arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2004.05122cond-mat.str-elcond-mat.supr-con
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高压下Cu2OSeO3体相的室温Skyrmion相

Room-temperature skyrmion phase in bulk Cu2OSeO3 under high pressures

Liangzi Deng, Hung-Cheng Wu, Alexander P. Litvinchuk, Noah F. Q. Yuan, Jey-Jau Lee, Rabin Dahal, Helmuth Berger, Hung-Duen Yang, Ching-Wu Chu

摘要:

在非中心对称helimagnet的skyrmion状态显示拓扑保护的自旋纹理与高密度信息存储,超快自旋电子学和有效的微波器件的深刻的技术意义。通常,其在体helimagnet中的平衡态仅发生在非常有限的磁场-温度相空间上,并且通常发生在磁转变温度Tc附近的低温区域。我们在42.1 GPa的压力下,通过从立方P2(_1)3 →正交P2(_1)2(_1)2(_1)→单斜P2(_1)→三斜P1的一系列相变,将单晶Cu_2 O_SeO_3的skyrmion相区从55-58.5 K扩展到5-300 K,使用我们新开发的超灵敏高压磁化技术结果与我们的Ginzburg-Landau自由能分析一致,表明压力倾向于稳定skyrmion状态,并在较高的温度下。观测结果还表明,skyrmion状态可以在更高的温度下在各种晶体对称性中实现,这表明skyrmion对底层晶格的不敏感性,从而可能在helimagnets中更普遍存在skyrmion。

英文摘要:

A skyrmion state in a non-centrosymmetric helimagnet displays topologically protected spin textures with profound technological implications for high density information storage, ultrafast spintronics, and effective microwave devices. Usually, its equilibrium state in a bulk helimagnet occurs only over a very restricted magnetic-field--temperature phase space and often in the low temperature region near the magnetic transition temperature Tc. We have expanded and enhanced the skyrmion phase region from the small range of 55-58.5 K to 5-300 K in single-crystalline Cu2OSeO3 by pressures up to 42.1 GPa through a series of phase transitions from the cubic P2(_1)3, through orthorhombic P2(_1)2(_1)2(_1) and monoclinic P2(_1), and finally to the triclinic P1 phase, using our newly developed ultrasensitive high-pressure magnetization technique. The results are in agreement with our Ginzburg-Landau free energy analyses, showing that pressures tend to stabilize the skyrmion states and at higher temperatures. The observations also indicate that the skyrmion state can be achieved at higher temperatures in various crystal symmetries, suggesting the insensitivity of skyrmions to the underlying crystal lattices and thus the possible more ubiquitous presence of skyrmions in helimagnets.

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