红外场对乙炔双化反应的严格非绝热量子控制
Strictly Non-Adiabatic Quantum Control of the Acetylene Dication Using an Infrared Field
摘要：
我们证明了在乙炔双金属的去质子化过程中存在严格的非绝热控制路径。通过在离子符合实验中测量动能位移，实验地识别该路径。我们使用TDSE仿真来确定哪些属性最强烈地影响我们的控制。我们发现，共振控制周围的锥形交叉点是有限的速度的非绝热动力学。
英文摘要：
We demonstrate the existence of a strictly non-adiabatic control pathway in deprotonation of the acetylene dication. This pathway is identified experimentally by measuring a kinetic energy shift in an ion coincidence experiment. We use a TDSE simulation to identify which properties most strongly affect our control. We find that resonant control around conical intersections is limited by the speed of non-adiabatic dynamics.
机构、总结、中文摘要均由AI分析而来，可能存在错误，请以论文正文为准。
