We explore the formation and collective modes of Bose-Einstein condensate of Dirac magnons (Dirac BEC). While we focus on two-dimensional Dirac magnons, an employed approach is general and could be used to describe Bose-Einstein condensates with linear quasiparticle spectrum in various systems. By using a phenomenological multicomponent model of pumped boson population together with bosons residing at Dirac nodes, the formation and time evolution of condensates of Dirac bosons is investigated. The condensate coherence and its multicomponent nature are manifested in the Rabi oscillations whose period is determined by the gap in the spin-wave spectrum. A Dirac nature of the condensates could be also probed by the spectrum of collective modes. It is shown that the Haldane gap provides an efficient means to tune between the gapped and gapless collective modes as well as controls their stability.
We present a microscopic theory of magnon transport in ferromagnetic insulators (FIs). Using magnon injection through microwave pumping, we propose a way to generate magnon dc currents and show how to enhance their amplitudes in hybrid ferromagnetic insulating junctions. To this end focusing on a single FI, we first revisit microwave pumping at finite (room) temperature from the microscopic viewpoint of magnon injection. Next, we apply it to two kinds of hybrid ferromagnetic insulating junctions. The first is the junction between a quasi-equilibrium magnon condensate and magnons being pumped b…
We clarify the condition for the occurrence of magnon Bose-Einstein condensation (BEC) in spin pumping systems without using external pumping magnetic fields. The Goldstone model is generalized and the stability of the vacuum is closely investigated. By applying the generalized Goldstone model to spin pumping systems, the condition for the experimental realization of the stable magnon BEC in spin pumping systems is theoretically proposed.
We theoretically investigate spin transfer between a system of quasiequilibrated Bose-Einstein condensed magnons in an insulator in direct contact with a conductor. While charge transfer is prohibited across the interface, spin transport arises from the exchange coupling between insulator and conductor spins. In normal insulator phase, spin transport is governed solely by the presence of thermal and spin-diffusive gradients; the presence of Bose-Einstein condensation (BEC), meanwhile, gives rise to a temperature-independent condensate spin current. Depending on the thermodynamic bias of the sy…
We experimentally identify coherent spin pumping in the magnon-magnon hybrid modes of permalloy/yttrium iron garnet (Py/YIG) bilayers. Using broadband ferromagnetic resonance, an "avoided crossing" is observed between the uniform mode of Py and the spin wave mode of YIG due to the fieldlike interfacial exchange coupling. We also identify additional linewidth suppression and enhancement for the in-phase and out-of-phase hybrid modes, respectively, \textcolor{black}{which can be interpreted as concerted dampinglike torque from spin pumping}. Our analysis predicts inverse proportionality of both …
The combination of parametric pumping and spin-transfer torque is a powerful approach that enables high-level control over magnetic excitations in thin-film ferromagnets. The excitation parameters, such as pumping power and external field strength, affect the instabilities of individual magnon modes. We theoretically explore how the simultaneous effects of parametric pumping and spin transfer torque influence these magnetic instabilities in a thin-film ferromagnet. Within the Landau-Lifshitz-Gilbert framework, we perform micromagnetic simulations of magnon excitations in yttrium iron garnet by…
We demonstrate how a magnon chemical potential is generated in parametric parallel pumping. We study how a time-periodic magnetic field of this pumping affects magnon properties of a ferrimagnet in a nonequilibrium steady state. We show that the magnon distribution function of our nonequilibrium steady state becomes the Bose distribution function with $μ=ω_{\textrm{p}}/2$, where $μ$ is the magnon chemical potential and $ω_{\textrm{p}}$ is the pumping frequency. This result is distinct from the absence of the magnon chemical potential in the standard theory and can qualitatively explain its gen…
On the basis of the Schwinger-Keldysh formalism, we have closely investigated the temperature dependence of quantum spin pumping by electron spin resonance. We have clarified that three-magnon splittings excite non-zero modes of magnons and characterize the temperature dependence of quantum spin pumping. Our theoretical result qualitatively agrees with the experiment by Czeschka et al. that the mixing conductance is little influenced by temperature [F. D. Czeschka et al., Phys. Rev. Lett., 107, 046601 (2011)].
A phenomenological theory is developed, that accounts for the collective dynamics of a Bose-Einstein condensate of magnons. In terms of such description we discuss the nature of spontaneous macroscopic interference between magnon clouds, highlighting the close relation between such effects and the well known Josephson effects. Using those ideas we present a detailed calculation of the Josephson oscillations between two magnon clouds, spatially separated in a magnonic Josephson junction.
We experimentally show that exchange magnons can be detected using a combination of spin pumping and inverse spin-Hall effect (iSHE) proving its wavelength integrating capability down to the sub-micrometer scale. The magnons were injected in a ferrimagnetic yttrium iron garnet film by parametric pumping and the iSHE-induced voltage was detected in an attached Pt layer. The role of the density, wavelength, and spatial localization of the magnons for the spin pumping efficiency is revealed. This study opens the field of the magnon-based information processing to magnons with nano-scale wavelengt…
We propose to excite a large number of coherent magnons with high momentum in optical cavities. This is achieved by two counterpropagating optical modes that are detuned by the frequency of a selected magnon, similar to stimulated Raman scattering. In sub-mm size yttrium iron garnet spheres, a mW laser input power generates 10^6-10^8 coherent magnons. The large magnon population enhances Brillouin light scattering, a probe suitable to access their quantum properties.
We formulate a microscopic linear response theory of nonequilibrium magnonic torques and magnon pumping applicable to multiple-magnonic-band uniform ferromagnets with Dzyaloshinskii-Moriya interactions. From the linear response theory, we identify the extrinsic and intrinsic contributions where the latter is expressed via the Berry curvature of magnonic bands. We observe that in the presence of a time-dependent magnetization Dzyaloshinskii-Moriya interactions can act as fictitious electric fields acting on magnons. We study various current responses to this fictitious field and analyze the rol…
The magnon pumping effect in ferromagnetic insulators under an external time-dependent transverse magnetic field is theoretically studied. Generation of a magnon current is discussed by calculating the magnon source term in the spin continuity equation. This term represents the non-conservation of magnons arising from an applied transverse magnetic field. The magnon source term has a resonance structure as a function of the angular frequency of the transverse field, and this fact is useful to enhance the pumping effect.
The richness in both the dispersion and energy of antiferromagnetic magnons has spurred the magnetism community to consider antiferromagnets for future spintronic/magnonic applications. However, the excitation and control of antiferromagnetic magnons remains challenging, especially when compared to ferromagnetic counterparts. A middle ground is found with synthetic antiferromagnet metamaterials, where acoustic and optical magnons exist at GHz frequencies. In these materials, the magnon energy spectrum can be tuned by static symmetry-breaking external fields or dipolar interactions hybridizing …
Thermalization of a parametrically driven magnon gas leading to the formation of a Bose-Einstein condensate at the bottom of a spin-wave spectrum was studied by time- and wavevector-resolved Brillouin light scattering spectroscopy. It has been found that the condensation is preceded by the conversion of initially pumped magnons into a second group of frequency degenerated magnons, which appear due to parametrically stimulated scattering of the initial magnons to a short-wavelength spectral region. In contrast to the first magnon group, which wavevectors are orthogonal to the wavevectors of the…
We theoretically propose quantum spin pumping mediated by magnons, under a time-dependent transverse magnetic field, at the interface between a ferromagnetic insulator and a non-magnetic metal. The generation of a spin current under a thermal equilibrium condition is discussed by calculating the spin transfer torque, which breaks the spin conservation law for conduction electrons and operates the coherent magnon state. Localized spins lose spin angular momentum by emitting magnons and conduction electrons flip from down to up by absorbing the momentum. The spin transfer torque has a resonance …
We study the exchange between electron and magnon spins at the interface of an antiferromagnet and a heavy metal at finite temperatures. The underlying physical mechanism is based on spin torque associated with the creation/annihilation of thermal magnons with right-hand and left-hand polarization. The creation/annihilation process depends strongly on the relative orientation between the polarization of the electron and the magnon spins. For a sufficiently strong spin transfer torque (STT), the conversion process becomes nonlinear, generating a nonzero net spin pumping current in the AFM that …
We study pumping of magnons to the Dirac points of magnon's Brillouin zone of a ferromagnet on a honeycomb lattice. In particular, we consider second-order Suhl process, when due to interaction between magnons, a pair of magnons is created due to absorption of two electromagnetic wave quanta. We introduce a bosonic analog of the Cooper ladder for the magnon pair, which is shown to enhance the pairing of magnons at the Dirac points. As a result of pairing of the Dirac magnons, the system becomes unstable towards formation of a magnetic state with zero or reduced magnetization - the Dirac magnon…
The quanta of magnetic excitations - magnons - are known for their unique ability to undergo Bose-Einstein condensation at room temperature. This fascinating phenomenon reveals itself as a spontaneous formation of a macroscopic coherent state under the influence of incoherent stimuli. Spin currents have been predicted to offer electronic control of magnon Bose-Einstein condensates, but this phenomenon has not been experimentally evidenced up to now. Here we experimentally show that current-driven Bose-Einstein condensation can be achieved in nanometer-thick films of magnetic insulators with ta…
We establish a general formulation for spin current pumped by magnons at the interface between a normal metal and a magnetic insulator, valid for any non-collinear magnetic configuration in the linear spin wave regime. This current is generated by driving the system in a non-equilibrium state, covering setups such as thermal spin injection (spin Seebeck effect) or spin voltage by irradiation of the insulator (spin pumping). We illustrate the formula in the special case of a honeycomb topological ferromagnet, for simplicity, and cover both the spin Seebeck and spin-pumping setups. We show how t…
Chiral spin pumping is the generation of a unidirectional spin current in half of ferromagnetic films or conductors by dynamic dipolar stray fields from close-by nanomagnets. We formulate a general theory of long-range chiral interactions between magnets mediated by unidirectional traveling waves, e.g., spin waves in a magnetic film or microwaves in a waveguide. The traveling waves emitted by an excited magnet can be perfectly trapped by a second, initially passive, magnet by a dynamical interference effect. When both magnets are excited by a uniform microwave, the chiral interaction between t…
We microscopically analyze thermal spin pumping mediated by magnons, at the interface between a ferromagnetic insulator and a non-magnetic metal, in the semiclassical regime. The generation of a spin current is discussed by calculating the thermal spin transfer torque, which breaks the spin conservation law for conduction electrons and operates the coherent magnon state. Inhomogeneous thermal fluctuations between conduction electrons and magnons induce a net spin current, which is pumped into the adjacent non-magnetic metal. The pumped spin current is proportional to the temperature difference…
Motivated by recent experiments on spin pumping from a ferromagnet into organic materials in which the charge transport is due to hopping, we study theoretically the generation and propagation of spin current in a hopping insulator. Unlike metals, the spin polarization at the boundary with ferromagnet is created as a result of magnon absorption within pairs of localized states and it spreads following the current-currying resistor network (although the charge current is absent). We consider a classic resonant mechanism of the ac absorption in insulators and adapt it to the absorption of magnon…
Magnonic spontaneous oscillation induced by parametric pumping
Argonne National Laboratory（阿贡国家实验室）；Carthage College（卡里斯学院）；University of Illinois Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校）；University of Colorado Colorado Springs（科罗拉多大学科泉分校）
The spectral distribution of parametrically excited dipole-exchange magnons in an in-plane magnetized epitaxial film of yttrium-iron garnet was studied by means of frequency- and wavevector-resolved Brillouin light scattering spectroscopy. The experiment was performed in a parallel pumping geometry where an exciting microwave magnetic field was parallel to the magnetizing field. It was found that for both dipolar and exchange spectral areas parallel pumping excites the lowest volume magnon modes propagating in the film plane perpendicularly to the magnetization direction. In order to interpret…
An easy-plane ferromagnetic insulator in a uniform external magnetic field and in contact with a phonon bath and a normal metal bath is studied theoretically in the presence of dc spin current injection via the spin Hall effect in the metal. The Keldysh path integral formalism is used to model the magnon gas driven into a nonequilibrium steady state by mismatched bath temperatures and/or electrical injection, and we analyze the magnon system in the normal (uncondensed) state, but close to the instability to Bose-Einstein condensation (BEC), within the self-consistent Hartree-Fock approximation…
Local temperature control of magnon frequency and direction of supercurrents in a magnon Bose-Einstein condensate
Rheinland-Pfälzische Technische Universität Kaiserslautern-Landau（莱茵兰-普法尔茨技术大学凯泽斯劳滕-兰道）；Weizmann Institute of Science（魏茨曼科学研究所）；Fraunhofer Institute for Industrial Mathematics ITWM（弗劳恩霍夫工业数学研究所）
We theoretically study spin pumping from a layered van der Waals antiferromagnet in its canted ground state into an adjacent normal metal. We find that the resulting dc spin pumping current bears contributions along all spin directions. Our analysis allows for detecting intra- and cross-sublattice spin-mixing conductances via measuring the two in-plane spin current components. We further show that sublattice symmetry-breaking Gilbert damping can be realized via interface engineering and induces a dissipative coupling between the optical and acoustic magnon modes. This realizes magnon level att…
Magnonics and magnon spintronics aim at the utilization of spin waves and magnons, their quanta, for the construction of wave-based logic networks via the generation of pure all-magnon spin currents and their interfacing with electrical charge transport. The promise of efficient parallel data processing and low power consumption renders this field one of the most promising research areas in spintronics. In this context, the process of parallel parametric amplification, i.e., the conversion of microwave photons into magnons at one half of the microwave frequency, has proven to be a versatile to…
Bose-Einstein condensation (BEC) of magnons is one of few macroscopic quantum phenomena observable at room temperature. Due to competition of the exchange and the magnetic dipole interactions the minimum-energy magnon state is doubly degenerate and corresponds to two antiparallel non-zero wavevectors. Correspondingly, magnon BEC differs essentially from other condensates, since it takes place simultaneously at +/-k_min. The degeneracy of BEC and interaction between its two components have significant impact on the condensate properties. Phase locking of the two condensates causes formation of …
We formulate a phenomenological description of thin ferromagnetic layers with inversion asymmetry where the single-domain magnetic dynamics experiences magnon current-induced torques and leads to magnon-motive forces. We first construct a phenomenological theory based on irreversible thermodynamics, taking into account the symmetries of the system. Furthermore, we confirm that these effects originate from Dzyaloshinskii-Moriya interactions from the analysis based on the stochastic Landau-Lifshitz-Gilbert equation. Our phenomenological results generalize to a general form of Dzyaloshinskii-Mori…
Using the Aharonov-Casher (A-C) phase, we present a microscopic theory of the Josephson and persistent spin currents in quasi-equilibrium Bose-Einstein condensates (BECs) of magnons in ferromagnetic insulators. Starting from a microscopic spin model that we map onto a Gross-Pitaevskii Hamiltonian, we derive a two-state model for the Josephson junction between the weakly coupled magnon-BECs. We then show how to obtain the alternating-current (ac) Josephson effect with magnons as well as macroscopic quantum self-trapping in a magnon-BEC. We next propose how to control the direct-current (dc) Jos…
Sub-picosecond magnetisation manipulation via femtosecond optical pumping has attracted wide attention ever since its original discovery in 1996. However, the spatial evolution of the magnetisation is not yet well understood, in part due to the difficulty in experimentally probing such rapid dynamics. Here, we find evidence of rapid magnetic order recovery in materials with perpendicular magnetic anisotropy via nonlinear magnon processes. We identify both localisation and coalescence regimes, whereby localised magnetic textures nucleate and subsequently evolve in accordance with a power law fo…
We report on the experimental observation of excitation and detection of parametric spin waves and spin currents in the bulk acoustic wave resonator. The hybrid resonator consists of ZnO piezoelectric film, yttrium iron garnet (YIG) films on gallium gadolinium garnet substrate, and a heavy metal Pt layer. Shear bulk acoustic waves are electrically excited in the ZnO layer due to piezoeffect at the resonant frequencies of the resonator. The magnetoelastic interaction in the YIG film emerges magnons (spin waves) excitation by acoustic waves either on resonator's eigenfrequencies or the half-valu…
We investigate the spin-pumping-induced electric current on the surface of a three-dimensional topological insulator hybridized with a ferromagnet, namely, ferromagnetic topological insulator. In order to do this, we establish the microscopic formalism and construct the perturbation theory using a Keldysh Green's function approach. We analyze how this electric current is generated by an exchange interaction and an external ac magnetic field, which is the driving force of ferromagnetic resonance as well as the spin pumping. The mechanism is as follows. First, the ferromagnetic resonance is driv…
"Pumping" of phonons by a dynamic magnetization promises to extend the range and functionality of magnonic devices. We explore the impact of phonon pumping on room-temperature ferromagnetic resonance (FMR) spectra of bilayers of thin yttrium iron garnet (YIG) films on thick gadolinium gallium garnet substrates over a wide frequency range. At low frequencies the Kittel mode hybridizes coherently with standing ultrasound waves of a bulk acoustic resonator to form magnon polarons that induce rapid oscillations of the magnetic susceptibility, as reported before. At higher frequencies, the phonon r…
The formation of a Bose condensate of magnons in a perpendicularly magnetized film of yttrium iron garnet under radio-frequency pumping in a strip line is studied experimentally. The characteristics of nonlinear magnetic resonance and the spatial distribution of the Bose condensate of magnons in the magnetic field gradient are investigated. In these experiments, the Bosonic system of magnons behaves similarly to the Bose condensate of magnons in the antiferromagnetic superfluid 3He-B, which was studied in detail earlier. Magnonic BEC forms a coherently precessing state with the properties of m…
Using newly developed quantum-classical hybrid framework, we investigate interaction between spin-polarized conduction electrons and a single spin wave (SW) coherently excited within a metallic ferromagnetic nanowire. When the nanowire hosting SW is attached to two normal metal (NM) leads, with no dc bias voltage applied between them, the SW pumps chiral electronic charge and spin currents into the leads---their direction is tied to the direction of SW propagation and they scale linearly with the frequency of the precession. This is in contrast to: standard pumping by the uniform precession mo…
We investigate the stability of the recently discovered room temperature Bose-Einstein condensate (BEC) of magnons in Ytrrium Iron Garnet (YIG) films. We show that magnon-magnon interactions depend strongly on the external field orientation, and that the BEC in current experiments is actually metastable - it only survives because of finite size effects, and because the BEC density is very low. On the other hand a strong field applied perpendicular to the sample plane leads to a repulsive magnon-magnon interaction; we predict that a high-density magnon BEC can then be formed in this perpendicul…
Bose-Einstein condensation of quasi-equilibrium magnons is one of few macroscopic quantum phenomena observed at room temperature. Since its discovery, it became an object of intense research, which led to the observation of many exciting phenomena such as quantized vortices, second sound, and Bogolyubov waves. However, for a long time it remained unclear, what physical mechanisms can be responsible for the spatial stability of the magnon condensate. Indeed, since magnons are believed to exhibit attractive interaction, it is generally expected that the magnon condensate should be unstable with …
We explore routes to realize electrically driven Bose-Einstein condensation of magnons in insulating antiferromagnets. Even in insulating antiferromagnets, the localized spins can strongly couple to itinerant spins in adjacent metals via spin-transfer torque and spin pumping. We describe the formation of steady-state magnon condensates controlled by a spin accumulation polarized along the staggered field in an adjacent normal metal. Two types of magnons exist in antiferromagnets, which carry opposite magnetic moments. Consequently, and in contrast to ferromagnets, Bose-Einstein condensation ca…
Spintronics is the science and technology of electric control over spin currents in solid-state-based devices. Recent advances have demonstrated a coupling between electronic spin currents in non-magnetic metals and magnons in magnetic insulators. The coupling is due to spin transfer and spin pumping at interfaces between the normal metals and magnetic insulators. In this Chapter, we review these developments and the prospects they raise for electric control of quasi-equilibrium magnon Bose-Einstein condensates and spin superfluidity.
We propose inducing Bose-Einstein condensation of magnons in a magnetic insulator by a heat flow oriented toward its boundary. At a critical heat flux, the oversaturated thermal gas of magnons accumulated at the boundary precipitates the condensate, which then grows gradually as the thermal bias is dialed up further. The thermal magnons thus pumped by the magnonic bulk (spin) Seebeck effect must generally overcome both the local Gilbert damping associated with the coherent magnetic dynamics as well as the radiative spin-wave losses toward the magnetic bulk, in order to achieve the threshold of…
We would like to point out the blind spots of the approach combining the spin pumping theory proposed by Tserkovnyak et al. with the Landau-Lifshitz-Gilbert equation; this method has been widely used for interpreting vast experimental results. The essence of the spin pumping effect is the quantum fluctuation. Thus, localized spin degrees of freedom should be quantized, i.e. be treated as magnons not as classical variables. Consequently, the precessing ferromagnet can be regarded as a magnon battery. This point of view will be useful for further progress of spintronics.
We propose a stabilizing mechanism for the Bose-Einstein condensation (BEC) of interacting magnons in ferrimagnets and ferromagnets. By studying the effects of the magnon-magnon interaction on the stability of the magnon BEC in a ferrimagnet and two ferromagnets, we show that the magnon BEC remains stable even in the presence of the magnon-magnon interaction in the ferrimagnet and ferromagnet with a sublattice structure, whereas it becomes unstable in the ferromagnet without a sublattice structure. This indicates that the existence of a sublattice structure is the key to stabilizing the BEC of…
We propose a mechanism for destabilizing or stabilizing Bose-Einstein condensation (BEC) of interacting magnons in an antiferromagnet. We study how the interaction between magnons affects the magnon BEC in a two-sublattice antiferromagnet without and with an external magnetic field. We show that in the absence of the magnetic field the magnon BEC is destabilized by the attractive interband interaction, which is larger than the repulsive intraband interaction. We also show that in the presence of the magnetic field the magnon BEC is stabilized only if the magnetic field is large enough to make …
