We study the expansion of a cold, non-neutral ion plasma into the vacuum. The plasma is made from cold rubidium atoms in a magneto-optical trap (MOT) and is formed via ultraviolet photoionization. We employ time-delayed plasma extraction and imaging onto a position- and time-sensitive micro-channel plate detector to analyze the plasma. We report on the formation and persistence of plasma shock shells, pair correlations in the plasma, and external-field-induced plasma focusing effects. We also develop trajectory and fluid descriptions to model the data and to gain further insight. The simulations verify the formation of shock shells and correlations, and allow us to model time- and position-dependent density, temperature, and Coulomb coupling parameter, $Γ({\bf{r}},t)$. This analysis both reaffirms the presence of shock shells and verifies that the experimental plasma is strongly coupled.
Employing recent developed magneto-optical trap recoil ion momentum spectroscopy (MOTRIMS) combining cold atom, strong laser pulse, and ultrafast technologies, we study momentum distributions of the multiply ionized cold rubidium (Rb) induced by the elliptically polarized laser pulses (35 fs, $1.3 \times 10^{15}$ W/cm$^2$). The complete vector momenta of Rbn+ ions up to charge state n = 4 are recorded with extremely high resolution (0.12 a.u. for Rb$^+$). Variations of characteristic multi-bands displayed in momentum distributions, as the ellipticity varies from the linear to circular polariza…
The effect of microwave radiation on the resonance fluorescence of a cloud of cold $^{85}Rb$ atoms in a magnetooptical trap is studied. The radiation frequency was tuned near the hyperfine splitting frequency of rubidium atoms in the 5S ground state. The microwave field induced magnetic dipole transitions between the magnetic sublevels of the 5S(F=2) and 5S(F=3) states, resulting in a change in the fluorescence signal. The resonance fluorescence spectra were recorded by tuning the microwave radiation frequency. The observed spectra were found to be substantially dependent on the transition und…
We report the production of a continuous, slow, and cold beam of 87-Rb atoms with an unprecedented flux of 3.2 x 10^12 atoms/s and a temperature of a few milliKelvin. Hot atoms are emitted from a Rb candlestick atomic beam source and transversely cooled and collimated by a 20 cm long atomic collimator section, augmenting overall beam flux by a factor of 50. The atomic beam is then decelerated and longitudinally cooled by Zeeman slowing.
This paper presents a setup capable of producing a high-flux continuous beam of cold rubidium atoms for cavity QED experiments in the regime of strong coupling. A 2 $D^+$ MOT, loaded by rubidium getters in a dry film coated vapor cell, fed a secondary moving-molasses MOT (MM-MOT) at a rate of 1.5 x $10^{10}$ atoms/sec. The MM-MOT provided a continuous beam with tunable velocity. This beam was then directed through the waist of a 280 $μ$m cavity resulting in a Rabi splitting of more than +/- 10 MHz. The presence of sufficient number of atoms in the cavity mode also enabled splitting in the pola…
A brief perspective on light scattering in dense and cold atomic rubidium is presented. We particularly focus on the influence of auxiliary applied fields on the system response to a weak and nearly resonant probe field. Auxiliary fields can strongly disturb light propagation; in addition to the steady state case, dynamically interesting effects appear clearly in both the time domain, and in the optical polarization dependence of the processes. Following a general introduction, two examples of features found in such studies are presented. These include nonlinear optical effects in (a) comparat…
We perform high-resolution measurements of momentum distribution on Rb$^{n+}$ recoil ions up to charge state $n=4$, where laser-cooled rubidium atoms are ionized by femtosecond elliptically polarized lasers with the pulse duration of 35 fs and the intensity of 3.3$\times$10$^{15}$ W/cm$^2$ in the over-barrier ionization (OBI) regime. The momentum distributions of the recoil ions are found to exhibit multi-band structures as the ellipticity varies from the linear to circular polarizations. The origin of these band structures can be explained quantitatively by the classical OBI model and dedicat…
Atoms in highly excited (Rydberg) states have a number of unique properties which make them attractive for applications in quantum information. These are large dipole moments, lifetimes and polarizabilities, as well as strong long-range interactions between Rydberg atoms. Experimental methods of laser cooling and precision spectroscopy enable the trapping and manipulation of single Rydberg atoms and applying them for practical implementation of quantum gates over qubits of a quantum computer based on single neutral atoms in optical traps. In this paper, we give a review of the experimental and…
Light-assisted reactive collisions between laser-cooled Ba+ ions and Rb atoms were studied in an ion-atom hybrid trap. The reaction rate was found to strongly depend on the electronic state of the reaction partners with the largest rate constant (7(2) x 10^-11 cm^3 s^-1) obtained for the excited Ba+(6s)+Rb(5p) reaction channel. Similar to the previously studied Ca+ + Rb system, charge transfer and radiative association were found to be the dominant reactive processes. The generation of molecular ions by radiative association could directly be observed by their sympathetic cooling into a Coulom…
Experiments on the spectroscopy of the Förster resonance Rb(37P)+Rb(37P) -> Rb(37S)+Rb(38S) and microwave transitions nP -> n'S, n'D between Rydberg states of cold Rb atoms in a magneto-optical trap have been performed. Under ordinary conditions, all spectra exhibited a 2-3 MHz line width independently of the interaction time of atoms with each other or with microwave radiation, although the ultimate resonance width should be defined by the inverse interaction time. Analysis of the experimental conditions has shown that the main source of the line broadening was the inhomogeneous electric fiel…
Using a blue detuned laser shaped in a Laguerre-Gaussian donut mode we highly collimate the output of a two dimensional magneto-optical trap. The resulting atomic beam has a 1 mm diameter, its divergence is reduced from 40 down to 3 mrad and the atomic density is increased by a factor of 200. The collimation effect has been studied versus the order of the Laguerre-Gaussian mode (up to 10) and the laser atom frequency detuning (2 to 120 GHz). The 2D-colli-MOT study allows us to determine the best conditions which minimize the atom heating due to residual light absorption and optimize the collim…
The integration of cold atomic systems with optical nanofibres is an increasingly important experimental platform. Here, we report on the spectra observed during a strongly driven, single-frequency, two-photon excitation of cold rubidium atoms near an optical nanofibre. At resonance, two competitive processes, namely a higher excitation rate and stronger pushing of atoms from the nanofibre due to resonance scattering, need to be considered. We discuss the processes that lead to the observed two-peak profile in the fluorescence spectrum as the excitation laser is scanned across the resonance, n…
Photoionization of the rubidium (Rb) atoms cooled in a magneto-optical trap, characterized by the coexistence of the ground 5$S_{1/2}$ and the excited 5$P_{3/2}$ states, is investigated experimentally and theoretically with the 400 nm femtosecond laser pulses at intensities of $I=3\times10^9$ W/cm$^2$ - $4.5\times10^{12}$ W/cm$^2$. Recoil-ion momentum distribution (RIMD) of Rb$^+$ exhibits rich ring-like structures and their energies correspond to one-photon ionization of the 5$P_{3/2}$ state, two-photon and three-photon ionizations of the 5$S_{1/2}$ state, respectively. With the increasing of…
Photoionization of a cold atomic sample offers intriguing possibilities to observe collective effects at extremely low temperatures. Irradiation of a rubidium condensate and of cold rubidium atoms within a magneto-optical trap with laser pulses ionizing through 1-photon and 2-photon absorption processes has been performed. Losses and modifications in the density profile of the remaining trapped cold cloud or the remaining condensate sample have been examined as function of the ionizing laser parameters. Ionization cross-sections were measured for atoms in a MOT, while in magnetic traps losses …
We employ an accurate, ab initio potential energy surface (PES) which describes the electronic interaction energy between the molecular anion OH$^-$ ($^1Σ^+$) and the neutral rubidium atom Rb ($^2S$), to evaluate the elastic and inelastic cross sections over a range of energies representative of the conditions of low-T experiments in MOT traps, when combined with laser-cooled rubidium gas. The system is considered to be in its vibrational ground state, while the first four rotational levels are taken to be involved in the cooling and heating collisional processes that are computed here. The co…
We study the expansion of a strongly coupled, non-neutral, and cylindrically arranged ion plasma into the vacuum. The plasma is made from cold rubidium atoms in a magneto-optical trap (MOT) and is formed via ultraviolet photoionization. Higher-density and lower-density plasmas are studied to exhibit different aspects indicative of strong coupling. In a higher-density regime, we report on the formation and persistence of plasma shock fronts, as well as external-field-induced plasma focusing effects. In the lower-density regime, conditions are ideal to observe the development and evolution of ne…
We realize a laser with a cloud of cold rubidium atoms as gain medium, placed in a low-finesse cavity. Three different regimes of laser emission are observed corresponding respectively to Mollow, Raman and Four Wave Mixing mechanisms. We measure an output power of up to 300 $μ$W and present the main properties of these different lasers in each regime.
We observe the shift of Rydberg levels of rubidium close to a copper surface when atomic clouds are repeatedly deposited on it. We measure transition frequencies of rubidium to S and D Rydberg states with principal quantum numbers n between 31 and 48 using the technique of electromagnetically induced transparency. The spectroscopic measurement shows a strong increase of electric fields towards the surface that evolves with the deposition of atoms. Starting with a clean surface, we measure the evolution of electrostatic fields in the range between 30 and 300 \mum from the surface. We find that …
When applying two counter-propagating laser beams to a cold cloud of Rubidium atoms, we observe the spontaneous formation of intensity patterns associated with a spatial structuration of the atomic spins. We study the average number of defects in these patterns as a function of the sweep time employed to cross the transition threshold. We observe a power-law decrease of the number of defects with increasing sweep time, typical of the Kibble-Zurek mechanism. The measured exponent is consistent with the prediction for a supercritical bifurcation.
The electric field in mm-sized clouds of cold Rb^+-ions is measured using the Stark effect of Rydberg atoms embedded in the ion clouds. The ion clouds are produced by UV photoionization of laser-cooled rubidium atoms in a magneto-optic trap. In very dense ion clouds, the Rydberg atom excitation spectra reflect the presence of a neutral plasma core and a positively charged ion shell.
We demonstrate subpicosecond-time-scale population transfer between the pair of hyperfine ground states of atomic rubidium using a single laser-pulse. Our scheme utilizes the geometric and dynamic phases induced during Rabi oscillation through the fine-structure excited state in order to construct an $X$ rotation gate for the hyperfine-state qubit system. Experiment performed with a femtosecond laser and cold rubidium atoms, in a magneto-optical trap, shows over 98\% maximal population transfer between the clock states.
We show that the resonance shifts in the fluorescence of a cold gas of rubidium atoms substantially differ from those of thermal atomic ensembles that obey the standard continuous medium electrodynamics. The analysis is based on large-scale microscopic numerical simulations and experimental measurements of the resonance shifts in a steady-state response in light propagation.
The potential energy curves, permanent and transition dipole moments, and the static dipolar polarizability, of molecular ions composed of one alkali-metal atom and a Strontium ion are determined with a quantum chemistry approach. The molecular ions are treated as effective two-electron systems and are treated using effective core potentials including core polarization, large gaussian basis sets, and full configuration interaction. In the perspective of upcoming experiments aiming at merging cold atom and cold ion traps, possible paths for radiative charge exchange, photoassociation of a cold …
We have measured the asymptotic expansion velocities of ultra-cold plasmas (UNPs) which evolve from cold, dense, samples of Rydberg rubidium atoms using ion time-of-flight spectroscopy. From this, we have obtained values for the initial plasma electron temperature as functions of the original Rydberg atom density and binding energy. Our results show that the electron temperature is determined principally by the plasma environment when the UNP decouples from the Rydberg atoms, which occurs when the plasma electrons become too cold to ionize the remaining Rydberg population. Furthermore, the dep…
Enhanced sensitivity in electromagnetically induced transparency (EIT) can be obtained by the use of noise correlation spectroscopy between the fields involved in the process. Here, we investigate EIT in a cold ($< 1$ mK) rubidium vapor and demonstrate sensitivity to detect weak light-induced forces on the atoms. A theoretical model is developed and shows good agreement with our measurements, enabling the attribution of the observed effects to the coupling of the atomic states to their motion. The effects remain unnoticed on the measurement of the mean fields but are clearly manifest in their …
We perform a comprehensive investigation of the coupling between a Rydberg-dressed atomic gas and an ultra-cold plasma. Using simultaneous time-resolved measurements of both neutral atoms and ions, we show that plasma formation occurs via a Coulomb anti-blockade mechanism, in which background ions DC Stark shift nearby atoms into resonance at specific distances. The result is a highly correlated growth of the Rydberg population that shares some similarities with that previously observed for van der Waals interactions. We show that a rate equation model that couples the laser-driven Rydberg gas…
We report the sympathetic cooling and Coulomb crystallization of molecular ions above the surface of an ion-trap chip. N$_2^+$ and CaH$^+$ ions were confined in a surface-electrode radiofrequency ion trap and cooled by the interaction with laser-cooled Ca$^{+}$ ions to secular translational temperatures in the millikelvin range. The configuration of trapping potentials generated by the surface electrodes enabled the formation of planar bicomponent Coulomb crystals and the spatial separation of the molecular from the atomic ions on the chip. The structural and thermal properties of the Coulomb …
The recent observation of coherent backscattering (CBS) of light by atoms has emphasized the key role of the velocity spread and of the quantum internal structure of the atoms. Firstly, using highly resonant scatterers imposes very low temperatures of the disordered medium in order to keep the full contrast of the CBS interference. This criterion is usually achieved with standard laser cooling techniques. Secondly, a non trivial internal atomic structure leads to a dramatic decrease of the CBS contrast. Experiments with Rubidium atoms (with a non trivial internal structure) and with Strontium …
Nowadays the development of novel particle accelerators is a hot topic for both experimental and theoretical sciences. In the CERN-AWAKE experiment electrons are accelerated in a cold rubidium plasma, generated by a short, intense laser pulse. We describe the corresponding photoionisation process with ab initio quantum mechanical calculations. In this paper we primarily investigate how the frequency chirping of the applied laser pulse influences the photoionisation. Secondarily we also study how the results of the numerical simulations depend on the shape of the envelope of the laser pulse. Ba…
Reciprocity is fundamental to light transport and is a concept that holds also in rather complex systems. Yet, reciprocity can be switched off even in linear, isotropic and passive media by setting the material structure into motion. In highly dispersive multilayers this leads to a fairly large forward-backward asymmetry in the pulse transmission. Moreover, in multilevel systems, this transport phenomenon can be all-optically enhanced. For atomic multilayer structures made of three-level cold Rubidium 87 atoms, for instance, forward-backward transmission contrast around 95 per cent can be obta…
A glass ultrahigh vacuum chamber with rubidium alkali metal dispensers and non-evaporable getter pumps has been developed and used to create a cold atomic sample in a chamber that operates with only passive vacuum pumps. The ion-mass spectrum of evaporated gases from the alkali metal dispenser has been recorded as a function of dispenser current. The efficacy of the non-evaporable getter pumps in promoting and maintaining vacuum has been characterized by observation of the Rb vapor optical absorption on the D2 transition at 780 nm and vacuum chamber pressure rate of rise tests. We have demonst…
A physics package for a compact cold atomic clock is hereby presented. The uniqueness of this package is its small dimensions that enable, for the first time, implementation of a primary cold atomic clock in a standard package of 3U height (=133mm). These dimensions are made possible by using an in-vacuum Microwave (MW) Loop Gap Resonator (LGR) whose length and diameter can be reduced from those of a typical resonator. Following our presentation of the design, we analyze the homogeneity of the MW field amplitude and phase. We find that the expected clock instability due to non-uniformity of th…
One of the most striking features of the strong interactions between Rydberg atoms is the dipole blockade effect, which allows only a single excitation to the Rydberg state within the volume of the blockade sphere. Here we present a method that spatially visualizes this phenomenon in an inhomogeneous gas of ultra-cold rubidium atoms. In our experiment we scan the position of one of the excitation lasers across the cold cloud and determine the number of Rydberg excitations detected as a function of position. Comparing this distribution to the one obtained for the number of ions created by a two…
We propose and analyze a new scheme to produce ultracold neutral plasmas deep in the strongly coupled regime. The method exploits the interaction blockade between cold atoms excited to high-lying Rydberg states and therefore does not require substantial extensions of current ultracold plasma experiments. Extensive simulations reveal a universal behavior of the resulting Coulomb coupling parameter, providing a direct connection between the physics of strongly correlated Rydberg gases and ultracold plasmas. The approach is shown to reduce currently accessible temperatures by more than an order o…
Here we report of a design and the performance of an optimized micro-fabricated conveyor belt for precise and adiabatic transportation of cold atoms. A theoretical model is presented to determine optimal currents in conductors used for the transportation. We experimentally demonstrate a fast adiabatic transportation of Rubidium ($^{87}$Rb) cold atoms with minimal loss and heating with as few as three conveyor belt conductors. This novel design of a multilayered conveyor belt structure is fabricated in aluminium nitride ($AlN$) because of its outstanding thermal and electrical properties. This …
We report a detailed investigation on the properties of correlation spectra for cold atoms under the condition of Electromagnetically Induced Transparency (EIT). We describe the transition in the system from correlation to anti-correlation as the intensity of the fields increases. Such transition occurs for laser frequencies around the EIT resonance, which is characterized by a correlation peak. The transition point between correlation and anti-correlation is independent of power broadening and provides directly the ground-state coherence time. We introduce a method to extract in real time the…
We present the realization of a compact micro-wave frequency synthesizer for an atom interferometer based on stimulated Raman transitions, applied to transportable inertial sensing. Our set-up is intended to address the hyperfine transitions of Rubidium 87 atoms at 6.8 GHz. The prototype is evaluated both in the time and the frequency domain by comparison with state-of-the-art frequency references developed at LNE-SYRTE. In free-running mode, it features a residual phase noise level of -65 dBrad$^2.Hz^{-1} at 10-Hz offset frequency and a white phase noise level in the order of -120 dBrad^2.Hz^…
