We investigate two-dimensional atomic arrays as a platform to modify the electromagnetic environment of individual quantum emitters. Specifically, we demonstrate that control over emission linewidths, resonant frequency shifts, and local enhancement of driving fields is possible due to strong dipole-dipole interactions within ordered, subwavelength atom configurations. We demonstrate that these effects can be used to dramatically enhance coherent dipole-dipole interactions between distant quantum emitters within an atom array. Possible experimental realizations and potential applications are discussed.
We explore the features of an equally-spaced array of two-level quantum emitters, that can be either natural atoms (or molecules) or artificial atoms, coupled to a field with a single continuous degree of freedom (such as an electromagnetic mode propagating in a waveguide). We investigate the existence and characteristics of bound states, in which a single excitation is shared among the emitters and the field. We focus on bound states in the continuum, occurring in correspondence of excitation energies in which a single excited emitter would decay. We characterize such bound states for an arbi…
We study the existence of bound states in the continuum for a system of n two-level quantum emitters, coupled with a one-dimensional boson field, in which a single excitation is shared among different components of the system. The emitters are fixed and equally spaced. We first consider the approximation of distant emitters, in which one can find degenerate eigenspaces of bound states corresponding to resonant values of energy, parametrized by a positive integer. We then consider the full form of the eigenvalue equation, in which the effects of the finite spacing and the field dispersion relat…
The single-photon scattering in a rectangular waveguide by a V-type three-level emitter is studied for large range of input-photon energy beyond the single-mode region. By using Lippmann-Schwinger formalism, the necessary and sufficient conditions of complete transmission and complete reflection are derived analytically. In the single-mode region, the complete transmission caused by electromagnetically induced transparency (EIT) and the complete reflection due to Fano resonance can both be achieved by adjusting the emitter's parameters. But in the multi-mode region, except that the input-state…
Encoding high-dimensional quantum information into single photons can provide a variety of benefits for quantum technologies, such as improved noise resilience. However, the efficient generation of on-demand, high-dimensional entanglement was thought to be out of reach for current and near-future photonic quantum technologies. We present a protocol for the near-deterministic generation of $N$-photon, $d$-dimensional photonic Greenberger-Horne-Zeilinger (GHZ) states using an array of $d$ non-interacting single-photon emitters. We analyse the impact on performance of common sources of error for …
We introduce spatial deformations to an array of light sources and study how the estimation precision of the interspacing distance, d, changes with the sources of light used. The quantum Fisher information (QFI) is used as the figure of merit in this work to quantify the amount of information we have on the estimation parameter. We derive the generator of translations, G, in d due to an arbitrary homogeneous deformation applied to the array. We show how the variance of the generator can be used to easily consider how different deformations and light sources can effect the estimation precision.…
We show that with a new family of pyramidal site-controlled InGaAsN quantum dots it is possible to obtain areas containing as much as 15% of polarization-entangled photon emitters - a major improvement if compared to the small fraction achievable by other quantum dot systems. Entanglement is attested by a two-photon polarization state density matrix and the parameters obtained from it. Emitters showing fidelities up to 0.721+-0.043 were found.
We discuss the scattering of photons from a three-level emitter in a one-dimensional waveguide, where the transport is governed by the interference of spontaneously emitted and directly transmitted waves. The scattering problem is solved in closed form for different level structures. Several possible applications are discussed: The state of the emitter can be switched deterministically by Raman scattering, thus enabling applications in quantum computing such as a single photon transistor. An array of emitters gives rise to a photonic band gap structure, which can be tuned by a classical drivin…
An outstanding challenge in quantum photonics is scalability, which requires positioning of single quantum emitters in a deterministic fashion. Site positioning progress has been made in established platforms including defects in diamond and self-assembled quantum dots, albeit often with compromised coherence and optical quality. The emergence of single quantum emitters in layered transition metal dichalcogenide semiconductors offers new opportunities to construct a scalable quantum architecture. Here, using nanoscale strain engineering, we deterministically achieve a two-dimensional lattice o…
Over the last decade, conditions for perfect state transfer in quantum spin chains have been discovered, and their experimental realizations addressed. In this paper, we consider an extension of such studies to quantum state transfer in a coupled cavity array including the effects of atoms in the cavities which can absorb and emit photons as they propagate down the array. Our model is equivalent to previously examined spin chains in the one-excitation sector and in the absence of emitters. We introduce a Monte Carlo approach to the inverse eigenvalue problem which allows the determination of t…
An array of $N$ closely spaced dipole coupled quantum emitters exhibits super- and subradiance with characteristic tailorable spatial radiation patterns. Optimizing their geometry and distance with respect to the spatial profile of a near resonant optical cavity mode allows to increase the ratio between light scattering into the cavity mode and free space by several orders of magnitude. This leads to a distinct nonlinear particle number scaling of the relative strength of coherent light-matter interactions versus decay. In particular, for subradiant states the collective cooperativity increase…
We describe applications of two-dimensional subwavelength quantum emitter arrays as efficient optical elements in the linear regime. For normally incident light, the cooperative optical response, stemming from emitter-emitter dipole exchanges, allows the control of the array's transmission, its resonance frequency, and bandwidth. Operations on fully polarized incident light, such as generic linear and circular polarizers as well as phase retarders can be engineered and described in terms of Jones matrices. Our analytical approach and accompanying numerical simulations identify optimal regimes …
Dipole-coupled subwavelength quantum emitter arrays respond cooperatively to external light fields as they may host collective delocalized excitations (a form of excitons) with super- or subradiant character. Deeply subwavelength separations typically occur in molecular ensembles, where in addition to photon-electron interactions, electron-vibron couplings and vibrational relaxation processes play an important role. We provide analytical and numerical results on the modification of super- and subradiance in molecular rings of dipoles including excitations of the vibrational degrees of freedom.…
Whenever several quantum light emitters are brought in proximity with one another, their interaction with common electromagnetic fields couples them, giving rise to cooperative shifts in their resonance frequency. Such collective line shifts are central to modern atomic physics, being closely related to superradiance on one hand and the Lamb shift on the other. Although collective shifts have been theoretically predicted more than fifty years ago, the effect has not been observed yet in a controllable system of a few isolated emitters. Here, we report a direct spectroscopic observation of the …
We examine the dissipative dynamics of N00N states with an arbitrary photon number N in two architectures of fiber-coupled optical ring resonators (RRs) interacting with two-level quantum emitters. One architecture consists of a two-way cascaded array of emitter-cavity systems, while in the other architecture we consider two fiber-coupled RRs each coupled to multiple dipole-dipole interacting (DDI) quantum emitters (QEs). Our focus in this paper is to study how am initially prepared multiple excitation atomic N00N states transfers to the RRs and then how rapidly it decays in these open cavity …
Anisotropic nanophotonic structures can couple the levels of a quantum emitter through the quantum interference effect. In this paper we study the coupling of quantum emitters excited states through the modes of a fully anisotropic structure: a structure for which all directions are physically nonequivalent. We consider an anisotropic metasurface as an illustrative example of such a structure. We point out a novel degree of freedom in controlling the temporal dynamics and spectral profiles of quantum emitters: namely, we show that a combination of the metasurface anisotropy and tilt of the emi…
Ordered lattices of emitters with subwavelength periodicities support unconventional forms of light-matter interactions arising from collective effects. Here, we propose the realization and control of subradiant optical states within the radiation continuum in two-dimensional lattices. We show how bound states in the continuum (BICs) which are completely decoupled from radiative states emerge in non-Bravais lattices of emitters. Symmetry breaking results in quasi-BICs with greatly extended lifetimes, which can be exploited for quantum information storage. The analytical derivation of a general…
We propose a nanophotonic platform for topological quantum optics. Our system is composed of a two-dimensional lattice of non-linear quantum emitters with optical transitions embedded in a photonic crystal slab. The emitters interact through the guided modes of the photonic crystal, and a uniform magnetic field gives rise to large topological band gaps and an almost completely flat topological band. Topological edge states arise on the boundaries of the system that are protected by the large gap against missing lattice sites and to the inhomogeneous broadening of emitters. These results pave t…
We develop a scattering theory to investigate the multi-photon transmission in a one-dimensional waveguide in the presence of quantum emitters. It is based on a path integral formalism, uses displacement transformations, and does not require the Markov approximation. We obtain the full time-evolution of the global system, including the emitters and the photonic field. Our theory allows us to compute the transition amplitude between arbitrary initial and final states, as well as the S-matrix of the asymptotic in- and out- states. For the case of few incident photons in the waveguide, we also re…
A primary motivation for studying topological matter regards the protection of topological order from its environment. In this work, we study a topological emitter array coupled to an electromagnetic environment. The photon-emitter coupling produces nonlocal interactions between emitters. Using periodic boundary conditions for all ranges of environment-induced interactions, the chiral symmetry inherent to the emitter array is preserved. This chiral symmetry protects the Hamiltonian, and induces parity in the Lindblad operator. A topological phase transition occurs at a critical photon-emitter …
We show how to realize a single-photon Dicke state in a large one-dimensional array of two- level systems, and discuss how to test its quantum properties. Realization of single-photon Dicke states relies on the cooperative nature of the interaction between a field reservoir and an array of two-level-emitters. The resulting dynamics of the delocalized state can display Rabi-like oscillations when the number of two-level emitters exceeds several hundred. In this case the large array of emitters is essentially behaving like a mirror-less cavity. We outline how this might be realized using a multi…
Regular arrays of two-level emitters at distances smaller that the transition wavelength collectively scatter, absorb and emit photons. The strong inter-particle dipole coupling creates large energy shifts of the collective delocalized excitations, which generates a highly nonlinear response at the single and few photon level. This should allow to implement nanoscale non-classical light sources via weak coherent illumination. At the generic tailored examples of regular chains or polygons we show that the fields emitted perpendicular to the illumination direction exhibit a strong directional co…
We describe a realistic scheme for coupling atoms or other quantum emitters with an array of coupled optical cavities. We consider open Fabry-Perot microcavities coupled to the emitters. Our central innovation is to connect the microcavities to waveguide resonators, which are in turn evanescently coupled to each other on a photonic chip to form a coupled cavity chain. In this paper, we describe the components, their technical limitations and the factors that need to be determined experimentally. This provides the basis for a detailed theoretical analysis of two possible experiments to realize …
Anomalous mobility edges and extended-localized transition in a quasiperiodic emitter-cavity array
School of Physics and Optoelectronic Engineering & Institute of Theoretical Physics, Ludong University（鲁东大学物理与光电工程学院暨理论物理研究所）；Center for Quantum Sciences, Northeast Normal University（东北师范大学量子科学中心）
The flourishing field of two-dimensional (2D) nanophotonics has generated much excitement in the quantum technologies community after the identification of quantum emitters (QEs) in layered materials (LMs). LMs offer many advantages as platforms for quantum circuits, such as integration within hybrid technologies, valley degree of freedom and strong spin-orbit coupling. QEs in LMs, however, suffer from uncontrolled occurrences, added to the uncertainty over their origin, which has been linked to defects and strain gradients. Here, we report a scalable method to create arrays of single-photon e…
Multiple emitters coherently interacting with an electromagnetic mode give rise to collective effects such as correlated decay and coherent exchange interaction, depending on the separation of the emitters. By diagonalizing the effective non-Hermitian many-body Hamiltonian we reveal the complex-valued eigenvalue spectrum encoding the decay and interaction characteristics. We show that there are significant differences in the emerging effects for an array of interacting anharmonic oscillators compared to those of two-level systems and harmonic oscillators. The bosonic decay rate of the most sup…
Dicke superradiance is an example of emergence of macroscopic quantum coherence via correlated dissipation. Starting from an initially incoherent state, a collection of excited atoms synchronizes as they decay, generating a macroscopic dipole moment and emitting a short and intense pulse of light. While well understood in cavities, superradiance remains an open problem in extended systems due to the exponential growth of complexity with atom number. Here we show that Dicke superradiance is a universal phenomenon in ordered arrays. We present a theoretical framework -- which circumvents the exp…
We present protocols to generate arbitrary photonic graph states from quantum emitters that are in principle deterministic. We focus primarily on two-dimensional cluster states of arbitrary size due to their importance for measurement-based quantum computing. Our protocols for these and many other types of two-dimensional graph states require a linear array of emitters in which each emitter can be controllably pumped, rotated about certain axes, and entangled with its nearest neighbors. We show that an error on one emitter produces a localized region of errors in the resulting graph state, whe…
We derive a generalized master equation for multiphoton pulses interacting with multiple emitters in a waveguide-quantum electrodynamics system where the emitter frequency can be modulated and the effects of non-guided modes can also be considered. Based on this theory, we can calculate the real-time dynamics of an array of interacting emitters driven by an incident photon pulse which can be vacuum, a coherent state, a Fock state or their superpositions. Moreover, we also derive generalized input-output relations to calculate the reflectivity and transmissivity of this system. We can also calc…
We theoretically study how to control transport, bound states, and resonant states of a single photon in a one-dimensional coupled-cavity array. We find that the transport of a single photon in the cavity array can be controlled by tuning the frequency of either one or two cavities. If one of the cavities in the array has a tunable frequency, and its frequency is tuned to be larger (or smaller) than those of other cavities, then there is a photon bound state above (or below) the energy band of the coupled cavity array. However, if two cavities in the array have tunable frequencies, then there …
We experimentally demonstrate the control of the spontaneous emission rate and the radiation pattern of colloidal quantum dots deterministically positioned in a plasmonic patch antenna. The antenna consists of a thin gold microdisk 30 nm above a thick gold layer. The emitters are shown to radiate through the entire patch antenna in a highly directional and vertical radiation pattern. Strong acceleration of spontaneous emission is observed, depending of the antenna size. Considering the double dipole structure of the emitters, this corresponds to a Purcell factor up to 80 for dipoles perpendicu…
High-order quantum correlations in nonlinear waveguide quantum electrodynamics
Academia Sinica（中央研究院）；National Central University（中央大学）；University of Mataram（马塔兰大学）；National Center for Theoretical Sciences（国家理论科学中心）；Hon Hai Research Institute（鸿海研究院）；National Taiwan University（台湾大学）
We propose a heralded quantum repeater based on the scattering of photons off single emitters in one-dimensional waveguides. We show the details by implementing nonlocal entanglement generation, entanglement swapping, and entanglement purification modules with atoms in waveguides, and discuss the feasibility of the repeater with currently achievable technology. In our scheme, the faulty events can be discarded by detecting the polarization of the photons. That is, our protocols are accomplished with fidelity of 100% in principle, which is advantageous for implementing realistic long-distance q…
We address the problem of optically controlling and quantifying the dissipative dynamics of quantum and classical correlations in a set-up of individual quantum emitters under external laser excitation. We show that both types of correlations, the former measured by the quantum discord, are present in the system's evolution even though the emitters may exhibit an early stage disentanglement. In the absence of external laser pumping,we demonstrate analytically, for a set of suitable initial states, that there is an entropy bound for which quantum discord and entanglement of the emitters are alw…
