Vectorially structured light has emerged as an enabling tool in many diverse applications, from communication to imaging, exploiting quantum-like correlations courtesy of a non-separable spatially varying polarization structure. Creating these states at the source remains challenging and is presently limited to two-dimensional vectorial states by customized lasers. Here we invoke ray-wave duality in a simple laser cavity to produce polarization marked multi-path modes that are non-separable in three degrees of freedom and in eight dimensions. As a topical example, we use our laser to produce the complete set of Greenberger-Horne-Zeilinger (GHZ) basis states, mimicking high-dimensional multi-partite entanglement with classical light, which we confirm by a new projection approach. We offer a complete theoretical framework for our laser based on SU(2) symmetry groups, revealing a rich parameter space for further exploitation. Our approach requires only a conventional laser with no special optical elements, is easily scaleable to higher dimensions, and offers a simple but elegant solution for at-the-source creation of classically entangled states of structured light, opening new applications in simulating and enhancing high-dimensional quantum systems.
Given the multitude of applications of vector vortex beams there is a need for robust tools to measure them. Here we exploit the non-separability of such beams, akin to entanglement of quantum states, to apply tools traditionally associated with quantum measurements to these classical fields. We apply three measures of non-separability: a Bell inequality, a concurrence, and an entanglement entropy to define the "vectorness" of such beams. In addition to providing novel tools for the analysis of vector beams, we also introduce the concept of classical entanglement to explain why these tools are…
One of the most prominent features of quantum entanglement is its invariability under local unitary transformations, which implies the degree of entanglement remains constant during free-space propagation. While this is true for quantum and classically--entangled modes, here we demonstrate a novel type of classically-entangled modes that experience an entanglement decay upon free-space propagation. We show this by numerical simulations and corroborate experimentally. Our results evinces novel properties of classically-entangled modes, which pave the way to novel applications.
Tracking the kinematics of fast-moving objects is an important diagnostic tool for science and engineering. Existing optical methods include high-speed CCD/CMOS imaging, streak cameras, lidar, serial time-encoded imaging and sequentially timed all-optical mapping. Here, we demonstrate an entirely new approach to positional and directional sensing based on the concept of classical entanglement in vector beams of light. The measurement principle relies on the intrinsic correlations existing in such beams between transverse spatial modes and polarization. The latter can be determined from intensi…
Complex vector light modes, classically-entangled in their spatial and polarisation degrees of freedom (DoF), havebecome ubiquitous in a vast diversity of research fields. Crucially, while polarisation is limited to a bi-dimensionalspace, the spatial mode is unbounded, it can be specified by any of the sets of solutions the wave equation can supportin the different coordinate systems. Here we report on a class of vector beams with elliptical symmetry where thespatial DoF is encoded in the Ince-Gaussian modes of the cylindrical elliptical coordinates. We outline their geometricrepresentation on…
Einstein, Podolsky and Rosen's prediction on incompleteness of quantum mechanics was overturned by experimental tests on Bell's inequality that confirmed the existence of quantum entanglement. In X-ray optics, entangled photon pairs can be generated by X-ray parametric down conversion (XPDC), which has certain wavelength window. Meanwhile, free electron laser (FEL) has successfully lased at X-ray frequencies recently. However, FEL is usually seen as a classical light source, and its quantum effects are considered minor corrections to the classical theory. Here we investigate entangled X-ray ph…
Entangled photon sources (EPS), the major building block for a variety of quantum communication protocols, are commonly developed by utilizing the spontaneous parametric down-conversion (SPDC) in $χ^{2}$ nonlinear bulk optical materials. While high nonlinearity and long interaction length have established the superiority of the periodically poled crystals for EPSs, the phase-matching condition of such crystals is very sensitive to the fluctuation of the crystal temperature and the laser wavelength. As a result, deploying such sources outside the laboratory, for example, satellite-based applica…
In single-particle or intraparticle entanglement, two degrees of freedom of a single particle, e.g., momentum and polarization of a single photon, are entangled. Single-particle entanglement (SPE) provides a source of non classical correlations which can be exploited both in quantum communication protocols and in experimental tests of noncontextuality based on the Kochen-Specker theorem. Furthermore, SPE is robust under decoherence phenomena. Here, we show that single-particle entangled states of single photons can be produced from attenuated sources of light, even classical ones. To experimen…
We show that a strong infrared laser beam obliquely incident on graphene can experience a parametric instability with respect to decay into lower-frequency (idler) photons and THz surface plasmons. The instability is due to a strong in-plane second-order nonlinear response of graphene which originates from its spatial dispersion. The parametric decay leads to efficient generation of THz plasmons and gives rise to quantum entanglement of idler photons and surface plasmon states. A similar process can be supported by surface states of topological insulators such as Bi$_2$Se$_3$.
In the course of the high-frequency upgrade of GEO 600, its optical configuration was extended by a squeezed-light laser [1]. Recently, a non-classically enhanced measurement sensitivity of GEO 600 was reported [2]. In this paper, a characterization of the squeezed-light laser is presented. Thereupon, the status of the integration into GEO 600 is reviewed, focussing on the sources of optical loss limiting the shot noise reduction by squeezing at the moment. Finally, the possibilities for a future loss reduction are discussed.
In this paper we describe a test of Bell inequalities using a non- maximally entangled state, which represents an important step in the direction of eliminating the detection loophole. The experiment is based on the creation of a polarisation entangled state via the superposition, by use of an appropriate optics, of the spontaneous fluorescence emitted by two non-linear crystals driven by the same pumping laser.
We report on a test of Bell inequalities using a non-maximally entangled state, which represents an important step in the direction of eliminating the detection loophole. The experiment is based on the creation of a polarisation entangled state via the superposition, by use of an appropriate optics, of the spontaneous fluorescence emitted by two non-linear crystals driven by the same pumping laser. The alignment has profitably taken advantage from the use of an optical amplifier scheme, where a solid state laser is injected into the crystals together with the pumping laser. In principle a very…
Emission of pairs of photons in the interface metal-dielectric under the laser excitation arising due to the time-dependent perturbation of the zero-point fluctuations of the electromagnetic field by photons of the laser is considered. The enhancement of this emission by surface plasmons may be used for getting polarization-entangled photons. A possibility to compensate the energy of the zero-point fluctuations of bosons by other fluctuations with negative energy is discussed.
Spontaneous down conversion in metal-dielectric interface in case of oblique laser excitation is considered. In this case it is possible to generate pairs of polarization entangled surface plasmon polaritons with high efficiency if to use excitation angle corresponding to the Kretschmann configuration for generated plasmons. The efficiency can be additionally enlarged if to use properly nanostructured metallic film allowing one to directly excite surface plasmon polaritons and to fulfill phase matching condition of them with generated surface plasmon polaritons.
We study the quantum properties of light propagating through an array of coupled nonlinear waveguides and forming a discrete soliton. We demonstrate that it is possible to use certain types of quasi-solitons to form continuous variables entanglement between the certain pair of waveguides. This entanglement generation process occurs even with a very large number of photons in the laser field used, so it does not require a special material with an extremely high nonlinearity coefficient. Also absorption in the waveguide media does not influence it too much.
Bright sources of polarization-entangled photon pairs are essential components for quantum information technologies. In general, it is necessary to introduce a resonator that combines active optical components such as an electric optical modulator to enhance the stimulated emission of polarization-entangled photons. It is technically difficult to perform the time series operation to output the stimulated entangled photons in the resonator by synchronizing laser pulses. In this paper, we propose a scheme to scale up the stimulated emission of polarization-entangled photon pairs using a resonato…
We report on the realisation of a new test of Bell inequalities using the superposition of type I parametric down conversion produced in two different non-linear crystals pumped by the same laser, but with different polarisation. The produced state is non-maximally entangled. We discuss the advantages and the possible developments of this configuration.
We report on the first realisation of a test of Bell inequalities using non-maximally entangled states. It is based on the superposition of type I parametric down conversion produced in two different non-linear crystals pumped by the same laser, but with different polarisations. We discuss the advantages and the possible developments of this configuration.
Without developing a correct theory, the rate of the production of entangled photon pairs in the X-ray region by high energy electrons is estimated for experimental parameters used in a few experiments on X-ray parametric down conversion. Taking into account the need for X-ray entangled X-ray photons, it is proposed to begin the experimental study of such mechanism of nonlinear X-ray optics before the launch of the X-ray free electron lasers.
We show, both classically and quantum mechanically, enantioselective orientation of gas phase chiral molecules excited by laser fields with twisted polarization. Counterintuitively, the induced orientation, whose direction is laser controllable, does not disappear after the excitation, but stays approximately constant long after the end of the laser pulses, behavior unique to chiral systems. We computationally demonstrate this long-lasting orientation using propylene oxide molecules (${\rm CH_{3}CHCH_{2}O}$, or PPO) as an example, and consider two kinds of fields with twisted polarization: a p…
Spontaneous emission of the quantum system driven by a high intensity classical laser field is analyzed. The study is based on the accurate consideration of quantum system interaction with vacuum quantized field modes in the first order of perturbation theory, while the intense laser field is considered classically beyond the perturbation theory. It is demonstrated that the spectrum of the spontaneous emission can be used for analyzing of the strong-field dynamics and structure of the energy spectrum of the atomic system. The obtained data are compared with that obtained in the frames of semic…
Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and temporal-frequency resolutions, increased cross sections for multiphoton and nonlinear measurements, and new abilities in inducing or measuring quantum correlations. A critical step in enabling entangled photon spectroscopies is the creation of high-flux entangled sources that can use conventional detectors, as well as provide redundancy for the losses in realistic sampl…
