We present the possibility of spin-dependent Kapitza-Dirac scattering based on a two-photon interaction only. The interaction scheme is inspired from a Compton scattering process, for which we explicitly show the mathematical correspondence to the spin-dynamics of an electron diffraction process in a standing light wave. The spin effect has the advantage that it already appears in a Bragg scattering setup with arbitrary low field amplitudes, for which we have estimated the diffraction count rate in a realistic experimental setup at available X-ray free-electron laser facilities.
We analyze the Bragg regime of the two-particle Kapitza-Dirac arrangement, completing the basic theory of this effect. We provide a detailed evaluation of the detection probabilities for multi-mode states, showing that a complete description must include the interaction time in addition to the usual dimensionless parameter w. The arrangement can be used as a massive two-particle beam splitter. In this respect, we present a comparison with Hong-Ou-Mandel-type experiments in quantum optics. The analysis reveals the presence of dips for massive bosons and a differentiated behavior of distinguisha…
Interactions between atoms and light fields are usually described in the electric-dipole approximation. We show that electric-quadrupole terms are important in the Kapitza-Dirac arrangement for light gratings on resonance with a quadrupole atomic transition. We derive the diffraction patterns, which in some cases are experimentally verifiable with the same techniques used with dipole transitions.
We theoretically demonstrate the feasibility of producing electron beam splitter using Kapitza-Dirac diffraction on bichromatic standing waves which are created by the fundamental frequency and the third harmonic. The relativistic electron in Bragg regime absorbs three photons with frequency of w and emits a photon with frequency of 3w, four-photon Kapitza-Dirac effect. In this four-photon Kapitza-Dirac effect distinct spin effects arise in different polarizations of the third harmonic laser beam. It is shown that the shape of Rabi oscillation between initial and scattered states is changed an…
Kapitza-Dirac scattering of nonrelativistic electrons from counterpropagating bichromatic laser waves of linear polarization is studied. The focus lies on the electronic spin dynamics in the Bragg regime when the laser fields possess a frequency ratio of two. To this end, the time-dependent Pauli equation is solved numerically, both in coordinate space and momentum space. Our numerical results are corroborated by analytical derivations. We demonstrate that, for certain incident electron momenta, the scattering crucially relies on the electron spin which undergoes characteristic Rabi-like oscil…
Spin-dependent Kapitza-Dirac scattering of electron beams from counterpropagating bichromatic laser waves in various polarization geometries is studied. The corresponding scattering probabilities are obtained by analytical and numerical solutions of the time-dependent Dirac equation, assuming a field frequency ratio of 2. When the fundamental field mode is circular-polarized, we show that spin dynamics are generally suppressed at low intensities, but can become distinct at high intensities. Conversely, when a linearly or elliptically polarized fundamental mode is combined with a second harmoni…
Computational methods are indispensable to study the quantum dynamics of relativistic light-matter interactions in parameter regimes where analytical methods become inapplicable. We present numerical methods for solving the time-dependent Dirac equation and the time-dependent Klein-Gordon equation and their implementation on high performance graphics cards. These methods allow us to study tunneling from hydrogen-like highly charged ions in strong laser fields and Kapitza-Dirac scattering in the relativistic regime.
The Kapitza-Dirac effect, which refers to electron scattering at standing light waves, is studied in the Bragg regime with counterpropagating elliptically polarized electromagnetic waves with the same intensity, wavelength, and degree of polarization for two different setups. In the first setup, where the electric-field components of the counterpropagating waves have the same sense of rotation, we find distinct spin effects. The spins of the scattered electrons and of the nonscattered electrons, respectively, precess with a frequency that is of the order of the Bragg-reflection Rabi frequency.…
We extend the study of Kapitza-Dirac diffraction to the case of two-particle systems. Due to the exchange effects the shape and visibility of the two-particle detection patterns show important differences for identical and distinguishable particles. We also identify a novel quantum statistics effect present in momentum space for some values of the initial particle momenta, which is associated with different numbers of photon absorptions compatible with the final momenta.
Electron spin dynamics in Kapitza-Dirac scattering from a standing laser wave of high frequency and high intensity is studied. We develop a fully relativistic quantum theory of the electron motion based on the time-dependent Dirac equation. Distinct spin dynamics, with Rabi oscillations and complete spin-flip transitions, is demonstrated for Kapitza-Dirac scattering involving three photons in a parameter regime accessible to future high-power X-ray laser sources. The Rabi frequency and, thus, the diffraction pattern is shown to depend crucially on the spin degree of freedom.
We analyze the diffraction of elementary systems as the electron by light gratings when they are described by charge distributions instead of the usual point-like form. The treatment of the problem is based on the introduction, in analogy with atomic polarizability, of state-dependent non-permanent multi-pole moments for the charge. The diffraction patterns can provide bounds on these moments. With this approach we can experimentally explore some aspects of the interpretation of the wave picture of single charges.
In this paper we present an analysis of the spin behavior of electrons propagating through a laser field. We present an experimentally realizable scenario in which spin-dependent effects of the interaction between the laser and the electrons are dominant. The laser interaction strength and incident electron velocity are in the nonrelativistic domain. This analysis may thus lead to novel methods of creating and characterizing spin-polarized nonrelativistic femtosecond electron pulses.
The Kapitza - Dirac effect is the diffraction of a well - collimated particle beam by a standing wave of light. Why is this interesting? Comparing this situation to the introductory physics textbook example of diffraction of a laser beam by a grating, the particle beam plays the role of the incoming wave and the standing light wave the role of the material grating, highlighting particle - wave duality. Apart from representing such a beautiful example of particle - wave duality, the diffracted particle beams are coherent. This allows the construction of matter interferometers and explains why t…
We theoretically investigate the influence of a longitudinal laser polarization component from beam focusing on spin dynamics in Kapitza-Dirac scattering by solving the relativistic Dirac equation with time-dependent perturbation theory. The transverse spacial dependence of the longitudinal beam polarization component is accounted for, by approximating a Gaussian beam with plane-wave components. We find that corrections from a longitudinal laser beam polarization component approximately scale with the second power of the diffraction angle $ε$, from which we conclude that a related influence fr…
Harmonic oscillators count among the most fundamental quantum systems with important applications in molecular physics, nanoparticle trapping, and quantum information processing. Their equidistant energy level spacing is often a desired feature, but at the same time a challenge if the goal is to deterministically populate specific eigenstates. Here, we show how interference in the transition amplitudes in a bichromatic laser field can suppress the sequential climbing of harmonic oscillator states (Kapitza-Dirac blockade) and achieve selective excitation of energy eigenstates, Schrödinger cats …
In the Kapitza-Dirac effect, atoms, molecules, or swift electrons are diffracted off a standing wave grating of the light intensity created by two counter-propagating laser fields. In ultrafast electron optics, such a coherent beam splitter offers interesting perspectives for ultrafast beam shaping. Here, we study, both analytically and numerically, the effect of the inclination angle between two laser fields on the diffraction of pulsed, low-energy electron beams. For sufficiently high light intensities, we observe a rich variety of complex diffraction patterns. These do not only reflect inte…
Kapitza-Dirac-Talbot-Lau interferometry (KDTLI) has recently been established for demonstrating the quantum wave nature of large molecules. A phase space treatment permits us to derive closed equations for the near-field interference pattern, as well as for the Moire-type pattern that would arise if the molecules were to be treated as classical particles. The model provides a simple and elegant way to account for the molecular phase shifts related to the optical dipole potential as well as for the incoherent effect of photon absorption at the second grating. We present experimental results for…
Coherent regime of Kapitza-Dirac effect with electrons
Faculty of Mathematics and Physics, Charles University（查理大学数学物理学院）；Institute of Physics, Czech Academy of Sciences（捷克科学院物理研究所）；Carl Zeiss Microscopy GmbH（卡尔蔡司显微镜有限公司）
The stationary eigenstates and eigenvalues for the ponderomotive potential of an optical crystal confined in a one-dimensional infinite square well are numerically obtained. The initial states of the incoming particles taken as Gaussian, are expanded in the basis of the stationary eigenstates of the ponderomotive potential, to obtain the subsequent time evolution of the wave function of the particle during the interaction with the optical crystal. From the results of the time evolution of the probability density, it is observed that the particles get localized at equidistant positions in the t…
Research on matter waves is a thriving field of quantum physics and has recently stimulated many investigations with electrons, neutrons, atoms, Bose-condensed ensembles, cold clusters and hot molecules. Coherence experiments with complex objects are of interest for exploring the transition to classical physics, for measuring molecular properties and they have even been proposed for testing new models of space-time. For matter-wave experiments with complex molecules, the strongly dispersive effect of the interaction between the diffracted molecule and the grating wall is a major challenge beca…
It is shown that the Kapitza-Dirac effect with atoms, which has been considered to be evidence of their wavelike character, can be interpreted as a scattering of pointlike objects by the periodic laser field.
We theoretically discuss several aspects of sequential superradiant scattering from atomic Bose-Einstein condensates. Our treatment is based on the semiclassical description of the process in terms of the Maxwell-Schroedinger equations for the coupled matter-wave and optical fields. First, we investigate sequential scattering in the weak-pulse regime and work out the essential mechanisms responsible for bringing about the characteristic fan-shaped side-mode distribution patterns. Second, we discuss the transition between the Kapitza-Dirac and Bragg regimes of sequential scattering in the stron…
Diffraction of walking drops by a standing Faraday wave
Department of Mathematics, MIT（麻省理工学院数学系）；Department of Mechanical Engineering, Boston University（波士顿大学机械工程系）；Department of Mathematics, UNC, Chapel Hill（北卡罗来纳大学教堂山分校数学系）
We consider optical systems where propagation of light can be described by a Dirac-like equation with $PT$-symmetric Hamiltonian. In order to construct exactly solvable configurations, we extend the confluent Crum-Darboux transformation for the one-dimensional Dirac equation. The properties of the associated intertwining operators are discussed and the explicit form for higher-order transformations is presented. We utilize the results to derive a multi-parametric class of exactly solvable systems where the balanced gain and loss represented by the $PT$-symmetric refractive index can imply loca…
We theoretically study the optical properties of a Fermi-Dirac gas in the presence of a superfluid state. We calculate the leading quantum-statistical corrections to the standard column density result of the electric susceptibility. We also consider the Bragg diffraction of atoms by means of light-stimulated transitions of photons between two intersecting laser beams. Bardeen-Cooper-Schrieffer pairing between atoms in different internal levels magnifies incoherent scattering processes. The absorption linewidth of a Fermi-Dirac gas is broadened and shifted. Bardeen-Cooper-Schrieffer pairing int…
We demonstrate the theoretical feasibility of spin-dependent diffraction and spin-polarization of an electron in two counter-propagating, circularly polarized laser beams. The spin-dynamics appears in a two-photon process of the Kapitza-Dirac effect in the Bragg regime. We show the spin-dependence of the diffraction process by comparison of the time-evolution of a spin-up and spin-down electron in a relativistic quantum simulation. We further discuss the spin properties of the scattering by studying an analytically approximated solution of the time-evolution matrix. A classification scheme in …
We report an experimental demonstration of engineering phase wraps for sub-wavelength structure in a Bose-Einstein condensate (BEC) with two-dimensional optical lattices. A short lattice pulse is applied on BEC working in the Kapitza-Dirac (or Raman-Nath) regime, which corresponds to phase modulation imprint on matter wave. When the phase modulation on matter wave is larger than $2π$ in a lattice cell, there appears phase wraps with multiple $2π$ jumps, generating the sub-wavelength phase structure. The phase wraps for sub-wavelength structure are measured in momentum space via the time-of-fli…
The electron spin degree of freedom can play a significant role in relativistic scattering processes involving intense laser fields. In this contribution we discuss the influence of the electron spin on (i) Kapitza-Dirac scattering in an x-ray laser field of high intensity, (ii) photo-induced electron-positron pair production in a strong laser wave and (iii) multiphoton electron-positron pair production on an atomic nucleus. We show that in all cases under consideration the electron spin can have a characteristic impact on the process properties and their total probabilities. To this end, spin…
Decoherence can be provided by a dissipative environment as described by the Caldeira-Leggett equation. This equation is foundational to the theory of quantum dissipation. However, no experimental test has been performed that measures for one physical system both the dissipation and the decoherence. Anglin and Zurek predicted that a resistive surface could provide such a dissipative environment for a free electron wave passing close to it. We propose that the electron wave's coherence and energy loss can be measured simultaneously by using Kapitza-Dirac scattering for varying light intensity.
We analyze the diffraction regime of the Kapitza-Dirac effect for particles entangled in momentum. The detection patterns show two-particle interferences. In the single-mode case we identify a discontinuity in the set of joint detection probabilities, associated with the disconnected character of the space of non-separable states. For Gaussian multi-mode states we derive the diffraction patterns, providing an example of the dependence of the light-matter interaction on entanglement. When the particles are identical, we can explore the relation between exchange and entanglement effects. We find…
We provide support for the claim that momentum is conserved for individual events in the electron double slit experiment. The natural consequence is that a physical mechanism is responsible for this momentum exchange, but that even if the fundamental mechanism is known for electron crystal diffraction and the Kapitza-Dirac effect, it is unknown for electron diffraction from nano-fabricated double slits. Work towards a proposed explanation in terms of particle trajectories affected by a vacuum field is discussed. The contentious use of trajectories is discussed within the context of oil droplet…
The present work theoretically investigates the probability of generation of entangled electron-photon pair in high-energy Compton scattering of unpolarized electrons and photons due to scattering-channel-exchange mechanism. The study suggests that the scattering of unpolarized electrons and photons with nearly equal energy of the order of MeV at cross-channel can create entangled pair of up-spin electron and RCP photon or down-spin electron and LCP photon. The entanglement is quite strong exhibiting jump-concurrence for particular directions of scattering however not limited by the Kapitza-Di…
We study the effects of strong inter-particle interaction on diffraction of a Bose-Einstein condensate of $^6Li_2$ molecules from a periodic potential created by pulses of a far detuned optical standing wave. For short pulses we observe the standard Kapitza-Dirac diffraction, with the contrast of the diffraction pattern strongly reduced for very large interactions due to interaction dependent loss processes. For longer pulses diffraction shows the characteristic for matter waves impinging on an array of tubes and coherent channeling transport. We observe a slowing down of the time evolution go…
The secular dynamics of a non-relativistic charged particle in an electromagnetic wave can be described by the ponderomotive potential. Although ponderomotive electron-laser interactions at relativistic velocities are important for emerging technologies from laser-based particle accelerators to laser-enhanced electron microscopy, the effects of special relativity on the interaction have only been studied theoretically. Here, we use a transmission electron microscope to measure the position-dependent phase shift imparted to a relativistic electron wave function when it traverses a standing lase…
