arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2005.02054cond-mat.str-elcond-mat.supr-con
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大极化子作为SrTiO3和SrTiO3-based异质结中的关键准粒子

Large polarons as key quasiparticles in SrTiO3 and SrTiO3-based heterostructures

Andrey Geondzhian, Alessia Sambri, Gabriella M. De Luca, Roberto Di Capua, Emiliano Di Gennaro, Davide Betto, Matteo Rossi, Ying Ying Peng, Roberto Fumagalli, N… 展开作者

Andrey Geondzhian, Alessia Sambri, Gabriella M. De Luca, Roberto Di Capua, Emiliano Di Gennaro, Davide Betto, Matteo Rossi, Ying Ying Peng, Roberto Fumagalli, Nicholas B. Brookes, Lucio Braicovich, Keith Gilmore, Giacomo Ghiringhelli, Marco Salluzzo

摘要:

尽管SrTiO $_3$(STO)的结构简单,电子相关性低,但它具有与电荷输运相关的集体现象,并最终具有超导性,这些现象尚未得到充分解释。因此,需要更好地了解准粒子的性质,塑造STO的电子和导电性能。利用Ti L $_3$边缘共振非弹性X射线散射研究了体相STO和LaAlO $_{3}$ /SrTiO $_{3}$二维电子气(2DEG)的低能激发.在所有样品中,我们发现极化子的特征是强烈的$dd$ +声子激发,以及从绝缘到高导电STO单晶和异质结构时LO 3模式电子-声子耦合的减少。这两个结果都归因于大极化子自激极化的动态屏蔽,表明STO和基于STO的2DEG的低温物理由大极化子准粒子主导。

英文摘要:

Despite its simple structure and low degree of electronic correlation, SrTiO$_3$ (STO) features collective phenomena linked to charge transport and, ultimately, superconductivity, that are not yet fully explained. Thus, a better insight in the nature of the quasiparticles shaping the electronic and conduction properties of STO is needed. We studied the low energy excitations of bulk STO and of the LaAlO$_{3}$/SrTiO$_{3}$ two dimensional electron gas (2DEG) by Ti L$_3$ edge resonant inelastic x-ray scattering. In all samples, we find the hallmark of polarons in the form of intense $dd$+phonon excitations, and a decrease of the LO3-mode electron-phonon coupling when going from insulating to highly conducting STO single crystals and heterostructures. Both results are attributed to the dynamic screening of the large polaron self-induced polarization, showing that the low temperature physics of STO and STO-based 2DEGs is dominated by large polaron quasiparticles.

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