酶的趋化性和增强扩散的非平衡理论
Nonequilibrium theory of enzyme chemotaxis and enhanced diffusion
摘要：
在过去的十年中，在几个实验中报道了酶的增强扩散和抗趋化性，在应用和基础层面上开辟了生物纳米科学研究的全新途径。在这里，我们介绍了一个新的理论框架，植根于催化循环的非平衡效应的特点，解释了所有的观察到目前为止，在这一领域。此外，我们的理论预测了全新的效应，如耗散诱导的抗趋化和趋化行为之间的转换。
英文摘要：
Enhanced diffusion and anti-chemotaxis of enzymes have been reported in several experiments in the last decade, opening up entirely new avenues of research in the bio-nanosciences both at the applied and fundamental level. Here, we introduce a novel theoretical framework, rooted in non-equilibrium effects characteristic of catalytic cycles, that explains all observations made so far in this field. In addition, our theory predicts entirely novel effects, such as dissipation-induced switch between anti-chemotactic and chemotactic behavior.
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