L $1_0$ FePt是一种用于一系列新型数据存储应用的技术上重要的材料。在有序的FePt结构中,通常非磁性的Pt离子获得磁矩,其取决于源自相邻Fe原子的局部场。在这项工作中,FePt的模型构建,其中诱导Pt力矩模拟使用组合的纵向和旋转自旋动力学。该模型被参数化,包括一个线性变化的时刻与交换场,使在Pt网站的磁矩取决于Fe的顺序。居里温度的FePt的计算和同意以及类似的模型,将Pt的动力学通过一个有效的Fe-唯一的哈密顿。通过计算动态关联函数,提取了一定温度范围内的各向异性场和吉尔伯特阻尼。各向异性与温度呈指数$n\approx2.1$的幂律关系。这与实验观察到的结果一致,并且它是在不包括其他方法中的两个离子各向异性项的情况下获得的。我们的工作表明,将纵向涨落自旋动力学计算是至关重要的理解材料的诱导力矩的性质。
英文摘要:
L$1_0$ FePt is a technologically important material for a range of novel data storage applications. In the ordered FePt structure the normally non-magnetic Pt ion acquires a magnetic moment, which depends on the local field originating from the neighboring Fe atoms. In this work a model of FePt is constructed, where the induced Pt moment is simulated by using combined longitudinal and rotational spin dynamics. The model is parameterized to include a linear variation of the moment with the exchange field, so that at the Pt site the magnetic moment depends on the Fe ordering. The Curie temperature of FePt is calculated and agrees well with similar models that incorporate the Pt dynamics through an effective Fe-only Hamiltonian. By computing the dynamic correlation function the anisotropy field and the Gilbert damping are extracted over a range of temperatures. The anisotropy exhibits a power-law dependence with temperature with exponent $n\approx2.1$. This agrees well with what observed experimentally and it is obtained without including a two-ion anisotropy term as in other approaches. Our work shows that incorporating longitudinal fluctuations into spin dynamics calculations is crucial for understanding the properties of materials with induced moments.
Observation of the Nernst effect driven by longitudinal spin fluctuations
National Institute for Materials Science(国立材料研究所);Research Institute for Interdisciplinary Science, Okayama University(冈山大学交叉科学研究所);Department of Advanced Materials Science, Graduate School of Frontier Sciences, The University of Tokyo(东京大学前沿科学研究生院先进材料科学系)
An ab initio effective Hamiltonian for magnetism including longitudinal spin fluctuations
我们讨论了使用的磁力定理(MFT)使用不同的参考状态后,微扰的方法是基于。使用无序局域矩(DLM)状态,人们发现在3d磁体Fe、Co(fcc)、Mn、Cr中的平面自旋螺旋具有良好的居里(或Neel)温度和良好的能量学。另一方面,铁磁参考态为Fe,Co和Ni中的小$θ$自旋螺旋提供了极好的能量,并在磁容假设下扩展了磁振子能量。然而,平面自旋螺旋能量和转变温度为镍,铁,锰,铬显示较差的协议。这是因为,并为fcc公司的情况下,当两种方法都工作得很好进行了讨论。我们进一步提供了一个扩展的映射的量子问题,包括纵向波动,并讨论它们将在磁相变中发挥的作用。使用平面自旋螺旋测试这种力矩,其中${\bf q}$是固定的,但允许力矩释放。结果表明,从磁力定理的方法和直接计算的{ \it ab initio}值的结果非常一致。
First-principles study of magnetic and spin-dependent transport properties of Mn2VZ (Z = Al, Ga) with negative spin polarization using a disordered local moment approach at finite temperatures
Max-Planck-Institute for Chemical Physics of Solids(德国马克斯·普朗克固体化学物理研究所);Tohoku University, Center for Science and Innovation in Spintronics(日本东北大学自旋科学创新中心)