The spin-1/2 Heisenberg kagome antiferromagnet is one of the paradigmatic playgrounds for frustrated quantum magnetism, with an extensive number of competing resonating valence bond (RVB) states emerging at low energies, including gapped and gapless spin liquids and valence bond crystals. Here we revisit the crossover from this quantum RVB phase to a semiclassical regime brought about by anisotropic Kitaev interactions, and focus on the precise mechanisms underpinning this crossover. To this end, we introduce a simple parametrization of the classical ground states (GSs) in terms of emergent Ising-like variables, and use this parametrizaton: i) to construct an effective low-energy description of the order-by-disorder mechanism operating in a large part of the phase diagram, and ii) to contrast, side by side, exact diagonalization data obtained from the full basis with that obtained from the restricted (orthonormalized) basis of classical GSs. The results reveal that fluctuation corrections from states outside the restricted basis are strongly quenched inside the semiclassical regime (due to the large anisotropy spin gaps), and that the RVB phase survives up to a relatively large value of Kitaev anisotropy $K$. We further find that the pure Kitaev model admits a subextensive number of one-dimensional symmetries, which explains naturally the absence of classical and quantum order by disorder reported previously.
The Kitaev-Heisenberg model on the honeycomb lattice has been studied for the purpose of finding exotic states such as quantum spin liquid and topological orders. On the kagome lattice, in spite of a spin-liquid ground state in the Heisenberg model, the stability of the spin-liquid state has hardly been studied in the presence of the Kitaev interaction. Therefore, we investigate the ground state of the classical and quantum spin systems of the kagome Kitaev-Heisenberg model. In the classical system, we obtain an exact phase diagram that has an eight-fold degenerated canted ferromagnetic phase …
Frustrated quantum spin systems such as the Heisenberg and Kitaev models on various lattices, have been known to exhibit various exotic properties not only at zero temperature but also for finite temperatures. Inspired by the remarkable development of the quantum frustrated spin systems in recent years, we investigate the finite-temperature properties of the $S=1/2$ Kitaev-Heisenberg models on kagome and triangular lattices by means of finite-temperature Lanczos methods with improved accuracy. In both lattices, multiple peaks are confirmed in the specific heat. To find the origin of the multip…
The Kitaev-Heisenberg (KH) model has been proposed to capture magnetic interactions in iridate Mott insulators on the honeycomb lattice. We show that analogous interactions arise in many other geometries built from edge-sharing IrO_6 octahedra, including the pyrochlore and hyperkagome lattices relevant to Ir2O4 and Na4Ir3O8 respectively. The Kitaev spin liquid exact solution does not generalize to these lattices. However, a different exactly soluble point of the honeycomb lattice KH model, obtained by a four-sublattice transformation to a ferromagnet, generalizes to all these lattices. A Klein…
The exploration of quantum spin liquids (QSLs) has been guided by different approaches including the resonating valence bond (RVB) picture, deconfined lattice gauge theories and the Kitaev model. More recently, a spin liquid ground state was numerically established on the ruby lattice, inspired by the Rydberg blockade mechanism. Here we unify these varied approaches in a single parent Hamiltonian, in which local fluctuations of anyons stabilize deconfinement. The parent Hamiltonian is defined on kagomé triangles -- each hosting four RVB-like states -- and includes only Ising interactions and s…
We study an exactly solvable quantum spin model of Kitaev type on the kagome lattice. We find a rich phase diagram which includes a topological (gapped) chiral spin liquid with gapless chiral edge states, and a gapless chiral spin liquid phase with a spin Fermi surface. The ground state of the current model contains an odd number of electrons per unit cell which qualitatively distinguishes it from previously studied exactly solvable models with a spin Fermi surface. Moreover, we show that the spin Fermi surface is stable against weak perturbations.
We study bond energy correlation functions in an exactly solvable quantum spin model of Kitaev type on the kagome lattice with stable Fermi surface of partons proposed recently by Chua et al, Ref.\[arXiv:1010.1035]. Even though any spin correlations are ultra-short ranged, we find that the bond energy correlations have power law behavior with a $1/|{\bm r}|^3$ envelope and oscillations at incommensurate wavevectors. We determine the corresponding singular surfaces in momentum space, which provide a gauge-invariant characterization of this gapless spin liquid.
We study the quantum spin liquid phase in a variant of the Kitaev model where the bonds of the honeycomb lattice are distributed in a Kekulé pattern. The system supports gapped and gapless Z_2 quantum spin liquids with interesting differences from the original Kitaev model, the most notable being a gapped Z_2 spin liquid on a Kagome lattice. Perturbing the exactly solvable model with antiferromagnetic Heisenberg perturbations, we find a magnetically ordered phase stabilized by a quantum `order by disorder' mechanism, as well as an exotic continuous phase transition between the topological spin…
Perfect deporalization of the Loudon-Fleury inelastic visible-light scattering in the Kitaev honeycomb model is well known. Though it happens in Heisenberg Kagome and triangular antiferromagnets as well, yet we prove it to be of geometric origin rather than peculiar to quantum spin liquids. A Kitaev spin liquid in the square planar geometry indeed exhibits polarized Raman spectra containing defferent symmetry species, each brought by symmetry-compatible spinon geminate excitations, i.e. arising from symmetry-compatible direct-product representations made of double-valued irreducible representa…
Disorder-induced spin-cluster magnetism in a doped kagome spin liquid candidate
Georgia Institute of Technology（佐治亚理工学院）；Naval Research Laboratory（海军研究实验室）；Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所）；University of Chinese Academy of Sciences（中国科学院大学）；University of Virginia（弗吉尼亚大学）；Songshan Lake Materials Laboratory（松山湖材料实验室）；Massachusetts Institute of Technology（麻省理工学院）
By using the variational Monte Carlo method, we study the magnetization process of the Kitaev honeycomb model in a magnetic field. Our trial wavefunction is a generalized Bardeen-Cooper-Schrieffer wave function with the Jastrow correlation factor, which exactly describes the ground state of the Kitaev model at zero magnetic field using the Jordan-Wigner (JW) transformation. We find that two phase transitions occur for the antiferromagnetic Kitaev coupling, while only one phase transition occurs for the ferromagnetic Kitaev coupling. For the antiferromagnetic Kitaev coupling, we also find that …
The magnetization process of the isotropic Heisenberg antiferromagnet on the kagome lattice is studied. Data obtained from the numerical-diagonalization method are reexamined from the viewpoint of the derivative of the magnetization with respect to the magnetic field. We find that the behavior of the derivative at approximately one-third of the height of the magnetization saturation is markedly different from that for the cases of typical magnetization plateaux. The magnetization process of the kagome-lattice antiferromagnet reveals a new phenomenon, which we call the "magnetization ramp".
Kagome Chern Magnets are lattices which host a Chern state when they are non-magnetic and a Chern Gap when they become magnetic. These Chern gaps can host fractional Chern Fermions. There has been extensive research in the RMn$_6$Sn$_6$ system which hosts a small Chern gap with many trivial bands surrounding them. RMn$_6$Ge$_6$ is studied theoretically in order to find a more insulating Kagome magnetic with fewer bands near the Chern gap.
Kitaev quantum spin liquids have been the focus of intense research effort thanks to the discovery of various materials (e.g., RuCl3) that approximate their intriguing physics. In this paper we construct a mean-field approximation for a moir`e superlattice emerging in twisted Kitaev bilayers in terms of solutions of commensurate bilayers. We show that the band structure of deconfined spinons, defined on the mini-Brillouin zone of the superlattice, is greatly modified. The system exhibits a hyper-magic manifold: a series of nearly perfectly-flat bands appear at energies above the lowest gap, ex…
Magnetization plateaus in quantum spin systems emerges in two-dimensional frustrated systems such as kagome lattice. The spin-1/2 antiferromagnetic Heisenberg model on square-kagome lattice is also appropriate for the study of magnetization plateau. Motivated by recent experimental finding of such a square-kagome lattice with nonequivalent three bonds, we investigate the phase diagrams and magnetization plateaus of the lattice by the exact diagonalization method. In addition to previously reported the 1/3 and 2/3 plateaus in the model with two equivalent bonds, we find a new 2/3 plateau whose …
The magnetization of two spin-1/2 kagome antiferromagnets, volborthite and vesignieite, has been measured in pulsed magnetic fields up to 68 T. A magnetization plateau is observed for each compound near the highest magnetic field. Magnetizations at saturation are approximately equal to 0.40Ms for both compounds, where Ms is the fully saturated magnetization, irrespective of a difference in the distortion of the kagome lattice between the two compounds. It should be noted that these values of magnetizations are significantly larger than Ms/3 predicted theoretically for the one-third magnetizati…
Spin-1/2 Heisenberg model on kagome lattice is a typical frustrated quantum spin system. A basic structure of kagome lattice is also present in kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus study the magnetization plateaus of the spin-1/2 Heisenberg model on a kagome-strip chain with three-independent antiferromagnetic exchange interactions by the density-matrix renormalization group method. In a certain range of exchange parameters, we find twelve kinds of magnetization plateaus, nine of which have magnetic structures breaking either translati…
Frustrated one-dimensional quantum spin systems are known to exhibit a variety of quantum ground states due to the effects of quantum fluctuations and frustrations. In a spin-1/2 kagome-strip chain, which is one of the frustrated one-dimensional spin systems, many quantum phases have been found. However, the magnetic phase diagrams of the kagome-strip chain under magnetic field have not been fully understood. We construct magnetic phase diagrams at 0, 1/5, 3/10, 1/3, 2/5, 7/15, 3/5, and 4/5 magnetization ratio in the kagome-strip chain and investigate magnetic properties in each phase using th…
Kagome materials often host exotic quantum phases, including spin liquids, Chern gap, charge order, and superconductivity. Existing scanning microscopy studies of the kagome charge order have been limited to non-kagome surface layers. Here we tunnel into the kagome lattice of FeGe to uncover features of the charge order. Our spectroscopic imaging identifes a 2x2 charge order in the magnetic kagome lattice, resembling that discovered in kagome superconductors. Spin-mapping across steps of unit-cell-height demonstrates that this charge order emerges from spin-polarized electrons with an antiferr…
Materials that realize Kitaev spin models with bond-dependent anisotropic interactions have long been searched for, as the resulting frustration effects are predicted to stabilize novel forms of magnetic order or quantum spin liquids. Here we explore the magnetism of $γ$-Li$_2$IrO$_3$, which has the topology of a 3D Kitaev lattice of inter-connected Ir honeycombs. Using resonant magnetic x-ray diffraction we find a complex, yet highly-symmetric incommensurate magnetic structure with non-coplanar and counter-rotating Ir moments. We propose a minimal Kitaev-Heisenberg Hamiltonian that naturally …
A range of honeycomb-lattice compounds has been proposed and investigated in the search for a topological Kitaev spin liquid. However, sizable Heisenberg interactions and additional symmetry-allowed exchange anisotropies in the magnetic Hamiltonian of these potential Kitaev materials push them away from the pure Kitaev spin-liquid state. Particularly the Kitaev-to-Heisenberg coupling ratio is essential in this respect. With the help of advanced quantum-chemistry methods, we explore how the magnetic coupling ratios depend on pressure in several honeycomb compounds (Na$_2$IrO$_3$, $β$-Li$_2$IrO$…
We investigate the ground state properties of the spin S=1 Kitaev honeycomb model under a magnetic field based on the density matrix renormalization group (DMRG) calculation. With the time reversal symmetry breaking due to the magnetic field, a gapped Kitaev spin liquid is identified for both ferromagnetic (FM) and antiferromagnetic (AFM) Kitaev couplings. The topological nature of such Kitaev spin liquid is manifested by the nearly quantized Wilson loop, degeneracy in the entanglement spectra and existence of edge modes. While the FM Kitaev spin liquid is destroyed by a weaker magnetic field …
In this Letter, we identify a noncoplanar chiral spin texture on the distorted kagomé-lattice antiferromagnets induced by the presence of a magnetic field applied perpendicular to the distorted kagomé plane. The noncoplanar chiral spin texture has a nonzero scalar spin chirality similar to a chiral quantum spin liquid with broken time-reversal symmetry. In the noncoplanar regime we observe nontrivial topological magnetic excitations and thermal Hall response through the emergent field-induced scalar spin chirality in contrast to collinear ferromagnets in which the Dzyaloshinskii-Moriya (DM) sp…
Kagome magnet usually hosts nontrivial electronic or magnetic states drawing great interests in condensed matter physics. In this paper, we report a systematic study on transport properties of kagome magnet TmMn$_6$Sn$_6$. The prominent topological Hall effect (THE) has been observed in a wide temperature region spanning over several magnetic phases and exhibits strong temperature and field dependence. This novel phenomenon due to non-zero spin chirality indicates possible appearance of nontrival magnetic states accompanying with strong fluctuations. The planar applied field drives planar Hall…
The spin-1/2 kagome antiferromagnets are key prototype materials for studying frustrated magnetism. Three isostructural kagome antiferromagnets LnCu$_3$(OH)$_6$Cl$_3$ (Ln = Gd, Tb, Dy) have been successfully synthesized by the hydrothermal method. LnCu$_3$(OH)$_6$Cl$_3$ adopts space group $P\overline{3}m1$ and features the layered Cu-kagome lattice with lanthanide Ln$^{3+}$ cations sitting at the center of the hexagons. Although heavy lanthanides (Ln = Gd, Tb, Dy) in LnCu$_3$(OH)$_6$Cl$_3$ provide a large effective magnetic moment and ferromagnetic-like spin correlations compared to light-lant…
The magnetic field response of the Mott-insulating honeycomb iridate Na$_{2}$IrO$_{3}$ is investigated using torque magnetometry measurements in magnetic fields up to 60 tesla. A peak-dip structure is observed in the torque response at magnetic fields corresponding to an energy scale close to the zigzag ordering ($\approx 15~K$) temperature. Using exact diagonalization calculations, we show that such a distinctive signature in the torque response constrains the effective spin models for these classes of Kitaev materials to ones with dominant ferromagnetic Kitaev interactions, while alternative…
We have explored the hidden symmetries of a generic four-parameter nearest-neighbor spin model, allowed in honeycomb lattice compounds under trigonal compression. Our method utilizes a systematic algorithm to identify all dual transformations of the model that map the Hamiltonian on itself, changing the parameters and providing exact links between different points in its parameter space. We have found the complete set of points of hidden SU(2) symmetry at which seemingly highly anisotropic model can be mapped back on the Heisenberg model and inherits therefore its properties such as the presen…
We clarify the existence of several magnetization plateaux for the kagome $S=1/2$ antiferromagnetic Heisenberg model in a magnetic field. Using approximate or exact localized magnon eigenstates, we are able to describe in a similar manner the plateau states that occur for magnetization per site $m=1/3$, $5/9$, and $7/9$ of the saturation value. These results are confirmed using large-scale Exact Diagonalization on lattices up to 63 sites.
The hole-doped kagome lattice of Cu2+ ions in LaCuO2.66 was investigated by nuclear quadrupole resonance (NQR), electron spin resonance (ESR), electrical resistivity, bulk magnetization and specific heat measurements. For temperatures above ~180 K, the spin and charge properties show an activated behavior suggestive of a narrow-gap semiconductor. At lower temperatures, the results indicate an insulating ground state which may or may not be charge ordered. While the frustrated spins in remaining patches of the original kagome lattice might not be directly detected here, the observation of coexi…
Kagome magnets provide a fascinating platform for a plethora of topological quantum phenomena. Here, utilizing angle-resolved photoemission spectroscopy, we demonstrate Weyl lines with strong out-of-plane dispersion in an A-A stacked kagome magnet TbxGd1-xMn6Sn6. On the Gd rich side, the Weyl line remains nearly spin-orbit-gapless due to a remarkable cooperative interplay between Kane-Mele spin-orbit-coupling, low site symmetry and in-plane magnetic order. Under Tb substitution, the kagome Weyl line gaps due to a magnetic reorientation to out-of-plane order. Our results illustrate the magnetic…
In recent years, there has been an intense search for materials realizing the Kitaev quantum spin liquid model. A number of edge-shared compounds with strong spin-orbit coupling, such as RuCl$_3$ and iridates, have been proposed to realize this model. Nevertheless, an effective spin Hamiltonian derived from the microscopic model relevant to these compounds generally contains terms that are antagonistic toward the quantum spin liquid. This is consistent with the fact the zero magnetic field ground state of these materials is generally magnetically ordered. It is a pressing issue to identify pro…
Recent discovery of the half quantized thermal Hall conductivity in $α$-RuCl$_3$, a candidate material for the Kitaev spin liquid, suggests the presence of a highly entangled quantum state in external magnetic fields. This field induced phase appears between the low field zig-zag magnetic order and the high field polarized state. Motivated by this experiment, we study possible field induced quantum phases in theoretical models of the Kitaev magnets, using the two dimensional tensor network approach or infinite tensor product states. We find various quantum ground states in addition to the chir…
Mn3V2O8 is a magnetic system in which S = 5/2 Mn2+ is found in the kagome staircase lattice. Here we report the magnetic phase diagram for temperatures above 2 K and applied magnetic fields below 9 T, characterized by measurements of the magnetization and specific heat with field along the three unique lattice directions. At low applied magnetic fields, the system first orders magnetically below Tm1 ~ 21 K, and then shows a second magnetic phase transition at Tm2 ~ 15 K. In addition, a phase transition that is apparent in specific heat but not seen in magnetization is found for all three appli…
We study periodically driven pure Kitaev model and ferromagnetic phase of the Kitaev-Heisenberg model on the honeycomb lattice by off-resonant linearly and circularly-polarized lights at zero magnetic field. Using a combination of linear spin wave and Floquet theories, we show that the effective time-independent Hamiltonians in the off-resonant regime map onto the corresponding anisotropic static spin model, plus a tunable photoinduced magnetic field along the $[111]$ direction, which precipitates Floquet topological magnons and chiral magnon edge modes. They are tunable by the light amplitude…
The ground state of the simple Heisenberg nearest-neighbor quantum kagome antiferromagnetic model is a magnetically disordered spin liquid, yet various perturbations may lead to fundamentally different states. Here we disclose the origin of magnetic ordering in the structurally-perfect kagome material YCu$_3$(OH)$_6$Cl$_3$, which is free of the widespread impurity problem. {\it Ab-initio} calculations and modeling of its magnetic susceptibility reveal that, similar to the archetypal case of herbertsmithite, the nearest-neighbor exchange is by far the dominant isotropic interaction. Dzyaloshins…
Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel insight into different contributions to its magnetism. At low temperatures, two distinct types of defects with different magnetic couplings to the kagome spins are found. Surprisingly, their magnetic response contradicts the three-fold symmetry of the ideal kagome lattice, suggesting the presence of a global structural distortion that may be related to the establi…
An anomalous Hall insulator without magnetic long-range ordering is theoretically reported in the absence of the relativistic spin-orbit coupling. It is realized in itinerant electrons coupled with the Ising spins on a <111> kagome plane of pyrochlore spin ice in applied magnetic field. We find that the kagome-ice type local spin correlation in the magnetization plateau state opens a charge gap without magnetic ordering, which results in quantization of the Hall conductivity. By Monte Carlo simulation, we identify the anomalous Hall insulating region in the magnetic phase diagram, in addition …
We investigated the crystal structure of Rb$_2$Cu$_3$SnF$_{12}$ and its magnetic properties using single crystals. This compound is composed of Kagome layers of corner-sharing CuF$_{6}$ octahedra with a 2a x 2a enlarged cell as compared with the proper Kagome layer. Rb$_2$Cu$_3$SnF$_{12}$ is magnetically described as an $S$=1/2 modified Kagome antiferromagnet with four kinds of neighboring exchange interaction. From magnetic susceptibility and high-field magnetization measurements, it was found that the ground state is a disordered singlet with the spin gap, as predicted from a recent theory. …
The magnetization and specific heat measurements have been performed on single-crystalline Gd_3_Ru_4_Al_12_ with a distorted Kagome lattice structure. This spin system is regarded as an antiferromagnetic triangular lattice of XY like Heisenberg model at low temperatures. The magnetic phase diagrams indicate the existence of frustration and Z_2_ degeneracy. The magnetization and specific heat imply the successive phase transitions with partial disorder and a T-shaped spin structure in the ground state.
We study the response of the Kitaev spin liquid (KSL) to a local magnetic field perpendicular to the Kitaev honeycomb lattice. The local magnetic field induces a dynamical excitation of a flux pair in the spin liquid and the system can be described by a generally particle-hole asymmetric interacting resonant level model. The dynamical excitation of the flux pair closes the flux gap in the spectrum of the spin correlation function locally for the gapless KSL even from the perturbative response to a weak magnetic field. Beyond the perturbative regime, the p-h asymmetry competes with the magnetic…
The insulating honeycomb magnet $α$-RuCl$_{3}$ exhibits fractionalized excitiations that signal its proximity to a Kitaev quantum spin liquid (QSL) state, however, at $T=0$, fragile long-range magnetic order arises from non-Kitaev terms in the Hamiltonian. Spin vacancies in the form of Ir$^{3+}$ substituted for Ru are found to destabilize this long-range order. Neutron diffraction and bulk characterization of Ru$_{1-x}$Ir$_{x}$Cl$_{3}$ show that the magnetic ordering temperature is suppressed with increasing $x$ and evidence of zizag magnetic order is absent for $x>0.3$. Inelastic neutron scat…
The Kitaev model exhibits a Quantum Spin Liquid hosting emergent fractionalized excitations. We study the Kitaev model on the honeycomb lattice coupled to a magnetic field along the [111] axis. Utilizing large scale matrix product based numerical models, we confirm three phases with transitions at different field strengths depending on the sign of the Kitaev exchange: a non-abelian topological phase at low fields, an enigmatic intermediate regime only present for antiferromagnetic Kitaev exchange, and a field-polarized phase. For the topological phase, we numerically observe the expected cubic…
Recent experiments on Kitaev spin liquid candidate materials reported non-monotonic behavior of thermal conductivity as a function of magnetic field, which lead to conflicting interpretations of its origin. Motivated by this development, we study the magnetic field dependence of thermal conductivity of a generalized Kitaev model, which allows the phase transitions between different flux sectors as a function of the magnetic field. The thermal conductivity due to Majorana fermions shows dip-bump structures as the magnetic field increases, which is caused by either the transitions between differ…
We consider the spin-1/2 antiferromagnetic Heisenberg model on the two-dimensional square-kagome lattice with almost dispersionless lowest magnon band. For a general exchange coupling geometry we elaborate low-energy effective Hamiltonians which emerge at high magnetic fields. The effective model to describe the low-energy degrees of freedom of the initial frustrated quantum spin model is the (unfrustrated) square-lattice spin-1/2 $XXZ$ model in a $z$-aligned magnetic field. For the effective model we perform quantum Monte Carlo simulations to discuss the low-temperature properties of the squa…
We investigate the possible regular magnetic order (RMO) for the spin models with global O(3) spin rotation, based on a group theoretical approach for triangular and kagome lattices. The main reason to study these RMOs is that they are good variational candidates for the ground states of many specific models. In this work, we followed the prescription introduced by Messio et al. (L. Messio, C. Lhuillier, and G. Misguich, Phys. Rev. B, 2011, 83, 184401) for the p6m group and extended their work for different subgroups of p6m, i.e., p6, p3, p3m1, and p31m. We have listed all the possible regular…
Magnetic properties of the spin-1/2 kagome-like compound volborthite are studied using a high-quality polycrystalline sample. It is evidenced from magnetization and specific heat measurements that the spins on the kagome lattice still fluctuate at low temperature, down to T = 60 mK that corresponds to 1/1500 of the nearest-neighbor antiferromagnetic interaction, exhibiting neither a conventional long-range order nor a spin gap. In contrast, 51V NMR experiments revealed a sharp peak at 1 K in relaxation rate, which indicates that a certain exotic order occurs. Surprisingly, we have observed thr…
We consider the quasi-two-dimensional pseudo-spin-1/2 Kitaev - Heisenberg model proposed for A2IrO3 (A=Li, Na) compounds. The spin-wave excitation spectrum, the sublattice magnetization, and the transition temperatures are calculated in the random phase approximation (RPA) for four different ordered phases, observed in the parameter space of the model: antiferomagnetic, stripe, ferromagnetic, and zigzag phases. The Néel temperature and temperature dependence of the sublattice magnetization are compared with the experimental data on Na2IrO3.
Relevance of on-site and intersite Coulomb interactions in the Kitaev-Heisenberg magnet Na$_3$Co$_2$SbO$_6$
Institute for Theoretical Solid State Physics, Leibniz IFW Dresden（德累斯顿亥姆霍兹中心莱布尼茨研究所理论固态物理研究所）；Department of Physics, Karpagam Academy of Higher Education（卡尔帕甘高等教育学院物理系）；Centre for Computational Physics, Karpagam Academy of Higher Education（卡尔帕甘高等教育学院计算物理中心）；School of Physics, University of Melbourne（墨尔本大学物理学院）；Department of Physics, Technical University Dresden（德累斯顿工业大学物理系）
The coupled cluster method is applied to a spin-half model at zero temperature ($T=0$), which interpolates between Heisenberg antiferromagnets (HAF's) on a kagome and a square lattice. With respect to an underlying triangular lattice the strengths of the Heisenberg bonds joining the nearest-neighbor (NN) kagome sites are $J_{1} \geq 0$ along two of the equivalent directions and $J_{2} \geq 0$ along the third. Sites connected by $J_{2}$ bonds are themselves connected to the missing NN non-kagome sites of the triangular lattice by bonds of strength $J_{1}' \geq 0$. When $J_{1}'=J_{1}$ and $J_{2}…
The layered honeycomb magnet $α$-Li$_2$IrO$_3$ has been theoretically proposed as a candidate to display novel magnetic behaviour associated with Kitaev interactions between spin-orbit entangled $j_{\rm eff}=1/2$ magnetic moments on a honeycomb lattice. Here we report single crystal magnetic resonant x-ray diffraction combined with powder magnetic neutron diffraction to reveal an incommensurate magnetic order in the honeycomb layers with Ir magnetic moments counter-rotating on nearest-neighbour sites. This type of magnetic structure has not been reported experimentally before in honeycomb magn…
We study the ground state properties of a quantum antiferromagnet in the kagome lattice in the presence of a magnetic field, paying particular attention to the stability of the plateau at magnetization 1/3 of saturation. While the plateau is reinforced by certain deformations of the lattice, like the introduction of structural defect lines and against an Ising anisotropy, ground state correlations are seen to be quite different and the undistorted SU(2) case appears to be rather special.
