The quantum states of light in an integrated photonics platform provide an important resource for quantum information processing and takes advantage of the scalability and practicality of silicon photonics. Integrated resonators have been well explored in classical and quantum optics. However, to encode multiple information through integrated quantum optics requires broader utilization of the available degrees of freedom on a chip. Here, we studied the quantum interference between photon pairs of the same higher order whispering gallery modes populated by spontaneous four-wave mixing in an integrated silicon micro-disk resonator. The quantum interference between the photon pairs of the first two quasi-TE0 and quasi-TE1 radial modes was measured to be Vnet ~ 98 + 0.8 % and Vnet ~ 94 + 2.6 %, respectively. The results are promising for achieving higher-dimensional quantum states using the higher-order radial modes of a micro-disk resonator coupled with an integrated waveguide.
We report on light emission from high-Q neodymium-implanted silica microtoroids. Following the description of the fabrication process of microtoroids, neodymium light emission is analysed. This emission is coupled to various cavity modes. Using evanescent wave coupling we achieve selective detection of Whispering Gallery Modes of a microtoroid.
By direct application of the fluctuation-dissipation theorem, we numerically calculate the fundamental dimensional fluctuations of crystalline CaF2 whispering gallery resonators in the case of structural damping, and the limit that this noise imposes on the frequency stability of such resonators at both room and cryogenic temperatures. We analyze elasto-optic noise - the effect of Brownian dimensional fluctuation on frequency via the strain-dependence of the refractive index - a noise term that has so far not been considered for whispering-gallery resonators. We find that dimensional fluctuati…
We report the direct observation of the electromagnetic-field distribution of whispering?gallery modes in silica microcavities (spheres and toroids). It is revealed by their excitation efficiency with a tapered fiber coupler swept along the meridian. The originality of this method lies in the use of the coupler itself for the near field mapping, eliminating the need of additional tools used in previous work. This method is successfully applied to microspheres and microtoroids
We demonstrate for the first time natural phase matching for optical frequency doubling in a high-Q whispering gallery mode resonator made of Lithium Niobate. A conversion efficiency of 9% is achieved at 30 micro Watt in-coupled continuous wave pump power. The observed saturation pump power of 3.2 mW is almost two orders of magnitude lower than the state-of-the-art. This suggests an application of our frequency doubler as a source of non-classical light requiring only a low-power pump, which easily can be quantum noise limited. Our theoretical analysis of the three-wave mixing in a whispering …
Stimulated Brillouin scattering recently allowed experimental excitation of surface acoustic resonances in micro-devices, enabling vibration at rates in the range of 50 MHz to 12 GHz. The experimental availability of such mechanical whispering gallery modes in photonic-MEMS raises questions on their structure and spectral distribution. Here we calculate the form and frequency of such vibrational surface whispering gallery modes, revealing diverse types of surface vibrations including longitudinal, transverse, and Rayleigh-type deformations. We parametrically investigate these various modes by …
We demonstrate a method to perform spectroscopy of near-infrared single photons without the need of dispersive elements. This method is based on a photon energy resolving transition edge sensor and is applied for the characterization of widely wavelength tunable narrow-band single photons emitted from a crystalline whispering gallery mode resonator. We measure the emission wavelength of the generated signal and idler photons with an uncertainty of up to 2 nm.
Current theoretical treatment of mode splitting and scattering loss resulting from sub-wavelength scatterers attached to the surface of high-quality-factor whispering-gallery-mode microresonators is not satisfactory. Different models have been proposed for two distinct scatterer regimes, i.e., a-few- and many-scatterers. In addition, many experimental results seem difficult to understand within the existing theoretical framework. Here we develop a unified approach that applies to an arbitrary number of scatterers, which reveals the applicable conditions and the limits of the existing theoretic…
Optical parametric downconversion has proven to be a valuable source of nonclassical light. The process is inherently able to produce twin beam correlations along with individual intensity squeezing of either parametric beam, when pumped far above threshold. Here, we present for the first time the direct observation of intensity squeezing of -1.2 dB of each of the individual parametric beams in parametric downconversion by use of a high quality whispering gallery mode disk resonator. In addition we observed twin beam quantum correlations of -2.7 dB with this cavity. Such resonators feature str…
Whispering-gallery microcavity laser possesses ultralow threshold, whereas convenient free-space optical excitation and collection suffer from low efficiencies due to its rotational symmetry. Here we analytically study a three-dimensional microsphere coupled to a nano-sized scatterer in the framework of quantum optics. It is found that the scatterer is capable of coupling light in and out of the whispering-gallery modes (WGMs) without seriously degrading their high-Q properties, while the microsphere itself plays the role of a lens to focus the input beam on the scatterer and vice versa. Our a…
We propose a series of conformal mappings for designing directional emission whispering gallery modes. The mappings transform circular cavity into quasi-polygonal transformation cavity. Anisotropic emission is demonstrated in the so-designed cavities.
A review of hollow core whispering gallery resonators (WGRs)is given. After a short introduction to the topic of whispering gallery resonators we provide a description of whispering gallery modes in hollow or liquid core WGRs. Next, whispering gallery mode (WGM) sensing mechanisms are outlined and some fabrication methods for microbubbles, microcapillaries and other tubular WGM devices are discussed. We then focus on the most common applications of hollow core WGRs, namely refractive index and temperature sensing, gas sensing, force sensing, biosensing, and lasing. The review highlights some o…
We simulate light propagation in perturbed whispering-gallery mode microcavities using a two-dimensional finite-difference beam prop- agation method in a cylindrical coordinate system. Optical properties of whispering-gallery microcavities perturbed by polystyrene nanobeads are investigated through this formulation. The light perturbation as well as quality factor degradation arising from cavity ellipticity are also studied.
We propose a kind of plasmonic whispering gallery modes highly localized on the exterior surface of a metal-coated microresonator. This exterior (EX) surface mode possesses high quality factors at room temperature, and can be efficiently excited by a tapered fiber. The EX mode can couple to an interior (IN) mode and this coupling produces a strong anti-crossing behavior, which not only allows conversion of IN to EX modes, but also forms a long-lived anti-symmetric mode. As a potential application, the EX mode could be used for a biosensor with a sensitivity high up to 500 nm per refraction ind…
We report a highly efficient source of narrow-band photon pairs based on parametric down-conversion in a crystalline whispering gallery mode resonator. Remarkably, each photon of a pair is strictly emitted into a single spatial and temporal mode, as witnessed by Glaubers autocorrelation function. We explore the phase-matching conditions in spherical geometries, and determine the requirements of the single-mode operation. Understanding these conditions has allowed us to experimentally demonstrate a single-mode pair-detection rate of $0.97 \cdot 10^6$ pairs/s per mW pump power per 20 MHz bandwid…
We study the Rayleigh scattering induced by a diamond nanocrystal in a whispering-gallery-microcavity--waveguide coupling system, and find that it plays a significant role in the photon transportation. On one hand, this study provides a new insight into future solid-state cavity quantum electrodynamics toward strong coupling physics. On the other hand, benefitting from this Rayleigh scattering, novel photon transportation such as dipole induced transparency and strong photon antibunching can occur simultaneously. As potential applications, this system can function as high-efficiency photon tur…
We have observed for the first time a new photonic quantum ring emission of anti-whispering gallery modes from a negative mesa-type toroid cavity due to semiconductor photonic corrals.
We have theoretically studied the photon statistical properties in a nonlinear whispering-gallery-mode microresonator coupled with two nanoparticles. By tuning the relative position of two nanoparticles, the photon statistical features of the system can be modified remarkably. Interestingly, a controllable switching between unconventional and conventional photon blockade can be realized by manipulating the angular positions of two nanoparticles. We also investigate the influence of the Kerr effect on the second order correlation function and find that there is an optimal choice for the relativ…
In this paper concave surface scanning method based on x-ray scattering in whispering gallery effect is considered. The capabilities of this method are studied based on ray-tracing computer simulation. The dependence of the output x-ray beam on the RMS roughness and minimum detectable imperfection height estimations were obtained.
We investigate the single-photon transport problem in the system of a Whispering-Gallery mode microresonator directionally coupled with a two-level quantum emitter (QE). This QE-microresonator coupling system can usually be studied by cavity quantum electrodynamics and the single-photon transport methods. However, we find that if we treat a two-level QE as a single-photon phase-amplitude modulator, we can also deal with such systems using the transfer matrix method. Further, in theory, we prove that these three methods are equivalent. The corresponding relations of respective parameters among …
We report a theoretical study showing that rogue waves can emerge in whispering gallery mode resonators as the result of the chaotic interplay between Kerr nonlinearity and anomalous group-velocity dispersion. The nonlinear dynamics of the propagation of light in a whispering gallery-mode resonator is investigated using the Lugiato-Lefever equation, and we evidence a range of parameters where rare and extreme events associated with a non-gaussian statistics of the field maxima are observed.
We propose asymmetric resonant cavities with rational caustics and experimentally demonstrate interior whispering gallery modes in monolithic silicon mesoscopic microcavities. These microcavities demonstrate unique robustness of cavity quality factor (Q) against roughness Rayleigh scattering. Angle-resolved tapered fiber measurements and near-field images observe distinct resonant families and asymmetric emission from interior whispering gallery modes, which can be used for microcavity laser and CQED applications.
In this paper we discuss the force exerted by the field of an optical cavity on a polarizable dipole. We show that the modification of the cavity modes due to interaction with the dipole significantly alters the properties of the force. In particular, all components of the force are found to be non-conservative, and cannot, therefore, be derived from a potential energy. We also suggest a simple generalization of the standard formulas for the optical force on the dipole, which reproduces the results of calculations based on the Maxwell stress tensor.
Second order nonlinearities in whispering gallery mode resonators are highly investigated for their many applications such as wavelength converters, entangled photon sources and generation of frequency combs. In such systems, depending on the material under scrutiny, the derivation of quasi-phase matching equations can lead to the appearance of additional quanta in the selection rule on the azimuthal confinement order. Here, we demonstrate that these additional quanta show up due to the Berry phase experienced by the transverse spin angular momentum components of the whispering gallery modes d…
Stimulated Brillouin scattering with both pump and Stokes beams in resonance with whispering gallery modes of an ultra high Q CaF_2 resonator is demonstrated for the first time. The resonator is pumped with 1064 nm light and has a Brillouin lasing threshold of 3.5 microwatt. Potential applications include optical generation of microwaves and sensitive gyros.
We experimentally studied whispering-gallery modes(WGMs) and demonstrated resonance enhancement of optical forces evanescently exerted on dielectric microspheres. We showed that the resonant light pressure can be used for optical sorting of microparticles with extraordinary uniform resonant properties that is unachievable by conventional sorting techniques.
We present a first principle derivation of the coupled nonlinear Schrödinger equations that govern the interaction between two families of modes with different transverse profiles in a generic whispering-gallery-mode resonator. We find regions of modulational instability and the existence of trains of bright solitons both in the normal and in the anomalous dispersion regime.
Numerical evolutions of whispering gallery modes of both isotropic and anisotropic spheroidal resonators are presented and used to build analytical approximations of these modes. Such approximations are carried out mainly to have the possibility to have a manageable analytic formulas for the eigenmodes and eigenfrequencies of anisotropic resonators. A qualitative analysis of ellipsoidal anisotropic modes in term of superposition of spherical modes is also presented.
A surface acoustic wave (SAW) creates its own high-Q ultra-small volume whispering gallery modes (WGMs), different from usual bulk acoustic WGMs, in an optical dielectric WGM resonator. We show that it is possible to realize an externally controllable, efficient triply-resonant opto-mechanical interaction between two optical WGMs and the SAW WGM and to use such an interaction in various sensor applications.
Quasiclassical approach and geometric optics allow to describe rather accurately whispering gallery modes in convex axisymmetric bodies. Using this approach we obtain practical formulas for the calculation of eigenfrequencies and radiative Q-factors in dielectrical spheroid and compare them with the known solutions for the particular cases and with numerical calculations. We show how geometrical interpretation allows expansion of the method on arbitrary shaped axisymmetric bodies.
Different applications of crystalline whispering gallery mode resonators call for different properties of the resonator host material. We report on our recent study of resonators made out of sapphire, diamond, and quartz crystals and discuss possible applications of these resonators. In particular, we demonstrate Kerr frequency comb generation in sapphire microresonators.
Typical microresonators exhibit a large frequency spacing between resonances and a limited tunability. This impedes their use in a large class of applications which require a resonance of the microcavity to coincide with a predetermined frequency. Here, we experimentally overcome this limitation with highly prolate-shaped whispering-gallery-mode "bottle microresonators" fabricated from standard optical glass fibers. Our resonators combine an ultra-high quality factor of 360 million, a small mode volume, and near lossless fibre coupling, characteristic of whispering-gallery-mode resonators, wit…
An analytic solution for an uniaxial spherical resonator is presented using the method of Debye potentials. This serves as a starting point for the calculation of whispering gallery modes (WGM) in such a resonator. Suitable approximations for the radial functions are discussed in order to best characterize WGMs. The characteristic equation and its asymptotic expansion for the anisotropic case is also discussed, and an analytic formula with a precision of the order $O[ν^{-1}]$ is also given. Our careful treatment of both boundary conditions and asymptotic expansions makes the present work a par…
Whispering gallery modes are known for having orbital angular momentum, however the interplay of local spin density, orbital angular momentum, and the near-field interaction with quantum emitters is much less explored. Here, we study the spin-orbital interaction of a circularly polarized dipole with the whispering gallery modes (WGMs) of a spherical resonator. Using an exact dyadic Green's function approach, we show that the near-field interaction between the photonic spin of a circularly polarized dipole and the local spin density of whispering gallery modes gives rise to unidirectional behav…
We report on tuning the optical whispering gallery modes in a poly dimethyl siloxane-based (PDMS) microsphere resonator by more than a THz. The PDMS microsphere system consists of a solid spherical resonator directly formed with double stems on either side. The stems act like tie-rods for simple mechanical stretching of the microresonator over tens of microns, resulting in tuning of the whispering gallery modes by one free spectral range. Further investigations demonstrate that the whispering gallery mode shift has a higher sensitivity (0.13 nm/μN) to an applied force when the resonator is in …
We demonstrated the tuning of whispering gallery modes (WGMs) of a silica microsphere during optical levitation through the annealing process. We determined the annealing temperature from the power balance between the CO2 laser light heating and several cooling processes. Cooling caused by heat conduction through the surrounding air molecules is the dominant process. We achieved a blue shift of the WGMs as large as 1 \%, which was observed in the white-light scattering spectrum from the levitated microsphere.
We consider an optical fiber with nanoscale variation of the effective fiber radius supporting whispering gallery modes slowly propagating along the fiber, and reveal that the radius variation can be designed to support reflectionless propagation of these modes. We show that reflectionless modulations can realize control of transmission amplitude and temporal delay, while enabling close packing due to the absence of cross-talk, in contrast to conventional potentials.
We experimentally demonstrate the use of a novel liquid state, whispering-gallery-mode optical resonator as a highly sensitive humidity sensor. The optical resonator used consists of a droplet made of glycerol, a transparent liquid that enables high optical quality factor, doped with rhodamine 6G, which acts as fluorescent emitter. As glycerol is highly hygroscopic, the refractive index and radius of the droplet change with ambient humidity. This produces a shift on the whispering gallery modes wavelengths, which modulates the emission of rhodamine 6G. This easily-made device has an unpreceded…
We propose an original method to couple light into a whispering-gallery mode resonator. This method benefits from the mode selectivity and robustness of the prism-coupling along with the single-mode propagation of the fiber taper. It consists in a prism shaped crystal with a waveguide inscribed inside it. The waveguide is self-inscribed in-situ by beam self-trapping to allow an optimum coupling to a given resonator.
We developed a new method for fabricating crystalline whispering gallery mode cavities based on laser-heated pedestal growth. We fabricated sapphire cavities and obtained a Q factor of 16000 with a cavity whose diameter was about 240 um. We showed numerically that the cross-sectional shape of the cavity is sensitive to the cavity Q, and we controlled it successfully by changing the growth condition in the molten zone, without significantly degrading the crystal structure.
We develop a compact whispering-gallery-mode (WGM) sensing system by integrating multiple components, including a tunable laser, a temperature controller, a function generator, an oscilloscope, a photodiode detector, and a testing computer, into a phone-sized embedded system. We demonstrate a thermal sensing experiment by using this portable system. Such a system successfully eliminates bulky measurement equipment required for characterizing optical resonators and will open up new avenues for practical sensing applications by using ultra-high Q WGM resonators.
We demonstrate the efficient coupling (99.5%) of a silica whispering gallery mode microresonator directly with a silicon chip by using a silicon photonic crystal waveguide as a coupler. The efficient coupling is attributed to the small effective refractive index difference between the two devices. The large group index of the photonic crystal waveguide mode also contributes to the efficient coupling. A coupling Q of 2.68*10^6 is obtained, which allows us to achieve the critical coupling of a silica whispering gallery mode with an intrinsic Q of close to 10^7 with a Si chip.
We investigated the whispering gallery modes of cavities with a hexagonal cross-section. We found two different modes, namely perturbed and quasi-WGMs, of which the former exhibits the higher Q when the corner radius is large. We studied the dependence of Q on the curvature radius of the polygonal cavities and found that the coupling between the two modes determines the Q of the cavity. In addition we fabricated a cavity by employing laser heated pedestal growth and demonstrated a high Q.
Whispering gallery modes (WGMs), circulating modes near the surface of a spheroidal material, have been known to exhibit high quality factors for both acoustic and electromagnetic waves. Here, we report an electro-optomechanical system, where the overlapping WGMs of acoustic and optical waves along the equator of a dielectric sphere strongly couple to each other. The triple-resonance phase-matching condition provides a large enhancement of the Brillouin scattering only in a single sideband, and conversion from the input radio-frequency signal exciting the acoustic mode to the output optical si…
Whispering gallery mode microdisk cavities fabricated by direct laser writing are studied using dark-field imaging and spectroscopy in the visible spectral range. {Dark-field imaging allows us to directly visualize the spatial intensity distribution of whispering gallery modes. We extract their azimuthal and radial mode indices from dark-field images, and find the axial mode number from the dispersion relation. The scattering spectrum obtained in the confocal arrangement provides information on the density of optical states in the resonator. The proposed technique is a simple non-invasive way …
The relative intensity noise (RIN) of a solid state whispering-gallery-mode class-B laser is studied both theoretically and experimentally under different pumping regimes. In particular, we show that harmonics of the spiking frequency are observed in the RIN spectrum. A rate equation model including Langevin forces and the nonlinear coupling between inverted ion and photon number fluctuations has been developed to reproduce the experimental results and to extract relevant physical parameters from the fitting of the RIN spectrum.
Using quasiclassical approach rather precise analytical approximations for the eigenfrequencies of whispering gallery modes in convex axisymmetric bodies may be found. We use the eikonal method to analyze the limits of precision of quasiclassical approximation using as a practical example spheroidal dielectric cavity. The series obtained for the calculation of eigenfrequencies is compared with the known series for dielectric sphere and with numerical calculations. We show how geometrical interpretation allows expansion of the method on arbitrary shaped axisymmetric bodies.
We propose and demonstrate a direct method to observe higher-order whispering-gallery modes in vertical cavity surface emitting lasers (VCSELs) at room temperature. Instead of introducing any defect mode, we show that suppression of lower-order cavity modes can be achieved by destroying vertical reflectors with a surface micro-structure. Up to the 23rd azimuthal order whispering-gallery mode confined laterally by the native oxide layers is observed in experiments through collecting near-field radiation patterns. Various vertical emission transverse modes are identified by the spectrum in exper…
We demonstrate a miniature self-injection locked DFB laser using resonant optical feedback from a high-Q crystalline whispering gallery mode resonator. The linewidth reduction factor is greater than 10,000, with resultant instantaneous linewidth less than 200 Hz. The minimal value of the Allan deviation for the laser frequency stability is 3x10^(-12) at the integration time of 20 us. The laser possesses excellent spectral purity and good long term stability.
We have tuned the whispering gallery modes of a fused silica microresonator over nearly 1 nm at 800 nm, i.e. over 0.5 FSR or 10^6 linewidths of the resonator. This has been achieved by a new method based on the stretching of a two-stem microsphere. The devices described below will permit new Cavity-QED experiments with this high-Q optical resonator when it is desirable to optimize its coupling to emitters with given transition frequencies. The tuning capability demonstrated here is compatible with both UHV and low temperature operation, which should be useful for future experiments with laser …
We study whispering gallery modes in triple microdisks of equilateral and isosceles triangular configurations. The characteristic properties of resonant modes in three microdisks on vertices of an equilateral triangle are explained by discrete rotational symmetry of the triangle. The avoided crossings of resonant modes in three microdisks on vertices of an isosceles triangle are also studied in terms of a combination of single and coupled microdisks. Finally, we propose the matrix models which well explain the resonant modes in triple microdisks.
Transmission electron microscopy is an excellent experimental tool to study the interaction of free electrons with nanoscale light fields. However, up to now, applying electron microscopy to quantum optical investigations was hampered by the lack of experimental platforms which allow a strong coupling between fast electrons and high-quality resonators. Here, as a first step, we demonstrate the broad-band excitation of optical whispering-gallery modes in silica microresonators by fast electrons. In the emitted coherent cathodoluminescence spectrum, a comb of equidistant peaks is observed, resul…
We show that electric field on the plane surface of truncated sphere or cylinders (so called Janus particles) have sharp resonances versus the depth of removed segment of a sphere or cylinder. These resonances are related to the excited whispering gallery waves caused by truncation. It is a new mechanism of the field localization. Optimization of this effect for cylinders permits to reach a super resolution in the line thickness what can be used for contacting optical lithography.
Chaotic whispering-gallery modes have significance both for optical applications and for our understanding of the interplay between wave phenomena and the classical ray limit in the presence of chaotic dynamics and openness. In strongly non-convex geometries, a theorem by Mather rules out the existence of invariant curves in phase space corresponding to rays circulating in whispering-gallery patterns, so that no corresponding modes of this type are expected. Here we discuss numerical computations of the electromagnetic fields in planar dielectric cavities that are strongly non-convex becauseth…
We outline a full-vectorial three-dimensional multi-mode matching technique in a cylindrical coordinate system that addresses the mutual coupling among multiple modes copropagating in a perturbed whispering-gallery-mode microcavity. In addition to its superior accuracy in respect to our previously implemented single-mode matching technique, this current technique is suitable for modelling waveguide-to-cavity coupling where the influence of multi-mode coupling is non-negligible. Using this methodology, a robust scheme for hybrid integration of a microcavity onto a silicon-on-insulator platform …
Whispering gallery mode biosensors allow selective unlabelled detection of single proteins and, combined with quantum limited sensitivity, the possibility for noninvasive realtime observation of motor molecule motion. However, to date technical noise sources, most particularly low frequency laser noise, have constrained such applications. Here we introduce a new technique for whispering gallery mode sensing based on direct detection of back-scattered light. This experimentally straightforward technique is immune to frequency noise in principle, and further, acts to suppress thermorefractive no…
High-$Q$ whispering gallery mode microresonators are cornerstones to develop compact coherent sources like single frequency lasers or frequency combs. This work reports a detailed characterization of a whispering gallery mode microsphere in the near ultraviolet. Light coupling in the resonator is obtain thanks to a robust angle-polished fiber allowing to investigate the different coupling regimes. An intrinsic $Q_0$-factor of $2.2 \times 10^8$ and a finesse of $7.3 \times 10^4$ are reported at a wavelength of 420 nm. Physical mechanisms contributing to the $Q_0$-factor are discussed and routes…
Coupled-mode induced transparency is realized in a single microbubble whispering gallery mode resonator. Using aerostatic tuning, we find that the pressure induced shifting rates are different for different radial order modes. A finite element simulation considering both the strain and stress effects shows a GHz/bar difference and this is confirmed by experiments. A transparency spectrum is obtained when a first order mode shifts across a higher order mode through precise pressure tuning. The resulting lineshapes are fitted with the theory. This work lays a foundation for future applications i…
