Spectrally reconfigurable quantum emitters enabled by optimized fast modulation
Daniil M. Lukin, Alexander D. White, Rahul Trivedi, Melissa A. Guidry, Naoya Morioka, Charles Babin, Öney O. Soykal, Jawad Ul Hassan, Nguyen Tien Son, Takeshi O… 展开作者
Daniil M. Lukin, Alexander D. White, Rahul Trivedi, Melissa A. Guidry, Naoya Morioka, Charles Babin, Öney O. Soykal, Jawad Ul Hassan, Nguyen Tien Son, Takeshi Ohshima, Praful K. Vasireddy, Mamdouh H. Nasr, Shuo Sun, Jean-Phillipe W. MacLean, Constantin Dory, Emilio A. Nanni, Jörg Wrachtrup, Florian Kaiser, Jelena Vučković
The ability to shape photon emission facilitates strong photon-mediated interactions between disparate physical systems, thereby enabling applications in quantum information processing, simulation and communication. Spectral control in solid state platforms such as color centers, rare earth ions, and quantum dots is particularly attractive for realizing such applications on-chip. Here we propose the use of frequency-modulated optical transitions for spectral engineering of single photon emission. Using a scattering-matrix formalism, we find that a two-level system, when modulated faster than its optical lifetime, can be treated as a single-photon source with a widely reconfigurable photon spectrum that is amenable to standard numerical optimization techniques. To enable the experimental demonstration of this spectral control scheme, we investigate the Stark tuning properties of the silicon vacancy in silicon carbide, a color center with promise for optical quantum information processing technologies. We find that the silicon vacancy possesses excellent spectral stability and tuning characteristics, allowing us to probe its fast modulation regime, observe the theoretically-predicted two-photon correlations, and demonstrate spectral engineering. Our results suggest that frequency modulation is a powerful technique for the generation of new light states with unprecedented control over the spectral and temporal properties of single photons.
Understanding the properties of novel solid-state quantum emitters is pivotal for a variety of applications in field ranging from quantum optics to biology. Recently discovered defects in hexagonal boron nitride are especially interesting, as they offer much desired characteristics such as narrow emission lines and photostability. Here, we study the dependence of the emission on the excitation wavelength. We find that, in order to achieve bright single photon emission with high quantum efficiency, the excitation wavelength has to be matched to the emitter. This is a strong indication that the …
We show how to create maximal entanglement between spectrally distinct solid-state emitters embedded in a waveguide interferometer. By revealing the rich underlying structure of multi-photon scattering in emitters, we show that a two-photon input state can generate deterministic maximal entanglement even for emitters with significantly different transition energies and line-widths. The optimal frequency of the input is determined by two competing processes: which-path erasure and interaction strength. We find that smaller spectral overlap can be overcome with higher photon numbers, and quasi-m…
We demonstrate how to create maximal entanglement between two qubits that are encoded in two spectrally distinct solid-state quantum emitters embedded in a waveguide interferometer. The optical probe is provided by readily accessible squeezed light, generated by parametric down-conversion. By continuously illuminating the emitters, the photon scattering and incremental path-erasure builds up entanglement. Our method does not require perfectly identical emitters, and accommodates spectral variations due to the fabrication process. Furthermore, for some line-width and energy ratios, the entangle…
Scalable spin-to-photon interfaces require quantum emitters with strong optical transition dipole moment and low coupling to phonons and stray electric fields. It is known that particularly for coupling to stray electric fields, these conditions can be simultaneously satisfied for emitters that show inversion symmetry. Here, we show that inversion symmetry is not a prerequisite criterion for a spectrally stable quantum emitter. We find that identical electron density in ground and excited states can eliminate the coupling to the stray electric fields. Further, a strong optical transition dipol…
A single photon in a strongly nonlinear cavity is able to block the transmission of the second photon, thereby converting incident coherent light into anti-bunched light, which is known as photon blockade effect. On the other hand, photon anti-pairing, where only the entry of two photons is blocked and the emission of bunches of three or more photons is allowed, is based on an unconventional photon blockade mechanism due to destructive interference of two distinct excitation pathways. We propose quantum plexcitonic systems with moderate nonlinearity to generate both anti-bunched and anti-paire…
Solid-state single-photon emitters are attractive for realization of integrated quantum systems due to their experimental convenience and scalability. Unfortunately, however, their complex mesoscopic environments cause photons from different emitters to be spectrally distinguishable. Here we demonstrate spectral alignment of two solid-state single-photon emitters by utilizing the strain gradient. Multiple germanium vacancy (GeV) color centers in diamond are created in fabricated diamond microcantilevers using focused ion beam implantation. The strain response of the electronic energy levels of…
We present a driving scheme for solid-state quantum emitters using frequency-swept pulses containing a spectral hole resonant with the optical transition in the emitter. Our scheme enables high-fidelity state inversion, exhibits robustness to variations in the laser pulse parameters and is immune to phonon-mediated excitation-induced dephasing, benefits that derive from the the insensitivity of the adiabaticity condition to variations in the experimental parameters. Our resonant driving approach could be combined with spectral filtering of the scattered pump light and photonic devices for enha…
The future of quantum photonic technology depends on the realization of efficient sources of single photons, the ideal carriers of quantum information. Parametric downconversion (PDC) is a promising route to create highly coherent, spectrally pure single photons for quantum photonics using versatile group-velocity matching (GVM) and tailored nonlinearities. However, the functionality to actively control the poling period of nonlinear crystals used in PDC is currently missing, yet would enable to dynamically modify the wavelength of single photons produced in the PDC process. Here a detailed GV…
In a quantum network, coherent emitters can be entangled over large distances using photonic channels. In solid-state devices, the required efficient light-emitter interface can be implemented by confining the light in nanophotonic structures. However, fluctuating charges and magnetic moments at the nearby interface then lead to spectral instability of the emitters. Here we avoid this limitation when enhancing the photon emission up to 70(12)-fold using a Fabry-Perot resonator with an embedded 19 micrometer thin crystalline membrane, in which we observe around 100 individual erbium emitters. I…
Resonant excitation of solid-state quantum emitters enables coherent control of quantum states and generation of coherent single photons, which are required for scalable quantum photonics applications. However, these systems can often decay to one or more intermediate dark states or spectrally jump, resulting in the lack of photons on resonance. Here, we present an optical co-excitation scheme which uses a weak non-resonant laser to reduce transitions to a dark state and amplify the photoluminescence from quantum emitters in hexagonal boron nitride (hBN). Utilizing a two-laser repumping scheme…
The interaction of quantum emitters with structured baths modifies both their individual and collective dynamics. In González-Tudela \emph{et al} we show how exotic quantum dynamics emerge when QEs are spectrally tuned around the middle of the band of a two-dimensional structured reservoir, where we predict the failure of perturbative treatments, anisotropic interactions and novel super and subradiant behaviour. In this work, we provide further analysis of that situation, together with a complete analysis for the quantum emitter dynamics in spectral regions different from the center of the ban…
We present a proof-of-principle experimental demonstration of a reconfigurable entanglement distribution scheme utilizing a poled fiber-based source of broadband polarization-entangled photon pairs and dense wavelength-division multiplexing. A large bandwidth (> 90 nm, centered at 1555 nm) and highly spectrally correlated nature of the entangled source can be exploited to allow for the generation of more than 25 frequency-conjugate entangled pairs when aligned to the standard 200 GHz ITU grid. In this work, three frequency-conjugate entangled pairs are used to demonstrate quantum key distribut…
Scalable photonic quantum computing architectures pose stringent requirements on photonic processing devices. The need for low-loss high-speed reconfigurable circuits and near-deterministic resource state generators are some of the most challenging requirements. Here we develop an integrated photonic platform based on thin-film lithium niobate and interface it with deterministic solid-state single-photon sources based on quantum dots in nanophotonic waveguides. The generated photons are processed with low-loss circuits programmable at speeds of several GHz. We realize a variety of key photonic…
The efficient interaction of light with quantum emitters is crucial to most applications in nano and quantum photonics, such as sensing or quantum information processing. Effective excitation and photon extraction are particularly important for the weak signals emitted by a single atom or molecule. Recent works have introduced novel collection strategies, which demonstrate that large efficiencies can be achieved by either planar dielectric antennas combined with high numerical-aperture objectives or optical nanostructures that beam emission into a narrow angular distribution. However, the firs…
For a scalable photonic device producing entangled photons, it is desirable to have multiple quantum emitters in an ensemble that can be collectively excited, despite their spectral variability. For quantum dots, Rabi rotation, the most popular method for resonant excitation, cannot assure a universal, highly efficient excited state preparation, because of its sensitivity to the excitation parameters. In contrast, Adiabatic Rapid Passage (ARP), relying on chirped optical pulses, is immune to quantum dot spectral inhomogeneity. Here, we advocate the robustness of ARP for simultaneous excitation…
Efficient, high rate photon sources with high single photon purity are essential ingredients for quantum technologies. Single photon sources based on solid state emitters such as quantum dots are very advantageous for integrated photonic circuits, but they can suffer from a high two-photon emission probability, which in cases of non-cryogenic environment cannot be spectrally filtered. Here we propose two temporal purification-by-heralding methods for using a two photon emission process to yield highly pure and efficient single photon emission, bypassing the inherent problem of spectrally overl…
Monolayer WSe$_2$ hosts bright single-photon emitters. Because of its compliance, monolayer WSe$_2$ conforms to patterned substrates without breaking, thus creating the potential for large local strain, which is one activation mechanism of its intrinsic quantum emitters. Here, we report an approach to creating spatially and spectrally isolated quantum emitters from WSe$_2$ monolayers with few or no detrimental sources of emission. We show that a bilayer of hexagonal boron nitride (hBN) and WSe$_2$ placed on a nanostructured substrate can be used to create and shape wrinkles that communicate lo…
The integration of quantum emitters with integrated photonics enables complex quantum photonic circuits that are necessary for photonic implementation of quantum simulators, computers, and networks. Thin-film lithium niobate is an ideal material substrate for quantum photonics because it can tightly confine light in small waveguides and has a strong electro-optic effect that can switch and modulate single photons at low power and high speed. However, lithium niobite lacks efficient single-photon emitters, which are essential for scalable quantum photonic circuits. We demonstrate deterministic …
Tunable WS$_2$ Micro-Dome Open Cavity Single Photon Source
Carl von Ossietzky Universität Oldenburg（奥尔登堡卡尔·冯·奥西茨基大学）；Sapienza University of Rome（罗马智慧大学）；Friedrich Schiller University Jena（耶拿弗里德里希·席勒大学）；National Institute for Materials Science（国立材料研究所）；National Research Council（国家研究委员会）
Quantum photonics technologies like wavelength division multiplexing (WDM) for high-rate quantum key distribution require narrowband, spectrally tunable single photon emitters. Physical methods that rely on the application of large mechanical strain to epitaxial quantum dots or electric and magnetic fields to color centers in 2D metal dichalcogenides provide limited spectral tunability. Here we adopt a chemical approach to synthesize a family of colloidal mixed-cation perovskite quantum dots ($\text{Cs}_{1-x}\text{FA}_{x}\text{PbBr}_3$) that show highly photo-stable, compositionally tunable si…
In this work we study the quantum dynamics emerging when quantum emitters exchange excitations with a two-dimensional bosonic bath with hexagonal symmetry. We show that a single quantum emitter spectrally tuned to the middle of the band relaxes following a logarithmic law in time due to the existence of a singular point with vanishing density of states, i.e., the Dirac point. Moreover, when several emitters are coupled to the bath at that frequency, long-range coherent interactions between them appear which decay inversely proportional to their distance without exponential attenuation. We anal…
We create and isolate single-photon emitters with a high brightness approaching $10^5$ counts per second in commercial silicon-on-insulator (SOI) wafers. The emission occurs in the infrared spectral range with a spectrally narrow zero phonon line in the telecom O-band and shows a high photostability even after days of continuous operation. The origin of the emitters is attributed to one of the carbon-related color centers in silicon, the so-called G center, allowing purification with the $^{12}$C and $^{28}$Si isotopes. Furthermore, we envision a concept of a highly-coherent scalable quantum p…
Photon-mediated coupling between distant matter qubits may enable secure communication over long distances, the implementation of distributed quantum computing schemes, and the exploration of new regimes of many-body quantum dynamics. Nanophotonic devices coupled to solid-state quantum emitters represent a promising approach towards realization of these goals, as they combine strong light-matter interaction and high photon collection efficiencies. However, the scalability of these approaches is limited by the frequency mismatch between solid-state emitters and the instability of their optical …
Optical nanostructures have proven to be meritorious for tailoring the emission properties of quantum emitters. However, unavoidable fabrication imperfections may represent a nuisance. Quite remarkably, disorder offers new opportunities since light can be efficiently confined by random multiple scattering leading to Anderson localization. Here we investigate the effect of such disorder-induced cavities on the emission dynamics of single quantum dots embedded in disordered photonic-crystal waveguides. We present time-resolved measurements of both the total emission from Anderson-localized cavit…
A highly promising route to scale millions of qubits is to use quantum photonic integrated circuits (PICs), where deterministic photon sources, reconfigurable optical elements, and single-photon detectors are monolithically integrated on the same silicon chip. The isolation of single-photon emitters, such as the G centers and W centers, in the optical telecommunication O-band, has recently been realized in silicon. In all previous cases, however, single-photon emitters were created uncontrollably in random locations, preventing their scalability. Here, we report the controllable fabrication of…
Hexagonal boron nitride (h-BN), a prevalent insulating crystal for dielectric and encapsulation layers in two-dimensional (2D) nanoelectronics and a structural material in 2D nanoelectromechanical systems (NEMS), has also rapidly emerged as a promising platform for quantum photonics with the recent discovery of optically active defect centers and associated spin states. Combined with measured emission characteristics, here we propose and numerically investigate the cavity quantum electrodynamics (cavity-QED) scheme incorporating these defect-enabled single photon emitters (SPEs) in h-BN microd…
Quantum emitters interacting with two-dimensional photonic-crystal baths experience strong and anisotropic collective dissipation when they are spectrally tuned to 2D Van-Hove singularities. In this work, we show how to turn this dissipation into coherent dipole-dipole interactions with tuneable range by breaking the lattice degeneracy at the Van-Hove point with a superlattice geometry. Using a coupled-mode description, we show that the origin of these interactions stems from the emergence of a qubit-photon bound state which inherits the anisotropic properties of the original dissipation, and …
We investigate the emission properties of a single semiconductor quantum dot deterministically coupled to a confined optical mode in the weak coupling regime. A strong pulling, broadening and narrowing of the cavity mode emission is evidenced when changing the spectral detuning between the emitter and the cavity. These features are theoretically accounted for by considering the phonon assisted emission of the quantum dot transition. These observations highlight a new situation for cavity quantum electrodynamics involving spectrally broad emitters.
The nitrogen-vacancy center (NV) in diamond, with its exceptional spin coherence and convenience in optical spin initialization and readout, is increasingly used both as a quantum sensor and as a building block for quantum networks. Employing photonic structures for maximizing the photon collection efficiency in these applications typically leads to broadened optical linewidths for the emitters, which are commonly created via nitrogen ion implantation. With studies showing that only native nitrogen atoms contribute to optically coherent NVs, a natural conclusion is to either avoid implantation…
We characterize the coherent dynamics of a two-level quantum emitter driven by a pair of symmetrically-detuned phase-locked pulses. The promise of dichromatic excitation is to spectrally isolate the excitation laser from the quantum emission, enabling background-free photon extraction from the emitter. Paradoxically, we find that excitation is not possible without spectral overlap between the exciting pulse and the quantum emitter transition for ideal two-level systems due to cancellation of the accumulated pulse area. However, any additional interactions that interfere with cancellation of th…
Photon-mediated interactions between quantum systems are essential for realizing quantum networks and scalable quantum information processing. We demonstrate such interactions between pairs of silicon-vacancy (SiV) color centers strongly coupled to a diamond nanophotonic cavity. When the optical transitions of the two color centers are tuned into resonance, the coupling to the common cavity mode results in a coherent interaction between them, leading to spectrally-resolved superradiant and subradiant states. We use the electronic spin degrees of freedom of the SiV centers to control these opti…
Reconfigurable photonic circuits have applications ranging from next-generation computer architectures to quantum networks, coherent radar and optical metamaterials. However, complete reconfigurability is only currently practical on millimetre-scale device footprints. Here, we overcome this barrier by developing an on-chip high quality microcavity with resonances that can be electrically tuned across a full free spectral range (FSR). FSR tuning allows resonance with any source or emitter, or between any number of networked microcavities. We achieve it by integrating nanoelectronic actuation wi…
We demonstrate the remote all-optical control of the spontaneous emission (SE) of quantum dots using coupled photonic crystal cavities. By spectrally tuning a Fabry-Perot cavity in resonance with a target cavity, the quality factor and the local density of states experienced by emitters in the target cavity are modified, leading to a change in the SE rate. From the theoretical analysis of the coupled-cavity quantum electrodynamics system, the SE rate change can be higher than the quality factor change due to a reduction of the vacuum field at the emitter's position when the two cavities are br…
Solid state quantum emitters have shown strong potential for applications in quantum information, but spectral inhomogeneity of these emitters poses a significant challenge. We address this issue in a cavity-quantum dot system by demonstrating cavity-stimulated Raman spin flip emission. This process avoids populating the excited state of the emitter and generates a photon that is Raman shifted from the laser and enhanced by the cavity. The emission is spectrally narrow and tunable over a range of at least 125 GHz, which is two orders of magnitude greater than the natural linewidth. We obtain t…
Monolithic integration of quantum emitters in nanoscale plasmonic circuitry requires low-loss plasmonic configurations capable of confining light well below the diffraction limit. We demonstrate on-chip remote excitation of nanodiamond-embedded single quantum emitters by plasmonic modes of dielectric ridges atop colloidal silver crystals. The nanodiamonds are produced to incorporate single germanium-vacancy (GeV) centers, providing bright, spectrally narrow and stable single-photon sources suitable for highly integrated circuits. Using electron-beam lithography with hydrogen silsesquioxane (HS…
