Scattering theory is a standard tool for the description of transport phenomena in mesoscopic systems. Here, we provide a detailed derivation of this method for nano-scale conductors that are driven by oscillating electric or magnetic fields. Our approach is based on an extension of the conventional Lippmann-Schwinger formalism to systems with a periodically time dependent Hamiltonian. As a key result, we obtain a systematic perturbation scheme for the Floquet scattering amplitudes that describe the transition of a transport carrier through a periodically driven sample. Within a general multi-terminal setup, we derive microscopic expressions for the mean values and time-integrated correlation functions, or zero-frequency noise, of matter and energy currents, thus unifying the results of earlier studies. We show that this framework is inherently consistent with the first and the second law of thermodynamics and prove that the mean rate of entropy production vanishes only if all currents in the system are zero. As an application, we derive a generalized Green-Kubo relation, which makes it possible to express the response of any mean currents to small variations of temperature and chemical potential gradients in terms of time integrated correlation functions between properly chosen currents. Finally, we discuss potential topics for future studies and further reaching applications of the Floquet scattering approach to quantum transport in stochastic and quantum thermodynamics.
We calculate the low-frequency current noise for AC biased mesoscopic chaotic cavities and diffusive wires. Contrary to what happens for the admittance, the frequency dispersion is not dominated by the electric response time (the "RC" time of the circuit), but by the time that electrons need to diffuse through the structure (dwell time or diffusion time). Frequency dispersion of noise stems from fluctuations of the Fermi distribution function that preserve charge neutrality. Our predictions can be verified with present experimental technology.
A short summary of the drift-diffusion-Langevin formalism for calculating finite-frequency shot noise in diffusive conductors is presented. Two new results are included in this presentation. First, we arrive at a simple (but accurate) phenomenological expression for the semiclassical distribution function of electrons in the presence of electron-electron scattering. Second, it is shown that in thin samples, low-frequency shot noise may be large even if the sample length is much larger than the electron-phonon relaxation length.
Periodically driven coherent conductors provide a universal platform for the development of quantum transport devices. Here, we lay down a comprehensive theory to describe the thermodynamics of these systems. We first focus on moderate thermo-electrical biases and low driving frequencies. For this linear response regime, we establish generalized Onsager-Casimir relations and an extended fluctuation-dissipation theorem. Furthermore, we derive a family of thermodynamic bounds proving that any local matter or heat current puts a non-trivial lower limit on the overall dissipation rate of a coheren…
Classically, the power generated by an ideal thermal machine cannot be larger than the Carnot limit. This profound result is rooted in the second law of thermodynamics. A hot question is whether this bound is still valid for microengines operating far from equilibrium. Here, we demonstrate that a quantum chiral conductor driven by AC voltage can indeed work with efficiencies much larger than the Carnot bound. The system also extracts work from common temperature baths, violating Kelvin-Planck statement. Nonetheless, with the proper definition, entropy production is always positive and the seco…
We study fluctuations of spin-polarized currents in a three-terminal spin-valve system consisting of a diffusive normal metal wire connected by tunnel junctions to three ferromagnetic terminals. Based on a spin-dependent Boltzmann-Langevin equation, we develop a semiclassical theory of charge and spin currents and the correlations of the currents fluctuations. In the three terminal system, we show that current fluctuations are strongly affected by the spin-flip scattering in the normal metal and the spin polarizations of the terminals, which may point in different directions. We analyze the de…
Theoretical and experimental work concerned with dynamic fluctuations has developed into a very active and fascinating subfield of mesoscopic physics. We present a review of this development focusing on shot noise in small electric conductors. Shot noise is a consequence of the quantization of charge. It can be used to obtain information on a system which is not available through conductance measurements. In particular, shot noise experiments can determine the charge and statistics of the quasiparticles relevant for transport, and reveal information on the potential profile and internal energy…
Mesoscopic systems provide us a unique experimental stage to address non-equilibrium quantum statistical physics. By using a simple tunneling model, we describe the electron exchange process via a quantum coherent conductor between two reservoirs, which yields the fluctuation theorem (FT) in mesoscopic transport. We experimentally show that such a treatment is semi-quantitatively validated in the current and noise measurement in an Aharonov-Bohm ring. The experimental proof of the microreversibility assumed in the derivation of FT is presented.
In order to specify a nonequilibrium steady state of a quantum wire (QWR), one must connect reservoirs to it. Since reservoirs should be large 2d or 3d systems, the total system is a large and inhomogeneous 2d or 3d system, in which e-e interactions have the same strength in all regions. However, most theories of interacting electrons in QWR considered simplified 1d models, in which reservoirs are absent or replaced with noninteracting 1d leads. We first discuss fundamental problems of such theories in view of nonequilibrium statistical mechanics. We then present formulations which are free fr…
When a biased conductor is put in proximity with an unbiased conductor a drag current can be induced in the absence of detailed balance. This is known as the Coulomb drag effect. However, even in this situation far away from equilibrium where detailed balance is explicitly broken, theory predicts that fluctuation relations are satisfied. This surprising effect has, to date, not been confirmed experimentally. Here we propose a system consisting of a capacitively coupled double quantum dot where the nonlinear fluctuation relations are verified in the absence of detailed balance.
Quantum Kinetic Uncertainty Relations in Mesoscopic Conductors at Strong Coupling
University of Geneva（日内瓦大学）；Instituto de Física Interdisciplinar y Sistemas Complejos IFISC (CSIC-UIB)（交叉物理与复杂系统研究所 IFISC (CSIC-UIB)）；ICFO-Institut de Ciències Fotòniques, The Barcelona Institute of Science and Technology（ICFO-光子科学研究所，巴塞罗那科学技术研究院）；Department of Metal and Semiconductor Physics, NTU “Kharkiv Polytechnic Institute”（哈尔科夫理工学院金属与半导体物理系）
We calculate the distribution of current fluctuations in two simple exclusion models. Although these models are classical, we recover even for small systems such as a simple or a double barrier, the same distibution of current as given by traditionnal formalisms for quantum mesoscopic conductors. Due to their simplicity, the full counting statistics in exclusion models can be reduced to the calculation of the largest eigenvalue of a matrix, the size of which is the number of internal configurations of the system. As examples, we derive the shot noise power and higher order statistics of curren…
We analyze high-field current fluctuations in degenerate conductors by mapping the electronic Fermi-liquid correlations at equilibrium to their semiclassical non-equilibrium form. Our resulting Boltzmann description is applicable to diffusive mesoscopic wires. We derive a non-equilibrium connection between thermal fluctuations of the current and resistive dissipation. In the weak-field limit this is the canonical fluctuation- dissipation theorem. Away from equilibrium, the connection enables explicit calculation of the excess ``hot-electron'' contribution to the thermal spectrum. We show that …
We summarize the main results of a microscopically based kinetic theory, applicable to open quantum point contacts (QPCs) driven up to high fields. The governing role of gauge invariance -- and the many-body sum rules for the electron gas -- lead to stringent constraints on both transport and fluctuations. These constraints exert a dominant influence on the observable properties of QPCs and similar open mesoscopic conductors. We illustrate this in the context of certain predictions within purely phenomenological models of mesoscopic transport.
We propose a two-terminal method to measure shot noise in mesoscopic systems based on an instability in the current-voltage characteristic of an on-chip detector. The microscopic noise drives the instability, which leads to random switching of the current between two values, the telegraph process. In the Gaussian regime, the shot noise power driving the instability may be extracted from the I-V curve, with the noise power as a fitting parameter. In the threshold regime, the extreme value statistics of the mesoscopic conductor can be extracted from the switching rates, which reorganize the comp…
We derive a closed equation of motion for the one particle density matrix of a quantum system coupled to multiple baths using the Redfield master equation combined with a mean-field approximation. The steady-state solution may be found analytically with perturbation theory. Application of the method to a one-dimensional non-interacting quantum wire yields an expression for the current that reproduces the celebrated Landauer's formula. Nonlinear rectification is found for the case of a mesoscopic three-dimensional semiconductor p-n junction. The results are in good agreement with numerical simu…
We present a theoretical investigation of shot-noise properties in nondegenerate elastic diffusive conductors. Both Monte Carlo simulations and analytical approaches are used. Two new phenomena are found: (i) the display of enhanced shot noise for given energy dependences of the scattering time, and (ii) the recovery of full shot noise for asymptotic high applied bias. The first phenomenon is associated with the onset of negative differential conductivity in energy space that drives the system towards a dynamical electrical instability in excellent agreement with analytical predictions. The en…
Entropy Production in Mesoscopic Electronic Transport Beyond Weak-Coupling
Instituto de Física Teórica, Universidade Estadual Paulista (UNESP)（圣保罗州立大学理论物理研究所）；Instituto de Física, Universidade Federal do Rio de Janeiro（里约热内卢联邦大学物理研究所）；Institut für Theoretische Physik, Universität Regensburg（雷根斯堡大学理论物理研究所）
