We have studied the nearest neighbor Heisenberg model with added Dzyaloshinskii-Moriya interaction using Schwinger boson mean field theory considering in-plane component as well as out-of-plane component. Motivated by experimental result of Vesigniete that the ground state is in Q = 0 long range order state, we first looked at the classical ground state of the model and consider the mean field ansatz which mimics the classical ground state in the large S limit. We have obtained the ground state phase diagram of this model and calculated properties of different phases. We have also studied the above model numerically using exact diagonalization up to a system size N = 30. We have compared the obtained results from these two approaches. Our results are in agreement with the experimental result of the Vesigniete.
We study the Heisenberg model on the pinwheel distorted kagome lattice as observed in the material Rb_2Cu_3SnF_12. Experimentally relevant thermodynamic properties at finite temperatures are computed utilizing numerical linked-cluster expansions. We also develop a Lanczos-based, zero-temperature, numerical linked cluster expansion to study the approach of the pinwheel distorted lattice to the uniform kagome-lattice Heisenberg model. We find strong evidence for a phase transition before the uniform limit is reached, implying that the ground state of the kagome-lattice Heisenberg model is likely…
A brief review is provided of earlier work on the low temperature phases of $S=1$ kagome and triangular lattice antiferromagnets in which there is sufficiently strongly single-ion anisotropy $D$ that dominates over the antiferromagnetic exchange $J$.
The magnetization process of the isotropic Heisenberg antiferromagnet on the kagome lattice is studied. Data obtained from the numerical-diagonalization method are reexamined from the viewpoint of the derivative of the magnetization with respect to the magnetic field. We find that the behavior of the derivative at approximately one-third of the height of the magnetization saturation is markedly different from that for the cases of typical magnetization plateaux. The magnetization process of the kagome-lattice antiferromagnet reveals a new phenomenon, which we call the "magnetization ramp".
Spin-1/2 Heisenberg model on kagome lattice is a typical frustrated quantum spin system. A basic structure of kagome lattice is also present in kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus study the magnetization plateaus of the spin-1/2 Heisenberg model on a kagome-strip chain with three-independent antiferromagnetic exchange interactions by the density-matrix renormalization group method. In a certain range of exchange parameters, we find twelve kinds of magnetization plateaus, nine of which have magnetic structures breaking either translati…
We study the ground state of a spin-half Heisenberg antiferromagnet on the stacked kagome lattice by using a spin-rotation-invariant Green's-function method. Since the pure two-dimensional kagome antiferromagnet is most likely a magnetically disordered quantum spin liquid, we investigate the question whether the coupling of kagome layers in a stacked three-dimensional system may lead to a magnetically ordered ground state. We present spin-spin correlation functions and correlation lengths. For comparison we apply also linear spin wave theory. Our results provide strong evidence that the system…
The anyonic excitations of a spin-liquid can feature fractional quantum numbers under space-group symmetries. Detecting these fractional quantum numbers, which are analogs of the fractional charge of Laughlin quasiparticles, may prove easier than the direct observation of anyonic braiding and statistics. Motivated by the recent numerical discovery of spin-liquid phases in the kagome Heisenberg antiferromagnet, we theoretically predict the pattern of space group symmetry fractionalization in the kagome lattice chiral spin liquid. We provide a method to detect these fractional quantum numbers in…
We have studied the effect of the Dzyaloshinskii-Moriya interaction on kagome Heisenberg anti-ferromagnet using Schwinger boson mean field theory (SBMFT). Within SBMFT framework, Messio et al had argued that the ground state of kagome antiferromagnet is possibly a chiral topological spin liquid (Phys. Rev. Lett. 108, 207204 (2012)). Thus, we have computed zero-temperature ground state phase diagram considering the time-reversal breaking states as well as fully symmetric Ansätze. We discuss the relevance of these results in experiments and other studies. Finally, we have computed the static and…
We study the phase diagram of the spin-1 quantum bilinear-biquadratic antiferromagnet on the kagome lattice using exact diagonalization and the density matrix renormalization group algorithm. The SU(3)-symmetric point of this model Hamiltonian is a spontaneously trimerized state whose qualitative nature persists even at the Heisenberg point, a finding that contrasts previous proposals. We report the ground state energy per site of the Heisenberg model to be -1.410(2) and establish the presence of a spin gap.
Motivated by recent numerical and experimental studies of the spin-1/2 Heisenberg antiferromagnet on kagome, we formulate a many-body model for fermionic spinons introduced by us earlier [Phys. Rev. Lett. 103, 187203 (2009)]. The spinons interact with an emergent U(1) gauge field and experience strong short-range attraction in the S=0 channel. The ground state of the model is generically a $Z_2$ liquid. We calculate the edge of the two-spinon continuum and compare the theory to the slave-fermion approach to the Heisenberg model.
We investigate the zero-temperature phase diagram of the nearest-neighbor kagome antiferromagnet in the presence of Dzyaloshinksii-Moriya interaction. We develop a theory for the transition between Z2 spin liquids with bosonic spinons and a phase with antiferromagnetic long-range order. Connections to recent numerical studies and experiments are discussed.
The coupled cluster method is applied to a spin-half model at zero temperature ($T=0$), which interpolates between Heisenberg antiferromagnets (HAF's) on a kagome and a square lattice. With respect to an underlying triangular lattice the strengths of the Heisenberg bonds joining the nearest-neighbor (NN) kagome sites are $J_{1} \geq 0$ along two of the equivalent directions and $J_{2} \geq 0$ along the third. Sites connected by $J_{2}$ bonds are themselves connected to the missing NN non-kagome sites of the triangular lattice by bonds of strength $J_{1}' \geq 0$. When $J_{1}'=J_{1}$ and $J_{2}…
We clarify the existence of several magnetization plateaux for the kagome $S=1/2$ antiferromagnetic Heisenberg model in a magnetic field. Using approximate or exact localized magnon eigenstates, we are able to describe in a similar manner the plateau states that occur for magnetization per site $m=1/3$, $5/9$, and $7/9$ of the saturation value. These results are confirmed using large-scale Exact Diagonalization on lattices up to 63 sites.
We construct a phenomenological Z_2 lattice gauge theory to describe the spin-liquid state of the S=1/2 kagome Heisenberg antiferromagnet in the sector with zero total spin. The model is a natural generalization of the Misguich-Serban-Pasquier Hamiltonian with added interactions that are strongly constrained by lattice symmetries. We are able to reproduce qualitatively many of the characteristic features observed in recent numerical studies. We also make connections to the previous works along similar lines.
Herbertsmithite (ZnCu3(OH)6Cl2) is often discussed as the best realization of the highly frustrated antiferromagnetic kagome lattice known so far. We employ density functional theory calculations to determine eight exchange coupling constants of the underlying Heisenberg Hamiltonian. We find the nearest neighbour coupling J1 to exceed all other couplings by far. However, next-nearest neighbour kagome layer couplings of 0.019 J1 and interlayer couplings of up to -0.035 J1 slightly modify the perfect antiferromagnetic kagome Hamiltonian. Interestingly, the largest interlayer coupling is ferromag…
Highly frustrated spin systems such as the kagome lattice (KL) are a treasure trove of new quantum states with large entanglements. We thus study the spin-$\frac{1}{2}$ Heisenberg model on a kagome-strip chain (KSC), which is one-dimensional KL, using the density-matrix renormalization group (DMRG) method. Calculating central charge and entanglement spectrum for the KSC, we find a novel gapless spin liquid state with doubly degenerate entanglement spectra in a 1/5 magnetization plateau. We also obtain a gapless low-lying continuum in the dynamic spin structure calculated by dynamical DMRG meth…
We consider the spin-1/2 antiferromagnetic Heisenberg model on the two-dimensional square-kagome lattice with almost dispersionless lowest magnon band. For a general exchange coupling geometry we elaborate low-energy effective Hamiltonians which emerge at high magnetic fields. The effective model to describe the low-energy degrees of freedom of the initial frustrated quantum spin model is the (unfrustrated) square-lattice spin-1/2 $XXZ$ model in a $z$-aligned magnetic field. For the effective model we perform quantum Monte Carlo simulations to discuss the low-temperature properties of the squa…
Motivated by recent experimental work on FeCrAs, we study the magnetic properties of classical spin models on the hexagonal Fe$_2$P/ZrNiAl structure (space group $P{\bar{6}}2m$). When both transition metal/rare earth sites carry magnetic moments, one has alternating distorted kagome and triangular lattice layers. Each point of the triangular lattice lies at the centre of a distorted hexagon and actually corresponds to three isolated magnetic atoms: a "trimer". We show that a simple model consisting of antiferromagnetically correlated Heisenberg spins on the frustrated distorted kagome lattice …
A preponderance of evidence suggests that the ground state of the nearest-neighbor $S = 1/2$ antiferromagnetic Heisenberg model on the kagome lattice is a gapless spin liquid. Many candidate materials for the realization of this model possess in addition a Dzyaloshinskii-Moriya (DM) interaction. We study this system by tensor-network methods and deduce that a weak but finite DM interaction is required to destabilize the gapless spin-liquid state. The critical magnitude, $D_c/J \simeq 0.012(2)$, lies well below the DM strength proposed in the kagome material herbertsmithite, indicating a need t…
Magnetization plateaus in quantum spin systems emerges in two-dimensional frustrated systems such as kagome lattice. The spin-1/2 antiferromagnetic Heisenberg model on square-kagome lattice is also appropriate for the study of magnetization plateau. Motivated by recent experimental finding of such a square-kagome lattice with nonequivalent three bonds, we investigate the phase diagrams and magnetization plateaus of the lattice by the exact diagonalization method. In addition to previously reported the 1/3 and 2/3 plateaus in the model with two equivalent bonds, we find a new 2/3 plateau whose …
In the search for spin-1/2 kagome antiferromagnets, the mineral volborthite has recently been the subject of experimental studies [Hiroi et al.,2001]. It has been suggested that the magnetic properties of this material are described by a spin-1/2 Heisenberg model on the kagome lattice with spatially anisotropic exchange couplings. We report on investigations of the Sp(N) symmetric generalisation of this model in the large N limit. We obtain a detailed description of the dependence of possible ground states on the anisotropy and on the spin length S. A fairly rich phase diagram with a ferrimagn…
Within the t-J model, we study the electronic properties of the doped antiferromagnet on the kagome lattice based on the framework of the self-consistent mean-field theory. At the half-filling, the spin-liquid ground-state energy per site of the kagome antiferromagnet is Eg/NJ=-0.859, which is in very good agreement with the numerical estimates. Away from the half-filling, the electron photoemission spectroscopy and density of states are discussed, and the results indicate that there is a gap in the normal-state of the system.
This paper is concerned with physics of the low energy singlet excitations found to exist below the spin gap in numerical studies of the Kagome lattice quantum Heisenberg antiferromagnet. Insight into the nature of these excitations is obtained by exploiting an approximate mapping to a fully frustrated transverse field Ising model on the dual dice lattice. This Ising model is shown to possess at least two phases - an ordered phase that also breaks translational symmetry with a large unit cell, and a paramagnetic phase. The former is argued to be a likely candidate for the ground state of the o…
The frustration of antiferromagnetic interactions on the loosely connected kagome lattice associated to the enhancement of quantum fluctuations for S=1/2 spins was acknowledged long ago as a keypoint to stabilize novel ground states of magnetic matter. Only very recently, the model compound Herbersmithite, ZnCu3(OH)6Cl2, a structurally perfect kagome antiferromagnet, could be synthesized and enables a close comparison to theories. We review and classify various experimental results obtained over the past years and underline some of the pending issues.
Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel insight into different contributions to its magnetism. At low temperatures, two distinct types of defects with different magnetic couplings to the kagome spins are found. Surprisingly, their magnetic response contradicts the three-fold symmetry of the ideal kagome lattice, suggesting the presence of a global structural distortion that may be related to the establi…
The low-energy singlet dynamics of the Quantum Heisenberg Antiferromagnet on the Kagome lattice is described by a quantitative Quantum Dimer Model. Using advanced numerical tools, the latter is shown to exhibit Valence Bond Crystal order with a large 36-site unit cell and hidden degeneracy between even and odd parities. Evidences are given that this groundstate lies in the vicinity of a $\mathbb{Z}_2$ dimer liquid region separated by a Quantum Critical Point. Implications regarding numerical analysis and experiments are discussed.
The recent NMR experiments on ZnCu3(OH)6Cl2 motivate our study of the effect of non- magnetic defects on the antiferromagnetic spin-1/2 kagome lattice. We use exact diagonalization methods to study the effect of two such defects on finite size systems. Our results, obtained without adjustable parameters, are in good quantitative agreement with recent Oxygen 17 NMR data. They provide support for the experimental interpretation of the presence of defects within the kagome layers due to Zn/Cu substitutions. Our results also show that disorder effects become relevant at lower temperatures, raising…
We study the zero-temperature phase diagram of the spin-$\frac{1}{2}$ Heisenberg model with breathing anisotropy (i.e., with different coupling strength on the upward and downward triangles) on the kagome lattice. Our study relies on large scale tensor network simulations based on infinite projected entangled-pair state and infinite projected entangled-simplex state methods adapted to the kagome lattice. Our energy analysis suggests that the U(1) algebraic quantum spin-liquid (QSL) ground-state of the isotropic Heisenberg model is stable up to very large breathing anisotropy until it breaks do…
Motivated by the unabating interest in the spin-1/2 Heisenberg antiferromagnetic model on the Kagome lattice, we investigate the energetics of projected Schwinger boson (SB) wave functions in the $J_1$--$J_2$ model with antiferromagnetic $J_2$ coupling. Our variational Monte Carlo results show that Sachdev's $Q_1=Q_2$ SB ansatz has a lower energy than the Dirac spin liquid for $J_2\gtrsim 0.08 J_1$ and the ${\bf q=0}$ Jastrow type magnetically ordered state. This work demonstrates that the projected SB wave functions can be tested on the same footing as their fermionic counterparts.
We propose a general non-perturbative scheme that quantitatively maps the low-energy sector of spin-1/2 frustrated Heisenberg antiferromagnets to effective Generalized Quantum Dimer Models. We develop the formal lattice independent frame and establish some important results on (i) the locality of the generated Hamiltonians (ii) how full resummations can be performed in this renormalization scheme. The method is then applied to the much debated kagome antiferromagnet for which a fully resummed effective Hamiltonian - shown to capture the essential properties and provide deep insights on the mic…
We study the quasi-one-dimensional limit of the spin-1/2 quantum Heisenberg antiferromagnet on the kagome lattice. The lattice is divided into antiferromagnetic spin-chains (exchange J) that are weakly coupled via intermediate "dangling" spins (exchange J'). Using one-dimensional bosonization, renormalization group methods, and current algebra techniques the ground state is determined in the limit J'<<J. We find that the dangling spins and chain spins form a spiral with O(1) and O(J'/J) static moments, respectively, atop of which the chain spins exhibit a smaller O[(J'/J)^2] antiferromagnetica…
Entanglement renormalization techniques are applied to numerically investigate the ground state of the spin-1/2 Heisenberg model on a kagome lattice. Lattices of N={36,144,inf} sites with periodic boundary conditions are considered. For the infinite lattice, the best approximation to the ground state is found to be a valence bond crystal (VBC) with a 36-site unit cell, compatible with a previous proposal. Its energy per site, E=-0.43221, is an exact upper bound and is lower than the energy of any previous (gapped or algebraic) spin liquid candidate for the ground state.
In this Letter, we identify a noncoplanar chiral spin texture on the distorted kagomé-lattice antiferromagnets induced by the presence of a magnetic field applied perpendicular to the distorted kagomé plane. The noncoplanar chiral spin texture has a nonzero scalar spin chirality similar to a chiral quantum spin liquid with broken time-reversal symmetry. In the noncoplanar regime we observe nontrivial topological magnetic excitations and thermal Hall response through the emergent field-induced scalar spin chirality in contrast to collinear ferromagnets in which the Dzyaloshinskii-Moriya (DM) sp…
We argue that the S=1/2 kagome antiferromagnet undergoes a quantum phase transition when the Dzyaloshinskii-Moriya coupling is increased. For $D<D_c$ the system is in a moment-free phase and for $D>D_c$ the system develops antiferromagnetic long-range order. The quantum critical point is found to be $D_c \simeq 0.1J$ using exact diagonalizations and finite-size scaling. This suggests that the kagome compound ZnCu$_3(OH)$_6$Cl$_3$ may be in a quantum critical region controlled by this fixed point.
The Kitaev-Heisenberg model on the honeycomb lattice has been studied for the purpose of finding exotic states such as quantum spin liquid and topological orders. On the kagome lattice, in spite of a spin-liquid ground state in the Heisenberg model, the stability of the spin-liquid state has hardly been studied in the presence of the Kitaev interaction. Therefore, we investigate the ground state of the classical and quantum spin systems of the kagome Kitaev-Heisenberg model. In the classical system, we obtain an exact phase diagram that has an eight-fold degenerated canted ferromagnetic phase …
We use $^{79}$Br nuclear quadrupole resonance (NQR) to demonstrate that ultra slow lattice dynamics set in below the temperature scale set by the Cu-Cu super-exchange interaction $J$~($\simeq160$~K) in the kagome lattice Heisenberg antiferromagnet Zn-barlowite. The lattice completely freezes below 50~K, and $^{79}$Br NQR lineshapes become twice broader due to increased lattice distortions. Moreover, the frozen lattice exhibits an oscillatory component in the transverse spin echo decay, a typical signature of pairing of nuclear spins by indirect nuclear spin-spin interaction. This indicates tha…
We investigate the extended Heisenberg model on the Kagome lattice by using Gutzwiller projected fermionic states and the variational Monte Carlo technique. In particular, when both second- and third-neighbor super-exchanges are considered, we find that a gapped spin liquid described by non-trivial magnetic fluxes and long-range chiral-chiral correlations is energetically favored compared to the gapless U(1) Dirac state. Furthermore, the topological Chern number, obtained by integrating the Berry curvature, and the degeneracy of the ground state, by constructing linearly independent states, le…
An effective spin-orbit Hamiltonian is derived for a spin-1/2 trimerized kagome antiferromagnet in the second-order of perturbation theory in the ratio of two coupling constants. Low-energy singlet states of the obtained model are mapped to a quantum dimer model on a triangular lattice. The quantum dimer model is dominated by dimer resonances on a few shortest loops of the triangular lattice. Characteristic energy scale for the dimer model constitutes only a small fraction of the weaker exchange coupling constant.
The ground state of the S=1/2 Heisenberg antiferomagnet on kagome can be viewed as a collection of fermionic spinons bound into small, heavy singlet pairs. Low-energy magnetic excitations in this system correspond to breaking the pairs into individual spinons. We calculate the structure factor for inelastic neutron scattering from independent spinon pairs.
We performed inelastic neutron scattering measurements on a polycrystalline sample of a classical kagome antiferromagnet NaBa$_{2}$Mn$_{3}$F$_{11}$ to investigate the possibility of a dispersionless zero-energy excitation associated with rotation of spins along the chains. The observed spectra indeed exhibit such an excitation with strong intensity at low energy, as well as dispersive excitations with weak intensity at high energy. Combining the measurements with calculations from linear spin-wave theory reveals that NaBa$_{2}$Mn$_{3}$F$_{11}$ is a good realization of the classical kagome anti…
With strong geometric frustration and quantum fluctuations, S=1/2 quantum Heisenberg antiferromagnets on the Kagome lattice has long been considered as an ideal platform to realize spin liquid (SL), a novel phase with no symmetry breaking and fractionalized excitations. A recent numerical study of Heisenberg S=1/2 Kagome lattice model (HKLM) show that in contrast to earlier studies, the ground state is a singlet-gapped SL with signatures of Z2 topological order. Motivated by this numerical discovery, we use projective symmetry group to classify all 20 possible Schwinger-fermion mean-field stat…
We present numerical evidence for the emergence of an extended valence bond solid (VBS) phase at $T=0$ in the kagome $S=1/2$ Heisenberg antiferromagnet with ferromagnetic further-neighbor interactions. The VBS is located at the boundary between two magnetically ordered regions and extends close to the nearest-neighbor Heisenberg point. It exhibits a diamond-like singlet covering pattern with a $12$-site unit-cell. Our results suggest the possibility of a direct, possibly continuous, quantum phase transition from the neighboring $\mathbf{q}=0$ coplanar magnetically ordered phase into the VBS ph…
We perform a Gutzwiller projected wavefunction study for the spin-1/2 Heisenberg model on the Kagome lattice to compare energies of several spin-liquid states. The result indicates that a U(1)-Dirac spin-liquid state has the lowest energy. Furthermore, even without variational parameters, the energy turns out to be very close to that found by exact diagonalization. We show that such a U(1)-Dirac state represents a quantum phase whose low energy physics is governed by four flavors of two-component Dirac fermions coupled to a U(1) gauge field. These results are discussed in the context of recent…
The spin wave excitations of the ideal S=5/2 Kagome lattice antiferromagnet KFe3(OH)6(SO4)2 have been measured using high-resolution inelastic neutron scattering. We directly observe a flat mode which corresponds to a lifted "zero energy mode," verifying a fundamental prediction for the Kagome lattice. A simple Heisenberg spin Hamiltonian provides an excellent fit to our spin wave data. The antisymmetric Dzyaloshinskii-Moriya interaction is the primary source of anisotropy and explains the low temperature magnetization and spin structure.
Motivated by recent experiments on ZnCu$_3$(OH)$_6$Cl$_2$, we study the inhomogeneous Knight shifts (local susceptibilities) of spin 1/2 Kagome antiferromagnet in the presence of nonmagnetic impurities. Using high temperature series expansion, we calculate the local susceptibility and its histogram down to about T=0.4J. At low temperatures, we explore a Dirac spin liquid proposal and calculate the local susceptibility in the mean field and beyond mean field using Gutzwiller projection, finding the overall picture to be consistent with the NMR experiments.
By using the density matrix renormalization group, we study the spin-liquid phases of spin-$1/2$ XXZ kagome antiferromagnets. We find that the emergence of spin liquid phase does not depend on the anisotropy of the XXZ interaction. In particular, the two extreme limits---Ising (strong $S^z$ interaction) and XY (zero $S^z$ interaction)---host the same spin-liquid phases as the isotropic Heisenberg model. Both the time-reversal-invariant spin liquid and the chiral spin liquid with spontaneous time-reversal symmetry breaking are obtained. We show they evolve continuously into each other by tuning…
Frustrated one-dimensional quantum spin systems are known to exhibit a variety of quantum ground states due to the effects of quantum fluctuations and frustrations. In a spin-1/2 kagome-strip chain, which is one of the frustrated one-dimensional spin systems, many quantum phases have been found. However, the magnetic phase diagrams of the kagome-strip chain under magnetic field have not been fully understood. We construct magnetic phase diagrams at 0, 1/5, 3/10, 1/3, 2/5, 7/15, 3/5, and 4/5 magnetization ratio in the kagome-strip chain and investigate magnetic properties in each phase using th…
Spin dynamics of the spin-1/2 kagome lattice antiferromagnet Cs$_2$Cu$_3$SnF$_{12}$ was studied using high-resolution, time-of-flight inelastic neutron scattering. The flat mode, a characteristic of the frustrated kagome antiferromagnet, and the low-energy dispersive mode, which is dominated by magnons, can be well described by the linear spin-wave theory. However, the theory fails to describe three weakly dispersive modes between 9 and 14 meV. These modes could be attributed to two-spinon bound states, which decay into free spinons away from the zone center and at a high temperature, giving r…
We study a class of disordered continuous classical spin systems including the kagome Heisenberg magnet. While each term in its local Hamiltonian can be independently minimised, we find {\it discrete} degenerate ground states whose number grows exponentially with system size. These states do not exhibit zero-energy `excitations' characteristic of highly frustrated magnets but instead are local minima of the energy landscape, albeit with an anomalously soft excitation spectrum. This represents a spin liquid version of the phenomenon of jamming familiar from granular media and structural glasses…
We report the crystal structure and unconventional magnetic ordering of Cs_2Cu_3CeF_{12}, which is composed of buckled kagome lattice of Cu^{2+} ions. The exchange network in the buckled kagome lattice is fairly anisotropic, so that the present spin system can be divided into two subsystems: alternating Heisenberg chains with strong antiferromagnetic exchange interactions and dangling spins. Although the direct exchange interactions between neighboring spins were found to be all antiferromagnetic, ferromagnetic magnetic ordering of the dangling spins was observed. Magnetization exhibits a plat…
The dc-magnetization of the unique S=1/2 kagome antiferromagnet Herbertsmithite has been measured down to 0.1K. No sign of spin freezing is observed in agreement with former muSR and ac-susceptibility results. The low temperature magnetic response is dominated by a defect contribution which exhibits a new energy scale $\simeq 1$ K, likely reflecting the coupling of the defects. The defect component is saturated at low temperature by H>8T applied magnetic fields which enables us to estimate an upper bound for the non saturated intrinsic kagome susceptibility at T=1.7K.
Motivated by a recent experiment on volborthite, a typical spin-$1/2$ antiferromagnet with a kagomé lattice structure, we study the magnetization process of a classical Heisenberg model on a spatially distorted kagomé lattice using the Monte Carlo (MC) method. We find a distortion-induced magnetization step at low temperatures and low magnetic fields. The magnitude of this step is given by $Δm_z=\left|1-α\right|/3α$ at zero temperature, where $α$ denotes the spatial anisotropy in exchange constants. The magnetization step signals a first-order transition at low temperatures, between two phases…
We provide strong numerical evidence, using improved variational wave functions, for a ground state with vanishing spin gap in the spin-$1/2$ quantum Heisenberg model on the kagome lattice. Starting from the algebraic $U(1)$ Dirac spin liquid state proposed by Y. Ran $et al.$ [Phys. Rev. Lett. $98$, $117205$ ($2007$)] and iteratively applying a few Lanczos steps, we compute the lowest $S=2$ excitation constructed by exciting spinons close to the Dirac nodes. Our results are compatible with a vanishing spin gap in the thermodynamic limit and in consonance with a power-law decay of long distance…
The antiferromagnetism in $α$-Cu$_3$Mg(OH)$_6$Br$_2$ was studied by magnetic-susceptibility, specific-heat and neutron-diffraction measurements. The crystal structure consists of Cu$^{2+}$ kagome layers with Mg$^{2+}$ ions occupying the centers of the hexagons, separated by Br$^{1-}$ ions. The magnetic system orders antiferromagnetically at 5.4 K with the magnetic moments aligned ferromagnetically within the kagome planes. The ordered moment is 0.94 $μ_B$, suggesting little quantum and geometrical fluctuations. By comparing the magnetic and specific-heat properties with those of the haydeeite,…
We propose in this work an effective field theory description of the chiral spin liquid state in Heisenberg spin system on kagomé lattice.To this end, we derive the low-energy effective theory of kagomé (isotropic) Heisenberg antiferromagnet around its ordered ground states found numerically and show that quantum fluctuations induced by further neighbor spin exchanges are equally strong as those from first neighbor.We use a chiral order parameter theory to argue for the occurrence of finite temperature chiral symmetry breaking transition into chiral ordered state in kagomé antiferromagnet with…
Density matrix renormalization group (DMRG) calculations on large systems (up to 3096 spins) indicate that the ground state of the Heisenberg model on a 3-chain Kagome strip is spontaneously dimerized. This system has degenerate ground states and a gap to triplet and singlet excitations. These results are in direct contradiction with recent results of Azaria et al (Phys. Rev. Lett. 81, 1694 (1998)) and suggest a need for a reexamination of the underlying field theory.
Through exact diagonalization study of the spin - 1/2 Heisenberg model on Kagome lattice with ring-exchange coupling $J_{r}$, we find the pure Heisenberg model with $J_{r}=0$ stands as a quantum critical point, as evidenced by avoided level crossing and divergence of the second derivative of the ground state energy with respect to $J_{r}$ at $J_{r}=0$. The pure Heisenberg model should thus be gapless in the thermodynamic limit, contrary to common beliefs. At the same time, the ring exchange coupling is found to drive the system into a state with more short ranged spin correlation and with a lo…
Magnetic excitations in the spin-$\frac{1}{2}$ distorted kagome lattice antiferromagnet Cs$_2$Cu$_3$SnF$_{12}$, which has an ordered ground state owing to the strong Dzyaloshinskii-Moriya interaction, were studied using inelastic neutron scattering. Although the spin-wave dispersion can be qualitatively understood in terms of linear spin-wave theory (LSWT), the excitation energies are renormalized by a factor of approximately 0.6 from those calculated by LSWT, almost irrespective of the momentum transfer. This inadequacy of LSWT, which is attributed to quantum fluctuations, provides evidence o…
