Understanding the thermodynamic properties of high-$T_c$ cuprate superconductors is a key step to establish a satisfactory theory of these materials. The electronic specific heat is highly unconventional, distinctly non-BCS, with remarkable doping-dependent features extending well beyond $T_c$. The pairon concept, bound holes in their local antiferromagnetic environment, has successfully described the tunneling and photoemission spectra. In this article, we show that the model explains the distinctive features of the entropy and specific heat throughout the temperature-doping phase diagram. Their interpretation connects unambiguously the pseudogap, existing up to $T^*$, to the superconducting state below $T_c$. In the underdoped case, the specific heat is dominated by pairon excitations, following Bose statistics, while with increasing doping, both bosonic excitations and fermionic quasiparticles coexist.
ARPES mesurements in cuprates have given key information on the temperature and angle dependence of the gap ($d$-wave order parameter, Fermi arcs and pseudogap). We show that these features can be understood in terms of a Bose condensation of interacting {\it pairons} (preformed hole pairs which form in their local antiferromagnetic environment). Starting from the basic properties of the pairon wavefunction, we derive the corresponding k-space spectral function. The latter explains the variation of the ARPES spectra as a function of temperature and angle up to T*, the onset temperature of pair…
Electron-phonon coupling (EPC) is one of the most common and fundamental interactions in solids. It not only dominates many basic dynamic processes like resistivity, thermal conductivity etc, but also provides the pairing glue in conventional superconductors. But in high-temperature superconductors (HTSC), it is still controversial whether or not EPC is in favor of paring. Despite the controversies, many experiments have provided clear evidence for EPC in HTSC. In this paper, we briefly review EPC in cuprate and iron-based superconducting systems revealed by Raman scattering. We introduce how …
Two contradictory phase diagrams have dominated the literature of high-$T_c$ cuprate superconductors. Does the pseudogap line cross the superconducting $T_c$-dome or not? To answer, we have revisited the experimental magnetic susceptibility and knight shift of four different compounds, La$_{1-x}$Sr$_x$CuO$_4$, Bi$_2$Sr$_2$Ca$_{1-x}$Y$_x$Cu$_2$O$_8$, Bi$_2$Sr$_2$CaCu$_2$O$_{8+y}$, and YBa$_2$Cu$_3$O$_{6+y}$, as a function of temperature and doping. The susceptibility can be described by the same function for all materials, having a magnetic and an electronic contributions. The former is the 2D …
We follow the line of reasoning that hidden broken symmetries are the root of quantum oscillations observed in underdoped superconductors and examine the role of bilayer splitting and incommensuration. This is a view that eschews the notion of a featureless Mott liquid as the source of complexity. Instead, our view is grounded in a conventional Fermi surface and quasiparticles. We show that bilayer splitting and/or incommensurate $d$-density wave order can lead to many interesting results, in particular a splitting of the main frequency of the quantum oscillations.
We present in-plane infrared reflectance measurement on two superconducting cuprates with relatively low T$_c$: a nearly optimally-doped Bi$_2$Sr$_{1.6}$La$_{0.4}$CuO$_{6+δ}$ with T$_c$=33 K and an underdoped La$_{1.89}$Sr$_{0.11}$CuO$_4$ with T$_c$=30 K. The measurement clearly reveals that the superconducting energy gap is distinct from the pseudogap. They have different energy scales and appear at different temperatures. The results suggest that the pseudogap is not a precursor to the superconducting state. The data also challenge the longstanding viewpoint that the superconductivity within…
We report an angular quantum oscillation study of Tl_2Ba_2CuO_{6+delta} for two different doping levels (Tc = 10K and 26 K) and determine the Fermi surface size and topology in considerable detail. Our results show that Fermi liquid behavior is not confined to the edge of the superconducting dome and is robust up to at least T_c^{max}/3.5. Superconductivity is found to survive up to a larger doping p_c = 0.31 than in La_{2-x}Sr_xCuO_4. Our data imply that electronic inhomogeneity does not play a significant role in the loss of superconductivity and superfluid density in overdoped cuprates, and…
We study the systematic doping evolution of nodal dispersions by in-situ angle-resolved photoemission spectroscopy on the continuously doped surface of a high-temperature superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$. We reveal that the nodal dispersion has three segments separated by two kinks, located at ~10 meV and roughly 70 meV, respectively. The three segments have different band velocities and different doping dependence. In particular, the velocity of the high-energy segment increases monotonically as the doping level decreases and can even surpass the bare band velocity. We propose tha…
Using resonant inelastic x-ray scattering (RIXS) at the Cu $L$-absorption edge, we have observed intense, dispersive spin excitations in highly overdoped Tl$_2$Ba$_2$CuO$_{6+δ}$ (superconducting $T_c =6$ K), a compound whose normal-state charge transport and thermodynamic properties have been studied extensively and shown to exhibit canonical Fermi-liquid behavior. Complementary RIXS experiments on slightly overdoped Tl$_2$Ba$_2$CuO$_{6+δ}$ ($T_c =89$ K) and on Y$_{1-x}$Ca$_{x}$Ba$_2$Cu$_3$O$_{6+δ}$ compounds spanning a wide range of doping levels indicate that these excitations exhibit energi…
Doping Evolution of Nodal Electron Dynamics in Trilayer Cuprate Superconductor Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ Revealed by Laser-Based Angle-Resolved Photoemission Spectroscopy
Recently, machine learning was applied to extract both the normal and the anomalous components of the self-energy from photoemission data at the antinodal points in Bi-based cuprate high-temperature superconductors [Y. Yamaji {\it et al.}, arXiv:1903.08060]. It was argued that both components do show prominent peaks near 50 meV, which hold information about the pairing glue, but the peaks are hidden in the actual data, which measure only the total self-energy. We analyze the self-energy within an effective fermion-boson theory. We show that soft thermal fluctuations give rise to peaks in both …
The Hall coefficient data for cuprates show that number of carriers exceeds external doping $x$ at higher $x$ and varies with temperature. Hence, spins on the Cu-sites are not conserved. Activation energy for thermally excited carriers equals the energy between the Fermi surface "arc" and the band bottom near the van Hove singularities. Crossover from marginal Fermi liquid- to pseudogap- regime happens at temperatures at which number of activated carriers gets comparable with the number of externally doped holes. Implications for the $(T,x)$-phase diagram of cuprates are discussed.
The representative cuprate, La$_{2-x}$M$_x$CuO$_4$, with M = Sr and $x = 1/8$ is studied via first-principles calculations in the high-temperature tetragonal (HTT), low-temperature orthorhombic (LTO), and low-temperature less-orthorhombic (LTLO) structures. By suppressing the magnetism and superconductivity, the LTLO phase, which has rarely been observed in La$_{2-x}$Sr$_x$CuO$_4$, is found to be the ground state, where the structural phase transitions, HTT$\rightarrow$LTO$\rightarrow$LTLO, can be understood via phonon instability. While the La-O composition is identified to be responsible for…
Inhomogeneous reduction-annealing effects on the electron-doped cuprate superconductor revealed by micro-focused angle-resolved photoemission spectroscopy
We use time- and angle-resolved photoemission to measure the nodal non-equilibrium electronic states in various dopings of Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$. We find that the initial pump-induced transient signal of these ungapped states is strongly affected by the onset of the superconducting gap at $T_c$, superconducting pairing fluctuations at $T_p$, and the pseudogap at $T^*$. Moreover, $T_p$ marks a suggestive threshold in the fluence-dependent transient signal, with the appearance of a critical fluence below $T_p$ that corresponds to the energy required to break apart all Cooper pairs. These…
We present an overview of angle-resolved photoemission spectroscopy (ARPES) studies of high-temperature cuprate superconductors aiming at elucidating the relationship between the superconductivity, the pseudogap, and the Fermi arc. ARPES studies of underdoped samples show a momentum dependence of the energy gap below Tc which deviates from a simple d-wave form, suggesting the coexistence of multiple energy scales in the superconducting state. Hence, two distinct energy scales have been introduced, namely, the gap near the node (characterized by Delta_0) and in the anti-nodal region (characteri…
In cuprate superconductors, high magnetic fields have been used extensively to suppress superconductivity and expose the underlying normal state. Early measurements revealed insulating-like behavior in underdoped material versus temperature $T$, in which resistivity increases on cooling with a puzzling $\log(1/T)$ form. We instead use microwave measurements of flux-flow resistivity in YBa$_2$Cu$_3$O$_{6+y}$ and Tl$_2$Ba$_2$CuO$_{6+δ}$ to study charge transport deep inside the superconducting phase, in the low temperature and low field regime. Here, the transition from metallic low-temperature …
The origin of the weak insulating behavior of the resistivity, i.e. $ρ_{xx}\propto\ln(1/T)$, revealed when magnetic fields ($H$) suppress superconductivity in underdoped cuprates has been a longtime mystery. Surprisingly, the high-field behavior of the resistivity observed recently in charge- and spin-stripe-ordered La-214 cuprates suggests a metallic, as opposed to insulating, high-field normal state. Here we report the vanishing of the Hall coefficient in this field-revealed normal state for all $T<(2-6)T_{\mathrm{c}}^{0}$, where $T_{\mathrm{c}}^{0}$ is the zero-field superconducting transit…
We demonstrated experimentally a direct way to probe a hidden propensity to the formation of spin density wave (SDW) in a non-magnetic metal with strong Fermi surface nesting. Substituting Fe for a tiny amount of Cu (1%) induced an incommensurate magnetic order below 20 K in heavily-overdoped La2-xSrxCuO4 (LSCO). Elastic neutron scattering suggested that this order cannot be ascribed to the localized spins on Cu or doped Fe. Angle-resolved photoemission spectroscopy (ARPES), combined with numerical calculations, revealed a strong Fermi surface nesting inherent in the pristine LSCO that likely …
Although phase diagrams can be leveraged to investigate high transition temperature (high-$T_c$) superconductivity, the issue has not been discussed thoroughly. In this study, we elucidate the phase diagram of the overdoped side of high-$T_c$ cuprates via systematic anisotropic transport measurements for Pb-doped Bi-2212 single crystals. We demonstrate that the characteristic temperatures of the "weak" pseudogap opening and electronic coherence cross each other at a critical doping level, while those of the "strong" pseudogap merges into that of superconducting fluctuations above the critical …
We present a combined soft x-ray and high-resolution vacuum-ultraviolet angle-resolved photoemission spectroscopy study of the electron-overdoped cuprate Pr$_{1.3-x}$La$_{0.7}$Ce$_{x}$CuO$_4$ (PLCCO). Demonstration of its highly two-dimensional band structure enabled precise determination of the in-plane self-energy dominated by electron-electron scattering. Through analysis of this self-energy and the Fermi-liquid cut-off energy scale, we find -- in contrast to hole-doped cuprates -- a momentum isotropic and comparatively weak electron correlation in PLCCO. Yet, the self-energies extracted fr…
The electron-doped cuprates are usually characterized by a more robust antiferromagnetic phase and a much narrower superconducting (SC) dome than those of the hole-doped counterparts. Recently, bulk single crystals of Pr1.3-xLa0.7CexCuO4-δ (PLCCO) prepared by the protect annealing method have been studied extensively and revealed many intriguing properties that were different from those obtained from samples annealed by the conventional methods. Here, we report on a systematic angle-resolved photoemission spectroscopy study of PLCCO single crystals after protect annealing. The results indicate…
Recent STM measurements have revealed the existence of periodic charge modulations at the surface of certain cuprate superconductors. Here we show that the observed patterns are compatible with the formation of a three-dimensional crystal of doped holes, with space correlations extending between different Cu-O layers. This puts severe constraints on the dynamical stability of the crystallised hole structure, resulting in a close relationship between the periodicity of the electronic modulation and the interlayer distance.
Using angle-resolved photoemission spectroscopy it is revealed that in the vicinity of optimal doping the electronic structure of La2-xSrxCuO4 cuprate undergoes an electronic reconstruction associated with a wave vector q_a=(pi, 0). The reconstructed Fermi surface and folded band are distinct to the shadow bands observed in BSCCO cuprates and in underdoped La2-xSrxCuO4 with x <= 0.12, which shift the primary band along the zone diagonal direction. Furthermore the folded bands appear only with q_a=(pi, 0) vector, but not with q_b= (0, pi). We demonstrate that the absence of q_b reconstruction i…
The correlated electronic structure of the infinite-layer compounds NdNiO$_2$ and SrCuO$_2$ at stoichiometry and with finite hole doping is compared. Key differences are elucidated from an advanced first-principles many-body perspective. Contrary to the charge-transfer insulating cuprate, the self-doped nickelate remains non-insulating even for large interaction strength, though the Ni-$d_{x^2-y^2}$ spectral weight is also gapped in that limit. Hybridization between Ni$(3d)$ and Nd$(5d)$ is crucial for the appearance of the self-doping band. Upon realistic hole doping, Sr$_{1-y}$CuO$_2$ shows …
We report detailed 17O, 139La, and 63Cu Nuclear Magnetic Resonance (NMR) and Nuclear Quadrupole Resonance (NQR) measurements in a stripe ordered La1.875Ba0.125CuO4 single crystal and in oriented powder samples of La1.8-xEu0.2SrxCuO4. We observe a partial wipeout of the 17O NMR intensity and a simultaneous drop of the 17O electric field gradient (EFG) at low temperatures where the spin stripe order sets in. In contrast, the 63Cu intensity is completely wiped out at the same temperature. The drop of the 17O quadrupole frequency is compatible with a charge stripe order. The 17O spin lattice relax…
The nature of the pseudogap and its relationship with superconductivity are one of the central issues of cuprate superconductors. Recently, a possible scenario has been proposed that the pseudogap state is a distinct phase characterized by spontaneous rotational symmetry breaking called "nematicity" based on transport and magnetic susceptibility measurements, where the symmetry breaking was observed below the pseudogap temperature $T^*$. Here, we report a temperature-dependent ARPES study of nematicity in slightly overdoped Bi${}_{1.7}$Pb${}_{0.5}$Sr${}_{1.9}$CaCu${}_2$O${}_{8+δ}$ triggered by…
We investigated the nature of the quasi-particle state in the vortex core by means of the flux-flow Hall effect measurements at 15.8 GHz. We measured the flux-flow Hall effect in cuprate superconductors, Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{y}$ and YBa$_{2}$Cu$_{3}$O$_{y}$ single crystals, whose equilibrium $B$-$T$ phase diagrams were different. As a result, we found that the Hall angle is independent of the magnetic field, and reaches an order of unity at low temperatures in BSCCO. However, in YBCO, the angle increases with increasing magnetic field even at low temperatures. We understood that this …
Understanding of the precise mechanisms of high-temperature superconductivity is elusive. In particular, in order to solve the puzzle of the pairing mechanism, it is important to understand the detailed nature of the excitations at energies around the superconducting gap. While measurements of the dynamics of excited electronic populations have been able to give some insight, they have largely neglected the intricate dynamics of quantum coherence. Here, we apply multidimensional coherent spectroscopy for the first time to a prototypical cuprate and report unprecedented coherent dynamics persis…
The spontaneous expulsion of applied magnetic field, the Meissner effect, is a defining feature of superconductors; in Type-II superconductors above the lower critical field, this screening takes the form of a lattice of magnetic flux vortices. Using implanted spin-1/2 positive muons, one can measure the vortex lattice field distribution through the spin precession and deduce key parameters of the superconducting ground state, and thereby fundamental properties of the superconducting pairing. Muon spin rotation/relaxation ($μ$SR) experiments have indeed revealed much interesting physics in the…
A central question in the high temperature cuprate superconductors is the fate of the parent Mott insulator upon charge doping. Here we use scanning tunneling microscopy to investigate the local electronic structure of lightly doped cuprate in the antiferromagnetic insulating regime. We show that the doped charge induces a spectral weight transfer from the high energy Hubbard bands to the low energy in-gap states. With increasing doping, a V-shaped density of state suppression occurs at the Fermi level, which is accompanied by the emergence of checkerboard charge order. The new STM perspective…
The recent development of x-ray scattering techniques revealed the charge-excitation spectrum in high-$T_c$ cuprate superconductors. While the presence of a dispersive signal in the high-energy charge-excitation spectrum is well accepted in the electron-doped cuprates, its interpretation and universality are controversial. Since charge fluctuations are observed ubiquitously in cuprate superconductors, the understanding of its origin is a pivotal issue. Here, we employ the layered $t$-$J$ model with the long-range Coulomb interaction and show that an acoustic-like plasmon mode with a gap at in-…
Microscopic mechanism of high-temperature superconductivity revealed by ab initio studies on hole-doped multilayer cuprates HgBa$_2$Ca$_2$Cu$_3$O$_8$ under pressure
Sophia University（上智大学）；The University of Tokyo（东京大学）
The electronic ground state in high-$T_{\rm c}$ cuprates where the superconducting state is suppressed by Ni substitution has been investigated in La$_{2-x}$Sr$_x$Cu$_{1-y}$Ni$_y$O$_4$ from the specific heat and muon spin relaxation measurements. It has been found that the ground state changes from a magnetically ordered state with the strong hole-trapping by Ni to a metallic state with the Kondo effect of Ni with increasing hole-concentration. Moreover, the analysis of the results has revealed that a phase separation into the magnetically ordered phase and the metallic phase occurs around the…
A new method to measure the superconducting stiffness tensor $\overlineρ_s$, without subjecting the sample to magnetic field, is applied to La$_{1.875}$Sr$_{0.125}$CuO$_4$ (LSCO). The method is based on the London equation $\bf{J}=-\overlineρ_s \bf{A}$, where $\bf{J}$ is the current density and $\bf{A}$ is the vector potential. Using rotor free $\bf{A}$ and measuring $\bf{J}$ via the magnetic moment of superconducting rings, we extract $\overlineρ_s$ at $T\rightarrow T_c$. The technique, named Stiffnessometer, is sensitive to very small stiffness, which translates to penetration depth on the o…
In strongly-correlated systems the electronic properties at the Fermi energy (EF) are intertwined with those at high energy scales. One of the pivotal challenges in the field of high-temperature superconductivity (HTSC) is to understand whether and how the high energy scale physics associated with Mott-like excitations (|E-E$_{F}$|>1 eV) is involved in the condensate formation. Here we show the interplay between the many-body high-energy CuO2 excitations at 1.5 and 2 eV and the onset of HTSC. This is revealed by a novel optical pump supercontinuum-probe technique, which provides access to the …
High magnetic field studies of the cuprate superconductors revealed a non-BCS temperature dependence of the upper critical field $H_{c2}(T)$ determined resistively by several groups. These determinations caused some doubts on the grounds of the contrasting effect of the magnetic field on the in-plane, $ρ_{ab}$, and out-of-plane, $ρ_{c}$ resistances reported for large sample of Bi2212. Here we present careful measurements of both $ρ_{ab}(B)$ and $ρ_{c}(B)$ of tiny Bi2212 crystals in magnetic fields up to 50 Tesla. None of our measurements revealed a situation when on field increase $ρ_c$ reache…
We have performed a systematic angle-resolved photoemission spectroscopy (ARPES) study of the high-Tc cuprates La2-xSrxCuO4, ranging from the underdoped insulator to the superconductor to the overdoped metal. We have revealed a systematic doping evolution of the band dispersions and (underlying) Fermi surfaces, pseudogap and quasi-particle features under the influence of strong electron-electron interaction and electron-phonon interaction. The unusual transport and thermodynamic properties are explained by taking into account the pseudogap opening and the Fermi arc formation, due to which the …
Recent neutron scattering experiments have revealed that the generic form of the magnetic excitations in the high-Tc cuprates of wide range of doping has the so-called "hourglass" shape; it features both upward and downward excitations at the incommensurate (IC) momenta spanning from the resonance peak at the commensurate momentum $(π,π)$. We propose the two-component spin-fermion model as a minimal phenomenological model which has both local spins and itinerant fermions as independent degrees of freedom. Our calculations of the dynamic spin correlation function provide good agreement with exp…
How coherent quasiparticles emerge by doping quantum antiferromagnets is a key question in correlated electron systems, whose resolution is needed to elucidate the phase diagram of copper oxides. Recent resonant inelastic X-ray scattering (RIXS) experiments in hole-doped cuprates have purported to measure high-energy collective spin excitations that persist well into the overdoped regime and bear a striking resemblance to those found in the parent compound, challenging the perception that spin excitations should weaken with doping and have a diminishing effect on superconductivity. Here we sho…
CeCoIn5 is a heavy fermion superconductor with strong similarities to the high-Tc cuprates, including quasi-two-dimensionality, proximity to antiferromagnetism, and probable d-wave pairing arising from a non-Fermi-liquid normal state. Experiments allowing detailed comparisons of their electronic properties are of particular interest, but in most cases are difficult to realize, due to their very different transition temperatures. Here we use low temperature microwave spectroscopy to study the charge dynamics of the CeCoIn5 superconducting state. The similarities to cuprates, in particular to ul…
The nature of the spin excitations in superconducting cuprates is a key question toward a unified understanding of the cuprate physics from long-range antiferromagnetism to superconductivity. The intense spin excitations up to the over-doped regime revealed by resonant inelastic X-ray scattering bring new insights as well as questions like how to understand their persistence or their relation to the collective excitations in ordered magnets (magnons). Here, we study the evolution of the spin excitations upon hole-doping the superconducting cuprate Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ by disentangling…
The parent compounds of the high-temperature cuprate superconductors are Mott insulators. It has been generally agreed that understanding the physics of the doped Mott insulators is essential to understanding the mechanism of high temperature superconductivity. A natural starting point is to elucidate the basic electronic structure of the parent compound. Here we report comprehensive high resolution angle-resolved photoemission measurements on Ca$_2$CuO$_2$Cl$_2$, a Mott insulator and a prototypical parent compound of the cuprates. Multiple underlying Fermi surface sheets are revealed for the …
We have performed angle-resolved photoemission and core-level x-ray photoemission studies of the single-layer cuprate Bi$_2$Sr$_{2-x}$La$_x$CuO$_{6+δ}$ (Bi2201) and revealed the doping evolution of the electronic structure from the lightly-doped to optimally-doped regions. We have observed the formation of the dispersive quasi-particle band, evolution of the Fermi ``arc'' into the Fermi surface and the shift of the chemical potential with hole doping as in other cuprates. The doping evolution in Bi2201 is similar to that in Ca$_{2-x}$Na$_{x}$CuO$_{2}$Cl$_2$ (Na-CCOC), where a rapid chemical po…
In the framework of the slave-boson approach to the $t-t'-t''-J$ model, it is found that for electron-doped high-$T_c$ cuprates, the staggered antiferromagnetic (AF) order coexists with superconducting (SC) order in a wide doping level ranged from underdoped to nearly optimal doping at the mean-field level. In the coexisting phase, it is revealed that the spin response is commensurate in a substantial frequency range below a crossover frequency $ω_{c}$ for all dopings considered, and it switches to the incommensurate structure when the frequency is higher than $ω_{c}$. This result is in agreem…
High magnetic field studies of cuprate superconductors revealed a non-BCS temperature dependence of the upper critical field $H_{c2}(T)$ determined resistively by several groups. These determinations caused some doubts on the grounds of both the contrasting effect of the magnetic field on the in-plane and out-of-plane resistances reported for large Bi2212 sample and the large Nernst signal \emph{well above} $T_{c}$. Here we present both $ρ_{ab}(B)$ and $ρ_{c}(B)$ of tiny Bi2212 crystals in magnetic fields up to 50 Tesla. None of our measurements revealed a situation when on the field increase …
It is proposed that the 50-70 meV dispersion anomaly (kink) in electron-doped cuprates revealed by recent angle-resolved photoemission spectroscopy experiments is caused by coupling with the spin fluctuation. We elaborate that the kink exists both along nodal and antinodal directions, and both in the superconducting and normal state. The renormalized effect for the density of states is also studied and the hump feature outside the superconducting coherent peak is established, consistent with recent scanning tunnelling microscopy experiments.
Superconductivity in cuprates peaks in the doping regime between a metal at high p and an insulator at low p. Understanding how the material evolves from metal to insulator is a fundamental and open question. Early studies in high magnetic fields revealed that below some critical doping an insulator-like upturn appears in the resistivity of cuprates at low temperature, but its origin has remained a puzzle. Here we propose that this 'metal-to-insulator crossover' is due to a drop in carrier density n associated with the onset of the pseudogap phase at a critical doping p*. We use high-field res…
Substitutional impurities in the CuO2 planes of the cuprates allow us to probe the electronic properties of the host material. The pseudo-gap in the underdoped regime is unmodified far from the impurities even though Tc is greatly reduced. The spin polarisation induced by magnetic impurities has an oscillatory behaviour reflecting the existing AF correlations between the Cu spins. Its influence on the NMR spectra opens a way to determine the q dependence of the static spin susceptibility and the T dependence of the AF correlation length. NMR measurements demonstrate that non-magnetic impuritie…
The exotic physics in condensed matter systems, such as high-Tc superconductivity in cuprates, is due to the properties of the elementary excitations and their interactions. The dispersion of the electronic states revealed by angle-resolved photoemission spectroscopy (ARPES) provides a chance to understand these excitations. Recently, a "high energy anomaly" or "waterfall-like" feature in cuprates' dispersion has been reported and studied theoretically. Most of the current views argue that it is the result of some many-body effect at a specific high energy scale (e.g. ~ 0.3eV), though there ar…
The discovery of superconductivity in a $d^{9-δ}$ nickelate has inspired disparate theoretical perspectives regarding the essential physics of this class of materials. A key issue is the magnitude of the magnetic superexchange, which relates to whether cuprate-like high-temperature nickelate superconductivity could be realized. We address this question using Ni L-edge and O K-edge spectroscopy of the reduced trilayer nickelate $d^{9-1/3}$ La4Ni3O8 and associated theoretical modeling. A magnon energy scale of ~80 meV resulting from a nearest-neighbor magnetic exchange of $J = 69(4)4$ meV is obs…
Using angle-resolved photoemission (ARPES), it is revealed that the low-energy electronic excitation spectra of highly underdoped superconducting and non-superconducting La(2-x)SrxCuO4 cuprates are gapped along the entire underlying Fermi surface at low temperatures. We show how the gap function evolves to a d(x2-y2) form as increasing temperature or doping, consistent with the vast majority of ARPES studies of cuprates. Our results provide essential information for uncovering the symmetry of the order parameter(s) in strongly underdoped cuprates, which is a prerequisite for understanding the …
