Proceedings of the National Conference on Nuclear Physics 2013, Sambalpur University, Sambalpur, India. arXiv admin note: text overlap with arXiv:1209.0281
We present a brief overview of nuclear multifragmentation reaction. Basic formalism of canonical thermodynamical model based on equilibrium statistical mechanics is described. This model is used to calculate basic observables of nuclear multifragmentation like mass distribution, fragment multiplicity, isotopic distribution and isoscaling. Extension of canonical thermodynamical model to a projectile fragmentation model is outlined. Application of the projectile fragmentation model for calculating average number of intermediate mass fragments and the average size of largest cluster at different $Z_{bound}$, differential charge distribution and cross-section of neutron rich nuclei of different projectile fragmentation reactions at different energies are described. Application of nuclear multifragmentation reaction in basic research as well as in other domains is outlined.
Nuclear multifragmentation is an important phenomenon, the study of which can throw light on reaction mechanism in heavy ion collisions at intermediate and high energies. Based on statistical and dynamical model studies, this thesis is concentrated mainly on, the following three aspects of nuclear multifragmentation reactions namely (i) production of exotic nuclei which are normally not available in the laboratory (ii) nuclear symmetry energy from heavy ion collisions at intermediate energies and (iii) Nuclear liquid-gas phase transition. In addition to these equivalence of statistical ensembl…
This review article is focused on the tremendous progress realized during the last fifteen years in the understanding of multifragmentation and its relationship to the liquid-gas phase diagram of nuclei and nuclear matter. The explosion of the whole nucleus, early predicted by Bohr [N. Bohr, Nature 137 (1936) 351], is a very complex and rich subject which continues to fascinate nuclear physicists as well as theoreticians who extend the thermodynamics of phase transitions to finite systems.
In nuclear reactions induced by hadrons and ions of high energies, nuclei can disintegrate into many fragments during a short time (~100 fm/c). This phenomenon known as nuclear multifragmentation was under intensive investigation last 20 years. It was established that multifragmentation is an universal process taking place in all reactions when the excitation energy transferred to nuclei is high enough, more than 3 MeV per nucleon, independently on the initial dynamical stage of the reactions. Very known compound nucleus decay processes (sequential evaporation and fission), which are usual for…
Isoscaling and isobaric yield ratio parameters are compared from canonical and grand canonical ensembles when applied to multifragmentation of finite nuclei. Source dependence of isoscaling parameters and source and isospin dependence of isobaric yield ratio parameters are examined in the framework of the canonical and the grand canonical models. It is found that as the nucleus fragments more, results from both the ensembles converge and observables calculated from the canonical ensemble coincide more with those obtained from the formulae derived using the grand canonical ensemble.
The fragment production in multifragmentation of finite nuclei is affected by the critical temperature of nuclear matter. We show that this temperature can be determined on the basis of the statistical multifragmentation model (SMM) by analyzing the evolution of fragment distributions with the excitation energy. This method can reveal a decrease of the critical temperature that, e.g., is expected for neutron-rich matter. The influence of isospin on fragment distributions is also discussed.
Distributions of the largest fragment charge, Zmax, in multifragmentation reactions around the Fermi energy can be decomposed into a sum of a Gaussian and a Gumbel distribution, whereas at much higher or lower energies one or the other distribution is asymptotically dominant. We demonstrate the same generic behavior for the largest cluster size in critical aggregation models for small systems, in or out of equilibrium, around the critical point. By analogy with the time-dependent irreversible aggregation model, we infer that Zmax distributions are characteristic of the multifragmentation time-…
Deviations from an idealized equilibrium phase transition picture in nuclear multifragmentation is studied in terms of the entropic index. We investigate different heat-capacity features in the canonical quantum statistical model of nuclear multifragmentation generalized in the framework of Tsallis nonextensive thermostatistics. We find that the negative branch of heat capacity observed in quasi-peripheral Au+Au collisions is caused primarily by the non-generic nonextensivity effects.
It is shown that the chemical equilibrium condition of the system can be unambiguously identified by analyzing the isospin evolution of fragments produced in nuclear multifragmentation process. As far as the chemical equilibrium is established, the isotope production can be used for finding properties of nuclear matter and fragments in the freeze-out volume, for example, via the isoscaling phenomenon.
The properties of the kinetic energy spectra of light isotopes produced in the breakup of a nuclear source and during the deexcitation of its products are examined. The initial stage, at which the hot fragments are created, is modeled by the Statistical Multifragmentation Model, whereas the Weisskopf-Ewing evaporation treatment is adopted to describe the subsequent fragment deexcita- tion, as they follow their classical trajectories dictated by the Coulomb repulsion among them. The energy spectra obtained are compared to available experimental data. The influence of the fusion cross-section en…
We show that the coalescence model for fragment formation leads to an approximate site percolation model. Features characteristic of a percolation model also appear in microscopic models of disassembly.
Nuclear multifragmentation in intermediate energy heavy ion collisions has long been associated with liquid-gas phase transition. We calculate the shear viscosity to entropy density ratio eta/s for an equilibrated system of nucleons and fragments produced in multifragmentation within an extended statistical multifragmentation model. The temperature dependence of eta/s exhibits surprisingly similar behavior as that for water. In the coexistence phase of fragments and light particles, the ratio eta/s reaches a minimum of comparable depth as that for water in the vicinity of the critical temperat…
The multifragmentation of excited spherical nuclear sources with various N/Z ratios and fixed mass number is studied within dynamical and statistical models. The dynamical model treats the multifragmentation process as a final stage of the growth of density fluctuations in unstable expanding nuclear matter. The statistical model makes a choice of the final multifragment configuration according to its statistical weight at a global thermal equilibrium. Similarities and differences in the predictions of the two models on the isotopic composition of the produced fragments are presented and the mo…
In peripheral collisions of relativistic heavy ions highly excited spectators containing Lambda-hyperons can be produced. Such strange spectator matter may undergo a break-up into many fragments (multifragmentation) as it is well established for ordinary nuclear systems. We generalize the statistical multifragmentation model, previously successfully used for the description of experimental data, for the case of hypernuclear systems. We predict relative yields of hypernuclei and the main characteristics of such a break-up. We point at a connection of this phenomenon with a liquid-gas phase tran…
Because of thermal expansion and residual interactions, hot nuclear fragments produced in multifragmentation reactions may have lower nucleon density than the equilibrium density of cold nuclei. In terms of liquid-drop model this effect can be taken into account by reducing the bulk energy of fragments. We study the influence of this change on fragment yields and isotope distributions within the framework of the statistical multifragmentation model. Similarities and differences with previously discussed modifications of symmetry and surface energies of nuclei are analyzed.
We assume that, in equilibrium, nuclear matter at reduced density and moderate finite temperature, breaks up into many fragments. A strong support to this assumption is provided by date accumulated from intermediate energy heavy ion collisions. The break-up of hot and expanded nuclear matter according to rules of equilibrium statistical mechanics is the multifragmentation model. The model gives a first order phase transition. This is studied in detail here. Phase-equilibrium lines for different degrees of asymmetry are computed.
The liquid-gas phase transition is analyzed from the topologic properties of the event distribution in the obervables space. A multi-canonical formalism allows to directly relate the standard phase transition with neutral particles to the case where the non saturating Coulomb interaction is present, and to interpret the effect of Coulomb as a deformation of the probability distributions and a rotation of the order parameter. This formalism is applied to a statistical multifragmentation model and consequences for the nuclear multifragmentation phase transitions are drawn.
We use a simplified model which is based on the same physics as inherent in most statistical models for nuclear multifragmentation. The simplified model allows exact calculations for thermodynamic properties of systems of large number of particles. This enables us to study a phase transition in the model. A first order phase transition can be tracked down. There are significant differences between this phase transition and some other well-known cases.
Experimental data for central collisions of $^{129}$Xe on $^{119}$Sn at beam energies of (a) 32 MeV/nucleon, (b) 39 MeV/nucleon, (c) 45 MeV/nucleon and (d) 50 MeV/nucleon are compared with results calculated using a hybrid model. We use a transport model (BUU) to obtain the excitation energy per nucleon in the center of mass of the multifragmenting system. The canonical thermodynamic model is then used to determine the temperature which would lead to this excitation energy. With this temperature we use the canonical thermodynamic model to calculate various experimental data such as multiplicit…
Using a recently proposed classification scheme for phase transitions in finite systems [Phys.Rev.Lett.{\bf 84},3511 (2000)] we show that within the statistical standard model of nuclear multifragmentation the predicted phase transition is of first order.
Within the statistical multifragmentation model we study modifications of the surface and symmetry energy of primary fragments in the freeze-out volume. The ALADIN experimental data on multifragmentation obtained in reactions induced by high-energy projectiles with different neutron richness are analyzed. We have extracted the isospin dependence of the surface energy coefficient at different degrees of fragmentation. We conclude that the surface energy of hot fragments produced in multifragmentation reactions differs from the values extracted for isolated nuclei at low excitation. At high frag…
We apply the canonical quantum statistical model of nuclear multifragmentation generalized in the framework of recently proposed Tsallis non-extensive thermostatistics for the description of nuclear multifragmentation process. The test calculation in the system with A=197 nucleons show strong modification of the 'critical' behaviour associated with the nuclear liquid-gas phase transition for small deviations from the conventional Boltzmann-Gibbs statistical mechanics.
We discuss the presence of both dynamical chaos and signals of a second--order phase transition in numerical Vlasov simulations of nuclear multifragmentation. We find that chaoticity and criticality are strongly related and play a crucial role in the process of fragments formation. This connection is not limited to our model and seems a rather general feature.
An exact analytical solution of the statistical multifragmentation model is found in thermodynamic limit. The system of nuclear fragments exhibits a 1-st order liquid-gas phase transition. The peculiar thermodynamic properties of the model near the boundary between the mixed phase and the pure gaseous phase are studied.
We point out similarity of thermodynamic conditions reached in intermediate energy nuclear collisions and in supernova explosions. We show that a statistical approach, which has been previously applied for nuclear multifragmentation reactions, can be very useful for description of electro-neutral stellar matter. Then properties of hot unstable nuclei extracted from analysis of multifragmentation data can be used for construction of a realistic equation of state of supernova matter.
Two instructive effects concerning fragment production at disintegration of finite nuclei are predicted with the statistical multifragmentation model: (1) a concentration of neutrons in intermediate mass fragments during the phase transition, (2) the break of the spatial symmetry of the fragment's isospin distribution, as well as of the symmetry of the fragment's emission from a statistical source, induced by the external Coulomb field.
Multiplicity fluctuations of intermediate-mass fragments are studied with the percolation model. It is shown that super-Poissonian fluctuations occur near the percolation transition and that this behavior is associated with the fragmentative nature of the percolation model. The consequences of various choices in defining and binning fragments are also evaluated. Several suggestions for experiments in nuclear fragmentation are presented.
Both simple and sophisticated models are frequently used in an attempt to understand how real nuclei breakup when subjected to large excitation energies, a process known as nuclear multifragmentation. Many of these models assume equilibriumthermodynamics and produce results often interpreted as evidence of a phase transition. This work examines one class of models and employs standard thermodynamical procedure to explore the possible existence and nature of a phase transition. The role of various terms, e.g. Coulomb and surface energy, is discussed.
The equation of state of nuclear matter suggests that at suitable beam energies the disassembling hot system formed in heavy ion collisions will pass through a liquid-gas coexistence region. Searching for the signatures of the phase transition has been a very important focal point of experimental endeavours in heavy ion collisions, in the last fifteen years. Simultaneously theoretical models have been developed to provide information about the equation of state and reaction mechanisms consistent with the experimental observables. This article is a review of this endeavour.
Clusters in the three-dimensional Ising model rigorously obey reducibility and thermal scaling up to the critical temperature. The barriers extracted from Arrhenius plots depend on the cluster size as $B \propto A^σ$ where $σ$ is a critical exponent relating the cluster size to the cluster surface. All the Arrhenius plots collapse into a single Fisher-like scaling function indicating liquid-vapor-like phase coexistence and the univariant equilibrium between percolating clusters and finite clusters. The compelling similarity with nuclear multifragmentation is discussed.
During the collapse of massive stars, and the supernova type-II explosions, stellar matter reaches densities and temperatures which are similar to the ones obtained in intermediate-energy nucleus-nucleus collisions. The nuclear multifragmentation reactions can be used for determination of properties of nuclear matter at subnuclear densities, in the region of the nuclear liquid-gas phase transition. It is demonstrated that the modified properties of hot nuclei (in particular, their symmetry energy) extracted from the multifragmentation data can essentially influence nuclear composition of stell…
We investigate the possibility to extract the symmetry energy from multifragmentation data. The applicability of the grandcanonical formula earlier proposed by Ono {\it et al.} [Phys. Rev. C {\bf 68}, 051601(R)] in the case of finite excited nuclei is tested within a microcanonical framework. Relatively good results are obtained except for large residual nuclei, especially when large sources are highly excited. Effects of secondary particle emission and the extent in which relevant information may be inferred from experimental observables are finally discussed.
A systematic comparison of different isotopic temperatures with the thermodynamical temperature of a multifragment system is made on the basis of the Statistical Multifragmentation Model. It is demonstrated that isotopic temperatures are strongly affected by the secondary decays of hot primary fragments and the population of particle-stable excited states in final fragments. The He-Li temperatures, measured recently by the ALADIN group, are reproduced fairly well both as a function of excitation energy and bound charge. Our analysis confirms the anomaly in the nuclear caloric curve.
We present a dynamical and dissipative lattice model, designed to mimic nuclear multifragmentation. Monte-Carlo simulations with this model show clear signature of critical behaviour and reproduce experimentally observed correlations. In particular, using techniques devised for finite systems, we could obtain two of its critical exponents, whose values are in agreement with those of the universality class to which nuclear multifragmentation is supposed to belong.
Some of the progress in determining the phase boundaries of the nuclear phase diagram, the location of the critical point of the nuclear fragmentation phase transition, and the values of the critical exponents of this transition is reviewed. The recently postulated connection of the size of the largest fragments as a function of their rank with Zipf's law known from linguistics is discussed, and an exact formula is derived. We show that Zipf's law is not strictly observed in nuclear fragmentation, but that one can derive useful approximations.
Statistical models based on canonical and grand canonical ensembles are extensively used to study intermediate energy heavy ion collisions. The underlying physical assumption behind canonical and grand canonical models is fundamentally different, and in principle agree only in the thermodynamical limit when the number of particles become infinite. Nevertheless, we show that these models are equivalent in the sense that they predict similar results if certain conditions are met even for finite nuclei. In particular, the results converge when nuclear multifragmentation leads to the formation of …
A systematic study of the effect of fragment$-$fragment interaction, quantum statistics, $γ$-feeding and collective flow is made in the extraction of the nuclear temperature from the double ratio of the isotopic yields in the statistical model of one-step (Prompt) multifragmentation. Temperature is also extracted from the isotope yield ratios generated in the sequential binary-decay model. Comparison of the thermodynamic temperature with the extracted temperatures for different isotope ratios show some anomaly in both models which is discussed in the context of experimentally measured caloric …
We investigate the average sizes of the $n$ largest fragments in nuclear multifragmentation events near the critical point of the nuclear matter phase diagram. We perform analytic calculations employing Poisson statistics as well as Monte Carlo simulations of the percolation type. We find that previous claims of manifestations of Zipf's Law in the rank-ordered fragment size distributions are not born out in our result, neither in finite nor infinite systems. Instead, we find that Zipf-Mandelbrot distributions are needed to describe the results, and we show how one can derive them in the infini…
We report the consequences of implementing momentum dependent interactions (MDI) on multifragmentation in heavy-ion reactions over entire collision geometry. The evolution of a single cold nucleus using static soft equation of state and soft momentum dependent equation of state demonstrates that inclusion of momentum dependence increases the emission of free nucleons. However, no heavier fragments are emitted artificially. The calculations performed within the framework of quantum molecular dynamics approach suggest that MDI strongly influence the system size dependence of fragment production.…
We study the disintegration of nuclei by strong electromagnetic fields induced by ultrarelativistic heavy ions. The proposed multi-step model includes 1) the absorption of a virtual photon by a nucleus, 2) intranuclear cascades of produced hadrons and 3) statistical decay of the excited residual nucleus. The combined model describes well existing data on projectile fragmentation at energy 200 GeV per nucleon. Electromagnetic multifragmentation of nuclei is predicted to be an important reaction mechanism at RHIC and LHC energies.
The possible usefulness of the renormalization group method in Nuclear Physics is pointed out in this talk in the context of the nuclear multifragmentation. The presentation is rather superficial and sketchy, to indicate the main lines only. But I believe that the idea is warrant of further, more careful studies.
We propose a new formulation of the statistical multifragmentation model based on the analysis of the virial expansion for a system of the nuclear fragments of all sizes. The developed model not only enables us to account for short-range repulsion, but also to calculate the surface free energy which is induced by the interaction between the fragments. We propose a new parameterization for the liquid phase pressure which allows us to introduce a compressible nuclear liquid into the statistical multifragmentation model. The resulting model is exactly solvable and has no irregular behavior of the…
We present an overview of concepts and results obtained with statistical models in study of nuclear multifragmentation. Conceptual differences between statistical and dynamical approaches, and selection of experimental observables for identification of these processes, are outlined. New and perspective developments, like inclusion of in-medium modifications of the properties of hot primary fragments, are discussed. We list important applications of statistical multifragmentation in other fields of research.
The agreement between the fragments' internal and kinetic temperatures with the breakup temperature is investigated using a Statistical Multifragmentation Model which makes no a priori as- sumption on the relationship between them. We thus examine the conditions for obtaining such agreement and find that, in the framework of our model, this holds only in a relatively narrow range of excitation energy. The role played by the qualitative shape of the fragments' state densities is also examined. Our results suggest that the internal temperature of the light fragments may be affected by this quant…
The ratio of symmetry energy coefficient to temperature $C_{sym}/T$ is extracted from different prescriptions using the isotopic as well as the isobaric yield distributions obtained in different projectile fragmentation reactions. It is found that the values extracted from our theoretical calculation agree with those extracted from the experimental data but they differ very much from the input value of the symmetry energy used. The best possible way to deduce the value of the symmetry energy coefficient is to use the fragment yield at the breakup stage of the reaction and it is better to use t…
A quantum statistical model of nuclear multifragmentation is proposed. The recurrence equation method used within the canonical ensemble makes the model solvable and transparent to physical assumptions and allows to get results without involving the Monte Carlo technique. The model exhibits the first order phase transition. Quantum statistics effects are clearly seen on the microscopic level of occupation numbers but are almost washed out for global thermodynamic variables and the averaged observables studied. In the latter case, the recurrence relations for multiplicity distributions of both …
The deexcitation of the primary hot fragments, produced in the breakup of an excited nuclear source, during their propagation under the influence of their mutual Coulomb repulsion is studied in the framework of a recently developed hybrid model. The latter is based on the Statistical Mul- tifragmentation Model (SMM), describing the prompt breakup of the source, whereas the particle emission from the hot fragments, that decay while traveling away from each other, is treated by the Weisskopf-Ewing evaporation model. Since this treatment provides an event by event descrip- tion of the process, in…
Density fluctuations of expanding nuclear matter are studied within a mean-field model in which fluctuations are generated by an external stochastic field. Fluctuations develop about a mean one-body phase-space density corresponding to a hydrodinamic motion that describes a slow expansion of the system. A fluctuation-dissipation relation suitable for a uniformly expanding medium is obtained and used to constrain the strength of the stochastic field. The distribution of the liquid domains in the spinodal decomposition is derived. Comparison of the related distribution of the fragment size with …
We include in statistical model calculations the facts that in the nuclear multifragmentation process the fragments are produced within a given volume and have a finite size. The corrections associated with these constraints affect the partition modes and, as a consequence, other observables in the process. In particular, we find that the favored fragmenting modes strongly suppress the collective flow energy, leading to much lower values compared to what is obtained from unconstrained calculations. This leads, for a given total excitation energy, to a nontrivial correlation between the breakup…
In multifragmentation of hot nuclear matter, properties of fragments embedded in a soup of nucleonic gas and other fragments should be modified as compared with isolated nuclei. Such modifications are studied within a simple model where only nucleons and one kind of heavy nuclei are considered. The interaction between different species is described with a momentum-dependent two-body potential whose parameters are fitted to reproduce properties of cold isolated nuclei. The internal energy of heavy fragments is parametrized according to a liquid-drop model with density and temperature dependent …
The experimental measures of the multiplicity derivatives, the moment parameters, the bimodal parameter, the fluctuation of maximum fragment charge number (NVZ), the Fisher exponent ($τ$) and Zipf's law parameter ($ξ$), are examined to search for the liquid-gas phase transition in nuclear multifragmention processes within the framework of the statistical multifragmentation model (SMM). The sensitivities of these measures are studied. All these measures predict a critical signature at or near to the critical point both for the primary and secondary fragments. Among these measures, the total mul…
Order parameter fluctuations (the largest cluster size distribution) are studied within a three-dimensional bond percolation model on small lattices. Cumulant ratios measuring the fluctuations exhibit distinct features near the percolation transition (pseudocritical point), providing a method for its identification. The location of the critical point in the continuous limit can be estimated without variation of the system size. This method is remarkably insensitive to finite-size effects and may be applied even for a very small system. The possibility of using various measurable quantities for…
The physics and the technical algorithms of the statistical de-excitation code ABLA07 are documented. The new developments of ABLA07 have been guided by the empirical knowledge obtained in a recent experimental campaign on the nuclide distributions measured at GSI, Darmstadt. Besides distinct signatures of very asymmetric binary splits, lighter systems show clear features of multifragmentation, while heavy systems reveal the influence of dynamics and microscopic structure on the fission process. ABLA07 includes elaborate but efficient descriptions of all these processes, with one set of the mo…
Nuclear collisions at intermediate, relativistic, and ultra-relativistic energies offer unique opportunities to study in detail manifold fragmentation and clustering phenomena in dense nuclear matter. At intermediate energies, the well known processes of nuclear multifragmentation -- the disintegration of bulk nuclear matter in clusters of a wide range of sizes and masses -- allow the study of the critical point of the equation of state of nuclear matter. At very high energies, ultra-relativistic heavy-ion collisions offer a glimpse at the substructure of hadronic matter by crossing the phase …
In this talk I discuss properties of hot stellar matter at sub-nuclear densities which is formed in supernova explosions. I emphasize that thermodynamic conditions there are rather similar to those created in the laboratory by intermediate-energy heavy-ion collisions. Theoretical methods developed for the description of multi-fragment final states in such reactions can be used also for description of the stellar matter. I present main steps of the statistical approach to the equation of state and nuclear composition, dealing with an ensemble of nuclear species instead of one "average" nucleus.
We show that the statistical multifragmentation model with the standard parameterization of the free volume predicts a constant pressure as density approaches the normal nuclear density. This is contrary to the Raduta&Raduta result obtained by disregarding the center of mass constraint. It is demonstrated that in finite nuclear systems the partitions with small number of fragments play an important role.
The study of liquid-gas phase transition in heavy ion collisions has generated a lot of interest amongst the nuclear physicists in the recent years. In heavy ion collisions, there is no direct way of measuring the state variables like entropy, pressure, energy and hence unambiguous characterization of phase transition becomes difficult. This work proposes new signatures of phase transition that can be extracted from the observables which are easily accessible in experiments. It is observed that the temperature dependence of the first order derivative of the order parameters in nuclear liquid g…
The density fluctuations of nuclear matter are studied within a mean-field model in wich fluctuations are generated by an external stochastic field. The constraints imposed on the random force by the fluctuation-dissipation theorem are analyzed. It is shown that in the proximity of the borders of the spinodal region the assumption of a white-noise stochastic field can be reliably used. The domain distribution of the liquid phase in the spinodal decomposition of nuclear matter is derived. The related distribution of fragment sizes compares favourably with the experimental fragment distribution …
