Purity monitor devices are increasingly used in noble gas time projection chambers to measure the lifetime of drifting electrons. Purity monitors work by emitting electrons from a photocathode material via the photoelectric effect. The electrons are then drifted towards an anode by means of an applied electric drift field. By measuring the difference in charge between the cathode and the anode, one can extract the lifetime of the drifting electrons in the medium. For the first time, we test the performance of different photocathode materials-- silver, titanium, and aluminium--and compare them to gold, which is the standard photocathode material used for purity monitors. Titanium and aluminium were found to have a worse performance than gold in vacuum, whereas silver showed a signal of the same order of magnitude as gold. Further tests in liquid argon were carried out on silver and gold with the conclusion that the signal produced by silver is about three times stronger than that of gold.
The Liquid Argon Purity Demonstrator was an R&D test stand designed to determine if electron drift lifetimes adequate for large neutrino detectors could be achieved without first evacuating the cryostat. We describe here the cryogenic system, its operations, and the apparatus used to determine the contaminant levels in the argon and to measure the electron drift lifetime. The liquid purity obtained by this system was facilitated by a gaseous argon purge. Additionally, gaseous impurities from the ullage were prevented from entering the liquid at the gas-liquid interface by condensing the gas an…
We report the measurement of longitudinal electron diffusion coefficients in liquid argon for electric fields between 100 and 2000 V/cm with a gold photocathode as a bright electron source. The measurement principle, apparatus, and data analysis are described. Our results, which are consistent with previous measurements in the region between 100 to 350 V/cm [1] , are systematically higher than the prediction of Atrazhev-Timoshkin[2], and represent the world's best measurement in the region between 350 to 2000 V/cm. The quantum efficiency of the gold photocathode, the drift velocity and longitu…
Measuring the argon purity is critical for all Ar-based rare event research experiments. Mass spectrometry is typically used to assess the uranium and thorium contamination in samples of the materials used to build low-background detectors; however, this technique has the potential to provide other valuable information that is currently not exploited. We have shown that, by ICP-MS, it is possible to identify and quantify common chemical contaminants in argon. Preliminary tests were done with the gas extracted from the experiments MicroBooNE at FNAL and ArDM at LSC. In the former case, we evide…
We demonstrate, for the time, the operation of a bubble-assisted Liquid Hole Multiplier (LHM) in liquid argon. The LHM, sensitive to both radiation-induced ionization electrons and primary scintillation photons, consists of a perforated electrode immersed in the noble liquid, with a stable gas-bubble trapped underneath. Electrons deposited in the liquid or scintillation-induced photoelectrons emitted from a photocathode on the electrode's surface, are collected into the holes; after crossing the liquid-gas interface, they induce electroluminescence within the bubble. After having validated in …
Presented here are first tests of a Gaseous Photomultiplier based on a cascade of Thick GEM structures intended for gamma-ray position reconstruction in liquid Argon. The detector has a MgF$_2$ window, transparent to VUV light, and a CsI photocathode deposited on the first THGEM. A gain of $8\cdot10^{5}$ per photoelectron and $\sim100\%$ photoelectron collection efficiency are measured at stable operation settings. The excellent position resolution capabilities of the detector (better than 100 $μ$m) at 100 kHz readout rate, is demonstrated at room temperature. Structural integrity tests of the…
Future giant liquid argon (LAr) time projection chambers (TPCs) require a purity of better than 0.1 parts per billion (ppb) to allow the ionised electrons to drift without significant capture by any electronegative impurities. We present a comprehensive study of the effects of electronegative impurity on gaseous and liquid argon scintillation light, an analysis of the efficacy of various purification chemicals, as well as the Liverpool LAr setup, which utilises a novel re-circulation purification system. Of the impurities tested - Air, O_2, H_2O, N_2 and CO_2 in the range of between 0.01 ppm t…
We describe the design of a 20-liter test stand constructed to study fundamental properties of liquid argon (LAr). This system utilizes a simple, cost-effective gas argon (GAr) purification to achieve high purity, which is necessary to study electron transport properties in LAr. An electron drift stack with up to 25 cm length is constructed to study electron drift, diffusion, and attachment at various electric fields. A gold photocathode and a pulsed laser are used as a bright electron source. The operational performance of this system is reported.
Procurement and Purification of Liquid Argon for the LEGEND-200 Experiment
Jagiellonian University（雅盖隆大学）；Technical University of Munich（慕尼黑工业大学）；Istituto Nazionale di Fisica Nucleare, Laboratori Nazionali del Gran Sasso（意大利国家核物理研究所，格兰萨索国家实验室）
We present a model for the Global Quantum Efficiency (GQE) of the MicroBooNE optical units. An optical unit consists of a flat, circular acrylic plate, coated with tetraphenyl butadiene (TPB), positioned near the photocathode of a 20.2-cm diameter photomultiplier tube. The plate converts the ultra-violet scintillation photons from liquid argon into visible-spectrum photons to which the cryogenic phototubes are sensitive. The GQE is the convolution of the efficiency of the plates that convert the 128 nm scintillation light from liquid argon to visible light, the efficiency of the shifted light …
Development of a novel high-sensivitiy LAr purity monitor based on an $α$-source
研制了一种新型的液氩纯度监测器，其灵敏度可达ppb级（O $_2$当量）。这种高纯度例如在LAr漂移室中是需要的。其原理是测量LAr中准自由电子的寿命，因为这是漂移室操作的重要参数。自由电子是通过用$α$ -粒子电离LAr产生的，该粒子由同位素$^{210}Pb$源的$^{210}Po$链子体发射。通过测量漂移路径开始和结束时电子云的电荷以及漂移时间，可以获得电子的寿命。$α$ -粒子具有约50 μ $m in LAr and the ionization density is very high, typically between $ 750 <$1500 \rm MeV/cm $, leading to a high recombination rate. To suppress the recombination of the argon ions with the electrons, the $ α $-source was put in a strong electric field of $ 40 <$150 $ kV/cm的非常短的范围。这是通过将源沉积在直径约为0.5 mm的球形高压阴极的表面上来实现的。阳极也被制成与阴极直径大致相同的球体，因此，靠近两个电极之间的轴，电漂移场近似为偶极场。
Experiments based on noble elements such as gaseous or liquid argon or xenon utilize the ionization and scintillation properties of the target materials to detect radiation-induced recoils. A requirement for high light and charge yields is to reduce electronegative impurities well below the ppb level. To achieve this, the target material is continuously circulated in the gas phase through a purifier and returned to the detector. Additionally, the low backgrounds necessary dictate low-Rn-emanation rates from all components that contact the gas. Since commercial pumps often introduce electronega…
In this paper, we report on the design and operation of the LongBo time projection chamber in the Liquid Argon Purity Demonstrator cryostat. This chamber features a 2 m long drift distance. We measure the electron drift lifetime in the liquid argon using cosmic ray muons and the lifetime is at least 14 ms at 95\% confidence level. LongBo is equipped with preamplifiers mounted on the detector in the liquid argon. Of the 144 channels, 128 channels were readout by preamplifiers made with discrete circuitry and 16 channels were readout by ASIC preamplifiers. For the discrete channels, we measure a…
This paper describes the design, realization and operation of a prototype liquid Argon Time Projection Chamber (LAr TPC) detector dedicated to the development of a novel online monitoring and calibration system exploiting UV laser beams. In particular, the system is intended to measure the lifetime of the primary ionization in LAr, in turn related to the LAr purity level. This technique could be exploited by present and next generation large mass LAr TPCs for which monitoring of the performance and calibration plays an important role. Results from the first measurements are presented together …
In this paper we describe the performance of a light detector for Ar scintillation light made of wavelength-shifting (WLS) fibers connected to Silicon-Photomultipliers (SiPM). The setup was conceived to be used as anti-Compton veto for high purity germanium (HPGe) detectors operated directly in liquid Argon (LAr). Background suppression efficiencies for different radioactive sources were measured in a test cryostat with about 800 kg LAr. This work was part of the R\&D effort for the GERDA experiment.
Voltages above a hundred kilo-volt will be required to generate the drift field of future very large liquid Argon Time Projection Chambers. The most delicate component is the feedthrough whose role is to safely deliver the very high voltage to the cathode through the thick insulating walls of the cryostat without compromising the purity of the argon inside. This requires a feedthrough that is typically meters long and carefully designed to be vacuum tight and have small heat input. Furthermore, all materials should be carefully chosen to allow operation in cryogenic conditions. In addition, el…
Particle detectors based on liquid argon (LAr) have recently become recognized as an extremely attractive technology for the direct detection of dark matter as well as the measurement of coherent elastic neutrino-nucleus scattering (CE$ν$NS). The Chinese argon group at Institute of High Energy Physics has been studying the LAr detector technology and a LAr detector has been operating steadily. A program of using a dual phase LAr detector to measure the CE$ν$NS at Taishang Nuclear Power Plant has been proposed and the R\&D work is ongoing. Considering the requirements of ultra-low radio-purity …
We report the results of the analyses of the cosmic ray data collected with a 4 tonne (3$\times$1$\times$1~m$^3$) active mass (volume) Liquid Argon Time-Projection Chamber (TPC) operated in a dual-phase mode. We present a detailed study of the TPC's response, its main detector parameters and performance. The results are important for the understanding and further developments of the dual-phase technology, thanks to the verification of key aspects, such as the extraction of electrons from liquid to gas and their amplification through the entire one square metre readout plain, gain stability, pu…
The model R5912-20MOD photomultiplier tube(PMT) is made for cryogenic application by Hamamatsu. In this paper, we report on the measurement of relative quantum efficiency (QE) of this model PMT at liquid argon(LAr) temperature. Furthermore, a specially designed setup and relevant test method are introduced. The relative QE is measured in visible wavelengths with the PMT emerged in high purity nitrogen atmosphere. The results show that the change of QE at LAr temperature is within about 5% compared with room temperature around 420 nm. However, the QE increases about 10% in the shorter wavelengt…
Particle detectors based on liquid argon are now recognised as an attractive technology for dark matter direct detection and coherent elastic neutrino-nucleus scattering measurement. A program using a dual-phase liquid argon detector with a fiducial mass of 200~kg to detect coherent elastic neutrino-nucleus scattering at Taishan Nuclear Power Plant has been proposed. SiPMs will be used as the photon sensor because of their high radio-purity and high photon detection efficiency. S13370-6050CN SiPM, made by Hamamatsu, is a candidate for the detector. In this paper, the characterisation of S13370…
The Deep Underground Neutrino Experiment (DUNE) will be a premier facility for exploring long-standing questions about the boundaries of the standard model. Acting in concert with the liquid argon time projection chambers underpinning the far detector design, the DUNE photon detection system will capture ultraviolet scintillation light in order to provide valuable timing information for event reconstruction. To maximize the active area while maintaining a small photocathode coverage, the experiment will utilize a design based on plastic light guides coated with a wavelength-shifting compound, …
In this paper we explore the potential improvements in neutrino event reconstruction that a 3D pixelated readout could offer over a 2D projective wire readout for liquid argon time projection chambers. We simulate and study events in two generic, idealized detector configurations for these two designs, classifying events in each sample with deep convolutional neural networks to compare the best 2D results to the best 3D results. In almost all cases we find that the 3D readout provides better reconstruction efficiency and purity than the 2D projective wire readout, with the advantages of 3D bei…
In this paper we report on measurements of the effects of dissolved methane upon argon scintillation light. We monitor the light yield from an alpha source held 20 cm from a cryogenic photomultiplier tube (PMT) assembly as methane is injected into a high-purity liquid argon volume. We observe significant suppression of the scintillation light yield by dissolved methane at the 10 part per billion (ppb) level. By examining the late scintillation light time constant, we determine that this loss is caused by an absorption process and also see some evidence of methane-induced scintillation quenchin…
Liquified noble gases are widely used as a target in direct Dark Matter searches. Signals from scintillation in the liquid, following energy deposition from the recoil nuclei scattered by Dark Matter particles (e.g. WIMPs), should be recorded down to very low energies by photosensors suitably designed to operate at cryogenic temperatures. Liquid Argon based detectors for Dark Matter searches currently implement photo multiplier tubes for signal read-out. In the last few years PMTs with photocathodes operating down to liquid Argon temperatures (87 K) have been specially developed with increasin…
Large (up to $\sim 100$ kt) liquid argon time-projection chamber detectors are presently being considered for proton decay searches and neutrino astrophysics, as well as for far detectors for the next generation of long-baseline neutrino oscillation experiments that aim to determine neutrino mass hierarchy and search for CP violation in the leptonic sector. These detectors rely on the capabilities to assemble large volumes of LAr in ultrahigh-purity conditions, possibly in an underground environment, and to achieve relatively long drifts for the ionization charge. Several proposals have been d…
For the first time, planar high-purity germanium detectors with thin amorphous germanium contacts were successfully operated directly in liquid nitrogen and liquid argon in a cryostat at the Max-Planck-Institut fuer Physics in Munich. The detectors were fabricated at the Lawrence Berkeley National Laboratory and the University of South Dakota, using crystals grown at the University of South Dakota. They survived long-distance transportation and multiple thermal cycles in both cryogenic liquids and showed reasonable leakage currents and spectroscopic performance. Also discussed are the pros and…
The movable temperature profiler is a 7 m vertical array of 24 sensors that measures cryogenic temperatures with a precision of a few mK. This precision is necessary to monitor the efficiency of re-circulation and purification of liquid-argon inside large liquid-argon based neutrino detectors. Liquid argon temperature impacts electron (signal) drift velocity, flow, purity distribution and thus the overall energy calibration. The temperature profiler is motorized and moves vertically, while in the detector, and cross-calibrates neighboring sensors. The temperature offsets between each sensor ca…
The China Dark Matter Experiment (CDEX) is a low background experiment at China Jinping Underground Laboratory (CJPL) designed to directly detect dark matter with a high-purity Germanium (HPGe) detector. In the second phase CDEX-10 with a 10 kg Germanium array detector system, the liquid argon (LAr) anti-compton active shielding and cooling system is proposed. For purpose of studying the properties of LAr detector, a prototype with an active volume of 7 liters of liquid argon was built and operated. The photoelectron yields, as a critically important parameter for the prototype detector, have …
We report on a measurement of the absorption length of scintillation light in liquid argon due to dissolved nitrogen at the part-per-million (ppm) level. We inject controlled quantities of nitrogen into a high purity volume of liquid argon and monitor the light yield from an alpha source. The source is placed at different distances from a cryogenic photomultiplier tube assembly. By comparing the light yield from each position we extract the absorption cross section of nitrogen. We find that nitrogen absorbs argon scintillation light with strength of $(1.51\pm 0.15)\times10^{-4} \;\mathrm{cm^{-…
The ICARUS T600 detector, the largest liquid Argon Time Projection Chamber (LAr-TPC) realized after many years of RD activities, was installed and successfully operated for 3 years at the INFN Gran Sasso underground Laboratory. One of the most important issues was the need of an extremely low residual electronegative impurity content in the liquid Argon, in order to transport the free electrons created by the ionizing particles with a very small attenuation along the drift path. The solutions adopted for the Argon re-circulation and purification systems have permitted to reach impressive resul…
We report on a measurement of the attenuation length for the scintillation light in the tonne size liquid argon target of the ArDM dark matter experiment. The data was recorded in the first underground operation of the experiment in single-phase operational mode. The results were achieved by comparing the light yield spectra from 39-Ar and 83m-Kr to a description of the ArDM setup with a model of full light ray tracing. A relatively low value close to 0.5 m was found for the attenuation length of the liquid argon bulk to its own scintillation light. We interpret this result as a presence of op…
The capabilities of liquid argon time projection chambers (LArTPCs) to reconstruct the spatial and calorimetric information of neutrino events have made them the detectors of choice in a number of experiments, specifically those looking to observe electron neutrino ($ν_e$) appearance. The LArTPC promises excellent background rejection capabilities, especially in this "golden" channel for both short and long baseline neutrino oscillation experiments. We present the first experimental observation of electron neutrinos and anti-neutrinos in the ArgoNeut LArTPC, in the energy range relevant to DUN…
A workshop was held at Fermilab on March 20-21, 2013 to discuss the development of liquid argon time projection chambers (LArTPC) in the United States. The workshop was organized under the auspices of the Coordinating Panel for Advanced Detectors, a body that was initiated by the American Physical Society Division of Particles and Fields. All presentations at the workshop were made in plenary sessions organized into seven topical categories: $i)$ Argon Purity, $ii)$ Cryogenics, $iii)$ TPC and High Voltage, $iv)$ Electronics, Data Acquisition and Triggering, $v)$ Scintillation Light Detection, …
The second workshop to discuss the development of liquid argon time projection chambers (LArTPCs) in the United States was held at Fermilab on July 8-9, 2014. The workshop was organized under the auspices of the Coordinating Panel for Advanced Detectors, a body that was initiated by the American Physical Society Division of Particles and Fields. All presentations at the workshop were made in six topical plenary sessions: $i)$ Argon Purity and Cryogenics, $ii)$ TPC and High Voltage, $iii)$ Electronics, Data Acquisition and Triggering, $iv)$ Scintillation Light Detection, $v)$ Calibration and Te…
In liquid argon-based particle detectors, slow wavelength shifters (WLSs) could be used alongside the common, nanosecond scale, WLS tetraphenyl butadiene (TPB) for background mitigation purposes. At room temperature, pyrene has a moderate fluorescence light yield (LY) and a time constant of the order of hundreds of nanoseconds. In this work, four pyrene-doped polystyrene films with various purities and concentrations were characterized in terms of LY and decay time constants in a range of temperature between 4 K and 300 K under ultraviolet excitation. These films were found to have a LY betwee…
We investigate the idea of detecting pure neutrino-hydrogen interactions in a multinuclear target using the transverse kinematic imbalance technique [Lu et al., Phys. Rev. D 92, 051302 (2015)] in a high-pressure time projection chamber (HPTPC). With full solid-angle acceptance, MeV-level proton tracking threshold, state-of-the-art tracking resolution, and an O(100 m^3) gas volume at 10 bar, an HPTPC could provide an opportunity to realize this technique. We propose the use of hydrogen-rich gases in the TPC to achieve high detection purity with large hydrogen mass. With the projected neutrino b…
Liquid argon time projection chamber technology is an attractive choice for large neutrino detectors, as it provides a high-resolution active target and it is expected to be scalable to very large masses. Consequently, it has been chosen as the technology for the first module of the DUNE far detector. However, the fiducial mass required for "far detectors" of the next generation of neutrino oscillation experiments far exceeds what has been demonstrated so far. Scaling to this larger mass, as well as the requirement for underground construction places a number of additional constraints on the d…
The MiniCLEAN dark matter experiment will exploit a single-phase liquid-argon detector instrumented with 92 photomultiplier tubes placed in the cryogen temperature with 4-$π$ coverage of a 500 kg (150 kg) target (fiducial) mass. The detector design strategy emphasizes scalability to target masses of order 10 tons or more. The detector is designed also for a liquid neon target that allows for an independent verification of signal and background and a test of the expected dependence of the WIMP-nucleus interaction rate. For MiniCLEAN, PMT stability and calibration are essential. The \textit{In-s…
Stanford University（斯坦福大学）；SLAC National Accelerator Laboratory（SLAC国家加速器实验室）
Liquid Argon Time Projection Chambers (LArTPCs) are high resolution particle imaging detectors, employed by accelerator-based neutrino oscillation experiments for high precision physics measurements. While images of particle trajectories are intuitive to analyze for physicists, the development of a high quality, automated data reconstruction chain remains challenging. One of the most critical reconstruction steps is particle clustering: the task of grouping 3D image pixels into different particle instances that share the same particle type. In this paper, we propose the first scalable deep lea…
In this paper we describe the design, construction, and operation of a first large area double-phase liquid argon Large Electron Multiplier Time Projection Chamber (LAr LEM-TPC). The detector has a maximum drift length of 60 cm and the readout consists of a $40\times 76$ cm$^2$ LEM and 2D projective anode to multiply and collect drifting charges. Scintillation light is detected by means of cryogenic PMTs positioned below the cathode. To record both charge and light signals, we have developed a compact acquisition system, which is scalable up to ton-scale detectors with thousands of charge read…
A 10 kilo-tonne dual-phase liquid argon TPC is one of the detector options considered for the Deep Underground Neutrino Experiment (DUNE). The detector technology relies on amplification of the ionisation charge in ultra-pure argon vapour and oers several advantages compared to the traditional single-phase liquid argon TPCs. A 4.2 tonne dual-phase liquid argon TPC prototype, the largest of its kind, with an active volume of 3x1x1 $m^3$ has been constructed and operated at CERN. In this paper we describe in detail the experimental setup and detector components as well as report on the operation…
Stanford University（斯坦福大学）；SLAC National Accelerator Laboratory（SLAC国家加速器实验室）
Liquid Argon Time Projection Chambers (LArTPC) are particle imaging detectors recording 2D or 3D images of trajectories of charged particles. Identifying points of interest in these images, namely the initial and terminal points of track-like particle trajectories such as muons and protons, and the initial points of electromagnetic shower-like particle trajectories such as electrons and gamma rays, is a crucial step of identifying and analyzing these particles and impacts the inference of physics signals such as neutrino interaction. The Point Proposal Network is designed to discover these spe…
The MicroBooNE liquid argon time projection chamber (LArTPC) maintains a high level of liquid argon purity through the use of a filtration system that removes electronegative contaminants in continuously-circulated liquid, recondensed boil off, and externally supplied argon gas. We use the MicroBooNE LArTPC to reconstruct MeV-scale radiological decays. Using this technique we measure the liquid argon filtration system's efficacy at removing radon. This is studied by placing a 500 kBq $^{222}$Rn source upstream of the filters and searching for a time-dependent increase in the number of radiolog…
Cosmic ray (CR) interactions can be a challenging source of background for neutrino oscillation and cross-section measurements in surface detectors. We present methods for CR rejection in measurements of charged-current quasielastic-like (CCQE-like) neutrino interactions, with a muon and a proton in the final state, measured using liquid argon time projection chambers (LArTPCs). Using a sample of cosmic data collected with the MicroBooNE detector, mixed with simulated neutrino scattering events, a set of event selection criteria is developed that produces an event sample with minimal contribut…
An accurate and efficient event reconstruction is required to realize the full scientific capability of liquid argon time projection chambers (LArTPCs). The current and future neutrino experiments that rely on massive LArTPCs create a need for new ideas and reconstruction approaches. Wire-Cell, proposed in recent years, is a novel tomographic event reconstruction method for LArTPCs. The Wire-Cell 3D imaging approach capitalizes on charge, sparsity, time, and geometry information to reconstruct a topology-agnostic 3D image of the ionization electrons prior to pattern recognition. A second novel…
