We describe degenerate square spin as an ensemble of magnetic monopoles coupled via an emergent entropic field that subsumes the effect of the underlying spin vacuum. We compute their effective free energy, entropic interaction, correlations, screening, and structure factors that coincide with the experimental ones. Unlike in pyrochlore ices, a dimensional mismatch between real and entropic interactions leads to weak singularities at the pinch points and algebraic correlations at long distance. This algebraic screening can be, however, camouflaged by a pseudo-screening regime.
We relate the anomalous noise found experimentally in spin ice to the subdiffusion of magnetic monopoles. Because monopoles are emergent particles, they do not move in a structureless vacuum. Rather, the underlying spin ensemble filters the thermal white noise, leading to non-trivial coevolution. Thus, monopoles can be considered as random walkers under the effect of stochastic forces only as long as those are not trivially white, but instead subsume the evolution of the spin vacuum. Via this conceptualization, we conjecture relations between the color of the noise and other observables, such …
We consider a pure square spin ice, that is a square ice where only nearest neighbors are coupled. A gauge-free duality between the perpendicular and collinear structure leads to a natural description in terms of topological currents and charges as the relevant degrees of freedom. That, in turn, can be expressed via a continuous field theory where the discrete spins are subsumed into entropic interactions among charges and currents. This approach produces structure factors, correlations, and susceptibilities for spins, monopoles, and currents. It also generalizes to non-zero temperature the he…
Proceeding from the more general to the more concrete, we propose an equilibrium field theory describing spin ice systems in terms of topological charges and magnetic monopoles. We show that for a spin ice on a graph, the entropic interaction in a Gaussian approximation is the inverse of the graph Laplacian matrix, while the screening function for external charges is the inverse of the screened laplacian. We particularize the treatment to square and pyrochlore ice. For square ice we highlight the gauge-free duality between direct and perpendicular structure in terms of symmetry between charges…
Magnetic monopole unpairing as a function of external magnetic fields is presented as a fingerprint of this emergent quasiparticles freedom in a two-dimensional artificial spin ice system. Such freedom, required for example for further application in magnetricity, is only possible due to ground-state degeneracy, which causes a decreasing of the string energy in rectangular geometries, designed to allow highest equidistance among nanomagnets. We show by simulations that spin correlation in different rectangular artificial spin ices evolves from antiferromagnetic ordered magnetic structure to a …
Current research on artificial spin ice (ASI) systems has revealed unique hysteretic memory effects and mobile quasi-particle monopoles controlled by externally applied magnetic fields. Here, we numerically demonstrate a strain-mediated multiferroic approach to locally control the ASI monopoles. The magnetization of individual lattice elements is controlled by applying voltage pulses to the piezoelectric layer resulting in strain-induced magnetic precession timed for 180 degree reorientation. The model demonstrates localized voltage control to move the magnetic monopoles across lattice sites, …
Artificial spin ices (ASIs) are interacting arrays of lithographically-defined nanomagnets in which novel frustrated magnetic phases can be intentionally designed. A key emergent description of fundamental excitations in ASIs is that of magnetic monopoles -- mobile quasiparticles that carry an effective magnetic charge. Here we demonstrate that the archetypal square ASI lattice can host, in specific regions of its magnetic phase diagram, high-density plasma-like regimes of mobile magnetic monopoles. By passively "listening" to spontaneous monopole noise in thermal equilibrium, we reveal their …
Magnetic analogue of an isolated free electric charge, i.e., a magnet with a single north or south pole, is a long sought-after particle which remains elusive so far. In magnetically frustrated pyrochlore solids, a classical analogue of monopole was observed as a result of excitation of spin ice vertices. Direct visualization of such excitations were proposed and later confirmed in analogous artificial spin ice (ASI) systems of square as well as Kagome geometries. However, such charged vertices are randomly created as they are thermally driven and are always associated with corresponding emerg…
The effect of the size of the system, aspect ratio and impurities concentration on the dynamic of emergent magnetic monopoles in artificial spin ice systems
Facultad de Ingeniería, Universidad Diego Portales（迭戈帕拉莱斯大学工程学院）
Artificial spin ice systems have been introduced as a possible mean to investigate frustration effects in a well-controlled manner by fabricating lithographically-patterned two-dimensional arrangements of interacting magnetic nanostructures. This approach offers the opportunity to visualize unconventional states of matter, directly in real space, and triggered a wealth of studies at the frontier between nanomagnetism, statistical thermodynamics and condensed matter physics. Despite the strong efforts made these last ten years to provide an artificial realization of the celebrated square ice mo…
In this paper we conduct Monte Carlo simulations to investigate the thermodynamic properties of a geometry of artificial spin ice recently proposed in the literature that had been termed "rewritable" spin ice, for its experimental realization allows total control over the microstates of the system. Our results show that in the thermodynamic limit a single phase transition between a fully magnetized state and a paramagnetic state exists, whereas for finite systems an intermediate phase also emerges, engendering a low temperature pseudo phase transition. This intermediate phase is characterized …
Designing and constructing model systems that embody the statistical mechanics of frustration is now possible using nanotechnology. We have arranged nanomagnets on a two-dimensional square lattice to form an artificial spin ice, and studied its fractional excitations, emergent magnetic monopoles, and how they respond to a driving field using X-ray magnetic microscopy. We observe a regime in which the monopole drift velocity is linear in field above a critical field for the onset of motion. The temperature dependence of the critical field can be described by introducing an interaction term into…
In the present Letter we discuss the origin of the vertex population inversion observed experimentally in the mediated Artificial Square Ice. An interaction modifier is a disc-shaped magnetic nanoisland (a dot) which is placed at the center of a vertex to mediate the interaction between the nearby islands. We show that the inversion is of entropic origin, and can be explained via the renormalization of the vertex configuration energies due to local interaction between the nanoislands and the dot. We show it in a model with mixed Heisenberg and Ising spins (a spin-dot interaction) that as a fun…
In this letter, we have constructed and experimentally investigated frustrated arrays of dipoles forming two-dimensional artificial spin ices with different lattice parameters (rectangular arrays with horizontal and vertical lattice spacings denoted by $a$ and $b$ respectively). Arrays with three different ratios $γ=a/b = \sqrt{2}$, $\sqrt{3}$ and $\sqrt{4}$ are studied. Theoretical calculations of low-energy demagnetized configurations for these same parameters are also presented. Experimental data for demagnetized samples confirm most of the theoretical results. However, the highest energy t…
We report here the results of micromagnetic simulations of square artificial spin ice (ASI) systems with defects. The defects are introduced by misaligning of a nanomagnet at the vertex. In these defective systems, we are able to stabilize emergent monopole-like state by applying a small external field. We observe a systematic change of dipolar energies of the systems with varying misalignment angle. The fields at which the emergent monopoles are created vary linearly with the dipolar energies of the systems. Our results clearly show that the magnetization reversal of the ASI systems is intric…
We study an artificial spin ice system consisting of two identical layers separated by a height offset $h$. For small separation, the layers are shown to attract each other, provided the whole system is in the ground state. Such an attraction comes about by means of a power-law force that we compare to van der Waals forces. When magnetic monopoles occur in one (or both) layers, the scenario becomes even more interesting and these layers may also repel each other. By tuning parameters like $h$ and monopole distance, switching between attraction and repulsion may be accomplished in a feasible wa…
Artificial ices enable the study of geometrical frustration by design and through direct observation. However, it has proven difficult to achieve tailored long-range ordering of their diverse configurations, limiting both fundamental and applied research directions. We designed an artificial spin structure that produces a magnetic charge ice with tunable long-range ordering of eight different configurations. We also developed a technique to precisely manipulate the local magnetic charge states and demonstrate write-read-erase multifunctionality at room temperature. This globally reconfigurable…
We introduce FePd$_{3}$ as a new material for studying thermally active artificial spin ice (ASI) systems and use it to investigate both the square and kagome ice geometries. We readily achieve perfect ground state ordering in the square lattice and demonstrate the highest yet degree of monopole charge-ordering in the kagome lattice. We find that smaller lattice constants in the kagome system generally produce larger domains of charge order. Monte Carlo simulations show excellent agreement with our data when a small amount of disorder is included in the simulation.
We report broadband spin-wave spectroscopy on kagome artificial spin ice (ASI) made of large arrays of interconnected Ni$_{80}$Fe$_{20}$ nanobars. Spectra taken in saturated and disordered states exhibit a series of resonances with characteristic magnetic field dependencies. Making use of micromagnetic simulations, we identify resonances that reflect the spin-solid-state and monopole-antimonopole pairs on Dirac strings. The latter resonances allow for the generation of highly-charged vertices in ASIs via microwave assisted switching. Our findings open further perspectives for fundamental studi…
We investigate spin dynamics of artificial spin ice (ASI) where topological defects confine magnon modes in Ni$_{81}$Fe$_{19}$ nanomagnets arranged on an interconnected kagome lattice. Brillouin light scattering microscopy performed on magnetically disordered states exhibit a series of magnon resonances which depend on topological defect configurations detected by magnetic force microscopy. Nanomagnets on a Dirac string and between a monopole-antimonopole pair show pronounced modifications in magnon frequencies both in experiments and simulations. Our work is key for the creation and annihilat…
Artificial spin ices are frustrated spin systems that can be engineered, wherein fine tuning of geometry and topology has allowed the design and characterization of exotic emergent phenomena at the constituent level. Here we report a realization of spin ice in a lattice of superconducting qubits. Unlike conventional artificial spin ice, our system is disordered by both quantum and thermal fluctuations. The ground state is classically described by the ice rule, and we achieve control over a fragile degeneracy point leading to a Coulomb phase. The ability to pin individual spins allows us to dem…
