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arXiv 2007.08268cond-mat.mtrl-sci
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磁性Weyl半金属Co3Sn2S2中本征和非本征共同驱动的33%巨反常霍尔电流

33% Giant Anomalous Hall Current Driven by both Intrinsic and Extrinsic Contributions in Magnetic Weyl Semimetal Co3Sn2S2

Jianlei Shen, Qingqi Zeng, Shen Zhang, Hongyi Sun, Qiushi Yao, Xuekui Xi, Wenhong Wang, Guangheng Wu, Baogen Shen, Qihang Liu, Enke Liu

摘要:

反常霍尔效应(AHE)可以由带内贝里相和杂质散射引起的非本征机制引起。最近发现的磁性Weyl半金属Co_3Sn_2S_2具有大的本征反常霍尔电导率(AHC)和巨大的反常霍尔角(AHA)。预测的这种材料中AHC的能量依赖性在1000 Ω-1 cm-1处表现出平台,能量宽度为100 meV,刚好低于EF,从而意味着大的本征AHC不会因小尺度能量扰动(如轻微的p掺杂)而显著改变。在这里,我们成功地触发外来原子散射的外在贡献,除了本征的原始材料通过引入少量的Fe掺杂剂,以取代Co在Co 3Sn 2S 2。我们的实验结果表明,由于TYJ模型所区分的内在和外在机制的协同贡献,AHC和AHA可以显著增强,分别达到1850 Ω-1 cm-1和33%。特别是,调谐的AHA在已知的磁性材料中保持低场的记录值。这项研究开辟了一条在磁性Weyl半金属中设计巨型AHE的途径,从而可能推进拓扑自旋电子学/Weyltronics。

英文摘要:

Anomalous Hall effect (AHE) can be induced by intrinsic mechanism due to the band Berry phase and extrinsic one arising from the impurity scattering. The recently discovered magnetic Weyl semimetal Co3Sn2S2 exhibits a large intrinsic anomalous Hall conductivity (AHC) and a giant anomalous Hall angle (AHA). The predicted energy dependence of the AHC in this material exhibits a plateau at 1000 Ω-1 cm-1 and an energy width of 100 meV just below EF, thereby implying that the large intrinsic AHC will not significantly change against small-scale energy disturbances such as slight p-doping. Here, we successfully trigger the extrinsic contribution from alien-atom scattering in addition to the intrinsic one of the pristine material by introducing a small amount of Fe dopant to substitute Co in Co3Sn2S2. Our experimental results show that the AHC and AHA can be prominently enhanced up to 1850 Ω-1 cm-1 and 33%, respectively, owing to the synergistic contributions from the intrinsic and extrinsic mechanisms as distinguished by the TYJ model. In particular, the tuned AHA holds a record value in low fields among known magnetic materials. This study opens up a pathway to engineer giant AHE in magnetic Weyl semimetals, thereby potentially advancing the topological spintronics/Weyltronics.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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