spin coupled to a bath of fermions, which can be realized with a strongly imbalanced mixture of ultracold atoms using currently available experimental tools. Radio-frequency driving can be used to induce tunneling between the spin states. The Rabi oscillations are modified due to the coupling of the quantum spin to the environment, which causes frequency renormalization and damping. The spin-bath coupling can be widely tuned by adjusting the scattering length through a Feshbach resonance. When the scattering potential creates a b…
We investigate the tunneling dynamics of an ultracold bosonic impurity species which interacts repulsively with a second, larger Bose gas. Both species are held in a finite-sized quasi-one-dimensional box potential. In addition, the impurity bosons experience a periodic potential generated by an optical lattice. We initially prepare our binary mixture in its ground state, such that the impurities and Bose gas are phase separated and the impurities localize pairwise in adjacent sites of the periodic potential, by tuning the interaction strengths and the lattice depth correspondingly. The dynami…
We present investigations of the formation rate and collisional stability of lithium Feshbach molecules in an ultracold three-component mixture composed of two resonantly interacting fermionic 6-Li spin states and bosonic 174-Yb. We observe long molecule lifetimes (> 100 ms) even in the presence of a large ytterbium bath and extract reaction rate coefficients of the system. We find good collisional stability of the mixture in the unitary regime, opening new possibilities for studies and probes of strongly interacting quantum gases in contact with a bath species.
We present a systematic investigation of the effects of "nonmagnetic" impurities on the $s$-wave BCS-BEC crossover in atomic Fermi gases within a pairing fluctuation theory. Both pairing and impurity scattering $T$-matrices are treated self-consistently at the same time. While the system is less sensitive to impurity scattering in the Born limit, for strong impurity scatterers, both the frequency and the gap function are highly renormalized, leading to significant suppression of the superfluid $T_c$, the order parameter and the superfluid density. We also find the formation of impurity bands a…
We show how impurity atoms can measure moments of ultracold atomic gas densities, using the example of bosons in a one-dimensional lattice. This builds on a body of work regarding the probing of systems by measuring the dephasing of an immersed qubit. We show this dephasing is captured by a function resembling characteristic functions of probability theory, of which the derivatives at short times reveal moments of the system operator to which the qubit couples. For a qubit formed by an impurity atom, in a system of ultracold atoms, this operator can be the density of the system at the location…
We have analyzed the behavior of a mobile quantum impurity in a bath formed by a two-leg bosonic ladder by a combination of field theory (Tomonaga-Luttinger liquid) and numerical (Density Matrix Renormalization Group) techniques. Computing the Green's function of the impurity as a function of time at different momenta, we find a power law decay at zero momentum, which signals the breakdown of any quasi-particle description of the impurity motion. We compute the exponent both for the limits of weak and strong impurity-bath interactions. At small impurity-bath interaction, we find that the impur…
We unravel the correlated quantum quench dynamics of a single impurity immersed in a bosonic environment confined in an one-dimensional double-well potential. A particular emphasis is placed on the structure of the time-evolved many-body wave function by relying on a Schmidt decomposition whose coefficients directly quantify the number of configurations that are macroscopically populated. For a non-interacting bosonic bath and weak postquench impurity-bath interactions, we observe the dynamical formation of a two-fold fragmented many-body state which is related to intra-band excitation process…
We study analytically and with the numerical time-evolving block decimation method the dynamics of an impurity in a bath of spinless fermions with nearest-neighbor interactions in a one-dimensional lattice. The bath is in a Mott insulator state with alternating sites occupied and the impurity interacts with the bath by repulsive on-site interactions. We find that when the magnitudes of the on-site and nearest-neighbor interactions are close to each other, the system shows excitations of two qualitatively distinct types. For the first type, a domain wall and an anti-domain wall of density propa…
We present a theoretical study based upon quantum Monte Carlo methods of the Bose polaron in one-dimensional systems with contact interactions. In this instance of the problem of a single impurity immersed in a quantum bath, the medium is a Lieb-Liniger gas of bosons ranging from the weakly interacting to the Tonks-Girardeau regime, whereas the impurity is coupled to the bath via a different contact potential producing both repulsive and attractive interactions. Both the case of a mobile impurity, having the same mass as the particles in the medium, and of a static impurity with infinite mass …
The impurities, introduced intentionally or accidentally into certain materials, can significantly modify their characteristics or reveal their intrinsic physical properties, and thus play an important role in solid-state physics. Different from those static impurities in a solid, the impurities realized in cold atomic systems are naturally mobile. Here we propose an effective theory for treating some unique behaviors exhibited by ultracold mobile impurities. Our theory reveals the interaction-induced transition between the extended and localized impurity states, and also explains the essentia…
Recent studies have demonstrated that higher than two-body bath-impurity correlations are not important for quantitatively describing the ground state of the Bose polaron. Motivated by the above, we employ the so-called Gross Ansatz (GA) approach to unravel the stationary and dynamical properties of the homogeneous one-dimensional Bose-polaron for different impurity momenta and bath-impurity couplings. We explicate that the character of the equilibrium state crossovers from the quasi-particle Bose polaron regime to the collective-excitation stationary dark-bright soliton for varying impurity m…
Mobile impurity interacting with a Hubbard chain and the role of Friedel oscillations
Pontificia Universidad Católica de Chile（智利天主教 Pontificia 大学）；Okinawa Institute of Science and Technology Graduate University（冲绳科学和技术大学院大学）；Universitat de Barcelona（巴塞罗那大学）
Decoherence of a quantum state coupled to an exterior environment is at the foundation of our understanding of the emergence of classical behavior from the quantum world, but how does it emerge in a finite closed quantum system? Here this is studied by modeling an isolated quantum system of a handful of ultracold atoms confined to a double well potential and coupled to a single atom of a different type. The ultracold atoms thermalize and serve as an environmental bath for the single atom. We observe accelerated decoherence of the single atom when ultracold atoms have thermalized. This is expla…
We study the correlated dynamics of few interacting bosonic impurities immersed in a one-dimensional harmonically trapped bosonic environment. The mixture is exposed to a time-dependent impurity-medium interaction pulse moving it across the relevant phase separation boundary. For modulation frequencies smaller than the trapping one, the system successively transits through the miscible/immiscible phases according to the driving of the impurity-medium interactions. For strong modulations, and driving from the miscible to the immiscible regime, a significant fraction of the impurities is expelle…
We unravel the many-body dynamics of a harmonically trapped impurity colliding with a bosonic medium confined in a double-well upon quenching the initially displaced harmonic trap to the center of the double-well. We reveal that the emerging correlation dynamics crucially depends on the impurity-medium interaction strength allowing for a classification into different dynamical response regimes. For strong attractive impurity-medium couplings the impurity is bound to the bosonic bath, while for intermediate attractions it undergoes an effective tunneling. In the case of weak attractive or repul…
We study a new type of Fermi polaron induced by an impurity interacting with an ultracold Fermi superfluid. Due to the three-component nature of the system, the polaron can become trimer-like with a non-universal energy spectrum. We identify multiple avoided crossings between impurity- and trimer-like solutions in both the attractive and the repulsive polaron spectra. In particular, the widths of avoided crossings gradually increase as the Fermi superfluid undergoes a crossover from the BCS side towards the BEC side, which suggests instabilities towards three-body losses. Such losses can be re…
An impurity atom immersed in an ultracold atomic Fermi gas can form a quasiparticle, so-called Fermi polaron, due to impurity-fermion interaction. We consider a three-dimensional homogeneous dipolar Fermi gas as a medium, where the interatomic dipole-dipole interaction (DDI) makes the Fermi surface deformed into a spheroidal shape, and, using a Chevy-type variational method, investigate the ground-state properties of the Fermi polaron: the effective mass, the momentum distribution of a particle-hole (p-h) excitation, the drag parameter, and the medium density modification around the impurity. …
We investigate the crossover of the impurity-induced dynamics, in trapped one-dimensional Bose polarons subject to radio frequency (rf) pulses of varying intensity, from an adiabatic to a diabatic regime. Utilizing adiabatic pulses for either weak repulsive or attractive impurity-medium interactions, a multitude of polaronic excitations or mode-couplings of the impurity-bath interaction with the collective breathing motion of the bosonic medium are spectrally resolved. We find that for strongly repulsive impurity-bath interactions, a temporal orthogonality catastrophe manifests in resonances i…
We investigate the quantum dynamics of a harmonically trapped particle (e.g. an ion) that is immersed in a Bose--Einstein condensate. The ultracold environment acts as a refrigerator, and thus, the influence on the motion of the ion is dissipative. We study the fully coupled quantum dynamics of particle and Bose gas in a linearized regime, treating the quasi-particle excitations of the gas as a (non-Markovian) environment for the particle dynamics. The density operator of the latter follows a known non-Markovian master equation with a highly non-trivial bath correlation function that we determ…
During the last 70 years, the quantum theory of angular momentum has been successfully applied to describing the properties of nuclei, atoms, and molecules, their interactions with each other as well as with external fields. Due to the properties of quantum rotations, the angular momentum algebra can be of tremendous complexity even for a few interacting particles, such as valence electrons of an atom, not to mention larger many-particle systems. In this work, we study an example of the latter: a rotating quantum impurity coupled to a many-body bosonic bath. In the regime of strong impurity-ba…
In ultracold atomic gases, a unique interplay arises between phenomena known from condensed matter physics, few-body physics and chemistry. Similar to an electron in a solid, an impurity in an ultracold gas can get dressed by excitations from the medium, forming a quasiparticle called the polaron. We study how dressing of an impurity leads to a modification of its chemical reactivity. Using a Gaussian state variational method in the frame of the impurity, we demonstrate that three-body correlations lead to an instability of the polaron. This instability is connected to an Efimov resonance, but…
Recent experimental realization of strongly imbalanced mixtures of ultracold atoms opens new possibilities for studying impurity dynamics in a controlled setting. We discuss how the techniques of atomic physics can be used to explore new regimes and manifestations of Anderson's orthogonality catastrophe (OC), which could not be accessed in solid state systems. We consider a system of impurity atoms localized by a strong optical lattice potential and immersed in a sea of itinerant Fermi atoms. Ramsey interference experiments with impurity atoms probe OC in the time domain, while radio-frequency…
Quantum probes are atomic-sized devices mapping information of their environment to quantum mechanical states. By improving measurements and at the same time minimizing perturbation of the environment, they form a central asset for quantum technologies. We realize spin-based quantum probes by immersing individual Cs atoms into an ultracold Rb bath. Controlling inelastic spin-exchange processes between probe and bath allows mapping motional and thermal information onto quantum-spin states. We show that the steady-state spin-population is well suited for absolute thermometry, reducing temperatur…
We explore the quantum dynamics of a one-dimensional trapped ultracold ensemble of bosonic atoms triggered by the sudden creation of a single ion. The numerical simulations are performed by means of the ab initio multiconfiguration time-dependent Hartree method for bosons which takes into account all correlations. The dynamics is analyzed via a cluster expansion approach, adapted to bosonic systems of fixed particle number, which provides a comprehensive understanding of the occurring many-body processes. After a transient during which the atomic ensemble separates into fractions which are unb…
Recent experimental advances enabled the realization of mobile impurities immersed in a Bose-Einstein condensate (BEC) of ultracold atoms. Here we consider impurities with two or more internal hyperfine states, and study their radio-frequency (RF) absorption spectra, which correspond to transitions between two different hyperfine states. We calculate RF spectra for the case when one of the hyperfine states involved interacts with the BEC, while the other state is non-interacting, by performing a non-perturbative resummation of the probabilities of exciting different numbers of phonon modes. In…
We investigate the properties of an impurity immersed in a dilute Bose gas at zero temperature using quantum Monte-Carlo methods. The interactions between bosons are modeled by a hard sphere potential with scattering length $a$, whereas the interactions between the impurity and the bosons are modeled by a short-range, square-well potential where both the sign and the strength of the scattering length $b$ can be varied by adjusting the well depth. We characterize the attractive and the repulsive polaron branch by calculating the binding energy and the effective mass of the impurity. Furthermore…
We present a detailed analysis of the usefulness of ultracold atomic collisions for sensing the strength of an external magnetic field as well as its spatial gradient. The core idea of the sensor, which we recently proposed in K. Jachymski \emph{et al.}, Phys. Rev. Lett. {\bf 120}, 013401 (2018), is to probe the transmission of the atoms through a set of quasi-one-dimensional waveguides that contain an impurity. Magnetic field-dependent interactions between the incoming atoms and the impurity naturally lead to narrow resonances that can act as sensitive field probes since they strongly affect …
We demonstrate that an ultracold many-body bosonic ensemble confined in a one-dimensional (1D) double-well (DW) potential can exhibit chaotic dynamics due to the presence of a single impurity. The non-equilibrium dynamics is triggered by a quench of the impurity-Bose interaction and is illustrated via the evolution of the population imbalance for the bosons between the two wells. While the increase of the post-quench interaction strength always facilitates the irregular motion for the bosonic population imbalance, it becomes regular again when the impurity is initially populated in the highly …
We discuss an even-odd effect for an impurity with an $N$-fold degenerate internal states immersed in a two-dimensional superfluid--Mott-insulator quantum critical bath, which is described by an spin-$S$ XY Bose-Kondo impurity model with $N=2S+1$. Using a dimensional- and momentum-cut off regularized renormalization group and unbiased large-scale Monte Carlo numerical simulations, we establish the phase diagram for the $S=1$ impurity with all the relevant terms included. We show that the $S=1$ impurity with 3-fold degeneracy is fully screened by the critical bath, in qualitative contrast to th…
We unravel the correlated tunneling dynamics of an impurity trapped in a double well and interacting repulsively with a majority species of lattice trapped bosons. Upon quenching the tilt of the double well it is found that the quench-induced tunneling dynamics depends crucially on the interspecies interaction strength and the presence of entanglement inherent in the system. In particular, for weak couplings the impurity performs a rather irregular tunneling process in the double well. Increasing the interspecies coupling it is possible to control the response of the impurity which undergoes a…
We investigate the system of a heavy impurity embedded in a paired two-component Fermi gas at the crossover from a Bose-Einstein condensate (BEC) to a Bardeen--Cooper--Schrieffer (BCS) superfluid via an extension of the functional determinant approach (FDA). FDA is an exact numerical approach applied to study manifestations of Anderson\textquoteright s orthogonality catastrophe (OC) in the system of a static impurity immersed in an ideal Fermi gas. Here, we extend the FDA to a strongly correlated superfluid background described by a BCS mean-field wavefunction. In contrast to the ideal Fermi g…
The Kondo effect in condensed-matter systems manifests itself most sharply in their transport measurements. Here we propose an analogous transport signature of the orbital Kondo effect realized with ultracold atoms. Our system consists of imbalanced Fermi seas of two components of fermions and an impurity atom of different species which is confined by an isotropic potential. We first apply a π/2 pulse to transform two components of fermions into two superposition states. Their interactions with the impurity atom then cause a "transport" of fermions from majority to minority superposition state…
